• Title/Summary/Keyword: Nuclear material detection

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A rapid and direct method for half value layer calculations for nuclear safety studies using MCNPX Monte Carlo code

  • Tekin, H.O.;ALMisned, Ghada;Issa, Shams A.M.;Zakaly, Hesham M.H.
    • Nuclear Engineering and Technology
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    • v.54 no.9
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    • pp.3317-3323
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    • 2022
  • Half Value Layer calculations theoretically need prior specification of linear attenuation calculations, since the HVL value is derived by dividing ln(2) by the linear attenuation coefficient. The purpose of this study was to establish a direct computational model for determining HVL, a vital parameter in nuclear radiation safety studies and shielding material design. Accordingly, a typical gamma-ray transmission setup has been modeled using MCNPX (version 2.4.0) general-purpose Monte Carlo code. The MCNPX code's INPUT file was designed with two detection locations for primary and secondary gamma-rays, as well as attenuator material between those detectors. Next, Half Value Layer values of some well-known gamma-ray shielding materials such as lead and ordinary concrete have been calculated throughout a broad gamma-ray energy range. The outcomes were then compared to data from the National Institute of Standards and Technology. The Half Value Layer values obtained from MCNPX were reported to be highly compatible with the HVL values obtained from the NIST standard database. Our results indicate that the developed INPUT file may be utilized for direct computations of Half Value Layer values for nuclear safety assessments as well as medical radiation applications. In conclusion, advanced simulation methods such as the Monte Carlo code are very powerful and useful instruments that should be considered for daily radiation safety measures. The modeled MCNPX input file will be provided to the scientific community upon reasonable request.

Assessment of Environmental Radioactivity Surveillance Results around Korean Nuclear Power Utilization Facilities in 2017

  • Kim, Cheol-Su;Lee, Sang-Kuk;Lee, Dong-Myung;Choi, Seok-Won
    • Journal of Radiation Protection and Research
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    • v.44 no.3
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    • pp.118-126
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    • 2019
  • Background: Government conducts environmental radioactivity surveillance for verification purpose around nuclear facilities based on the Nuclear Safety Law and issues a surveillance report every year. This study aims to evaluate the short and the long-term fluctuation of radionuclides detected above MDC and their origins using concentration ratios between these radionuclides. Materials and Methods: Sample media for verification surveillance are air, rainwater, groundwater, soil, and milk for terrestrial samples, and seawater, marine sediment, fish, and seaweed for marine samples. Gamma-emitting radionuclides including $^{137}Cs$, $^{90}Sr$, Pu, $^3H$, and $^{14}C$ are evaluated in these samples. Results and Discussion: According to the result of the environmental radioactivity verification surveillance in the vicinity of nuclear power facilities in 2017, the anthropogenic radionuclides were not detected in most of the environmental samples except for the detection of a trace level of $^{137}Cs$, $^{90}Sr$, Pu, and $^{131}I$ in some samples. Radioactivity concentration ratios between the anthropogenic radionuclides ($^{137}Cs/^{90}Sr$, $^{137}Cs/^{239+240}Pu$, $^{90}Sr/^{239+240}Pu$) were similar to those reported in the environmental samples, which were affected by the global fallout of the past nuclear weapon test, and Pu atomic ratios ($^{240}Pu/^{239}Pu$) in the terrestrial sample and marine sample showed significant differences due to the different input pathway and the Pu source. Radioactive iodine ($^{131}I$) was detected at the range of < $5.6-190mBq{\cdot}kg-fresh^{-1}$ in the gulfweed and sea trumpet collected from the area of Kori and Wolsong intake and discharge. A high level of $^3H$ was observed in the air (Sangbong: $0.688{\pm}0.841Bq{\cdot}m^{-3}$) and the precipitation (Meteorology Post: $199{\pm}126Bq{\cdot}L^{-1}$) samples of the Wolsong nuclear power plant (NPP). $^3H$ concentration in the precipitation and pine needle samples showed typical variation pattern with the distance and the wind direction from the stack due to the gaseous release of $^3H$ in Wolsong NPP. Conclusion: Except for the detection of a trace level of $^{137}Cs$, $^{90}Sr$, Pu, and $^{131}I$ in some samples, anthropogenic radionuclides were below MDC in most of the environmental samples. Overall, no unusual radionuclides and abnormal concentration were detected in the 2017's surveillance result for verification. This research will be available in the assessment of environment around nuclear facilities in the event of radioactive material release.

Determination of the Uranium Backgrounds in Lexan Films for Single Particle Analysis using FT-TIMS technique

  • Park, Su-Jin;Park, Jong-Ho;Lee, Myung-Ho;Song, Kyu-Seok
    • Mass Spectrometry Letters
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    • v.2 no.2
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    • pp.57-60
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    • 2011
  • As background significantly affects measurement accuracy and a detection limit in determination of the trace amounts of uranium, it is necessary to determine the impurities in the Lexan detector film for single particle measurements by thermal ionization mass spectrometry coupled with fission track technique (FT-TIMS). We have prepared various micro sizes of the blank Lexan detector film using a micromanipulation technique for uranium measurements by TIMS. Few tens of fg of uranium background with no remarkable dependency on the film sizes were observed in the blank Lexan films with the sizes from $50{\times}50\;{\mu}m^2$ to $300{\times}300\;{\mu}m^2$. Based on the determination of the uranium background in the Lexan film, any background correction is necessary in the isotopic analysis of a uranium single particle with micron sizes when the particle bearing Lexan film is dissected with less than $300{\times}300\;{\mu}m^2$ size. The isotopic analysis of a uranium particle in U030 standard material using TIMS was carried out to verify the applicability of the Lexan film to the single particle analysis with high accuracy and precision.

Multigrid Wavelet-Based Natural Pixel Method for Image Reconstruction in Emission Computed Tomography

  • Chang je park;Park, Jeong hwan;Cho, Nam-Zin
    • Proceedings of the Korean Nuclear Society Conference
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    • 1998.05b
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    • pp.705-710
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    • 1998
  • We describe a multigrid wavelet-based natural pixel (WNP) method for image reconstruction in emission computed tomography (ECT). The ECT is used to identify the tagged radioactive material's position in the body for detection of abnormal tissue such as tumor or cancer, as in SPECT and PET. With ECT methodology in parallel beam mode, we formulate a matrix-based reconstruction method for radionuclide sources in the human body. The resulting matrix for a practical problem is very large and nearly singular. To overcome this ill-conditioning, wavelet transform is considered in this study. Wavelets have inherent de-noising and multiscale resolution properties. Therefore, the multigrid wavelet-based natural pixel (WNP) method is very efficient to reconstruct image from projection data that is noisy and incomplete. We test this multigrid wavelet natural pixel (WNP) reconstruction method with the MCNP generated projection data for diagnosis of the simulated cancerous tumor.

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Complete Simultaneous Analysis of Uranium Isotopes in NUSIMEP-7 Microparticles Using SEM-TIMS

  • Park, Jong-Ho;Jeong, Kahee
    • Mass Spectrometry Letters
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    • v.7 no.3
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    • pp.64-68
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    • 2016
  • Scanning electron microscopy combined with thermal ionization mass spectrometry (SEM-TIMS) was used to determine the precise isotope ratios of ultra-trace levels of uranium contained in individual microparticles. An advanced multiple ion counter system consisting of three secondary ion multipliers and two compact discrete dynodes was used for complete simultaneous ion detection. For verification purposes, using TIMS with complete simultaneous measurement, isotopes were analyzed in 5 pg of uranium of a certified reference material. A microprobe in the SEM was used to transfer individual particles from a NUSIMEP-7 sample to TIMS filaments, which were then subjected to SEM-TIMS and complete simultaneous measurement. The excellent agreement in the resulting uranium isotope ratios with the certified NUSIMEP-7 values shows the validity of SEM-TIMS with complete simultaneous measurement for the analysis of uranium isotopes in individual particles. Further experimental study required for investigation of simultaneous measurement using the advanced multiple ion counter system is presented.

Isolation of Listeria monocytogenes by Immunomagnetic Separation and Atomic Force Microscopy

  • Mercanolu, Birce;Aykut, S.;Ergun, M.Ali;Tan, Erdal
    • Journal of Microbiology
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    • v.41 no.2
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    • pp.144-147
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    • 2003
  • Listeria monocytogenes is a pathogen of major concern to the food industry and the potential cause of severe infections such as listeriosis. Early detection of this foodborne pathogen is important in order to eliminate its potential hazards. So, immunomagnetic separation (IMS) has been suggested as a means of reducing the total analysis time and for improving the sensitivity of detection. Atomic force microscopy (AFM) has been used for measuring the topographic properties of sample surfaces at nanometer scale. In this study, we used AFM to confirm both the sensitivity and the specificity of IMS. Regarding AFM analysis, the length and the width of the bacteria, which were in agreement with literature values, were found to be 2.993 $\mu\textrm{m}$ and 0.837 $\mu\textrm{m}$, respectively. As a result, AFM helped us both characterize and measure the bacterial and bead structures.

Laboratory Tests of Chromium-51 Complexes for teak Detection in Pipes Carrying A Liquid Flow

  • Kim, You-Sun;Lee, Byung-Hyun
    • Nuclear Engineering and Technology
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    • v.6 no.4
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    • pp.231-237
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    • 1974
  • For detection and localization of leaks in closed vessels or pipes carrying liquid flow, $^{51}$ Cr-EDTA and $^{51}$ Cr-DTPA were synthesized and, the column and batch equilibrium experiments were carried out. In the column experiment, the recovery of $^{51}$ Cr-EDTA is 100% in quartz sand and 80.9% in steel sawdust, and that of $^{51}$ Cr-DTPA is 77.4% in quartz sand and 6.4% in steel sawdust. The recovery curve. $^{51}$ Cr-DTPA system in steel sawdust does not show a certain plateau, exceptionally. In general, $^{51}$ Cr-EDTA is adsorbed less than $^{51}$ Cr-DTPA. In the batch equilibrium experiment, the distribution coefficients (Kd) and effect of pH were investigated by using quartz sand, montmorillonite, steel sawdust, and mixed cement raw material as media. In general, the Kd values for $^{51}$ Cr-EDTA are lower than that of $^{51}$ Cr-DTPA. The Kd values for $^{51}$ Cr-EDTA are almost zero at pH 6.0, 7.0, and 8.0.

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Development of Ceramic Humidity Sensor for the Korean Next Generation Reactor

  • Lee, Na-Young;Hwang, Il-Soon;Song, Chang-Rock;Yoo, Han-Ill;Park, Sang-Duk;Yang, Jun-Seong
    • Nuclear Engineering and Technology
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    • v.30 no.5
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    • pp.435-443
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    • 1998
  • Leak-before-break(LBB) approach has been shown to be both cost effective and risk reductive when applied to high energy Piping in nuclear Power Plants. For the Korean Next Generation Reactor (KNGR) development, LBB application is considered for the Main Steam Line(MSL) piping inside containment. Unlike the primary system leakages, the MSL leak detection systems must be based on principles other than radioactivity measurements. Among humidity, heat and acoustic noise currently being considered as indicators of leakage, we explored humidity as an effective one and developed ceramic-based humidity sensor which can be qualified for LBB applications. The ceramic material, sintered and annealed MgCr$_2$O$_4$-TiO$_2$, is shown to increase its electrical conductivity drastically upon water vapor adsorption over the entire temperature range of interest. With this ceramic sensor specimen, we suggested installation-inside-the-piping method by which we can detect leakage more rapidly and sensitively. In this paper, we describe the progress in the development and characterization of ceramic humidity sensor for the LBB application to the MSL of KNGR.

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Computational mechanics and optimization-based prediction of grain orientation in anisotropic media using ultrasonic response

  • Kim, Munsung;Moon, Seongin;Kang, To;Kim, Kyongmo;Song, Sung-Jin;Suh, Myungwon;Suhr, Jonghwan
    • Nuclear Engineering and Technology
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    • v.53 no.6
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    • pp.1846-1857
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    • 2021
  • Ultrasonic nondestructive testing is important for monitoring the structural integrity of dissimilar metal welds (DMWs) in pressure vessels and piping in nuclear power plants. However, there is a low probability of crack detection via inspection of DMWs using ultrasonic waves because the grain structures (grain orientations) of the weld area cause distortion and splitting of ultrasonic beams propagating in anisotropic media. To overcome this issue, the grain orientation should be known, and a precise ultrasonic wave simulation technique in anisotropic media is required to model the distortion and splitting of the waves accurately. In this study, a method for nondestructive prediction of the DMW grain orientations is presented for accurate simulation of ultrasonic wave propagation behavior in the weld area. The ultrasonic wave propagation behavior in anisotropic media is simulated via finite-element analysis when ultrasonic waves propagate in a transversely isotropic material. In addition, a methodology to predict the DMW grain orientation is proposed that employs a simulation technique for ultrasonic wave propagation behavior calculation and an optimization technique. The simulated ultrasonic wave behaviors with the grain orientations predicted via the proposed method demonstrate its usefulness. Moreover, the method can be used to determine the focal law in DMWs.

Neutronic design of pulsed neutron facility (PNF) for PGNAA studies of biological samples

  • Oh, Kyuhak
    • Nuclear Engineering and Technology
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    • v.54 no.1
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    • pp.262-268
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    • 2022
  • This paper introduces a novel concept of the pulsed neutron facility (PNF) for maximizing the production of the thermal neutrons and its application to medical use based on prompt gamma neutron activation analysis (PGNAA) using Monte Carlo simulations. The PNF consists of a compact D-T neutron generator, a graphite pile, and a detection system using Cadmium telluride (CdTe) detector arrays. The configuration of fuel pins in the graphite monolith and the design and materials for the moderating layer were studied to optimize the thermal neutron yields. Biological samples - normal and cancerous breast tissues - including chlorine, a trace element, were used to investigate the sensitivity of the characteristic γ-rays by neutron-trace material interactions and the detector responses of multiple particles. Around 90 % of neutrons emitted from a deuterium-tritium (D-T) neutron generator thermalized as they passed through the graphite stockpile. The thermal neutrons captured the chlorines in the samples, then the characteristic γ-rays with specific energy levels of 6.12, 7.80 and 8.58 MeV were emitted. Since the concentration of chlorine in the cancerous tissue is twice that in the normal tissue, the count ratio of the characteristic g-rays of the cancerous tissue over the normal tissue is approximately 2.