• 제목/요약/키워드: nuclear reactions

검색결과 275건 처리시간 0.024초

Monte Carlo Analysis of the Accelerator-Driven System at Kyoto University Research Reactor Institute

  • Kim, Wonkyeong;Lee, Hyun Chul;Pyeon, Cheol Ho;Shin, Ho Cheol;Lee, Deokjung
    • Nuclear Engineering and Technology
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    • 제48권2호
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    • pp.304-317
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    • 2016
  • An accelerator-driven system consists of a subcritical reactor and a controllable external neutron source. The reactor in an accelerator-driven system can sustain fission reactions in a subcritical state using an external neutron source, which is an intrinsic safety feature of the system. The system can provide efficient transmutations of nuclear wastes such as minor actinides and long-lived fission products and generate electricity. Recently at Kyoto University Research Reactor Institute (KURRI; Kyoto, Japan), a series of reactor physics experiments was conducted with the Kyoto University Critical Assembly and a Cockcrofte-Walton type accelerator, which generates the external neutron source by deuteriu-metritium reactions. In this paper, neutronic analyses of a series of experiments have been re-estimated by using the latest Monte Carlo code and nuclear data libraries. This feasibility study is presented through the comparison of Monte Carlo simulation results with measurements.

Study on (n,p) reactions of 58,60,61,62,64Ni using new developed empirical formulas

  • Yigit, Mustafa
    • Nuclear Engineering and Technology
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    • 제52권4호
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    • pp.791-796
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    • 2020
  • Nuclear fusion seems to be a good choice of energy source in the future. Nickel is one of the crucial structural materials for fusion devices. In this work, the cross section data of 58Ni(n,p)58Co, 60Ni(n,p)60Co, 61Ni(n,p)61Co, 62Ni(n,p)62Co and 64Ni(n,p)64Co reactions were calculated using the nuclear codes ALICE/ASH, EMPIRE 3.2 and TALYS 1.8. In addition, the cross sections were calculated with the empirical formulas obtained in our previous paper at 14-15 MeV. The obtained results were compared with the measured values in the literature, and with the evaluated data files (JEFF-3.3, TENDL-2017, ENDF/B-VIII.0).

A new gas-solid reaction model for voloxidation process with spallation

  • Ryu, Je Ir;Woo, Seung Min
    • Nuclear Engineering and Technology
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    • 제50권1호
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    • pp.145-150
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    • 2018
  • A new methodology, the crack-spallation model, has been developed to analyze gas-solid reactions dominated by crack growth inside of the solid reactant and spallation phenomena. The new model physically represents three processes of the reaction progress: (1) diffusion of gas reactant through pores; (2) growth of product particle in pores; and (3) crack and spallation of solid reactant. The validation of this method has been conducted by comparison of results obtained in an experiment for oxidation of $UO_2$ and the shrinking core model. The reaction progress evaluated by the crack-spallation model shows better agreement with the experimental data than that evaluated by the shrinking core model. To understand the trigger point during the reaction progress, a detailed analysis has been conducted. A parametric study also has been performed to determine mass diffusivities of the gas reactant and volume increase constants of the product particles. This method can be appropriately applied to the gas-solid reaction based on the crack and spallation phenomena such as the voloxidation process.

Kinetic Studies on the Halide Exchange Reactions of Some Substituted Benzyl Chlorides

  • Lee, Ikchoon;Lee, Bon-Su;Yie, Jae-Eui
    • Nuclear Engineering and Technology
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    • 제3권4호
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    • pp.198-202
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    • 1971
  • 방사성동위원소로 표지된 할라이드 이온과 염화벤질간의 할로겐 교환반응을 아세톤 용액에서 반응속도론적으로 연구하였다. 결과로 전보에서 얻은 결론대로 교환반응속도가 기질과 할라이드 이온의 편극화율에 의하여 좌우됨을 알았다.

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양성자 에너지 변화에 따른 핵반응 생성핵종 분석 (Analysis of Proton Nuclear Reaction-Generated Nuclides for Different Proton Energy)

  • 이삼열
    • 한국방사선학회논문지
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    • 제13권5호
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    • pp.819-824
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    • 2019
  • 본 연구에서 서로 다른 양성자 에너지를 사용하여 핵반응에 의해 생성된 감마선의 차이를 통해 고에너지 양성자 Pb(p, nx) 핵반응에서 생성된 동위원소를 식별하는 방법을 제안했다. 한국원자력연구원의 100-M eV 양성자 선형 가속기에서 생성된 고 에너지 양성자를 이용하여 실험을 수행 하였다. 양성자 핵반응을 통해 생성된 다양한 핵종에 의해 생성된 감마선은 HPGe 검출기로 구성된 감마선 분광법 시스템을 사용하여 측정되었습니다. 감마선 표준선원은 감마선 검출기의 정확한 에너지교정 및 효율측정을 위해 사용되었습니다. 제안한 방법을 위하여 동일한 천연 납 시료에 서로 다른 100 및 60 MeV 양성자 에너지빔을 사용하였다. 이 방법은 동일한 시료에서 발생되는 감마선들을 서로 비교함으로써 생성된 핵종들을 확인하는데 매우 효과적임을 알 수 있었다. 이 연구의 결과는 향후 다른 양성자 핵반응 결과를 얻는데도 매우 효과적으로 적용될 것이라 생각된다.

RAIM - A MODEL FOR IODINE BEHAVIOR IN CONTAINMENT UNDER SEVERE ACCIDENT CONDITION

  • KIM, HAN-CHUL;CHO, YEONG-HUN
    • Nuclear Engineering and Technology
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    • 제47권7호
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    • pp.827-837
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    • 2015
  • Following a severe accident in a nuclear power plant, iodine is a major contributor to the potential health risks for the public. Because the amount of iodine released largely depends on its volatility, iodine's behavior in containment has been extensively studied in international programs such as International Source Term Programme-Experimental Program on Iodine Chemistry under Radiation (EPICUR), Organization for Economic Co-operation and Development (OECD)-Behaviour of Iodine Project, and OECD-Source Term Evaluation and Mitigation. Korea Institute of Nuclear Safety (KINS) has joined these programs and is developing a simplified, stand-alone iodine chemistry model, RAIM (Radio-Active Iodine chemistry Model), based on the IMOD methodology and other previous studies. This model deals with chemical reactions associated with the formation and destruction of iodine species and surface reactions in the containment atmosphere and the sump in a simple manner. RAIM was applied to a simulation of four EPICUR tests and one Radioiodine Test Facility test, which were carried out in aqueous or gaseous phases. After analysis, the results show a trend of underestimation of organic and molecular iodine for the gas-phase experiments, the opposite of that for the aqueous-phase ones, whereas the total amount of volatile iodine species agrees well between the experiment and the analysis result.

Model-based predictions for nuclear excitation functions of neutron-induced reactions on 64,66-68Zn targets

  • Yigit, M.;Kara, A.
    • Nuclear Engineering and Technology
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    • 제49권5호
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    • pp.996-1005
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    • 2017
  • In this paper, nuclear data for cross sections of the $^{64}Zn(n,2n)^{63}Zn$, $^{64}Zn(n,3n)^{62}Zn$, $^{64}Zn(n,p)^{64}Cu$, $^{66}Zn(n,2n)^{65}Zn$, $^{66}Zn(n,p)^{66}Cu$, $^{67}Zn(n,p)^{67}Cu$, $^{68}Zn(n,p)^{68}Cu$, and $^{68}Zn(n,{\alpha})^{65}Ni$ reactions were studied for neutron energies up to 40 MeV. In the nuclear model calculations, TALYS 1.6, ALICE/ASH, and EMPIRE 3.2 codes were used. Furthermore, the nuclear data for the (n,2n) and (n,p) reaction channels were also calculated using various cross-section systematics at energies around 14-15 MeV. The code calculations were analyzed and obtained using the different level densities in the exciton model and the geometry-dependent hybrid model. The results obtained from the excitation function calculations are discussed and compared with literature experimental data, ENDF/B-VII.1, and the TENDL-2015 evaluated data.

Study on (n, α) reactions for the production of 51Cr, 89Sr, 99Tc, 131I, 133Xe, 137Cs and 153Sm radioisotopes used in nuclear medicine

  • Hallo M. Abdullah;Ali H. Ahmed
    • Nuclear Engineering and Technology
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    • 제55권9호
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    • pp.3352-3358
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    • 2023
  • Nuclear medicine seems to be a decent choice of medicine in the recent decade. The radioactive isotopes 51Cr, 89Sr, 99Tc, 131I, 133Xe, 137Cs and 153Sm are extremely essential in nuclear medicine. The excitation functions of the 54Fe (n, α) 51Cr, 92Zr (n, α) 89Sr, 102Rh (n, α) 99Tc, 134Cs (n, α) 131I, 136Ba (n, α) 133Xe, 140La (n, α) 137Cs and 156Gd (n, α) 153Sm reactions were calculated in this study using the EMPIRE 3.2.3 and TALYS 1.95 nuclear codes. Additionally, the cross sections at 14-15 MeV were calculated using empirical formulae and the experimental data. The computer codes were compared to the experimental data and Empirical formulas as well as the evaluated data (TENDL 2021, JENDL 3.3, JENDL 5, JEFF 3.3, EAF 2010, CENDL 3.1, CENDL 3.2, ROSFOND 2010, FENDL 3.2 b, and BROND 3.1).