• Title/Summary/Keyword: radioactive isotopes

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Application of peak based-Bayesian statistical method for isotope identification and categorization of depleted, natural and low enriched uranium measured by LaBr3:Ce scintillation detector

  • Haluk Yucel;Selin Saatci Tuzuner;Charles Massey
    • Nuclear Engineering and Technology
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    • v.55 no.10
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    • pp.3913-3923
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    • 2023
  • Todays, medium energy resolution detectors are preferably used in radioisotope identification devices(RID) in nuclear and radioactive material categorization. However, there is still a need to develop or enhance « automated identifiers » for the useful RID algorithms. To decide whether any material is SNM or NORM, a key parameter is the better energy resolution of the detector. Although masking, shielding and gain shift/stabilization and other affecting parameters on site are also important for successful operations, the suitability of the RID algorithm is also a critical point to enhance the identification reliability while extracting the features from the spectral analysis. In this study, a RID algorithm based on Bayesian statistical method has been modified for medium energy resolution detectors and applied to the uranium gamma-ray spectra taken by a LaBr3:Ce detector. The present Bayesian RID algorithm covers up to 2000 keV energy range. It uses the peak centroids, the peak areas from the measured gamma-ray spectra. The extraction features are derived from the peak-based Bayesian classifiers to estimate a posterior probability for each isotope in the ANSI library. The program operations were tested under a MATLAB platform. The present peak based Bayesian RID algorithm was validated by using single isotopes(241Am, 57Co, 137Cs, 54Mn, 60Co), and then applied to five standard nuclear materials(0.32-4.51% at.235U), as well as natural U- and Th-ores. The ID performance of the RID algorithm was quantified in terms of F-score for each isotope. The posterior probability is calculated to be 54.5-74.4% for 238U and 4.7-10.5% for 235U in EC-NRM171 uranium materials. For the case of the more complex gamma-ray spectra from CRMs, the total scoring (ST) method was preferred for its ID performance evaluation. It was shown that the present peak based Bayesian RID algorithm can be applied to identify 235U and 238U isotopes in LEU or natural U-Th samples if a medium energy resolution detector is was in the measurements.

Characteristics of a Hydrogen Isotope Storage and Accountancy System (수소동위원소 저장 계량 장치 특성 연구)

  • KIM, YEANJIN;JUNG, KWANGJIN;GOO, DAESEO;PARK, JONGCHUL;JEON, MIN-GU;YUN, SEI-HUN;CHUNG, HONGSUK
    • Transactions of the Korean hydrogen and new energy society
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    • v.26 no.6
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    • pp.541-546
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    • 2015
  • Global energy shortage problem is expected to increase driven by strong energy demand growth from developing countries. Nuclear fusion power offers the prospect of an almost infinite source of energy for future generations. Hydrogen isotope storage and delivery system is a important subsystem of a nuclear fusion fuel cycle. Metal hydride is a method of the high-density storage of hydrogen isotope. For the safety storage of hydrogen isotope, depleted uranium (DU) has been widely proposed. But DU needs a safe test because It is a radioactive substance. The authors studied a small-scale DU bed and a medium-scale DU bed for the safety test. And then we made a large-scale DU bed and stored hydrogen isotopes in the bed. Before the hydriding/dehydriding, we tested it's heating and cooling properties and carried out an activation procedure. As a result, Reaction rate of DU-$H_2$ is more rapid than the other metal hydride ZrCo. Through the successful storage result of our large bed, the development possibility of the hydrogen isotope storage technology seems promising.

Evaluation of Radioactive Stack Air Effluents from the Advanced Fuel Science Building at KAERI (한국원자력연구원 새빛연료과학동 굴뚝방출 방사능 평가)

  • Chang, S.Y.;Kim, B.H.
    • Journal of Radiation Protection and Research
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    • v.33 no.3
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    • pp.121-126
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    • 2008
  • Radioactivities of the stack air effluents from the Advance Fuel Science Building (AFSB) at KAERI have been investigated and evaluated. In this AFSB, nuclear fuels for the HANARO research reactor have been fabricated and the advanced nuclear fuels have been studied. A stack air monitoring system has been continuously operating to monitor the stack air effluents from the facility to protect the environment. As the results of the periodical radioactivity measurement and both the gamma and alpha spectrometry for the millipore filters taken from the stack air monitor from January until March 2008, a trace amount of primordial $^{40}K$ and the short-lived decay products of natural borne $^{222}Rn$ and $^{220}Rn$ have been detected. However, the radioactivities have rapidly decayed to the level below the Minimum Detectable Activity (MDA) of the counting system. Therefore, it was evaluated that no uranium isotopes have been released to the atmosphere from the stack of the AFSB at KAERI.

Determining Sediment Rate Using Cesium-137 Fallout at the Larto Lake (137Cs 낙녹(落鹿)을 이용(利用)한 퇴사율(堆砂率) 측정(測定)에 관(關)하여)

  • Koh, Mun-Hwan;McHenry, J. Rogar
    • Korean Journal of Soil Science and Fertilizer
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    • v.15 no.4
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    • pp.207-212
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    • 1982
  • Soils and sediments have been uniquely tagged by radioactive isotopes as a result of nuclear test explosions in the 1950's and 1960's. Fallout $^{137}Cs$ strongly fixed to fine soil particles, was measured in sediment profiles in Larto Lake to calculate the sedimentation rate as a time dependence. The Lake sediment profiles indicated an average rate of 1.6 to 3.1 cm/yr of sediment deposition since 1958. The rate of sediment depositions clearly decreased with time. Particle size distribution in sediment was reflected almost fine particles in lake.

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Feasibility Study on Development of a Fiber-Optic Dual Detector to Measure Beta- and Gamma-rays Simultaneously (베타/감마 동시 측정용 광섬유 이중 검출기의 개발을 위한 기초연구)

  • Hong, Seunghan;Shin, Sang Hun;Sim, Hyeok In;Kim, Seon Geun;Jeon, Hyesu;Jang, Jaeseok;Kim, Jaeseok;Kwon, Guwon;Jang, Kyoung Won;Yoo, Wook Jae;Lee, Bongsoo
    • The Transactions of The Korean Institute of Electrical Engineers
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    • v.63 no.2
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    • pp.284-290
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    • 2014
  • A fiber-optic beta/gamma dual detector system with two types of sensing probes was fabricated to detect the beta- and gamma-rays simultaneously. As scintillators of the sensing probe type 1, two different inorganic scintillators, $CaF_2(Eu)$ and LYSO(Ce) crystals, were used to obtain the each scintillating efficiency with respect to beta-and gamma-rays and the inherent energy spectra of radioactive isotopes. In the case of the sensing probe type 2, which is composed of two identical inorganic scintillators and a beta shielding material based on the lead, it could discriminate beta- and gamma-rays using a subtraction method. In conclusion, we demonstrated that the proposed fiber-optic beta/gamma dual detector could measure and discriminate beta- and gamma-rays using both energy spectroscopy and subtraction method.

[ $^{99m}Tc$ ] Generator Safety Simulation Based on GEANT4 (GEANT4를 이용한 $^{99m}Tc$ Generator 안전성 시뮬레이션)

  • Kang, Sang-Koo;Han, Dong-Hyun;Kim, Chong-Yeal
    • Progress in Medical Physics
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    • v.19 no.1
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    • pp.1-8
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    • 2008
  • Technisium $(^{99m}Tc)$ is one of the most widely used radioactive isotopes for diagnosis in nuclear medicine. In general, technisium is produced inside the so called $^{99m}Tc$ generator which is usually made out of lead to shield relatively high energy radiation from $^{99}Mo$ and its daughter nuclide $^{99m}Tc$. In this paper, a GEANT4 simulation is carried out to test the safety of the $^{99m}Tc$ generator, taking the Daiichi product with radioactivity of 500 mCi as an example. According to the domestic regulation on radiation safety, the dose at 10 cm and 100 cm away from the surface of shielding container should not exceed 2.0 mSv/h and 0.02 mSv/h, respectively. The simulated dose turned out to be less than the limit, satisfying the domestic regulation.

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Diffuse Pigmented Villonodular Synovitis of the Knee: Case Report (무릎 관절의 미만형 색소 융모 활액막염: 증례 보고)

  • Choi, Sang-Gyu
    • Radiation Oncology Journal
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    • v.25 no.4
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    • pp.278-282
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    • 2007
  • Purpose: Diffuse pigmented villonodular synovitis (PVNS) is an uncommon aggressive synovial proliferative disorder of unknown etiology affecting the joint linings. Though a histologically benign inflammatory process, because of its aggressive growth with bone destruction or recurrence, it is frequently suggested to occur as a low malignant neoplasm. Optimal treatment is surgery, but the local recurrence rate after radical synovectomy for diffuse PVNS is relatively high due to the infiltrative growth pattern. External beam radiotherapy with moderate doses or intra-articular instillation of radioactive isotopes may improve the likelihood of local control and long-term function in patients with incompletely resected or recurrent diffuse PVNS. I report one case of diffuse PVNS of the right knee joint treated with arthroscopic synovectomy and external beam radiotherapy is presented.

Organ Dose Assessment of Nuclear Medicine Practitioners Using L-Block Shielding Device for Handling Diagnostic Radioisotopes (진단용 방사성동위원소 취급 시 L-block 차폐기구 사용에 따른 핵의학 종사자의 장기 선량평가)

  • Kang, Se-Sik;Cho, Yong-In;Kim, Jung-Hoon
    • Journal of radiological science and technology
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    • v.40 no.1
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    • pp.49-55
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    • 2017
  • In the case of nuclear medicine practitioners in medical institutions, a wide range of exposure dose to individual workers can be found, depending on the type of source, the amount of radioactivity, and the use of shielding devices in handling radioactive isotopes. In this regard, this study evaluated the organ dose on practitioners as well as the dose reduction effect of the L-block shielding device in handling the diagnostic radiation source through the simulation based on the Monte Carlo method. As a result, the distribution of organ dose was found to be higher as the position of the radiation source was closer to the handling position of a practitioner, and the effective dose distribution was different according to the ICRP tissue weight. Furthermore, the dose reduction effect according to the L-block thickness tended to decrease, which showed the exponential distribution, as the shielding thickness increased. The dose reduction effect according to each radiation source showed a low shielding effect in proportion to the emitted gamma ray energy level.

Fabrication and Characterization of a Fiber-Optic Alpha/Beta Detector for Nuclear Medicine Application (핵의학 적용을 위한 광섬유 기반의 알파/베타 검출기의 제작 및 특성분석)

  • Hong, Seung-Han;Yoo, Wook-Jae;Shin, Sang-Hun;Seo, Jeong-Ki;Han, Ki-Tek;Jeon, Da-Yeong;Cho, Seung-Hyun;Lee, Bong-Soo
    • Journal of Sensor Science and Technology
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    • v.21 no.5
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    • pp.367-373
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    • 2012
  • We fabricated a fiber-optic alpha/beta detector, which is composed of a sensing probe, a plastic optical fiber, a photomultiplier tube, and a multichannel analyzer, to obtain the energy spectra of radioactive isotopes. As inorganic scintillators of a sensing probe, a ZnS(Ag) film was coupled with a $CaF_2$(Eu) crystal for alpha and beta spectroscopy. In this study, $^{210}Po$ and $^{90}Sr$ were used as alpha and beta sources, respectively, and we measured the radiation energy spectra using a fiber-optic alpha/beta detector to identify alpha and beta emitting radionuclides for nuclear medicine application. Also, the variations of energy spectrum were obtained according to the length of plastic optical fiber.

Separation and Purification for the Determination of Zirconium and Its Isotopes in PWR Spent Nuclear Fuels (PWR 사용후핵연료 중 Zr 및 Zr 동위원소 정량을 위한 분리 및 정제)

  • Kim, Jung Suk;Jeon, Young Shin;Park, Yong Joon;Lee, Chang Heon;Kim, Won Ho
    • Analytical Science and Technology
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    • v.11 no.6
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    • pp.421-428
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    • 1998
  • A method has been studied to separate Zr from various fission products in PWR spent nuclear fuels. A solution containing metal ions in place of radioactive fission products was prepared. The Zr was separated with 5 M HCl followed by eluting metal ions such as Ce, Nd, Cs, Rb, Ba, Sr, Ru, Rh, Pd, Ag and Cd with 12 M HCl on Dowex $1{\times}8$, anion exchange resin. The recovery of Zr was more than 95%. The purification of Zr was carried out on anion exchange resin, Dowex $1{\times}8$, in 5 M HCl in order to remove Mo causing isobaric effect during mass spectrometry. The method was applied to separate Zr from a spent PWR fuel. From mass spectrometric measurement, the purified Zr portion was not showed the isobars from other elements such as Mo and Sr.

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