• Proceedings of the Korea Air Pollution Research Association Conference
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• 2006.04a
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• pp.55-56
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• 2006

This thesis describes the use of measured aerosol size distributions and size-resolved hygroscopic growth to examine the physical and chemical properties of several particle classes. The primary objective of this work was to investigate the optical and cloud forming properties of a range of ambient aerosol types measured in a number of different locations. The tool used for most of these analyses is a differential mobility analyzer / tandem differential mobility analyzer (DMA / TDMA) system developed in our research group. To collect the data described in two of the chapters of this thesis, an aircraft-based version of the DMA / TDMA was deployed to Japan and California. The data described in two other chapters were conveniently collected during a period when the aerosol of interest came to us. The unique aspect of this analysis is the use of these data to isolate the size distributions of distinct aerosol types in order to quantify their optical and cloud forming properties. I used collected data during the Asian Aerosol Characterization Experiment (ACE-Asia) to examine the composition and homogeneity of a complex aerosol generated in the deserts and urban regions of China and other Asian countries. An aircraft-based tandem differential mobility analyzer was used for the first time during this campaign to examine the size-resolved hygroscopic properties of particles having diameters between 40 and 586 nm. Asian Dust Above Monterey (ADAM-2003) study was designed both to evaluate the degree to which models can predict the long-range transport of Asian dust, and to examine the physical and optical properties of that aged dust upon reaching the California coast. Aerosol size distributions and hygroscopic growth are measured in College Station, TX to investigate the cloud nucleating and optical properties of a biomass burning aerosol generated from fires on the Yucatan Peninsula. Measured aerosol size distributions and size-resolved hygroscopicity and volatility were used to infer critical supersaturation distributions of the distinct particle types that were observed during this period. The predicted CCN concentrations were used in a cloud model to determine the impact of the different aerosol types on the expected cloud droplet concentration. RH-dependent aerosol extinction coefficients are calculated at a wavelength of 550 nm.

• Journal of Environmental Science International
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• v.10 no.3
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• pp.201-208
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• 2001

To investigate the physio-chemical components and properties of aerosol particles in urban area sampling of aerosol particles was carried out in the campus of Hokkaido University, Sapporo, Japan, during snowfall. Aerosol particles were collected on millipore filter papers using a low volume air sampler. Their shapes, sizes and chemical components were analyzed by a SEM(Scanning Electron Microscope) and an EDX(Energy Dispersive X-ray). As a results, ice crystals of dendrite and column types were predominantly shown at mature and developing stage of snowfall intensity. The denerite and sector plate types of ice crystals were mainly originated from the sea but column types were come from soil. Scavenging effect by snowfall was greatly also shown at dendrite type ice crystals that embryo was fully developd. Al, Si elements were shown at high frequencies as compared with others. Na, Cl components were especially shown at high frequencies under the sea-breeze wind during snowfall. Anthropogenic aerosol particles had shown with irregular shapes and sizes, relatively. Mainly 3-7$\mu$m aerosol particles were abundant and coarse particles also could be seen during snowfall. Ca, Zn, Fe components mainly caused by spike tires from vehicles in winter season were dominant before snowfall, however the element S mainly caused by human activity was rich after snowfall. The pH values of snow in Sapporo city were higher than those at coastal area. The concentration of chemical components in aerosol particles was also affected by surface winds. Aerosol particles in urban area, Sapporo were mainly affected by human activities like vehicles and combustion with wind system. And their types were related with snowfall intensity.

• Atmosphere
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• v.34 no.3
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• pp.233-255
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• 2024

This study analyzed the distribution of Aerosol Robotic Network (AERONET) Version 3 Level 2.0 data, spanning over two decades, across South Korea and its six administrative regions (Seoul metropolitan area, Chungcheong, Jeolla, Gangwon, Gyeongsang, and Jeju). The research assessed long-term trends in aerosol optical depth (AOD) and mass concentration of particulate matter (i.e., PM₁₀ and PM_2.5), using data from the AERONET direct sun product and AirKorea, respectively. Additionally, eight aerosol types were identified using the scattering Ångström exponent and absorption Ångström exponent from the AERONET inversion product. The study further explored their domestic and regional distributions. Findings indicated that AERONET data were predominantly concentrated in the western regions of South Korea, including the Seoul metropolitan area, Chungcheong, and Jeolla, with a higher frequency of data in spring, thus demonstrating spatial and temporal heterogeneity. The annual average AOD exhibited a declining trend of -0.006 yr^-1. Similarly, PM₁₀ and PM_2.5 mass concentrations decreased by -1.324 ㎍ m^-3 yr^-1 and -1.335 ㎍ m^-3 yr^-1, respectively. These trends in AOD and PM₁₀ (PM_2.5) demonstrated positive correlations, with correlation coefficients of 0.674 (0.753) and statistically significant low p-values of 0.00058 (0.03), respectively. The analysis also revealed that aerosols in South Korea predominantly consisted of black carbon (BC) or BC-mixed types (84.09%), with a notable presence of smaller, less absorbent aerosol types (13.11%).

• Journal of Korean Society for Atmospheric Environment
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• v.34 no.5
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• pp.668-676
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• 2018

This study has developed a technique to divide the aerosol optical depth of the entire aerosol (${\tau}_{total}$) into the dust optical depth (${\tau}_D$) and the pollution particle optical depth (${\tau}_P$) using the AERONET sun/sky radiometer data provided in Version 3. This method was applied to the analysis of AERONET data observed from 2006 to 2016 in Beijing, China, Seoul and Gosan, Korea and Osaka, Japan and the aerosol optical depth trends of different types of atmospheric aerosols in Northeast Asia were analyzed. The annual variation of ${\tau}_{total}$ showed a tendency to decrease except for Seoul where observation data were limited. However, ${\tau}_D$ tended to decrease when ${\tau}_{total}$ were separated as ${\tau}_D$ and ${\tau}_P$, but ${\tau}_P$ tended to increase except for Osaka. This is because the concentration of airborne aerosols, represented by Asian dust in Northeast Asia, is decreased in both mass concentration and optical concentration. However, even though the mass concentration of pollution particles generated by human activity tends to decrease, Which means that the optical concentration represented as aerosol optical depth is increasing in Northeast Asia.

• Korean Journal of Remote Sensing
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• v.29 no.4
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• pp.407-413
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• 2013

The Modified Aerosol Factor (MAF) derived from spectral Single-Scattering Albedo (SSA) values was created to express the light absorption properties according to aerosol types. As a factor of the MAF, slope of a linear regression line for SSA at four wavelengths shows positive value for dust aerosol, while negative values were found for mixing with other types of aerosol. The negative values were shown by anthropogenic and smoke aerosols. The modified SSA at 1020 nm was also calculated. MAF was calculated by summing the slope and modified SSA. MAF was -1.0 for the anthropogenic and smoke aerosol and 1.5 for the dust particles. Those values were decreased by increasing light absorption property.

• Food Science and Biotechnology
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• v.17 no.3
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• pp.664-668
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• 2008

The diffusivity of aerosol sanitizers may be determined by the weight and droplet size of the aerosol. To test the effects of droplet size, 2 types of aerosol sanitizers were prepared using different ultrasonic nebulizer frequencies (1.6 and 2.4 MHz) and their reduction activities were determined against Escherichia coli O157:H7, Listeria monocytogenes, and Salmonella typhimurium. A sodium hypochlorite aerosol was treated for 10, 30, or 60 min in a model aerosol cabinet. When the aerosol prepared by nebulizing at 1.6 MHz was treated for 30 min, a 0.2 log reduction was observed in E. coli O157:H7 and 0.3 log reductions were exhibited in L. monocytogenes and S. typhimurium, respectively. After 60 min, the 3 pathogens were reduced by 1.7, 0.6, and 0.8 log units, respectively. However, when the aerosol prepared by nubulizing at 2.4 MHz was treated, the microbes presented 1.6, 0.5, and 0.6 log reductions at 30 min, and 1.8, 0.9, and 1.1 log reductions at 60 min of treatment, respectively.

• Journal of Korean Society for Atmospheric Environment
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• v.34 no.3
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• pp.493-507
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• 2018

Due to high spatio-temporal variability of amount and optical/microphysical properties of atmospheric aerosols, satellite-based observations have been demanded for spatiotemporal monitoring the major aerosols. Observations of the heavy aerosol episodes and determination on the dominant aerosol types from a geostationary satellite can provide a chance to prepare in advance for harmful aerosol episodes as it can repeatedly monitor the temporal evolution. A new geostationary observation sensor, namely the Advanced Himawari Imager (AHI), onboard the Himawari-8 platform, has been observing high spatial and temporal images at sixteen wavelengths from 2016. Using observed spectral visible reflectance and infrared brightness temperature (BT), the algorithm to find major aerosol type such as volcanic ash (VA), desert dust (DD), polluted aerosol (PA), and clean aerosol (CA), was developed. RGB color composite image shows dusty, hazy, and cloudy area then it can be applied for comparing aerosol detection product (ADP). The CALIPSO level 2 vertical feature mask (VFM) data and MODIS level 2 aerosol product are used to be compared with the Himawari-8/AHI ADP. The VFM products can deliver nearly coincident dataset, but not many match-ups can be returned due to presence of clouds and very narrow swath. From the case study, the percent correct (PC) values acquired from this comparisons are 0.76 for DD, 0.99 for PA, 0.87 for CA, respectively. The MODIS L2 Aerosol products can deliver nearly coincident dataset with many collocated locations over ocean and land. Increased accuracy values were acquired in Asian region as POD=0.96 over land and 0.69 over ocean, which were comparable to full disc region as POD=0.93 over land and 0.48 over ocean. The Himawari-8/AHI ADP algorithm is going to be improved continuously as well as the validation efforts will be processed by comparing the larger number of collocation data with another satellite or ground based observation data.

• Journal of Korean Society for Atmospheric Environment
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• v.20 no.6
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• pp.811-821
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• 2004

Low-Z particle electron probe X-ray microanalysis (low-Z particle EPMA) was applied to characterize aerosol particles collected at Gosan in Jeju island during an IOP (intensive observation period) for an international ACE-Asia project in April, 2001. Various types of atmospheric particles such as organics, carbon-rich, aluminosilicates, silicon oxide, sodium nitrate, sodium chloride, and ammonium sulfate were observed. The reacted sea salt particles such as sodium nitrate were the most abundantly encountered, but original sea salt particles were rarely observed. Since the Low-Z particle EPMA can provide quantitative information on the chemical composition of aerosol particles, many different particle types on the basis of their chemical compositions were observed and identified. In this study, it is demonstrated that the Low-Z particle EPMA can provide detailed information on the chemical compositions for the aerosol particles collected for six consecutive days in April, 2001, at Gosan super-site.

• Journal of Environmental Science International
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• v.22 no.8
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• pp.1053-1062
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• 2013

The shortwave aerosol direct radiative forcing (SWARF) was analyzed using the Clouds and Earth's Radiant Energy System (CERES) data in the East Asian region from 2001 to 2010. In the Yellow Sea and the Korean Peninsula, located in the leeward side of China, significantly negative high SWARF at the top of atmosphere (TOA) occurs due to the long-range transport of anthropogenic (e.g. sulphate) and natural aerosols (e.g. mineral dust) from the East Asian continent. Conversely, eastern China has much higher levels of SWARF at the surface (SFC) due to anthropogenically emitted aerosol than in the Yellow Sea and the Korean Peninsula. Since the radiative forcing of aerosols in the atmosphere are different in type, aerosol types were classified into sea salt+sulphate, smoke, sulphate and dust by using satellite data. The analysis on the SWARF by the classified aerosol types indicated that sulphate occupies a predominant portion of the atmosphere in the Yellow Sea and the Korean Peninsula in the summer. In particular, the annual averages of the summer TOA SWARF increased in the Yellow Sea and the Korean Peninsula from 2001 to 2010.

• Proceedings of the Korea Air Pollution Research Association Conference
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• 1999.10a
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• pp.121-123
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• 1999

Bio-Aerosol Concentrator Inlets were made to collect particles of which size was $2\mu\textrm{m}$ as aerodynamic diameter or larger. The Concentrator Inlets were designed by using virtual impactors, because the virtual impactors are known for high efficiency. In a virtual impactor, the intake air is typically divided into two streams with the major and the minor flow. In this work, several types of the acceleration nozzles and collection probes were designed. Subsequently, the results were evaluated experimentally. It was found that if controled properly, the velocity can improve substantially the aerosol concentration performance. The diameter of acceleration nozzle and type of collection probe were varied to obtain the optimum design. Subsequently, the different designs were compared respectively and the best design among them was identified. It is expected that this new finding can help improve design of future Aerosol Concentrator for high concentration rate.