• Title/Summary/Keyword: natural radioactive materials

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Hydrochemistry and Occurrences of Natural Radioactive Materials from Groundwater in Various Geological Environment (다양한 지질환경에서 지하수의 수리화학 및 자연방사성물질 산출특성)

  • Jeong, Chan Ho;Lee, Yu Jin;Lee, Yong Cheon;Kim, Moon Su;Kim, Hyun Koo;Kim, Tae Seong;Jo, Byung Uk;Choi, Hyeon Young
    • The Journal of Engineering Geology
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    • v.26 no.4
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    • pp.531-549
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    • 2016
  • The purpose of this study is to analyze the relationship of hydrochemistry, geology, fault with occurrence of uranium and radon-222 from the groundwater in the Yeongdong area. In this study, 49 groundwater and 4 surface water samples collected in the study area were collected on two separate occasions. The surface radioactivities were measured at 40 points to know the relationship between the occurrence of uranium in groundwater and surface geology. The chemical composition of groundwater showed three types : $Ca-HCO_3$, $Na-HCO_3$ and $Ca-HCO_3(SO_4,\;NO_3)$. Two groundwater of 49 samples exceeded the maximum contaminant levels of uranium, $30{\mu}g/L$, proposed by the Ministry of Environment of Korea and 11 groundwater of 40 samples for Rn-222 concentrations exceeded the 148 Bq/L maximum contaminant level of US EPA. Most of unsuitable groundwater are located in the geological boundary related with the biotite gneiss and the surface radioactivities of rock samples showed no relationship with groundwater geochemical constituents. The strike-slip fault, Youngdong fault, is $N45^{\circ}E$ direction and the high concentrations of uranium in upper part of fault, consisted of granite and granitic gneiss are detected but in lower part, consisted of metamorphic sedimentary rock are not detected. It suggests that the natural radioactive concentrations are related with the geologic characteristics and the migration and diffusion of natural radioactive materials are affected by the fault.

Volume Reduction of Radioactive Liquid Waste by Pervaporation Method (투과증발법에 의한 방사성폐액의 감용)

  • Kang, Young-Ho;Kwon, Seon-Gil;Yang, Yeong-Seok;Hwang, Sung-Tai;Chang, In-Soon
    • Applied Chemistry for Engineering
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    • v.3 no.2
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    • pp.327-334
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    • 1992
  • As a promising method for the volume reduction of the low-level liquid waste, the pervaporation process was studied using a cellulose acetate membrane. Experimental results showed that the pervaporation method, usually applied to separation of organic materials, has a good decontamination effect for the volume reduction of liquid waste and the evaporation rate of water in this process was markedly faster than that of natural evaporation method, a wide-used process for the volume reduction of liquid waste. Depending on the feed solution conditions, the pervaporation characteristics were evaluated by the experimental results and the optimum conditions for preparation of the cellulose acetate membrane were established to increase the pervaporation flux through the membrane.

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Sensitivity Analysis of Thermal Parameters Affecting the Peak Cladding Temperature of Fuel Assembly

  • Ju-Chan Lee;Doyun Kim;Seung-Hwan Yu;Sungho Ko
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.21 no.3
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    • pp.359-370
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    • 2023
  • The thermal integrity of spent nuclear fuels has to be maintained during their long-term dry storage. The detailed temperature distributions of spent fuel assemblies are essential for evaluating the integrity of their dry storage systems. In this study, a subchannel analysis model was developed for a canister of a single fuel assembly using the COBRA-SFS code. The thermal parameters affecting the peak cladding temperature (PCT) of the spent fuel assembly were identified, and sensitivity analyses were performed based on these parameters. The subchannel analysis results indicated the presence of a recirculation flow, based on natural convection, between the fuel assembly and downcomer region. The sensitivity analysis of the thermal parameters indicated that the PCT was affected by the emissivity of the fuel cladding and basket, convective heat transfer coefficient, and thermal conductivity of the fluid. However, the effects of the wall friction factor of the canister, form loss coefficient of the grid spacers, and thermal conductivities of the solid materials, on the PCT were predominantly ignored.

Gamma-ray Exposure Rate Monitoring by Energy Spectra of NaI(Tl) Scintillation detectors

  • Lee, Mo Sung
    • Journal of Radiation Protection and Research
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    • v.42 no.3
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    • pp.158-165
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    • 2017
  • Background: Nuclear facilities in South Korea have generally adopted pressurized ion chambers to measure ambient gamma ray exposure rates for monitoring the impact of radiation on the surrounding environment. The rates assessed with pressurized ion chambers do not distinguish between natural and man-made radiation, so a further step is needed to identify the cause of abnormal variation. In contrast, using NaI(Tl) scintillation detectors to detect gamma energy rates can allow an immediate assessment of the cause of variation through an analysis of the energy spectra. Against this backdrop, this study was conducted to propose a more effective way to monitor ambient gamma exposure rates. Materials and Methods: The following methods were used to analyze gamma energy spectra measured from January to November 2016 with NaI detectors installed at the Korea Atomic Energy Research Institute (KAERI) dormitory and Hanbat University. 1) Correlations of the variation of rates measured at the two locations were determined. 2) The dates, intervals, duration, and weather conditions were identified when rates increased by $5nSv{\cdot}h^{-1}$ or more. 3) Differences in the NaI spectra on normal days and days where rates spiked by $5nSv{\cdot}h^{-1}$ or more were studied. 4) An algorithm was derived for automatically calculating the net variation of the rates. Results and Discussion: The rates measured at KAERI and Hanbat University, located 12 kilometers apart, did not show a strong correlation (coefficient of determination = 0.577). Time gaps between spikes in the rates and rainfall were factors that affected the correlation. The weather conditions on days where rates went up by $5nSv{\cdot}h^{-1}$ or more featured rainfall, snowfall, or overcast, as well as an increase in peaks of the gamma rays emitted from the radon decay products of $^{214}Pb$ and $^{214}Bi$ in the spectrum. This study assumed that $^{214}Pb$ and $^{214}Bi$ exist at a radioactive equilibrium, since both have relatively short half-lives of under 30 minutes. Provided that this assumption is true and that the gamma peaks of the 352 keV and 1,764 keV gamma rays emitted from the radionuclides have proportional count rates, no man-made radiation should be present between the two energy levels. This study proved that this assumption was true by demonstrating a linear correlation between the count rates of these two gamma peaks. In conclusion, if the count rates of these two peaks detected in the gamma energy spectrum at a certain time maintain the ratio measured at a normal time, such variation can be confirmed to be caused by natural radiation. Conclusion: This study confirmed that both $^{214}Pb$ and $^{214}Bi$ have relatively short half-lives of under 30 minutes, thereby existing in a radioactive equilibrium in the atmosphere. If the gamma peaks of the 352 keV and 1,764 keV gamma rays emitted from these radionuclides have proportional count rates, no man-made radiation should exist between the two energy levels.

Pore Characterisitics and Adsorption Performance Evaluation of Magnesium Oxide Matrix by Active Carbon Particle Size (활성탄소 입도에 따른 산화마그네슘 경화체의 공극특성과 흡착성능 평가)

  • Pyeon, Su-Jeong;Lee, Sang-Soo
    • Journal of the Korea Institute of Building Construction
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    • v.18 no.1
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    • pp.59-65
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    • 2018
  • Radon gas is a colorless, odorless, tasteless gas that occurs when uranium, a natural radioactive material in rocks and soils, collapses. 85% of the annual radiation exposure of the human body is due to natural radiation, of which 50% is radon. According to the US Environmental Protection Agency (EPA) survey, 62 out of 1,000 smokers and 7 out of 1,000 nonsmokers are exposed to lung cancer when exposed to radon gas for a long time. In order to reduce the risk of radon gas, activate carbon was used to fabricate matrix, and the pore properties and radon reduction properties were investigated. When the activate carbon was used, the radon gas concentration was drastically reduced and the graph was changed as the measurement period became longer. The pore distribution and microporous properties, which are one of the material properties of activate carbon, can be grasped.

Impact of Nuclear Tests on Deforestation in North Korea using Google Earth-Based Spatial Images

  • Ki, Junghoon;Sung, Minki;Choi, Choongik
    • Journal of People, Plants, and Environment
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    • v.22 no.6
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    • pp.563-573
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    • 2019
  • The North Korean government conducted its first nuclear test in 2006 and more recently the sixth nuclear test on September 3, 2017. In order to identify how North Korea's nuclear tests have affected the environment, a scientific approach is required. Although North Korea's nuclear tests and their environmental destruction are not a severe threat to the environment of the Korean Peninsula at this time, identifying environmental damage and taking countermeasures in advance are essential to minimize their potential threats to the environments. The purpose of this study is to study the environmental impact of North Korea's nuclear tests using Google Earth image analysis. As a method of the study, we compare Google Earth images taken before and after each nuclear test was conducted in North Korea. To overcome limitations of the suggested comparison method, we cross-checked our results with those of previous scientific research. After the 1st-3rd nuclear tests, green spaces were found to be considerably reduced. In particular, when comparing the Google Earth images before and after the second nuclear test, some ground subsidences were observed. Such subsidences can cause tunnels on the mountainsides and cracks in rocks around the mountains, leading to the release of radioactive materials and contaminating groundwater. Besides, after the 4th-6th nuclear tests, decay and deforestation were observed not in the nuclear test sites, but in their surrounding areas. Especially after the 5th and 6th nuclear tests, the topography and the forests of the surrounding areas were severely damaged. In relation to North Korea's nuclear tests and their impact on the natural environment, we need to prepare various policy measures to reduce North Korea's environmental pollution and natural environment destruction. Those policy measures include the establishment of various cooperative governance between the Korean government, the private sector, the academia, NGOs, and international organizations.

Sorption of aqueous uranium(VI) ion onto a cation-exchangeable K-birnessite colloid (양이온 교환능을 갖는 K-Birnessite 콜로이드에 의한 수용성 우라늄(VI) 이온의 흡착 연구)

  • Kang, Kwang-Cheol;Kim, Seung-Soo;Baik, Min-Hoon;Kwon, Soo-Han;Rhee, Seog-Woo
    • Analytical Science and Technology
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    • v.23 no.6
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    • pp.566-571
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    • 2010
  • This paper describes the sorption behaviors of aqueous uranium ions on the K-birnessite. K-birnessite was synthesized by adding a concentrated HCl to an aqueous solution of $KMnO_4$. Physicochemical characteristics of the K-birnessite, such as structure, specific surface area and surface charge, were investigated. K-birnessite is a layered material and the $K^+$ ions exist in the interlayer of layered K-birnessite. BET specific surface area of the K-birnessite was 38.30 m2/g. The surface charge of K-birnessite was $-1.65\;C/m^2$ at pH 5.00 and ionic strength of 0.010 M $NaClO_4$, at which the sorption experiments of uranium ions were carried out. Uranium ions were incorporated into the interlayer of the K-birnessite by cation-exchange reaction with $K^+$ ions, and the distribution coefficient is quite similar to those of common ion-exchange materials. The results might be applicable in the retardation of migration of radioactive materials from the underground disposal site of high-level radioactive waste.

Establishment of the Physicochemical and Radiological Database of Raw Materials and By-Products in Domestic Distribution (국내 유통중인 원료물질 및 공정부산물의 물리화학적 및 방사선적 특성 데이터베이스 구축)

  • Lim, Chung-Sup;Lim, Jong-Myoung;Park, Ji-Young;Chung, Kun Ho;Kim, Chang-Jong;Chang, Byung-Uck;Ji, Young-Yong
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.14 no.4
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    • pp.331-341
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    • 2016
  • To evaluate the physicochemical and radiological properties of raw materials and by-products in domestic distribution, about 220 samples with 16 species were prepared. We measured the energy spectrum and the chemical content, such as U, Th, and K, using a $LaBr_3$ scintillation detector and ED-XRF. In addition, HPGe detector was used to analyze the radioac-tivity of $^{234}Th$, $^{234}mPa$, and $^{214}Bi$ in uranium decay series and $^{228}Ac$, $^{212}Pb$, and $^{208}Tl$ in thorium decay series, and $^{40}K$. The correlation between characteristic variables, such as the count rate in several ROIs, chemical content, and radioactivity, was assessed to infer the radioactivity of natural radionuclides through a rapid screening method. Based on the results, a characteristic database for raw material and by-product in domestic distribution was established and it will provide useful information in the analysis procedure and improve the accuracy and reproducibility in the analysis of natural radionuclides.

Assessment of Physicochemical Properties of Domestic Bentonite and Zeolite as Candidate Materials for a Engineered Barrier in a Radwaste Repository (방사성폐기물 처분장 공학방벽 재료로서의 국산 벤토나이트 및 제올라이트에 대한 물리화학적 특성 평가)

  • 정찬호
    • The Journal of Engineering Geology
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    • v.9 no.2
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    • pp.89-100
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    • 1999
  • This study was carried out to assess the physicochemical properties of domestic bentonites and zeolites from Tertiary Formation as the candidate material for a engineered barrier of a radioactive waste repository. Natural bentonite and zeolite samples were collected from nine bentonite mines and six zeolite mines in Yeonil-Gampo area. The commercial products of bentonite and zeolite were obtained from local companies. The collected samples were investigated to study the following physicochemical properties: X-ray diffraction patterns, swelling, cation exchange capacity(CEC), specific surface area, montmorillonite content, pH, organic carbon content, thermal property, microstruciure and chemical composition. Based on the physicochemical properties of bentonite and zeolite, the bentonites from U-41 and G-46 mines and the zeolites from Daedo and Y-1 mines are regarded as the most desirable candidate materials.

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Case Study of Radiation Protection and Radiation Exposure (방사능 노출과 방사선 보호 사례 연구)

  • Young Sil Min
    • Advanced Industrial SCIence
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    • v.2 no.3
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    • pp.1-7
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    • 2023
  • Recently, it is increasing that a issue of concern about radiation exposure. It affects soil, water, air, crops, etc., and in the long term, environmental pollution and food pollution occur, and it is considered to cause social problems and economic damage. Radiation exposure causes diseases and health problems, but as a method for diagnosing diseases, nuclear medicine tests such as X-ray imaging, CT, and PET-CT are conducted, and radiation isotopes are exposed for the purpose of cancer treatment. A Hungarian case study on radiation in water, particularly drinking water, following the release of radioactive waste from Fukushima, and an examination of the Larsemann Hills area in Antarctica, found that it was within the prescribed radioactivity limits of drinking water recommended by the World Health Organization. We looked at radioprotective agents, focusing on DNA damage, cell and organ damage, and cancer, and also investigated various literatures on ACE inhibitors, antioxidants, and natural substances among restoration materials. Although exposed to radiation in everyday life, the reason why it can be safe is probably because there is a radiation protection material and a recovery material for radiation exposure, so we are trying to find possible materials.