• Title/Summary/Keyword: radionuclide migration

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Radionuclide Transport Mediated by Pseudo-Colloid in the fractured Rock Media : Model Development

  • Baik, Min-Hoon;Hahn, Phil-Soo
    • Proceedings of the Korean Nuclear Society Conference
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    • 1995.05b
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    • pp.769-774
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    • 1995
  • In this study, a transport model was developed in order to analyze and predict the transport behaviors of radionuclides mediated by pseudo-colloid in the fractured rock media. It was resulted that the transport of Pu-239 was faster than Ni-63 because pseudo-colloid formation constant of Pu-239 was greater than that of Ni-63. Also, the effect of pseudo-colloid formation on the transport of a radionuclide was shown to be very significant when the apparent pseudo colloid formation constant, $K_{ap}(m^{3}/kg)$, was greater than 100. Thus, it can be concluded that acceleration of radionuclide migration may be occurred because the pseudo-colloid formation of radionuclides increases the amount of mobile components in the solution and consequently decreases the amount of radionuclides adsorbed on the stationary solid medium.

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Development of the Numerical Model for Complex Transport of Radionuclide and Colloid in the Single Fractured Rock (단일 균열암반에서 핵종/콜로이드 복합이동에 대한 수치모델 개발)

  • Lee, Sanghwa;Kim, Jung-Woo;Jeong, Jongtae
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.10 no.4
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    • pp.237-246
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    • 2012
  • In this study, numerical model for transport of radionuclide and colloid was developed. In order to solve reaction-migration governing equation for colloid and radionuclide, Strang-splitting Sequential Non-Iterative (SNI), which is one of Operator Splitting Method, was used for numerical method and this was coded by MATLAB. From the verification by comparing the simulation results with analytical solution considering only solute transport and rock diffusion, the Pearson's correlation coefficient was greater than 0.99 which demonstrates the accuracy of the model.

Radionuclide (Tc-99m) Hysterosalpingography for Evaluation of Fallopian Tube Patency (동위원소(Tc-99m HAM)를 이용한 난관 조영술)

  • Park, Won;Kim, Chong-Soon;Park, Chang-Seo
    • The Korean Journal of Nuclear Medicine
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    • v.21 no.2
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    • pp.207-211
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    • 1987
  • A prospecitive study was performed to evaluate the efficacy of Radionuclide Hysterosalpingography (RNHSG), that was modified by McCalley, et al. for the evaluation of fallopian tube. Using spontaneous migration of Tc99m labelled human albumin microsphers (HAM) and images got with Gamma camera, the study was made in 20 gynecological patients (44 tubes) in an effort to confirm the anatomical patency or obstruction as well as functional one at the Department of Obstetrics and Gynecology, National Medical Center from January 1, 1986 to July 31, 1986. The efficacy was also compared with that of contrast hysterosalpingography and surgical observation. Results obtained were as follows; 1) The Radionuclide Hysterosalpingography appeared to be a simple and accurate procedure as a mean with which anatomical tubal patency, as well as functional patency can be detected, although it's some limit in showing anatomical details of uterine cavity and tubes in comparison with contrast hysterosalpingography. 2) The predicted value of tubal obstruction was 82.4%. and that of tubal patency was 88.9% respectively. Overall efficacy (percent of tube correctly classified) of Radionuclide Hysterosalpingography was 88.6%. 3) There was no nuclide related complication during and after the procedure.

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Simulation of the Migration of 3H and 14C Radionuclides on the 2nd Phase Facility at the Wolsong LILW Disposal Center

  • Ha, Jaechul;Son, Yuhwa;Cho, Chunhyung
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.18 no.4
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    • pp.439-455
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    • 2020
  • Numerical model was developed that simulates radionuclide (3H and 14C) transport modeling at the 2nd phase facility at the Wolsong LILW Disposal Center. Four scenarios were simulated with different assumptions about the integrity of the components of the barrier system. For the design case, the multi-barrier system was shown to be effective in diverting infiltration water around the vaults containing radioactive waste. Nevertheless, the volatile radionuclide 14C migrates outside the containment system and through the unsaturated zone, driven by gas diffusion. 3H is largely contained within the vaults where it decays, with small amounts being flushed out in the liquid state. Various scenarios were examined in which the integrity of the cover barrier system or that of the concrete were compromised. In the absence of any engineered barriers, 3H is washed out to the water table within the first 20 years. The release of 14C by gas diffusion is suppressed if percolation fluxes through the facility are high after a cover failure. However, the high fluxes lead to advective transport of 14C dissolved in the liquid state. The concrete container is an effective barrier, with approximately the same effectiveness as the cover.

Characterization of Groundwater Colloids From the Granitic KURT Site and Their Roles in Radionuclide Migration

  • Baik, Min-Hoon;Park, Tae-Jin;Cho, Hye-Ryun;Jung, Euo Chang
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.20 no.3
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    • pp.279-296
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    • 2022
  • The fundamental characteristics of groundwater colloids, such as composition, concentration, size, and stability, were analyzed using granitic groundwater samples taken from the KAERI Underground Research Tunnel (KURT) site by such analytical methods as inductively coupled plasma-mass spectrometry, field emission-transmission electron microscopy, a liquid chromatography-organic carbon detector, and dynamic light scattering technique. The results show that the KURT groundwater colloids are mainly composed of clay minerals, calcite, metal (Fe) oxide, and organic matter. The size and concentration of the groundwater colloids were 10-250 nm and 33-64 ㎍·L-1, respectively. These values are similar to those from other studies performed in granitic groundwater. The groundwater colloids were found to be moderately stable under the groundwater conditions of the KURT site. Consequently, the groundwater colloids in the fractured granite system of the KURT site can form stable radiocolloids and increase the mobility of radionuclides if they associate with radionuclides released from a radioactive waste repository. The results provide basic data for evaluating the effects of groundwater colloids on radionuclide migration in fractured granite rock, which is necessary for the safety assessment of a high-level radioactive waste repository.

Soil-to-Plant Transfer Factors and Migration of Radionuclides Applied onto Soli during Growing Season of Cucumber (오이의 재배기간중 처리한 방사성 핵종의 토양;작물체간 전이계수 및 지하이동)

  • Choi, Yong-Ho;Park, Hyo-Kook;Kim, Sang-Bog;Choi, Geun-Sik;Lee, Jeong-Ho
    • Korean Journal of Environmental Agriculture
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    • v.16 no.4
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    • pp.304-310
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    • 1997
  • In greenhouse, a mixed solution of Mn-54, Co-60, Sr-85 and Cs-137 was applied to the soil of culture boxes 2 days before sowing cucumber and at 4 different times during its growth for measuring their transfer factors (TFs) for fruit and migration in soil. TFs varied with radionuclide, application time and harvest time by factor of up to about 60. Variations in TFs with application time showed different patterns among radionuclides. TFs decreased on the whole in the order of Sr-85 > Mn-54 > Co-60 > Cs-137. TFs of Mn-54, Co-60 and Cs-137 mixed with topsoil before sowing were a little higher than those for the soil-surface application made at an early growth stage while no difference in Sr-85 TF was found. After harvest, soil concentrations of the radionuclides applied at an early growth stage were examined. They decreased with increasing soil depth and 80${\sim}$99% of the radioactivity remained in the top 3cm. Soil pemeation of the radionuclides migration decreased in the order of Sr-85 > Mn-54 > Co-60 > Cs-137. The present data can be utilized in estimating radionuclide concentration in cucumber fruit, taking proper measures for its harvest and consumption and designing the best way of soil decontamination following an radioactive deposition during the cucummber growing season.

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A Theoretical Study on the Radionuclide Transport Mediated by Pseudo-Colloid in the Fractured Rock Medium (균열 암반 매질에서 의사콜로이드에 의해 매개된 방사성 핵종의 이동에 대한 이론적 연구)

  • Baik, M.H.;Hahn, P.S.;Park, H.H.
    • Nuclear Engineering and Technology
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    • v.27 no.4
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    • pp.532-543
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    • 1995
  • In this study, a transport model was developed in order to analyze and predict the transport behaviors of radionuclides mediated by pseudo-colloid in the fractured rock media. The effect of pseudo-colloid formation on the transport of a radionuclide was shown to be tory significant when an ap-parent pseudo-colloid formation constant, $A_{ap}$ (㎥/kg), os greater than 100. It was resulted from example calculations that the transport of Pu-239 was faster than Ni-63 because pseudo-colloid formation constant of Pu-239 was venter than that of Ni-63. Thus, it can be concluded that acceleration of radionuclide migration may be occurred because the pseudo-colloid formation of radionuclides increases the amount of mobile components in the solution and consequently decreases the amount of radionuclides adsorbed on the stationary solid medium.

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CRITICALITY SAFETY OF GEOLOGIC DISPOSAL FOR HIGH-LEVEL RADIOACTIVE WASTES

  • Ahn, Joon-Hong
    • Nuclear Engineering and Technology
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    • v.38 no.6
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    • pp.489-504
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    • 2006
  • A review has been made for the previous studies on safety of a geologic repository for high-level radioactive wastes (HLW) related to autocatalytic criticality phenomena with positive reactivity feedback. Neutronic studies on geometric and materials configuration consisting of rock, water and thermally fissile materials and the radionuclide migration and accumulation studies were performed previously for the Yucca Mountain Repository and a hypothetical water-saturated repository for vitrified HLW. In either case, it was concluded that it would be highly unlikely for an autocatalytic criticality event to happen at a geologic repository. Remaining scenarios can be avoided by careful selection of a repository site, engineered-barrier design and conditioning of solidified HLW. Thus, criticality safety should be properly addressed in regulations and site selection criteria. The models developed for radiological safety assessment to obtain conservatively overestimated exposure dose rates to the public may not be used directly for the criticality safety assessment, where accumulated fissile materials mass needs to be conservatively overestimated. The models for criticality safety also require more careful treatment of geometry and heterogeneity in transport paths because a minimum critical mass is sensitive to geometry of fissile materials accumulation.

Method for Evaluating Radionuclide Transport in Biosphere by Calculating Elapsed Transport Time (이동 경과 시간 계산을 이용한 생물권에서의 방사성 핵종 이동 평가 방법)

  • Ko, Nak-Youl;Ji, Sung-Hoon
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.18 no.2_spc
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    • pp.305-315
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    • 2020
  • For geological disposal of radioactive wastes, a method was proposed to evaluate the radionuclide transport in the biosphere by calculating the elapsed time of nuclide migration. The radionuclides were supposed to be introduced from a natural barrier and reached a large surface water body following a groundwater flow in a shallow subsurface. The biosphere was defined as a shallow subsurface environment that included aquifers on a host rock. Using the proposed method, a calculation algorithm was established, and a computer code that implemented the algorithm was developed. The developed code was verified by comparing the simulation results of the simple cases with the results of the analytical solution and a public program, which has been widely used to evaluate the radiation dose using the radionuclide transport near the surface. A case study was constructed using the previous research for radionuclide transport from the hypothetical geological disposal repository. In the case study, the code calculated the mass discharge rate of radionuclide to a stream in the biosphere. Because the previous research only demonstrated the transport of radionuclides from the hypothetical repository to the host rock, the developed code in the present study could help identify the total transport of radionuclide along the complete pathway.

Roles and Importance of Microbes in the Radioactive Waste Disposal (방사성폐기물 처분에서 미생물의 역할과 중요성)

  • Baik, Min-Hoon;Lee, Seung-Yeop;Roh, Yeol
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.7 no.1
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    • pp.63-72
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    • 2009
  • Recently the importance and interest for the microbes has been increased because several important results for the effects of microbes on the radioactive waste disposal have been published continuously. In this study, research status and major results on the various roles and effects of microbes in the radioactive waste disposal have been investigated. We investigated and summarized the roles and major results of microbes in a multi-barrier system consisting of an engineered barrier and a natural barrier which is considered in radioactive waste disposal systems. For the engineered barrier, we discussed about the effects of microbes on the corrosion of a waste container and investigated the survival possibility and roles of microbes in a compacted bentonite buffer. For the natural barrier, the roles of microbes present in groundwaters and rocks were discussed and summarized with major results from natural analogue studies. Furthermore, we investigated and summarized the roles and various interactions processes of microbes and their effects on the radionuclide migration and retardation including recent research status. Therefore, it is expected that the effects and roles of microbes on the radioactive waste disposal can be rigorously evaluated if further researches are carried out for a long-term behavior of the disposal system in the deep geological environments and for the effects of microbes on the radionuclide migration through geological media.

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