• Title/Summary/Keyword: UO$_2$pellet

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초음파 공진 분석법을 이용한 건식공정 핵연료 소결체의 탄성계수 측정 (Elastic Modulus Measurement of a Dry Process Fuel Pellet by Resonant Ultrasound Spectroscopy)

  • 류호진;강권호;문제선;송기찬;정현규;정용무
    • 한국분말재료학회지
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    • 제11권4호
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    • pp.314-321
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    • 2004
  • The elastic moduli of simulated dry process fuels with varying composition and density were measured in order to analyze the mechanical properties of a dry process fuel pellet. Resonant ultrasound spectroscopy(RUS) which can determine all elastic moduli with one set of measurements for a rectangular parallelepiped sample was used to measure the elastic moduli of UO$_{2}$ and simulated dry process fuel. The simulated dry process fuel showed a higher value of Young's modulus than UO$_2$ due to the presence of metallic precipitates and solid solution elements in the UO$_{2}$ matrix. The correlation between Young's modulus and porosity(P) of simulated dry process fuel was found to be 231.4-651.8 P (GPa) at room temperature. Dry process fuel with a higher burnup showed higher Young's modulus because total content of fission product element was increased.

Investigation of nuclear material using a compact modified uniformly redundant array gamma camera

  • Lee, Taewoong;Kwak, Sung-Woo;Lee, Wonho
    • Nuclear Engineering and Technology
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    • 제50권6호
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    • pp.923-928
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    • 2018
  • We developed a compact gamma camera based on a modified uniformly redundant array coded aperture to investigate the position of a $UO_2$ pellet emitting characteristic X-rays (98.4 keV) and ${\gamma}-rays$ (185.7 keV). Experiments using an only-mask method and an antimask subtractive method were conducted, and the maximum-likelihood expectation maximization algorithm was used for image reconstruction. The images obtained via the antimask subtractive method were compared with those obtained using the only-mask method with regard to the signal-to-noise ratio. The reconstructed images of the antimask subtractive method were superior. The reconstructed images of the characteristic X-rays and the ${\gamma}-rays$ were combined with the obtained image using the optical camera. The combined images showed the precise position of the $UO_2$ pellet. According to the self-absorption ratios of the nuclear material and the minimum number of effective events for image reconstruction, we estimated the minimum detection time depending on the amount of nuclear material.

노내 손상 핵연료의 산화거동 및 핵연료 산화가 핵분열기체 방출에 미치는 효과 (Oxidation Kinetics of $UO_2$ Pellets in Defective Fuel Rods and Its Effect on Fission Gas Release)

  • Koo, Yang-Hyun;Sohn, Dong-Seong;Yoon, Young-Ku
    • Nuclear Engineering and Technology
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    • 제26권1호
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    • pp.90-99
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    • 1994
  • 손상 핵연료에서 발생하는 주요한 현상중의 하나는 수중기의 분해로 갭에 존재하는 산소에 의해 $UO_2$$UO_{2+}$x/로 산화되고, 이로 인해 결정립내에서의 핵분열기체 확산계수가 증가하여 결과적으로 핵분열 기체의 방출이 증대하는 현상이다. 본 논문은 일반적인 원자로 운전 조건하에서 원자로 및 손상 핵연료의 운전조건을 고려하여 소결체의 산화거동을 모사하고 이를 바탕으로 소결체 산화가 핵분열기체의 방출 중대에 미치는 영향을 분석하였다. 소결체 산화거동은 갭에는 150기압의 포화된 순수한 수증기만이 존재한다는 가정하에 분석하였고, 산화에 의한 핵분열기체의 방출 증대 효과를 정량적으로 분석하기 위해 방출중대 인자를 도입하였다. 실험 치와 비교한 결과 방출증대 인자는 소결체 산화에 의한 핵분열기체의 방출증대 효과를 잘 예측하였다.

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Effect of a Li2O Additive on the Sintering Behavior of UO2 in the H2 and CO2 Atmospheres

  • Kim, Si-Hyung;Joung, Chang-Young;Kim, Yeon-Gu;Lee, Soo-Chul;Kim, Ban-Soo;Na, Sang-Ho;Lee, Young-Woo;Suhr, Dong-Soo
    • 한국세라믹학회지
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    • 제41권8호
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    • pp.567-572
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    • 2004
  • The variation of the sintered density and grain size of UO$_2$ as a function of the Li$_2$O amount and sintering atmosphere was observed. Li$_2$O enhanced the grain growth of the UO$_2$ pellet in H$_2$, but rather hindered it in $CO_2$ atmosphere. Grain size of the UO$_2$ and UO$_2$-0.1 wt%Li$_2$O pellets was, respectively, 8 $\mu$m and 100 $\mu$m at 168$0^{\circ}C$ in the H$_2$ atmosphere, and that of each pellet was, respectively, 24 $\mu$m and 17 $\mu$m at the same temperature in the $CO_2$ atmosphere. As-received Li$_2$O powder, which had been composed of Li$_2$O and LiOH, was converted to the Li$_2$CO$_3$ phase after heating to 80$0^{\circ}C$ in $CO_2$. On the other hand, the Li$_2$O and LiOH phases remained unchanged in H$_2$ atmosphere. In the H$_2$, the as-received Li$_2$O powder began to evaporate at about 105$0^{\circ}C$ and then about 20 wt% residue was left at 150$0^{\circ}C$. But, most of the Li elements evaporated at 150$0^{\circ}C$ in the $CO_2$ atmosphere.

HIGH BURNUP FUEL TECHNOLOGY IN KOREA

  • Song, Kun-Woo;Jeong, Yong-Hwan;Kim, Keon-Sik;Bang, Je-Geon;Chun, Tae-Hyun;Kim, Hyung-Kyu;Song, Kee-Nam
    • Nuclear Engineering and Technology
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    • 제40권1호
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    • pp.21-36
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    • 2008
  • High bum-up fuel technology has been developed through a national R&D program, which covers key technology areas such as claddings, $UO_2$ pellets, spacer grids, performance code, and fuel assembly tests. New cladding alloys were developed through alloy designs, tube fabrication, out-of-pile test and in-reactor test. The new Zr-Nb tubes are found to be much better in their corrosion resistance and creep strength than the Zircaloy-4 tube, owing to an optimized composition and heat treatment of the new Zr-Nb alloys. A new fabrication technology for large grain $UO_2$ pellets was developed using various uranium oxide seeds and a micro-doping of Al. The uranium oxide seeds, which were added to $UO_2$ powder, were prepared by oxidizing and heat-treating scrap $UO_2$ pellets. A $UO_2$ pellet containing tungsten channels was fabricated for a thermal conductivity enhancement. For the fuel performance analysis, new high burnup models were developed and implemented in a code. This code was verified by an international database and our own database. The developed spacer grid has two features of contoured contact spring and hybrid mixing vanes. Mechanical and hydraulic tests showed that the spacer grid is superior in its rodsupporting, wear resistance and CHF performance. Finally, fuel assembly test technology was also developed. Facilities for mechanical and thermal hydraulic tests were constructed and are now in operation. Several achievements are to be utilized soon by the Korea Nuclear Fuel and thereby contribute to the economy and safety of PWR fuel in Korea

Oxidation Behavior of Unirradiated and Irradiated $UO_2$ in hir at $150-375^\circ{C}$

  • Kim, Keon-Sik;You, Gil-Sung;Min, Duck-Kee;Ro, Seung-Gy;Kim, Eun-Ka
    • Nuclear Engineering and Technology
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    • 제29권2호
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    • pp.93-98
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    • 1997
  • Air-oxidation experiments on unirradiated and irradiated UO$_2$ were performed at temperature from 150 to 375$^{\circ}C$ for investigating the long-term storage behavior of spent PWR fuel. The rate of oxidation was monitored by a thermogravimetric analyzer(TGA) and an X-ray diffraction(XRD). The correlation between the onset-time for U$_3$O$_{8}$ formation and temperature was given as follows, logt(hr) = -12.89+7650/T(K), 423$_2$ pellet, the oxidation rate of irradiated UO$_2$ increase more rapidly at the initial stage and shows a lower saturation point at the later Stage. The Oxidation rate of high bumup UO$_2$ and gadolinia-doped UO$_2$(Gd$_2$O$_3$-UO$_2$) were observed to be much slower than that of unirradiated UO$_2$ pellets.s.

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UO2 및 (U1-yCey)O2 소결체의 열팽창 측정 및 평가 (The Linear Thermal Expansion Measurements and Estimations for UO2 and (U1-yCey)O2 Pellet)

  • 김동주;김용수;이영우
    • 한국세라믹학회지
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    • 제42권5호
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    • pp.346-351
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    • 2005
  • The linear thermal expansions of $UO_2$ and $(U_{1-y}Ce_y)O_2$ pellet were measured from room temperature to $1400^{\circ}C$ as a function of Ce contents (0, 7.63, 14.84, and $21.68 mol\%$) by using the TMA(Thermo-Mechanical Analysis) method. From the measured data, the linear thermal expansion rate, the coefficient of linear thermal expansion and density variation with temperature were calculated, and the best-fitted temperature-dependent equations were recommended. It was shown that the rate and coefficient of $(U_{1-y}Ce_y)O_2$ thermal expansion increased and the density decreased with increasing Ce contents.

EFFECT OF $SiO_2-CaO-Cr_2O_3$ ON THE CREEP PROPERTY OF URANIUM DIOXIDE

  • RHEE YOUNG WOO;KANG KI WON;KIM KEON SIK;YANG JAE HO;KIM JONG HEON;SONG KUN WOO
    • Nuclear Engineering and Technology
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    • 제37권3호
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    • pp.287-292
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    • 2005
  • [ $\pi$ ]The effects of silica-based additives have been investigated to improve the creep property of a $UO_2$ pellet. The additive composition, $50wt\%SiO_2-47wt{\%}CaO-3wt\%Cr_2O_3$ (SCC), was selected according to the dihedral angle and the distribution of the second phase. It was observed that the creep rate of the $0.07 wt\%$ SCC-added $UO_2$ was slower than that of the pure $UO_2$. However, the creep rate of the $0.22 wt\%$ SCC-added $UO_2$ was about 3_48 times faster than that of the pure $UO_2$, depending on the applied stress in the lower stress range. In the case of the $0.35 wt\%$ SCC-added $UO_2$, the creep rate decreased in comparison with that of the $0.22 wt\%$ SCC-added $UO_2$. The observed enhancement in the creep rate might depend on a balance between the positive role of the viscous intergranular phase and the negative roles of the additives and the grain growth.