• Atmosphere
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• v.19 no.3
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• pp.243-253
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• 2009

In other to interpret the long-term variations of sunshine duration, cloud lifetime, and precipitation intensity observed in and around Seoul and Busan for the period from 1986 to 2005, aerosol indirect effect was employed and applied. For the identification of long-term trend of aerosol concentration, observed visibility and AOT of AERONET sunphotometer data were also used over the same regions. The result showed that the time series of visibility was decreased and those of AOT increased, especially trends were remarkable in 2000s. In both regions, occurrence frequencies of observed cloudiness (cloud amount ${\leq}6/10$) and strong precipitation (rain rate > $0.5mmhour^{-1}$) have been steadily increased while those of cloudiness (cloud amount > 7/10) and weak precipitation (rain rate ${\leq}0.2mmhour^{-1}$) decreased. These results are corresponding to the trend of both visibility and AERONET data, implying the aerosol indirect effect that makes size of cloud droplet reduce, cloud life-time longer and precipitation efficiency decreased. Our findings demonstrate that, although these phenomena are not highly significant, weather and climate system over Korean urban area have been changed toward longer lifetime of small cloudiness and increasing precipitation intensity as a result of increased aerosol indirect effect.

• Journal of Korean Society for Atmospheric Environment
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• v.22 no.2
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• pp.235-247
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• 2006

Aerosol indirect radiative forcing of climate change is considered the most uncertain forcing of climate change over the industrial period, despite numerous studies demonstrating such modification of cloud properties and several studies quantifying resulting changes in shortwave radiative fluxes. Detection of this effect is made difficult by the large inherent variability in cloud liquid water path (LWP): the dominant controlling influence of LWP on optical depth and albedo masks any aerosol influences. Here we have used ground-based remote sensing of cloud optical depth (${\tau}_c$) by narrowband radiometry and LWP by microwave radiometry to determine the dependence of optical depth on LWP, thereby permitting examination of aerosol influence. The method is limited to complete overcast conditions with liquid-phase single layer clouds, as determined mainly by millimeter wave cloud radar. The results demonstrate substantial (factor of 2) day-to-day variation in cloud drop effective radius at the ARM Southern Great Plains site that is weakly associated with variation in aerosol loading as characterized by light-scattering coefficient at the surface. The substantial scatter suggests the importance of meteorological influences on cloud drop size as well, which should be analyzed in the further intensive studies. Meanwhile, it is notable that the decrease in cloud drop effective radius results in marked increase in cloud albedo.

• Journal of Environmental Science International
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• v.29 no.11
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• pp.1065-1078
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• 2020

The statistical characteristics of aerosol-cloud interactions over East Asia were investigated using Moderate Resolution Imaging Spectroradiometer satellite data. The long-term relationship between various aerosol and cloud parameters was estimated using correlation analysis, principle component analysis, and Aerosol Indirect Effect (AIE) estimation. In correlation analysis, Aerosol Optical Depth (AOD) was positively Correlated with Cloud Condensation Nuclei (CCN) and Cloud Fraction (CF), but negatively correlated with Cloud Top Temperature (CTT) and Cloud Top Pressure (CTP). Fine Mode Fraction (FMF) and CCN were positively correlated over the ocean because of sea spray. In principle component analysis, AOD and FMF were influenced by water vapor. In particular, AOD was positively influenced by CF, and negatively by CTT and CTP over the ocean. In AIE estimation, the AIE value in each cloud layer and type was mostly negative (Twomey effect) but sometimes positive (anti-Twomey effect). This is related to regional, environmental, seasonal, and meteorological effects. Rigorous and extensive studies on aerosol-cloud interactions over East Asia should be conducted via micro- and macro-scale investigations, to determine chemical characteristics using various meteorological instruments.

• Journal of Environmental Science International
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• v.17 no.6
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• pp.623-631
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• 2008

Many recent studies have concentrated upon the radiative effects of atmospheric aerosols. Though their scattering and absorption of radiation, aerosols can also induce some other important environment effects. In this study, new radiation code and aerosol data within Atmosphere General Circulation Model (AGCM) is used to assess the aerosol radiative forcing and to analyze relative climate effects. The new Kangnung National University AGCM Stratospheric-15 (KNU AGCM ST15) was integrated by using two sets of radiative effect of aerosols: CTRL as not a radiative effect of aerosols and AERO as a radiative effect of aerosols. Two cases show the difference of net shortwave radiation budget at top-of-atmosphere (TOA) is found to be about $-3.4Wm^{-2}$, at the surface (SFC) is about $-5.6Wm^{-2}$. Consequently the mean atmospheric absorption due to aerosol layer in global is about $2.2Wm^{-2}$. This result confirms the existence of a negative forcing due to the direct effect of aerosols at the surface and TOA in global annual mean. In addition, it is found that cooling over at the surface air temperature due to radiative effect of aerosols is about $0.17^{\circ}C$. It is estimated that radiative forcing of the net upward longwave radiation taken as the indirect effect of aerosol is much smaller than that of the direct effect as there is about $0.2Wm^{-2}$ of positive forcing both at TOA and at SFC. From this study, It made an accurate estimation of considering effect of aerosols that is negative effect. This may slow the rate of projected global warming during the $21^{st}$ century.

• Atmosphere
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• v.22 no.4
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• pp.437-447
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• 2012

There is still large uncertainty in estimating aerosol indirect effect despite ever-escalating efforts and virtually exponential increase in published studies concerning aerosol-cloud-precipitation interactions (CAPI). Probably most uncertainty comes from a wide range of observational scales and different platforms inappropriately used, and inherent complex chains of CAPI. Therefore, well-designed field campaigns and data analysis are required to address how to attribute aerosol signals along with clouds and precipitation to the microphysical effects of aerosols. Basically, aerosol influences cloud properties at the microphysical scales, "process scale", but observations are generally made of bulk properties over a various range of temporal and spatial resolutions, "analysis scale" (McComiskey & Feingold, 2012). In the most studies, measures made within the wide range of scales are erroneously treated as equivalent, probably resulting in a large uncertainty in associated with CAPI. Therefore, issues associated with the disparities of the observational resolution particular to CAPI are briefly discussed. In addition, the dependence of CAPI on the cloud environment such as stability and adiabaticity, and observation characteristics with varying situations of CAPI are also addressed together with observation framework optimally designed for the Korean situation. Properly designed and observation-based CAPI studies will likely continue to accumulate new evidences of CAPI, to further help understand its fundamental mechanism, and finally to develop improved parameterization for cloud-resolving models and large scale models.

• Particle and aerosol research
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• v.5 no.2
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• pp.45-52
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• 2009

Black carbon, which is a by-product of combustion of fossil fuel and biomass burning, is the component that imposes the largest uncertainty on quantifying aerosol climate effect. The direct, indirect and semi-direct climate effects of black carbon depend on its state of the mixing with other water-soluble aerosol components. The process that transforms hydrophobic externally mixed black carbon particles into hygroscopic internally mixed ones is called "aging". In most climate models, simple parameterizations for the aging time scale are used instead of solving detailed dynamics equations on the aging process due to the computation cost. In this study, a new parameterization for the black carbon aging time scale due to condensation and coagulation is presented as a function of the concentration of hygroscopic atmospheric components and the black carbon particle size. It is shown that the black carbon aging time scale due to condensation of sulfuric acid vapors varies to a large extent depending on the sulfuric acid concentration and the black carbon particle size. This result indicates that the constant aging time scale values suggested in the literature cannot be directly applied to a global scale modeling. The aging time scale due to coagulation with internally mixed aerosol particles shows an even stronger dependency on particle size, which implies that the use of a particle-size-independent aging time scale may lead to a large error when the aging is dominated by coagulation.

• Korean Journal of Remote Sensing
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• v.33 no.3
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• pp.301-311
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• 2017

Aerosol optical properties as well as vertical location of layer can alter the radiative balance of the Earth by reflecting and absorbing solar radiation. In this study, radiative transfer model (RTM) and satellite-based analysis have been used to quantify the top-of-atmosphere (TOA) radiative effect of aerosol layers in the cloudy atmosphere of the northeast Asia. RTM simulation results show that the atmospheric warming effect of aerosols increases with their height in the presence of underlying cloud layer. This relationship is higher for stronger absorbing aerosols and higher surface albedo condition. Over study region ($20-50^{\circ}N$, $110-140^{\circ}E$) and aerosol event cases, it is possible to qualitatively identify absorbing aerosol effects in the presence of clouds by combining the UV Absorbing Aerosol Index (AAI) derived from Total Ozone Mapping Spectrometer (TOMS), cloud parameters derived from the Moderate Resolution Imaging Spectro-radiometer (MODIS), with TOA Upward Shortwave Flux (USF) from the Clouds and the Earth's Radiant Energy System (CERES). As the regional-mean radiative effect of aerosols, 6 - 26 % lower the USF between aerosols and cloud cover is taken into account. These results demonstrate the importance of estimation for the accurate quantification of aerosol's direct and indirect effect.

• Journal of the Korean earth science society
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• v.44 no.6
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• pp.578-593
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• 2023

Intense convective activity and heavy precipitation inundated Seoul and its metropolitan area on July 15, 2017. This study investigated the synoptic-scale meteorological drivers of cold cloud genesis of this event. The WRF-Chem (Weather Research and Forecasting model coupled with Chemistry) model was employed to explore the intricate interplay between meteorological factors and the indirect effects of PM_2.5 aerosols originating from eastern China. The PM_2.5 aerosols' indirect effect was quantified by contrasting outcomes between the comprehensive Aerosol Radiation Interaction experiment (encompassing aerosol radiation feedback, cloud chemistry processes, and wet scavenging in the WRF-Chem model) and ACR (Aerosol Cloud Radiation interaction) experiment. The ACR experiment specifically excluded aerosol radiation feedback while incorporating only cloud chemistry processes and wet scavenging. Results indicated that in the early hours of July 15, 2017, a convergence of warm, moisture-laden airflow originating from southeast China and the East China Sea unfolded over the Yellow Sea. This convergence was driven by the juxtaposition of a low-pressure system over the Chinese mainland and Northwest Pacific high. Notably, at approximately 12 km altitude, the resultant convective clouds were characterized by the presence of ice crystals, a hallmark of continental-origin cold clouds. The WRF-Chem model simulations elucidated the role of PM_2.5 aerosols from eastern China, attributing 5.7, 10.4, and 10.8% to cloud water, ice crystal column, and liquid water column formation, respectively, within the developing cold clouds. Thus, this study presented a meteorological mechanism elucidating the formation of deep convective clouds over the Yellow Sea and the indirect effects of PM_2.5 aerosols originating from eastern China.

• Journal of the Korean Association of Geographic Information Studies
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• v.5 no.2
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• pp.1-15
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• 2002

Atmospheric aerosols interact with sunlight and affect the global radiation balance that can cause climate change through direct and indirect radiative forcing. Because of the spatial and temporal uncertainty of aerosols in atmosphere, aerosol characteristics are not considered through GCMs (General Circulation Model). Therefor it is important physical and optical characteristics should be evaluated to assess climate change and radiative effect by atmospheric aerosols. In this study GMS-5 satellite data and surface measurement data were analyzed using a radiative transfer model for the Yellow Sand event of April 7~8, 2000 in order to investigate the atmospheric radiative effects of Yellow Sand aerosols, MODTRAN3 simulation results enable to inform the relation between satellite channel albedo and aerosol optical thickness(AOT). From this relation AOT was retreived from GMS-5 visible channel. The variance observations of satellite images enable remote sensing of the Yellow Sand particles. Back trajectory analysis was performed to track the air mass from the Gobi desert passing through Korean peninsular with high AOT value measured by ground based measurement. The comparison GMS-5 AOT to ground measured RSR aerosol optical depth(AOD) show that for Yellow Sand aerosols, the albedo measured over ocean surfaces can be used to obtain the aerosol optical thickness using appropriate aerosol model within an error of about 10%. In addition, LIDAR network measurements and backward trajectory model showed characteristics and appearance of Yellow Sand during Yellow Sand events. These data will be good supporting for monitoring of Yellow Sand aerosols.

• Korean Journal of Remote Sensing
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• v.26 no.2
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• pp.65-73
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• 2010

To observe and analyze the characteristics of cloud and precipitation properties, the Cloud physics Observation System (CPOS) has been operated from December 2003 at Daegwallyeong ($37.4^{\circ}N$, $128.4^{\circ}E$, 842 m) in the Taebaek Mountains. The major instruments of CPOS are follows: Forward Scattering Spectrometer Probe (FSSP), Optical Particle Counter (OPC), Visibility Sensor (VS), PARSIVEL disdrometer, Microwave Radiometer (MWR), and Micro Rain Radar (MRR). The former four instruments (FSSP, OPC, visibility sensor, and PARSIVEL) are for the observation and analysis of characteristics of the ground cloud (fog) and precipitation, and the others are for the vertical cloud characteristics (http://weamod.metri.re.kr) in real time. For verification of CPOS products, the comparison between the instrumental products has been conducted: the qualitative size distributions of FSSP and OPC during the hygroscopic seeding experiments, the precipitable water vapors of MWR and radiosonde, and the rainfall rates of the PARSIVEL(or MRR) and rain gauge. Most of comparisons show a good agreement with the correlation coefficient more than 0.7. These reliable CPOS products will be useful for the cloud-related studies such as the cloud-aerosol indirect effect or cloud seeding. The visibility value is derived from the droplet size distribution of FSSP. The derived FSSP visibility shows the constant overestimation by 1.7 to 1.9 times compared with the values of two visibility sensors (SVS (Sentry Visibility Sensor) and PWD22 (Present Weather Detect 22)). We believe this bias is come from the limitation of the droplet size range ($2{\sim}47\;{\mu}m$) measured by FSSP. Further studies are needed after introducing new instruments with other ranges.