• Title/Summary/Keyword: fission

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Application of Laser Ablation Inductively Coupled Plasma Mass Spectrometry for Characterization of U-7Mo/Al-5Si Dispersion Fuels

  • Lee, Jeongmook;Park, Jai Il;Youn, Young-Sang;Ha, Yeong-Keong;Kim, Jong-Yun
    • Nuclear Engineering and Technology
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    • v.49 no.3
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    • pp.645-650
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    • 2017
  • This technical note demonstrates the feasibility of using laser ablation inductively coupled plasma mass spectrometry for the characterization of U-7Mo/Ale5Si dispersion fuel. Our measurements show 5.0% Relative Standard Deviation (RSD) for the reproducibility of measured $^{98}Mo/^{238}U$ ratios in fuel particles from spot analysis, and 3.4% RSD for $^{98}Mo/^{238}U$ ratios in a NIST-SRM 612 glass standard. Line scanning allows for the distinction of U-7Mo fuel particles from the Al-5Si matrix. Each mass spectrum peak indicates the presence of U-7Mo fuel particles, and the time width of each peak corresponds to the size of that fuel particle. The size of the fuel particles is estimated from the time width of the mass spectrum peak for $^{98}Mo$ by considering the scan rate used during the line scan. This preliminary application clearly demonstrates that laser ablation inductively coupled plasma mass spectrometry can directly identify isotope ratios and sizes of the fuel particles in U-Mo/Al dispersion fuel. Once optimized further, this instrument will be a powerful tool for investigating irradiated dispersion fuels in terms of fission product distributions in fuel matrices, and the changes in fuel particle size or shape after irradiation.

A 235U mass measurement method for UO2 rod assembly based on the n/γ joint measurement system

  • Yang, Jianqing;Zhang, Quanhu;Su, Xianghua;Li, Sufen;Zhuang, Lin;Hou, Suxia;Huo, Yonggang;Zhou, Hao;Liu, Guorong
    • Nuclear Engineering and Technology
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    • v.52 no.5
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    • pp.1036-1042
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    • 2020
  • Fast-Neutron Multiplicity Counter based on Liquid Scintillator Detector can directly measure the fast neutron multiplicity emitted by UO2 rod. HPGe gamma spectrometer; which has superior energy resolution; is routinely used for the gamma energy spectrum measurement. Combing Fast-Neutron Multiplicity Counter and HPGe γ-spectrometer, the n/γ joint measurement system is developed. The fast neutron multiplicity and gamma energy spectrum of UO2 rod assemblies under different conditions are measured by the n/γ joint measurement system. The induced fission rate and the 235U abundance, thereby the 235U mass; can be obtained for UO2 rod assemblies. The 235U mass deviation of the measured value from the reference value is less than 5%. The results show that the n/γ joint measurement system is effective and applicable in the measurement of the 235U mass in samples.

Decay Heat Evaluation of Spent Fuel Assemblies in SFP of Kori Unit-1

  • Kim, Kiyoung;Kim, Yongdeog;Chung, Sunghwan
    • Proceedings of the Korean Radioactive Waste Society Conference
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    • 2018.11a
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    • pp.104-104
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    • 2018
  • Kori Unit 1 is the first permanent shutdown nuclear power plant in Korea and it is on June 18th, 2017. Spent fuel assemblies began to be discharged from the reactor core to the spent fuel pool(SFP) within one week after shutdown of Kori unit 1 and the campaign was completed on June 27th, 2017. The total number of spent nuclear fuel assemblies in SFP of Kori Unit-1 is 485 and their discharging date is different respectively. So, decay heat was evaluated considering the actual enrichment, operation history and cooling time of the spent fuel assemblies stored in SFP of the Kori Unit-1. The code used in the evaluation is the ORIGEN-based CAREPOOL system developed by KHNP. Decay heat calculation of PWR fuel is based on ANSI/ANS 5.1-2005, "Decay heat power in light water reactors" and ISO-10645, "Nuclear energy - Light water reactors - Calculation of the decay heat power in nuclear fuels. Also, we considered the contribution of fission products, actinide nuclides, neutron capture and radioactive material in decay heat calculation. CAREPOOL system calculates the individual and total decay heat of all of the spent fuel assemblies in SFP of Kori Unit-1. As a result, the total decay heat generated in SFP on June 28th, 2017 when the spent fuel assemblies were discharged from the reactor core, is estimated to be about 4,185.8 kw and to be about 609.5 kw on September 1st, 2018. It was also estimated that 119.6 kw is generated in 2050 when it is 32 years after the permanent shutdown. Figure 1 shows the trend of total decay heat in SFP of Kori Unit-1.

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Verification and validation of isotope inventory prediction for back-end cycle management using two-step method

  • Jang, Jaerim;Ebiwonjumi, Bamidele;Kim, Wonkyeong;Cherezov, Alexey;Park, Jinsu;Lee, Deokjung
    • Nuclear Engineering and Technology
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    • v.53 no.7
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    • pp.2104-2125
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    • 2021
  • This paper presents the verification and validation (V&V) of a calculation module for isotope inventory prediction to control the back-end cycle of spent nuclear fuel (SNF). The calculation method presented herein was implemented in a two-step code system of a lattice code STREAM and a nodal diffusion code RAST-K. STREAM generates a cross section and provides the number density information using branch/history depletion branch calculations, whereas RAST-K supplies the power history and three history indices (boron concentration, moderator temperature, and fuel temperature). As its primary feature, this method can directly consider three-dimensional core simulation conditions using history indices of the operating conditions. Therefore, this method reduces the computation time by avoiding a recalculation of the fuel depletion. The module for isotope inventory calculates the number densities using the Lagrange interpolation method and power history correction factors, which are applied to correct the effects of the decay and fission products generated at different power levels. To assess the reliability of the developed code system for back-end cycle analysis, validation study was performed with 58 measured samples of pressurized water reactor (PWR) SNF, and code-to-code comparison was conducted with STREAM-SNF, HELIOS-1.6 and SCALE 5.1. The V&V results presented that the developed code system can provide reasonable results with comparable confidence intervals. As a result, this paper successfully demonstrates that the isotope inventory prediction code system can be used for spent nuclear fuel analysis.

Log Count Rate Circuits for Checking Electronic Cards in Low Frequency Band Reactor Power Monitoring (저주파수대의 원자로 출력신호 점검을 위한 대수 카운트레이트 회로)

  • Kim, Jong-ho;Che, Gyu-shik
    • Journal of Advanced Navigation Technology
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    • v.24 no.6
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    • pp.557-565
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    • 2020
  • In order for thermal degradationIn, excore nuclear flux monitoring system, as a monitoring and signal processing methodology of reactor power, monitors neutron pulses generated during nuclear fission as frequency status, and converts them into DC voltage, and then log values resultantly. The methods realy applied in the nuclear power plant are to construct combination of counters and flip-flops, or diodes and capacitors up to now. These methodes are reliable for relative high frequencies, while not credible for reasonable low frequencies or extreme low values. Therefore, we developed the circuit that converts frequencies into DC voltages, into and into log DC values in the wide range from low Hz to several hundred high kHz. We proved their validities through testing them using real data used in nuclear power plant and analyzed their results. And, these methods will be used to measure the neutron level of excore nuclear flux monitoring system in nuclear power plant.

Sensitivity and uncertainty quantification of neutronic integral data in the TRIGA Mark II research reactor

  • Makhloul, M.;Boukhal, H.;Chakir, E.;El Bardouni, T.;Lahdour, M.;Kaddour, M.;Ahmed, Abdulaziz;Arectout, A.;El Yaakoubi, H.
    • Nuclear Engineering and Technology
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    • v.54 no.2
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    • pp.523-531
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    • 2022
  • In order to study the sensitivity and the uncertainty of the Moroccan research reactor TRIGA Mark II, a model of this reactor has been developed in our ERSN laboratory for use with the N-Particle MCNP Monte Carlo transport codes (version 6). In this article, the sensitivities of the effective multiplication factor of this reactor are evaluated using the ENDF/B-VII.0, ENDF/B-VII.1 and JENDL-4.0 libraries and in 44 energy groups, for the cross sections of the fuel (U-235 and U-238) and the moderator (H-1 and O-16). However, the quantification of the uncertainty of the nuclear data is performed using the nuclear code NJOY99 for the generation and processing of covariance matrices. On the one hand, the highest uncertainty deviations, calculated using the ENDFB-VII.1 and JENDL4.0 evaluations, are 2275, 386 and 330 pcm respectively for the reactions U235(n, f), $ U_{235}(n\bar{\nu})$ and H1(n, γ). On the other hand, these differences are very small for the neutron reactions of O-16 and U-238. Regarding the neutron spectra, in CT-mid plane, they are very close for the three evaluations (ENDF/B-VII.0, ENDF/B-VII.1 and JENDL-4.0). These spectra present two peaks (thermal and fission) around the energies 0.05 eV and 1 MeV.

Explore the possible advantages of using thorium-based fuel in a pressurized water reactor (PWR) Part 1: Neutronic analysis

  • Galahom, A. Abdelghafar;Mohsen, Mohamed Y.M.;Amrani, Naima
    • Nuclear Engineering and Technology
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    • v.54 no.1
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    • pp.1-10
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    • 2022
  • This study discusses the effect of using 232Th instead of 238U on the neutronic characteristics and the main operating parameters of the pressurized water reactor (PWR). MCNPX version 2.7 was used to compare the neutronic characteristics of UO2 with (Th, 235U)O2 and (Th, 233U) O2. Firstly, the infinity multiplication factor (Kinf), thermal neutron flux, and power distribution have been studied for the investigated fuel types. Secondly, the effect of Gd2O3 and Er2O3 on the Kinf and on the radial thermal neutron flux and thermal power has been investigated to distinguish which of them is more suitable than the other in reactivity management. Thirdly, to illustrate the effectiveness of 232Th in decreasing the inventory of both the actinides and non-actinides, the concentration of plutonium (Pu) isotopes and minor actinides (MAs) has been simulated with the fuel burnup. Besides, due to their large thermal neutron absorption cross-section, the concentrations of 135Xe, 149Sm, and 151Sm with the fuel burnup have been investigated. Finally, the main safety parameters such as the reactivity worth of the control rods (ρCR), the effective delayed neutron fraction βeff, and the Doppler reactivity coefficient (DRC) were calculated to determine to which extent these fuel types achieve the acceptable limits.

Theoretical simulation on evolution of suspended sodium combustion aerosols characteristics in a closed chamber

  • Narayanam, Sujatha Pavan;Kumar, Amit;Pujala, Usha;Subramanian, V.;Srinivas, C.V.;Venkatesan, R.;Athmalingam, S.;Venkatraman, B.
    • Nuclear Engineering and Technology
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    • v.54 no.6
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    • pp.2077-2083
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    • 2022
  • In the unlikely event of core disruptive accident in sodium cooled fast reactors, the reactor containment building would be bottled up with sodium and fission product aerosols. The behavior of these aerosols is crucial to estimate the in-containment source term as a part of nuclear reactor safety analysis. In this work, the evolution of sodium aerosol characteristics (mass concentration and size) is simulated using HAARM-S code. The code is based on the method of moments to solve the integro-differential equation. The code is updated to FORTRAN-77 and run in Microsoft FORTRAN PowerStation 4.0 (on Desktop). The sodium aerosol characteristics simulated by HAARM-S code are compared with the measured values at Aerosol Test Facility. The maximum deviation between measured and simulated mass concentrations is 30% at initial period (up to 60 min) and around 50% in the later period. In addition, the influence of humidity on aerosol size growth for two different aerosol mass concentrations is studied. The measured and simulated growth factors of aerosol size (ratio of saturated size to initial size) are found to be matched at reasonable extent. Since sodium is highly reactive with atmospheric constituents, the aerosol growth factor depends on the hygroscopic growth, chemical transformation and density variations besides coagulation. Further, there is a scope for the improvement of the code to estimate the aerosol dynamics in confined environment.

Validation of the neutron lead transport for fusion applications

  • Schulc, Martin;Kostal, Michal;Novak, Evzen;Czakoj, Tomas;Simon, Jan
    • Nuclear Engineering and Technology
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    • v.54 no.3
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    • pp.959-964
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    • 2022
  • Lead is an important material, both for fusion or fission reactors. The cross sections of natural lead should be validated because lead is a main component of lithium-lead modules suggested for fusion power plants and it directly affects the crucial variable, tritium breeding ratio. The presented study discusses a validation of the lead transport libraries by dint of the activation of carefully selected activation samples. The high emission standard 252Cf neutron source was used as a neutron source for the presented validation experiment. In the irradiation setup, the samples were placed behind 5 and 10 cm of the lead material. Samples were measured using a gamma spectrometry to infer the reaction rate and compared with MCNP6 calculations using ENDF/B-VIII.0 lead cross sections. The experiment used validated IRDFF-II dosimetric reactions to validate lead cross sections, namely 197Au(n, 2n)196Au, 58Ni(n,p)58Co, 93Nb(n, 2n)92mNb, 115In(n,n')115mIn, 115In(n,γ)116mIn, 197Au(n,γ)198Au and 63Cu(n,γ)64Cu reactions. The threshold reactions agree reasonably with calculations; however, the experimental data suggests a higher thermal neutron flux behind lead bricks. The paper also suggests 252Cf isotropic source as a valuable tool for validation of some cross-sections important for fusion applications, i.e. reactions on structural materials, e.g. Cu, Pb, etc.

Thermal-fluid-structure coupling analysis on plate-type fuel assembly under irradiation. Part-II Mechanical deformation and thermal-hydraulic characteristics

  • Li, Yuanming;Ren, Quan-yao;Yuan, Pan;Su, Guanghui;Yu, Hongxing;Zheng, Meiyin;Wang, Haoyu;Wu, Yingwei;Ding, Shurong
    • Nuclear Engineering and Technology
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    • v.53 no.5
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    • pp.1556-1568
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    • 2021
  • The plate-type fuel assembly adopted in nuclear research reactor suffers from complicated effect induced by non-uniform irradiation, which might affect stress conditions, mechanical behaviors and thermal-hydraulic performance of the fuel assembly. This paper is the Part II work of a two-part study devoted to analyzing the complex unique mechanical deformation and thermal-hydraulic characteristics for the typical plate-type fuel assembly under irradiation effect, which is on the basis of developed and verified numerical thermal-fluid-structure coupling methodology under irradiation in Part I of this work. The mechanical deformation, thermal-hydraulic performance and Mises stress have been analyzed for the typical plate-type fuel assembly consisting of support plates under non-uniform irradiation. It was interesting to observe that: the plate-type fuel assembly including the fuel plates and support plates tended to bend towards the location with maximum fission rate; the hot spots in the fuel foil appeared at the location with maximum thickness increment; the maximum Mises stress of fuel foil was located at the adjacent location with the maximum plate thickness increment et al.