• Title/Summary/Keyword: ${238}^U$

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Jurassic (~170Ma) Zircon U-Pb Age of a "Granite Boulder" in the Geumgang Limestone, Ogcheon Metamorphic Belt, Korea: Reinterpretation of its Origin (옥천변성대 금강석회암 내 "화강암 거력"의 쥬라기(~170 Ma) 저어콘 연대: 성인에 대한 재해석)

  • Cheong, Wonseok;Cho, Moonsup;Yi, Keewook;Lee, Min Sung;Kim, Yoonsup
    • The Journal of the Petrological Society of Korea
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    • v.25 no.1
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    • pp.29-37
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    • 2016
  • A "granite boulder", ~70 cm in size, was reported from the Geumgang Limestone, and has been considered as a glaciogenic dropstone. Since this interpretation has enormous implications for unraveling the evolution history of the Ogcheon Metamorphic Belt, we re-examined the contact relationship and structure of the "granite boulder", and estimated its emplacement age based upon SHRIMP U-Pb zircon dating. The weighted mean $^{206}Pb/^{238}U$ age pooled from 6 spot analyses of two specimens is $170{\pm}2Ma$ ($2{\sigma}$, MSWD=2.2). This zircon age suggests that the "granite boulder" in the Geumgang Limestone is a part of Jurassic granite, rather than a glaciogenic dropstone.

Application of Laser Ablation Inductively Coupled Plasma Mass Spectrometry for Characterization of U-7Mo/Al-5Si Dispersion Fuels

  • Lee, Jeongmook;Park, Jai Il;Youn, Young-Sang;Ha, Yeong-Keong;Kim, Jong-Yun
    • Nuclear Engineering and Technology
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    • v.49 no.3
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    • pp.645-650
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    • 2017
  • This technical note demonstrates the feasibility of using laser ablation inductively coupled plasma mass spectrometry for the characterization of U-7Mo/Ale5Si dispersion fuel. Our measurements show 5.0% Relative Standard Deviation (RSD) for the reproducibility of measured $^{98}Mo/^{238}U$ ratios in fuel particles from spot analysis, and 3.4% RSD for $^{98}Mo/^{238}U$ ratios in a NIST-SRM 612 glass standard. Line scanning allows for the distinction of U-7Mo fuel particles from the Al-5Si matrix. Each mass spectrum peak indicates the presence of U-7Mo fuel particles, and the time width of each peak corresponds to the size of that fuel particle. The size of the fuel particles is estimated from the time width of the mass spectrum peak for $^{98}Mo$ by considering the scan rate used during the line scan. This preliminary application clearly demonstrates that laser ablation inductively coupled plasma mass spectrometry can directly identify isotope ratios and sizes of the fuel particles in U-Mo/Al dispersion fuel. Once optimized further, this instrument will be a powerful tool for investigating irradiated dispersion fuels in terms of fission product distributions in fuel matrices, and the changes in fuel particle size or shape after irradiation.

Increased Plasma $PGE_2$ Levels after Administration of Radionuclides Used in Nuclear Medicine (핵의학 이용 방사핵종의 투여후 혈중 $PGE_2$의 변동)

  • Ryu, Yong-Wun
    • Journal of Radiation Protection and Research
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    • v.14 no.1
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    • pp.8-15
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    • 1989
  • After administration of $^{99m}TC,\;^{67}Ga,\;^{131}I,\;^{32}P\;and\;^{238}U(UO_2(NO_2)_3{\cdot}6H_2O)$, in male rats, toxic effects were examined by determining the biological materials in blood. Dosages of radio-nuclides injected are based on the amounts routinely administered to patients, and concentrations of BUN, creatinine, SGOT, SGPT and $PGE_2$ in plasma are determinated as indices to the biochemical response. No increase of creatinine was observed after injection of $^{99m}TC$. Concentrations of BUN, SGOT and $PGE_2$ were not significantly increased in comparison with before-administration. Administration of $^{67}Ga,\;^{131}I\;and\;^{32}P$, did not significantly change BUN, SGPT and SGOT, but largely increased $PGE_2$ than control levels. Besides, $^{238}U$ Showed the most severe toxicity. From the above results, we suggest that the determination of $PGE_2$ in plasma can be used as an index in case of elvaluating the effects of radiation toxicity by nuclides used in nuclear medicine.

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Study on the determination methods of the natural radionuclides (238U, 232Th) in building materials and processed living products (실내 건축자재 및 생활 가공제품 중 천연방사성핵종(238U, 232Th)의 농도 평가를 위한 분석법 연구)

  • Lee, Hyeon-Woo;Lim, Jong-Myoung;Lee, Hoon;Park, Ji-Young;Jang, Mee;Lee, Jin-Hong
    • Analytical Science and Technology
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    • v.31 no.4
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    • pp.149-160
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    • 2018
  • A large number of functional living products are being produced for eco-friendly or health-promoting purposes. In the manufacturing process, such products could be adulterated with raw materials with high radioactivity, such as monazite and tourmaline. Thus, it is essential to manage raw materials and products closely related to the public living. For proper management, an accurate radioactivity data of the processed products are needed. Therefore, it is essential to develop a rapid and validated analytical method. In this study, the concentration of the radioactive $^{238}U$ and $^{232}Th$ in building materials (e.g., tile, cement, paint, wall paper, and gypsum board) and living products (e.g., health products, textiles, and minerals) were determined and compared by ED-XRF and ICP-MS. By comparing the results of both methods, we confirmed the applicability of the rapid screening and precise analysis of ED-XRF and ICP-MS. In addition, $^{238}U$ and $^{232}Th$ levels were relatively lower in building materials than in living products. Particularly, $^{232}Th$ content in 6 of 47 living products exceeded (maximum $8.2Bq{\cdot}g^{-1}$) the standard limit of $^{232}Th$ content in raw material ($1.0Bq{\cdot}g^{-1}$).

Estimate of Particulate Organic Carbon Export Flux Using $^{234}Th/^{238}U$ Disequilibrium in the Southwestern East Sea During Summer (동해 서남해역에서 여름철 $^{234}Th/^{238}U$ 비평형을 이용한 입자상 유기탄소 침강플럭스 추정)

  • Kim, Dong-Seon;Choi, Man-Sik;Oh, Hae-Young;Kim, Kyung Hee;Noh, Jae-Hoon
    • The Sea:JOURNAL OF THE KOREAN SOCIETY OF OCEANOGRAPHY
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    • v.14 no.1
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    • pp.1-9
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    • 2009
  • Export fluxes of particulate organic carbon were estimated for the first time by using $^{234}Th/^{238}U$ disequilibrium in the southwestern East Sea during August 2007. They were calculated by multiplying POC/$^{234}Th_p$ ratios of sinking particles (larger than 0.7 ${\mu}m$) obtained from 150-200 m water depths to $^{234}Th$ fluxes that were estimated by integrating $^{234}Th/^{238}U$ disequilibrium from surface to 100 m water depth. Export fluxes ranged from 14 to 505 mg C $m^{-2}$ $day^{-1}$, with the highest value at station A2 and the lowest value at station D4. Primary production was well correlated with export flux, indicating that it was a major factor controlling export flux. Export flux in the East Sea was generally higher than those estimated in the open ocean and similar to or somewhat higher than those in the continental marginal seas. Export flux/primary production (EF/PP) ratios varied from 0.29 to 0.62, with an average of 0.43 and were somewhat higher in the basin area than in the coastal area. EF/PP ratio in the East Sea was rather similar to those estimated in the North Sea and Chukchi Sea, but much higher than those in the Labrador Sea, Barents Sea, and Gulf of Lions. Therefore, the East Sea is one of the major areas where a large amount of organic carbon produced in the euphotic zone sinks into the deep layer below 200 m water depth.

An analysis of the concentration of radioactivity of natural radionuclides (238U, 232Th, 40K) and gamma-ray emitting artificial radionuclides(137Cs, 60Co) present in the drinking water of the city of Busan, Republic of Korea, and the calculated absorbed dose of the residents

  • Kim, Chang-Soo;Kim, Jung-Hoon
    • International Journal of Contents
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    • v.8 no.2
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    • pp.60-66
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    • 2012
  • This study was designed to detect and measure the concentration of radioactivity of natural radionuclides ($^{238}U$, $^{232}Th$, $^{40}K$) and artificial radionuclides ($^{137}Cs$, $^{60}Co$) present in the drinking water of the city of Busan and surrounding areas in South Korea, and also to measure the absorbed dose of radiation caused by these elements in the residents so as to help better manage the risk that these radionuclides pose in the future. For the purposes of the study, a total of 42 samples of water were collected from three key water sources (19 samples of groundwater, 4 samples of tap water, and 19 samples of surface water) and their contents were analyzed for radioactivity concentration. The results revealed that two natural radionuclides, $^{238}U$ and $^{232}Th$, exist in the groundwater with an average concentration of radioactivity of 3.34 Bq/L and $8.28{\times}10^{-5}Bq/L$ respectively, while the surface water was found to contain the same two radionuclides with mean concentrations of 0.849 Bq/L and $1.103{\times}10^{-4}Bq/L$ respectively. In addition, of the 19 samples of the groundwater, $^{137}Cs$ was found in eight of them and $^{60}Co$ was detected in ten. Of the four samples of the tap water, $^{137}Cs$ was detected in all samples and $^{60}Co$ was detected in three. Both $^{137}Cs$ and $^{60}Co$ were detected in all 12 samples of surface water. As far as $^{40}K$ is concerned, this element was detected in three of the 19 groundwater samples, but was not detected in any surface or tap water sample. In addition, the absorbed dose of $^{238}U$ from the groundwater was $7.94{\times}10^{-8}Sv/y$, while the absorbed dose of $^{232}Th$ from the surface water was $9.33{\times}10^{-13}Sv/y$. The absorbed dose of $^{137}Cs$ from the tap water was $7.33{\times}10^{-5}Sv/y$, while the absorbed dose of $^{60}Co$ from the surface water was the highest at $4.23{\times}10^{-6}Sv/y$.

Determination of the exposure conversion coefficient for 3" X 3" NaI spectrum (3" X 3" NaI 스펙트럼의 조사선량 변환계수 결정)

  • Lee, M.S.
    • Journal of Radiation Protection and Research
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    • v.26 no.2
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    • pp.73-78
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    • 2001
  • In order to find the exposure conversion coefficients for 3"X3" NaI spectrum, we measured the exposure rates with the pressurized ion chamber at 29 different areas in the range of $4{\sim}23{\mu}R\;h^{-1}$, and also measured the gamma spectra with 3"X3" and 4"X4" NaI detectors, simultaneously. The exposure conversion coefficient of the total energy method was determined using the linear relation between the measured exposure rate and the gamma spectrum energy. In order to find the exposure conversion coefficients of the energy band method, we applied the exposure conversion coefficients recommended by NCRP to the 4"X4" NaI spectra, and calculated the exposure rates due to $^{40}K,\;^{238}U$, and $^{232}Th$ series respectively. Using the linearly proportional relation between the obtained $^{232}Th$ series exposure rate and peak area of 2614 keV that represents the $^{232}Th$ series, we obtained the exposure conversion coefficients for $^{232}Th$ series. We also determined the conversion coefficients for $^{238}U$ series and $^{40}K$ using a similar method.

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