• Title/Summary/Keyword: Nonlinear optical coefficient

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Optical Interferometric Characterization of Nonlinear Optical Polymer Thin Films

  • Wu, J.W.
    • Journal of the Korean Vacuum Society
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    • v.7 no.s1
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    • pp.149-155
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    • 1998
  • The linear electro-optic (EO) effect is one of the second-order nonlinear optical effects existing in a noncentrosymmetric macroscopic system. In a polymer thin film, the noncentrosymmetry is achieved by electric field poling. The magnitude of the linear EO response is determined through the orientational distribution function of hyperpolarizable molecular dipoles. The relation between the linear EO coefficient and the second-order nonlinear optical susceptibility is explained. Three different methods of measuring the linear EO coefficient of a poled nonliner optical polymer thin film are introduced and discussed. All of them make use of the interferometric technique, the difference being in the optical parameters which are interfering.

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Measurement of the Nonlinear Optical Properties by use of the Far-Field Phase Modulation Method (Far-field 위상 변조량 측정법을 이용한 광학매질의 비선형 특성 측정)

  • 김성훈;양준목;김용평;이영우;신동주;정영붕
    • Korean Journal of Optics and Photonics
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    • v.9 no.3
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    • pp.168-174
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    • 1998
  • We have measured nonlinear refractive index and nonlinear absorption coefficient of optical materials by using a far-field phase modulation technique. The phase variation of the probe beam in the nonlinear material is transformed into the spatial phase modulation in the far-field so that the spatial distribution of the optical intensity in conjunction with the computer simulation analysis can give the nonlinear optical constants. We have obtained the nonlinear refractive indices and nonlinear absorption coefficient of $CS_2$ and $BaF_2$ by fitting the experimental values and numerical simulation analysis of far-field measurements. The nonlinear refractive indices of $CS_2$ and $BaF_2$were obtained as $1.2{\times}10^{-11}$ esu and $1.0{\times}10^{-13}$ esu, respectively at 616 nm, and the nonlinear absorption coefficient of BaF$_2$as $5.0{\times}10^{-11}$cm/W at 308nm. These measured values were in good agreement with previous reports.

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Design of nonlinear photonic crystal fibers with ultra-flattened zero dispersion for supercontinuum generation

  • Kumar, Pranaw;Fiaboe, Kokou Firmin;Roy, Jibendu Sekhar
    • ETRI Journal
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    • v.42 no.2
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    • pp.282-291
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    • 2020
  • The study reports on the design and performance of two air-filled and two partial ethanol-filled photonic crystal fiber (PCF) structures with a tetra core for supercontinuum generation. The PCFs are nonlinear with ultra-flattened zero dispersion. Holes with smaller areas are used to create a tetra-core PCF structure. Ethanol is filled in the holes of smaller area while the larger holes of cladding region are airfilled. Optical properties including dispersion, effective mode area, confinement loss, normalized frequency, and nonlinear coefficient of the designed PCF structures are investigated via full vector finite difference time domain (FDTD) method. A PCF structure with lead silicate as wafer exhibits significantly better results than a PCF structure with silica as wafer. However, both structures report dispersion at a telecommunication wavelength corresponding to 1.55 ㎛. Furthermore, the PCF structure with lead silicate as wafer exhibits a very high nonlinear coefficient corresponding to 1375 W-1 km-1 at the same wavelength. This scheme can be used for optical communication systems and in optical devices by exploiting the principle of nonlinearity.

Synthesis and Characterization of Nonlinear Optical Polymers Having Quinoline-based Chromophores

  • Kim, Min-Ho;Jin, Jung-Il;Lee, Chul-Joo;Kim, Nak-Joong;Park, Ki-Hong
    • Bulletin of the Korean Chemical Society
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    • v.23 no.7
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    • pp.964-970
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    • 2002
  • We synthesized three kinds of chromophores incorporating aromatic quinoline unit as a $\pi-conjugated$ bridge in order to prepare more thermally stable nonlinear optical (NLO) chromophores than general stilbene unit. The NLO poly(methylmethacrylate) copolymer, polyimides, and polyester were successfully synthesized by these corresponding quinoline-based monomers. Their physical and optical properties were investigated by thermogravimetry, gel permeation chromatography, ultraviolet-visible spectroscopy, second harmonic generation (SHG) and electro-optic (EO) measurement. All the polymers exhibited better thermal stability,however their NLO activity was a little lower than that of general stilbene-based NLO polymers. Among three kinds of polymers, the PMMA copolymer with quinoline chromophores had the largest SHG coefficient d33 value of 27 pm/V (at 1.064 $\mu\textrm{m})$ and EO coefficient r33 value of 6.8 pm/V (at 1.3 $\mu\textrm{m}$).

Linear and Nonlinear Optical Properties of Vanadium Pentoxide Films Prepared by Pulsed-Laser Deposition

  • Cui, Liqi;Wang, Ruiteng;Wang, Weitian
    • Korean Journal of Materials Research
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    • v.31 no.7
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    • pp.382-385
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    • 2021
  • Well-crystallized vanadium pentoxide V2O5 thin films are fabricated on MgO single crystal substrates by using pulsed-laser deposition technique. The linear optical transmission spectra are measured and found to be in a wavelength range from 300 to 800 nm; the data are used to determine the linear refractive index of the V2O5 films. The value of linear refractive index decreases with increasing wavelength, and the relationship can be well explained by Wemple's theory. The third-order nonlinear optical properties of the films are determined by a single beam z-scan method at a wavelength of 532 nm. The results show that the prepared V2O5 films exhibit a fast third-order nonlinear optical response with nonlinear absorption coefficient and nonlinear refractive index of 2.13 × 10-10 m/W and 2.07 × 10-15 cm2/kW, respectively. The real and imaginary parts of the nonlinear susceptibility are determined to be 3.03 × 10-11 esu and 1.12 × 10-11 esu, respectively. The enhancement of the nonlinear optical properties is discussed.

Reliability and maximum transmission length analysis between adjacent optical solitons in nonlinear dispersive transmission materials (비선형 분산 광 전송 매질에 있어서 인접 광 솔리톤간의 신뢰도 및 최대 전송거리 분석)

  • 변승우;김종규;송재원
    • Electrical & Electronic Materials
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    • v.9 no.3
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    • pp.246-250
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    • 1996
  • In optical soliton transmission systems with nonlinear dispersive materials, which is utilized for ultra-long and high bit rate transmission, it is shown that the value of initial time difference between adjacent solitons is analyzed for optimum bit rate. The method is inducted by uncorrelation condition with minimum interaction forces in initial covariance coefficient between adjacent solitons. When the initial time difference is 6 times of soliton pulse width by the results, it is shown that the reliability is maintained with more than 90% within transmission length of soliton period. multiplied by 93.

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Green Generation and Investigation of Optical Properties of Amorphous BaTiO3 by Poling (폴링에 의한 비정질 BaTiO3 박막의 광학적 특성 조사 및 녹색광 발생)

  • Kim, Eung-Soo
    • The Journal of the Korea institute of electronic communication sciences
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    • v.15 no.1
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    • pp.39-44
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    • 2020
  • BaTiO3 thin films was deposited on the slide glass by RF sputter. We have investigated the optical properties of BaTiO3 film after corona poling process. The transmission characteristics was very good over 80% in visible region and second order nonlinear optical coefficient depends on the poling conditions. The nonlinear optical coefficient of poled BaTiO3 films was about 1.15pm/V. The relaxation of second order nonlinear optical was remained around 60% of the initial value for a long time. In addition we have observed the green light generation from BaTiO3 films.

Dispersion and Nonlinear Properties of Elliptical Air Hole Photonic Crystal Fiber

  • Rao, MP Srinivasa;Singh, Vivek
    • Current Optics and Photonics
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    • v.2 no.6
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    • pp.525-531
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    • 2018
  • The effect of eccentricity on dispersion and nonlinear properties of a photonic crystal fiber having elliptical air holes is investigated using a fully vectorial effective index method. It is found that the effective refractive index increases with increase of eccentricity. The dependence of dispersion and nonlinear properties of the PCF on the eccentricity of the air hole is investigated. It is revealed that eccentricity of the air hole affects the zero dispersion wavelength. Further, the nonlinear properties such as mode field area, nonlinear coefficient and self phase modulation of the Photonic crystal fibers are analyzed. The mode field area increases and the nonlinear coefficient decreases with increase in eccentricity. The variation of the self phase modulation with elliptical air hole is also discussed.

Anomalous Propagation Characteristics of an Airy Beam in Nonlocal Nonlinear Medium

  • Wu, Yun-Long;Ye, Qin;Shao, Li
    • Current Optics and Photonics
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    • v.5 no.2
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    • pp.191-197
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    • 2021
  • The anomalous propagation characteristics of a single Airy beam in nonlocal nonlinear medium are investigated by utilizing the split-step Fourier-transform method. We show that besides the normal straight propagation trajectory, the breathing solitons formed by the interaction between Airy beam and nonlocal nonlinear medium can propagate along the sinusoidal trajectory, and the anomalous trajectory can be modulated arbitrarily by altering the initial amplitude and the nonlocal nonlinear coefficient. In addition, the initial amplitude and the nonlocal nonlinear coefficient can have inverse impacts on the formation and transformation of the equilibrium state of spatial solitons, when the two parameters are larger than certain values. Therefore, the reversible transformation of the evolution dynamics of two soliton states can be realized by adjusting those two parameters properly. Finally, it is shown that the propagation properties of the solitons formed by the interaction between Airy beam and nonlocal nonlinear medium can be controlled arbitrarily, by adjusting the distribution factor and nonlocal coefficient.