• Title/Summary/Keyword: Aerosol modeling

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A Modeling Study on Aerosol Property Changes due to Sea-Salts (해염성분에 의한 에어로솔 물성변화 모사연구)

  • 김용표
    • Journal of Korean Society for Atmospheric Environment
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    • v.16 no.2
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    • pp.113-120
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    • 2000
  • Effects of sea-salts on the properties of aerosol collected in a coastal region were studied by applying a gas-particle equilibrium model SCAPE to the measurement data from Korea Cheju Island in summer 1994. It was found that the observed higher ammonium concentrations in fine particles (PM2.5) than in TSP were caused by forced evaporation of ammonium in coarse fraction of aerosol by sea-salts and the degree of evaporation was quantified through an application of SCAPE. By subtracting the sea-salt fraction from the measured concentra-tions the changes of aerosol property were also studied. The concentrations of nitrate at both TSP and PM2.5 decreased when alkaline sea-salt fraction was removed from the measured data. Estimates of aerosol acidity increased for most samples with sea salt loadings, However in some cases with high mass fractions of sea-salt components the aerosol acidity of PM2.5 decreased slightly. This is though to be related with the formation of solid salt with the removal of sea-salts.

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A Derivation of Aerosol Optical Depth Estimates from Direct Normal Irradiance Measurements

  • Yun Gon Lee;Chang Ki Kim
    • New & Renewable Energy
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    • v.20 no.1
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    • pp.79-87
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    • 2024
  • This study introduces a method for estimating Aerosol Optical Depth (AOD) using Broadband Aerosol Optical Depth (BAOD) derived from direct normal irradiance and meteorological factors observed between 2016 and 2017. Through correlation analyses between BAOD and atmospheric components such as Rayleigh scattering, water vapor, and tropospheric nitrogen dioxide, significant relationships were identified, enabling accurate AOD estimation. The methodology demonstrated high correlation coefficients and low Root Mean Square Errors (RMSE) compared to actual AOD500 measurements, indicating that the attenuation effects of water vapor and the direct impact of tropospheric nitrogen dioxide concentration are crucial for precise aerosol optical depth estimation. The application of BAOD for estimating AOD500 across various time scales-hourly, daily, and monthly-showed the approach's robustness in understanding aerosol distributions and their optical properties, with a high coefficient of determination (0.96) for monthly average AOD500 estimates. This study simplifies the aerosol monitoring process and enhances the accuracy and reliability of AOD estimations, offering valuable insights into aerosol research and its implications for climate modeling and air quality assessment. The findings underscore the viability of using BAOD as a surrogate for direct AOD500 measurements, presenting a promising avenue for more accessible and accurate aerosol monitoring practices, crucial for improving our understanding of aerosol dynamics and their environmental impacts.

Aerosol Direct Radiative Forcing by Three Dimensional Observations from Passive- and Active- Satellite Sensors (수동형-능동형 위성센서 관측자료를 이용한 대기 에어러솔의 3차원 분포 및 복사강제 효과 산정)

  • Lee, Kwon-Ho
    • Journal of Korean Society for Atmospheric Environment
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    • v.28 no.2
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    • pp.159-171
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    • 2012
  • Aerosol direct radiative forcing (ADRF) retrieval method was developed by combining data from passive and active satellite sensors. Aerosol optical thickness (AOT) retrieved form the Moderate Resolution Imaging Spectroradiometer (MODIS) as a passive visible sensor and aerosol vertical profile from to the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) as an active laser sensor were investigated an application possibility. Especially, space-born Light Detection and Ranging (Lidar) observation provides a specific knowledge of the optical properties of atmospheric aerosols with spatial, temporal, vertical, and spectral resolutions. On the basis of extensive radiative transfer modeling, it is demonstrated that the use of the aerosol vertical profiles is sensitive to the estimation of ADRF. Throughout the investigation of relationship between aerosol height and ADRF, mean change rates of ADRF per increasing of 1 km aerosol height are smaller at surface than top-of-atmosphere (TOA). As a case study, satellite data for the Asian dust day of March 31, 2007 were used to estimate ADRF. Resulting ADRF values were compared with those retrieved independently from MODIS only data. The absolute difference values are 1.27% at surface level and 4.73% at top of atmosphere (TOA).

Effect of Aerosol Feedback on Solar Radiation in the Korean Peninsula Using WRF-CMAQ Two-way Coupled Model (WRF-CMAQ 결합모델을 이용한 에어로졸 피드백 효과가 한반도 일사량에 미치는 영향 연구)

  • Yoo, Jung-Woo;Park, Soon-Young;Jeon, WonBae;Kim, Dong-Hyeok;Lee, HwaWoon;Lee, Soon-Hwan;Kim, Hyun-Goo
    • Journal of Korean Society for Atmospheric Environment
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    • v.33 no.5
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    • pp.435-444
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    • 2017
  • In this study, we investigated the effect of aerosol feedback on $PM_{10}$ simulation using a two-way coupled air quality model (WRF-CMAQ). $PM_{10}$ concentration over Korea in January 2014 was simulated, and the aerosol feedback effect on the simulated solar radiation was intensively examined. Two $PM_{10}$ simulations were conducted using the WRF-CMAQ model with (FB) and without(NFB) the aerosol feedback option. We find that the simulated solar radiation in the west part of Korea decreased by up to $-80MJ/m^2$ due to the aerosol feedback effect. The feedback effect was significant in the west part of Korea, showing high $PM_{10}$ estimates due to dense emissions and its long-range transport from China. The aerosol feedback effect contributed to the decreased rRMSE(relative Root Mean Square Error) for solar radiation (47.58% to 30.75%). Aerosol feedback effect on the simulated solar radiation was mainly affected by concentration of $PM_{10}$. Moreover, FB better matched the observed solar radiation and $PM_{10}$ concentration than NFB, implying that taking into account the aerosol direct effects resulted in the improved modeling performance. These results indicate that aerosol feedback effects can play an important role in the simulation of solar radiation over Korean Peninsula.

Theoretical simulation on evolution of suspended sodium combustion aerosols characteristics in a closed chamber

  • Narayanam, Sujatha Pavan;Kumar, Amit;Pujala, Usha;Subramanian, V.;Srinivas, C.V.;Venkatesan, R.;Athmalingam, S.;Venkatraman, B.
    • Nuclear Engineering and Technology
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    • v.54 no.6
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    • pp.2077-2083
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    • 2022
  • In the unlikely event of core disruptive accident in sodium cooled fast reactors, the reactor containment building would be bottled up with sodium and fission product aerosols. The behavior of these aerosols is crucial to estimate the in-containment source term as a part of nuclear reactor safety analysis. In this work, the evolution of sodium aerosol characteristics (mass concentration and size) is simulated using HAARM-S code. The code is based on the method of moments to solve the integro-differential equation. The code is updated to FORTRAN-77 and run in Microsoft FORTRAN PowerStation 4.0 (on Desktop). The sodium aerosol characteristics simulated by HAARM-S code are compared with the measured values at Aerosol Test Facility. The maximum deviation between measured and simulated mass concentrations is 30% at initial period (up to 60 min) and around 50% in the later period. In addition, the influence of humidity on aerosol size growth for two different aerosol mass concentrations is studied. The measured and simulated growth factors of aerosol size (ratio of saturated size to initial size) are found to be matched at reasonable extent. Since sodium is highly reactive with atmospheric constituents, the aerosol growth factor depends on the hygroscopic growth, chemical transformation and density variations besides coagulation. Further, there is a scope for the improvement of the code to estimate the aerosol dynamics in confined environment.

Study of aerosol-cloud interaction phenomena from satellite remote sensing and climate modeling

  • Nakajima, Teruyuki;Higurashi, Akiko;Kawamoto, Kazuaki;Okamoto, Hajime;Takemura, Toshihiko;Kuroda, Shunsuke
    • Proceedings of the KSRS Conference
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    • 1999.11a
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    • pp.100-102
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    • 1999
  • We have analyzed AVHRR global data set for obtaining aerosol and cloud microphysical parameters, i. e., optical thickness and size index of particle polydispersions. From the results, it is found that the cloud optical thickness increases with increasing aerosol column number, which seems to be caused mainly by decreasing cloud particle radius, The cloud liquid water path was observed to be relatively constant without a significant dependence on the aerosol number. Further comparison of the satellite results with a general circulation model simulation.

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Aerosol Generation Mechanism for Cutting Fluid in Turning (선삭에서 절삭유 미립화 생성 메카니즘)

  • 박성호;고태조;김희술
    • Proceedings of the Korean Society of Machine Tool Engineers Conference
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    • 2001.10a
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    • pp.179-184
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    • 2001
  • The mechanism of the aerosol generation consists of spin-off, splash, and evaporation/condensation. Most researchers showed some theoretical model for predicting the particulate size and generation rate without cutting in turning operation. These models were based on the spin-off mechanism and verified good for modeling the process. However, in real machining, the cutting tool destructs the spin-off process, and the majority of the mist is due to splash. In this paper, we show some experimental evidence the aerosol generation mechanism should be explained with splash model as well as spin-off.

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Experimental Verification of Aerosol Generation Mechanism for Cutting Fluid in Turning (선삭에서 절삭유 미립화 생성 메카니즘의 실험적 검증)

  • 고태조;오명석;박성호;김희술
    • Journal of the Korean Society for Precision Engineering
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    • v.19 no.12
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    • pp.93-99
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    • 2002
  • The mechanism of the aerosol generation generally consists of spin-off, splash, and evaporation/condensation. Most researchers showed some theoretical model for predicting the particulate size and generation rate without real cutting in turning operation. These models were based on the spin-off mechanism, and verified good for modeling the process. However, in real machining, the cutting tool destroys the spin-off process, and the majority of the mist is due to splash. In this paper, we show some experimental evidence that the aerosol generation mechanism in real machining should be explained with splash model as well as spin-off.

Estimation of Aerosol Vertical Profile from the MODIS Aerosol Optical Thickness and Surface Visibility Data (MODIS 에어러솔 광학두께와 지상에서 관측된 시정거리를 이용한 대기 에어러솔 연직분포 산출)

  • Lee, Kwon-Ho
    • Journal of the Korean Association of Geographic Information Studies
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    • v.16 no.2
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    • pp.141-151
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    • 2013
  • This study presents a modeling of aerosol extinction vertical profiles in Korea by using the Moderate Resolution Imaging Spectro-radiometer(MODIS) derived aerosol optical thickness(AOT) and ground based visibility observation data. The method uses a series of physical equations for the derivation of aerosol scale height and vertical profiles from MODIS AOT and surface visibility data. The modelled results under the standard atmospheric condition showed small differences with the standard aerosol vertical profile used in the radiative transfer model. Model derived aerosol scale heights for two cases of clean(${\tau}_{MODIS}=0.12{\pm}0.07$, visibility=$21.13{\pm}3.31km$) and hazy atmosphere(${\tau}_{MODIS}=1.71{\pm}0.85$, visibility=$13.33{\pm}5.66km$) are $0.63{\pm}0.33km$ and $1.71{\pm}0.84km$. Based on these results, aerosol extinction profiles can be estimated and the results are transformed into the KML code for visualization of dataset. This has implications for atmospheric environmental monitoring and environmental policies for the future.

Estimations of the Optical Properties and Direct Radiative Forcing of Aerosol Chemical Components in PM2.5 Measured at Aewol Intensive Air Monitoring Site on Jeju Island (제주 애월 대기오염집중측정소의 PM2.5 에어로졸 화학성분 자료를 이용한 광학특성 및 직접적 복사강제력 추정 연구)

  • Park, Yeon-Hee;Song, Sang-Keun;Kang, Chang-Hee;Song, Jung-Min
    • Journal of Korean Society for Atmospheric Environment
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    • v.33 no.5
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    • pp.458-472
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    • 2017
  • The optical properties and direct aerosol radiative forcing (DARF) of different aerosol components in $PM_{2.5}$ (water-soluble, insoluble, black carbon (BC), and sea-salt) were estimated using the hourly resolution data measured at Aewol intensive air monitoring site on Jeju Island during 2013, based on a modeling approach. In general, the water-soluble component was predominant over all other components with respect to its impact on the optical properties(except for absorbing BC) and DARF. The annual mean aerosol optical depth (AOD) at 500 nm for the water-soluble component was $0.14{\pm}0.14$ ($0.04{\pm}0.01$ for BC). The total DARF at the surface ($DARF_{SFC}$) and top of the atmosphere ($DARF_{TOA}$), and in the atmosphere ($DARF_{ATM}$) for most aerosol components(except for sea-salt) during the daytime were highest in spring and lowest in fall and/or summer. The maximum $DARF_{SFC}$ of most aerosol components occurred around noon (12:00~14:00 LST) during all seasons, while the maximum $DARF_{TOA}$ occurred in the afternoon (13:00~16:00 LST) during most seasons (except for spring). In addition, the estimated $DARF_{SFC}$ and $DARF_{ATM}$ of the water-soluble component were -20 to $-59W/m^2$ and +3.5 to $+14W/m^2$, respectively, while those of BC were -18 to $-29W/m^2$ and +23 to $+37W/m^2$, respectively.