• Title/Summary/Keyword: Aerosol extinction

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Characteristics of Visibility Impairment by Semi-Continuous Optical and Chemical Property Monitoring of Aerosols in Seoul (에어로졸의 광학 및 화학 특성 준실시간 모니터링을 통한 서울지역 시정 감쇄 분석)

  • Park, Jong-Sung;Park, Seung-Myung;Song, In-Ho;Shin, Hye-Jung;Hong, You-Deog
    • Journal of Korean Society for Atmospheric Environment
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    • v.31 no.4
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    • pp.319-329
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    • 2015
  • The characteristics of aerosol light extinction were investigated by comparing measured and calculated extinction coefficient to understand the contribution of air pollutants on visibility impairment for data during 4 months (Jan~ April), 2014. The integrated nephelometer and aethalometer system were installed to measure the scattering and absorption coefficients of aerosol as well as BAM 1020, MARGA, semi-continuous OCEC analyzer, and online-XRF to calculate the extinction coefficient. The IMPROVE_2005 equation was used to determine the contributions of different chemical components on visibility impairment in $PM_{2.5}$ and $PM_{10}$ due to highest correlation with measured data. Sulfate, nitrate, and organic mass by carbon (OMC) of fine aerosol were the major contributors affecting on visibility impairment. Total contributions to light extinction were calculated as $631.0Mm^{-1}$ for the worst-case and $64.4Mm^{-1}$ for the best-case. The concentrations of aerosol component for the worst-case were 38.4 times and 45.5 times larger than those of the best-case for $(NH_4)_2SO_4$ and $NH_4NO_3$, respectively. At lower visibility condition, in which extinction coefficient was higher than $400Mm^{-1}$, extinction coefficient varied according to the relative humidity variation regardless of $PM_{2.5}$.

Multi-wavelength Raman LIDAR for Use in Determining the Microphysical, Optical, and Radiative Properties of Mixed Aerosols

  • Lee, Kwon-Ho;Noh, Young Min
    • Asian Journal of Atmospheric Environment
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    • v.9 no.1
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    • pp.91-99
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    • 2015
  • The Multi-wavelength Raman LIDAR (MRL) system was developed to enable a better understanding of the complex properties of aerosols in the atmosphere. In this study, the microphysical, optical, and radiative properties of mixed aerosols were retrieved using the discrete aerosol observation products from the MRL. The dust mixing ratio, which is the proportion of dust particles to the total mixed, was derived using the particle depolarization ratio. It was employed in the retrieval of backscattering and extinction coefficient profiles for dust and non-dust particles. The vertical profiles of aerosol optical properties were then used as input parameters in the inversion algorithm for the retrieval of microphysical parameters including the effective radius, refractive index, and the single scattering albedo (SSA). Those products were successfully applied to an analysis of radiative flux using a radiative transfer model. The relationship between the MRL derived extinction and aerosol radiative forcing (ARF) in short-wavelength was assessed over Gwangju, Korea. The results clearly demonstrate that the MRL-derived extinction profiles are a good surrogate for use in the estimation of optical, microphysical, and radiative properties of aerosols. It is considered that the analytical results shown in this study can be used to provide a better understanding of air quality and the variation of local radiative effects due to aerosols.

Estimation of Aerosol Vertical Profile from the MODIS Aerosol Optical Thickness and Surface Visibility Data (MODIS 에어러솔 광학두께와 지상에서 관측된 시정거리를 이용한 대기 에어러솔 연직분포 산출)

  • Lee, Kwon-Ho
    • Journal of the Korean Association of Geographic Information Studies
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    • v.16 no.2
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    • pp.141-151
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    • 2013
  • This study presents a modeling of aerosol extinction vertical profiles in Korea by using the Moderate Resolution Imaging Spectro-radiometer(MODIS) derived aerosol optical thickness(AOT) and ground based visibility observation data. The method uses a series of physical equations for the derivation of aerosol scale height and vertical profiles from MODIS AOT and surface visibility data. The modelled results under the standard atmospheric condition showed small differences with the standard aerosol vertical profile used in the radiative transfer model. Model derived aerosol scale heights for two cases of clean(${\tau}_{MODIS}=0.12{\pm}0.07$, visibility=$21.13{\pm}3.31km$) and hazy atmosphere(${\tau}_{MODIS}=1.71{\pm}0.85$, visibility=$13.33{\pm}5.66km$) are $0.63{\pm}0.33km$ and $1.71{\pm}0.84km$. Based on these results, aerosol extinction profiles can be estimated and the results are transformed into the KML code for visualization of dataset. This has implications for atmospheric environmental monitoring and environmental policies for the future.

A Study of the Characteristics of Highly Spatially Resolved CW-laser-based Aerosol Lidar (고공간분해능 연속 광원을 이용한 미세먼지 라이다의 신호 특성에 관한 연구)

  • Sim, Juhyeon;Kim, Taekeong;Ju, Sohee;Noh, Youngmin;Kim, Dukhyeon
    • Korean Journal of Optics and Photonics
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    • v.33 no.1
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    • pp.1-10
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    • 2022
  • In this study we introduce a new method for high-spatial-resolution continuous wave (CW) aerosol lidar that has a high spatial resolution in the near field and a low spatial resolution at long distances. A normal lidar system uses a nanosecond-pulse laser and measures the round-trip TOF between the aerosol and laser to obtain range resolution. In this study, however, we propose a new type of spatially resolving aerosol lidar that uses laser-scattering images. Using a laser-light-scattering image, we have calculated the distance of each scattering aerosol image for a given pixel, and recovered the short-range aerosol extinction. For this purpose, we have calculated the distance image and the contribution range of the aerosol to the given one-pixel image, and finally we have calculated the extinction coefficients of the aerosol with range-resolved information. In the case of traditional aerosol lidar, we can only obtain the aerosol extinction coefficients above 400 m. Using our suggested method, it was possible to extend the range of the extinction coefficient lower then several tens of meters. Finally, we can remove the unknown short-range region of pulsed aerosol lidar using our method.

The KALION Automated Aerosol Type Classification and Mass Concentration Calculation Algorithm (한반도 에어로졸 라이다 네트워크(KALION)의 에어로졸 유형 구분 및 질량 농도 산출 알고리즘)

  • Yeo, Huidong;Kim, Sang-Woo;Lee, Chulkyu;Kim, Dukhyeon;Kim, Byung-Gon;Kim, Sewon;Nam, Hyoung-Gu;Noh, Young Min;Park, Soojin;Park, Chan Bong;Seo, Kwangsuk;Choi, Jin-Young;Lee, Myong-In;Lee, Eun hye
    • Korean Journal of Remote Sensing
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    • v.32 no.2
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    • pp.119-131
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    • 2016
  • Descriptions are provided of the automated aerosol-type classification and mass concentration calculation algorithm for real-time data processing and aerosol products in Korea Aerosol Lidar Observation Network (KALION, http://www.kalion.kr). The KALION algorithm provides aerosol-cloud classification and three aerosol types (clean continental, dust, and polluted continental/urban pollution aerosols). It also generates vertically resolved distributions of aerosol extinction coefficient and mass concentration. An extinction-to-backscatter ratio (lidar ratio) of 63.31 sr and aerosol mass extinction efficiency of $3.36m^2g^{-1}$ ($1.39m^2g^{-1}$ for dust), determined from co-located sky radiometer and $PM_{10}$ mass concentration measurements in Seoul from June 2006 to December 2015, are deployed in the algorithm. To assess the robustness of the algorithm, we investigate the pollution and dust events in Seoul on 28-30 March, 2015. The aerosol-type identification, especially for dust particles, is agreed with the official Asian dust report by Korean Meteorological Administration. The lidar-derived mass concentrations also well match with $PM_{10}$ mass concentrations. Mean bias difference between $PM_{10}$ and lidar-derived mass concentrations estimated from June 2006 to December 2015 in Seoul is about $3{\mu}g\;m^{-3}$. Lidar ratio and aerosol mass extinction efficiency for each aerosol types will be developed and implemented into the KALION algorithm. More products, such as ice and water-droplet cloud discrimination, cloud base height, and boundary layer height will be produced by the KALION algorithm.

Opto-Chemical Characteristics of Visibility Impairment Using Semi-Continuous Aerosol Monitoring in an Urban Area during Summertime (에어로졸의 준실시간 관측에 의한 여름철 도시지역 시정 감쇄 현상의 광ㆍ화학적인 특성 분석)

  • 김경원;김영준
    • Journal of Korean Society for Atmospheric Environment
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    • v.19 no.6
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    • pp.647-661
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    • 2003
  • For continuous monitoring of atmospheric visibility in the city of Kwanaju, Korea, a transmissometer system consisting of a transmitter and a receiver was installed at a distance of 1.91 km across the downtown Kwanaju. At the transmitter site an integrating nephelometer and an aethalometer were also installed to measure the scattering and absorption coefficients of the atmosphere, respectively. At the receiver site. an URG PM$_{2.5}$ cyclone sampler and an URG-VAPS (Versatile Air Pollutant Sampler) with three filter packs and two denuders were used to collect both PM$_{2.5}$ and PM$_{10}$ samples at a 2-hour or 12-hour sampling interval for aerosol chemical analysis. Sulfate, organic mass by carbon (OMC), nitrate, elemental carbon (EC) components of fine aerosol were the major contributors to visibility impairment. Diurnal variation of visibility during best-case days showed rapid improvement in the morning hours, while it was delayed until afternoon during the worst-case days. Aerosol mass concentration of each aerosol component for the worst-case was calculated to be 11.2 times larger than the best-case for (NH$_4$)$_2$SO$_4$(NHSO), 19.0 times for NH$_4$NO$_3$ (NHNO), 2.2 times for OMC, respectively. Also result shows that elemental carbon and fine soil (FS) were 3.7 and 2.2 times more than those of best-case. respectively- Sum of total contributions of wet NHSO and NHNO to light extinction was calculated to be 301 Mm$^{-1}$ for the worst-case. However, sum of contributions by dry NHSO and NHNO was calculated to be 123 Mm$^{-1}$ for the best case. Mass extinction efficiencies of fine and coarse particles were calculated to be 5.8$\pm$0.3 $m^2$/g and 1.8$\pm$0.1 $m^2$/g, respectively.ely.

Vertical Change in Extinction and Atmospheric Particle Size in the Boundary Layers over Beijing: Balloon-borne Measurement

  • Chen, Bin;Shi, Guang-Yu;Yamada, Maromu;Zhang, Dai-Zhou;Hayashi, Masahiko;Iwasaka, Yasunobu
    • Asian Journal of Atmospheric Environment
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    • v.4 no.3
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    • pp.141-149
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    • 2010
  • Aerosol size and number concentration were observed in the atmospheric boundary layer over Beijing (from near the ground to 1,200 m) on March 15 (a clear day) and 16 (a dusty day), 2005. The results were further compared with lidar measurements in order to understand the dependency of extinction on the particle size distribution and their vertical changes. The boundary layer atmosphere was composed of several sub-layers, and a dry air layer appeared between 400 and 1,000 m under the influence of dust event. In this dry air layer, the concentration of the fine-mode particles (diameter smaller than $1.0\;{\mu}m$) was slightly lower than the value on the clear day, while the concentration of coarse-mode particles (diameter larger than $1.0\;{\mu}m$) was remarkably higher than that on the clear day. This situation was attributed to the inflow of an air mass containing large amounts of Asian dust particles and a smaller amount of fine-mode particles. The results strongly suggest that the fine-mode particles affect light extinction even in the dusty atmosphere. However, quantitatively the relation between extinction and particle concentration is not satisfied under the dusty atmospheric conditions since laser beam attenuates in the atmosphere with high concentration of particles. Laser beam attenuation effect becomes larger in the relation between extinction and coarse particle content comparing the relation between extinction and fine particle content. To clarify this problem technically, future in situ measurements such as balloon-borne lidar are suggested. Here extinction was measured at 532 nm wavelength. Measurements of extinction at other wavelengths are desired in the future.

Retrieval of LIDAR Aerosol Parameter Using Sun/Sky Radiometer at Gangneung, Korea

  • Shin, Sung-Kyun;Lee, Kwon-Ho;Lee, Kyu-Tae
    • Current Optics and Photonics
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    • v.1 no.3
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    • pp.175-185
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    • 2017
  • The aerosol optical properties such as depolarization ratio (${\delta}$) and aerosol extinction-to-backscatter ratios (S, LIDAR ratio) and ${\AA}ngstr{\ddot{o}m$ exponent (${\AA}$) derived from measurement with AERONET sun/sky radiometer at Gangneung-Wonju National University (GWNU), Gangneung, Korea ($37.77^{\circ}N$, $128.87^{\circ}E$) during a winter season (December 2014 - February 2015) are presented. The PM concentration measurements are conducted simultaneously and used to identify the high-PM events. The observation period was divided into three cases according to the PM concentrations. We analysed the ${\delta}$, S, and ${\AA}$ during these high PM-events. These aerosol optical properties are calculated by the sun/sky radiometer data and used to classify a type of aerosols (e.g., dust, anthropogenic pollution). The higher values of ${\delta}$ with lower values of S and ${\AA}$ were measured for the dust particles. The mean values of ${\delta}$, S, and ${\AA}$ at 440-870 nm wavelength pair (${\AA}_{440-870}$) for the Asia dust were 0.19-0.24, 36-56 sr, and 0.48, respectively. The anthropogenic aerosol plumes are distinguished with the lower values of ${\delta}$ and higher values of ${\AA}$. The mean values of spectral ${\delta}$ and ${\AA}_{440-870}$ for this case varied 0.06-0.16 and 1.33-1.39, respectively. We found that aerosol columnar optical properties obtained from the sun/sky radiometer measurement are useful to identify the aerosol type. Moreover, the columnar aerosol optical properties calculated based on sun/sky radiometer measurements such as ${\delta}$, S, and ${\AA}$ will be further used for the validation of aerosol parameters obtained from LIDAR observation as well as for quantification of the air quality.

Measurement of Aerosol Parameters with Altitude by Using Two Wavelength Rotational Raman Signals

  • Song, Im-Kang;Kim, Yong-Gi;Baik, Sung-Hoon;Park, Seung-Kyu;Cha, Hyung-Ki;Choi, Sung-Chul;Chung, Chin-Man;Kim, Duk-Hyeon
    • Journal of the Optical Society of Korea
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    • v.14 no.3
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    • pp.221-227
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    • 2010
  • Aerosol size distribution provides good information for predicting weather changes and understanding cloud formation. Aerosol extinction coefficient and backscattering coefficient are measured by many scientists, but these parameters depend not only on aerosol size but on aerosol concentrations. An algorithm has been developed to measure aerosol parameters such as ${\AA}$ngstr$\ddot{o}$m exponent, color ratio, and LIDAR ratio without any assumptions by using two wavelength rotational Raman LIDAR signals. These parameters are good indicators for the aerosol size. And we can find ${\AA}$ngstr$\ddot{o}$m exponent, color ratio, and LIDAR ratio under various weather conditions. Finally, it can be seen that the ${\AA}$ngstr$\ddot{o}$m exponent has an inverse relationship to the particle size of the aerosol and the color ratio is linearly dependent on the aerosol size. An ${\AA}$ngstr$\ddot{o}$m exponent from 1.2 to 3.1, a color ratio from 0.28 to 1.04, and a LIDAR ratio 66.9 sr at 355 nm and 32.6 sr at 532 nm near the cloud were obtained.

3-D Perspectives of Atmospheric Aerosol Optical Properties over Northeast Asia Using LIDAR on-board the CALIPSO satellite (CALIPSO위성 탑재 라이다를 이용한 동북아시아 지역의 대기 에어러솔 3차원 광학특성 분포)

  • Lee, Kwon-Ho
    • Korean Journal of Remote Sensing
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    • v.30 no.5
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    • pp.559-570
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    • 2014
  • Backscatter signal observed from the space-borne Light Detection And Ranging (LIDAR) system is providing unique 3-dimensional spatial distribution as well as temporal variations for atmospheric aerosols. In this study, the continuous observations for aerosol profiles were analyzed during a years of 2012 by using a Cloud-Aerosol LIDAR with Orthogonal Polarization (CALIOP), carried on the Cloud-Aerosol LIDAR and Infrared Pathfinder Satellite Observation (CALIPSO) satellite. The statistical analysis on the particulate extinction coefficient and depolarization ratio for each altitude was conducted according to time and space in order to estimate the variation of optical properties of aerosols over Northeast Asia ($E110^{\circ}-140^{\circ}$, $N20^{\circ}$ $-50^{\circ}$). The most frequent altitudes of aerosols are clearly identified and seasonal mean aerosol profiles vary with season. Since relatively high particle depolarization ratios (>0.5) are found during all seasons, it is considered that the non-spherical aerosols mixed with pollution are mainly exists over study area. This study forms initial regional 3-dimensional aerosol information, which will be extended and improved over time for estimation of aerosol climatology and event cases.