• 제목/요약/키워드: fine aerosols

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라만-탄성 라이다를 이용한 황사 및 오염 에어러솔의 라이다 비 측정 연구 (Measurements of the Lidar Ratio for Asian Dust and Pollution Aerosols with a Combined Raman and Back-scatter Lidar)

  • 윤순창;이영지;김상우;김만해
    • 대기
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    • 제20권4호
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    • pp.483-494
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    • 2010
  • The vertical profiles of the extinction coefficient, the backscatter coefficient, and the lidar ratio (i.e., extinction-to-backscattering ratio) for Asian dust and pollution aerosols are determined from Raman (inelastic) and elastic backscatter signals. The values of lidar ratios during two polluted days is found between 52 and 82 sr (July 22, 2009) and 40~60 sr (July 31, 2009) at 52 nm, with relatively low value of particle depolarization ratio (<5%) and high value of sun photometer-derived Angstrom exponent (> 1.2). However, lidar ratios between 25 and 40 sr are found during two Asian dust periods (October 20, 2009 and March 15, 2010), with 10~20% of particle depolarization ratio and the relatively low value of sun photometer-derived Angstrom exponent (< 0.39). The lidar ratio, particle depolarization ratio and color ratio are useful optical parameter to distinguish non-spherical coarse dust and spherical fine pollution aerosols. The comparison of aerosol extinction profiles determined from inelastic-backscatter signals by the Raman method and from elastic-backscatter signals by using the Fernald method with constant value of lidar ratio (50 sr) have shown that reliable aerosol extinction coefficients cannot be determined from elastic-backscatter signals alone, because the lidar ratio varies with aerosol types. A combined Raman and elastic backscatter lidar system can provide reliable information about the aerosol extinction profile and the aerosol lidar ratio.

Comparison of Chemical Compositions of Size-segregated Atmospheric Aerosols between Asian Dust and Non-Asian Dust Periods at Background Area of Korea

  • Kim, Won-Hyung;Song, Jung-Min;Ko, Hee-Jung;Kim, Jin Seog;Lee, Joung Hae;Kang, Chang-Hee
    • Bulletin of the Korean Chemical Society
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    • 제33권11호
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    • pp.3651-3656
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    • 2012
  • The size-segregated atmospheric aerosols have been collected at 1100 m site of Mt. Halla in Jeju, a background area in Korea, using 8-stage cascade impact air sampler during Asian dust and non-Asian dust storm periods. Their ionic and elemental species were analyzed, in order to examine the pollution characteristics and composition change between Asian dust and non-Asian dust periods. The major ionic species such as nss-$SO_4{^{2-}}$, $NH_4{^+}$, and $K^+$ were predominantly distributed in the fine particles (below $2.1{\mu}m$ diameter), and besides the $NO_3{^-}$ was distributed more in coarse particle fraction than fine particle. On the other hand, the typical soil and marine species i.e., nss-$Ca^{2+}$, $Na^+$, $Cl^-$, and $Mg^{2+}$, were mostly existed in the coarse particles (over $2.1{\mu}m$ diameter). As well in the elemental analysis of aerosols, the major soil-originated Al, Fe, Ca, and others showed prominently high concentrations in the coarse particle fraction, whereas the anthropogenic S and Pb were relatively high in the fine particle fraction. From the comparison of aerosol compositions between Asian dust and non-Asian dust periods, the concentrations of the soil-originated species such as nss-$Ca^{2+}$, Al, Ca, Fe, Ti, Mn, Ba, Sr have increased as 2.7-4.2 times during the Asian dust periods. Meanwhile the concentrations of nss-$SO_4{^{2-}}$ and $NO_3{^-}$ have increased as 1.4 and 2.0 times, and on the contrary $NH_4{^+}$ concentrations have a little bit decreased during the Asian dust periods. Especially the concentrations of both soil-originated ionic and elemental species increased noticeably in the coarse particle mode during the dust storm periods.

Aerosol Observation with Raman LIDAR in Beijing, China

  • Xie, Chen-Bo;Zhou, Jun;Sugimoto, Nobuo;Wang, Zi-Fa
    • Journal of the Optical Society of Korea
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    • 제14권3호
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    • pp.215-220
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    • 2010
  • Aerosol observation with Raman LIDAR in NIES (National Institute for Environmental Studies, Japan) LIDAR network was conducted from 17 April to 12 June 2008 over Beijing, China. The aerosol optical properties derived from Raman LIDAR were compared with the retrieved data from sun photometer and sky radiometer observations in the Aerosol Robotic Network (AERONET). The comparison provided the complete knowledge of aerosol optical and physical properties in Beijing, especially in pollution and Asian dust events. The averaged aerosol optical depth (AOD) at 675 nm was 0.81 and the Angstrom exponent between 440 nm and 675 nm was 0.99 during experiment. The LIDAR derived AOD at 532 nm in the planetary boundary layer (PBL) was 0.48, which implied that half of the total AOD was contributed by the aerosol in PBL. The corresponding averaged LIDAR ratio and total depolarization ratio (TDR) were 48.5sr and 8.1%. The negative correlation between LIDAR ratio and TDR indicated the LIDAR ratio decreased with aerosol size because of the high TDR associated with nonspherical and large aerosols. The typical volume size distribution of the aerosol clearly demonstrated that the coarse mode radius located near 3 ${\mu}m$ in dust case, a bi-mode with fine particle centered at 0.2 ${\mu}m$ and coarse particle at 2 ${\mu}m$ was the characteristic size distribution in the pollution and clean cases. The different size distributions of aerosol resulted in its different optical properties. The retrieved LIDAR ratio and TDR were 41.1sr and 19.5% for a dust event, 53.8sr and 6.6% for a pollution event as well as 57.3sr and 7.2% for a clean event. In conjunction with the observed surface wind field near the LIDAR site, most of the pollution aerosols were produced locally or transported from the southeast of Beijing, whereas the dust aerosols associated with the clean air mass were transported by the northwesterly or southwesterly winds.

12-year LIDAR Observations of Tropospheric Aerosol over Hefei (31.9°N, 117.2°E), China

  • Wu, Decheng;Zhou, Jun;Liu, Dong;Wang, Zhenzhu;Zhong, Zhiqing;Xie, Chenbo;Qi, Fudi;Fan, Aiyuan;Wang, Yingjian
    • Journal of the Optical Society of Korea
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    • 제15권1호
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    • pp.90-95
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    • 2011
  • 12-year LIDAR observations of tropospheric aerosol vertical distribution using a Mie scattering LIDAR in Hefei ($31.9^{\circ}N$, $117.2^{\circ}E$) from 1998 to 2009 are presented and analyzed in this paper. Characters of temporal variation and vertical distribution of tropospheric aerosol over Hefei are summarized from the LIDAR measurements. The impacts of natural source and human activities on the aerosol vertical distribution over Hefei could be seen clearly. Dust particles from the north in spring could affect the aerosol distributions below about 12 km over Hefei, and aerosol scale height in April reaches $2.29{\pm}0.68\;km$. Both LIDAR measurements and surface visibility imply that aerosols in the lower troposphere have been increasing since about 2005.

우리 나라 배경농도지역의 1996~1997년 미세입자상 탄소성분 측정 결과 (Measurement of Carbonaceous Species in Fine Particles at the Background Sites in Korea During 1996 and 1997)

  • 김용표;이종훈
    • 한국대기환경학회지
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    • 제14권6호
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    • pp.621-630
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    • 1998
  • The concentrations of organic carbon (OC) and elemental carbon (EC) in fine aerosols were determined from the samples collected at the two background sites of Kosan in Cheju Island and Kangwha. Samplings were carried out during the spring and winter of 1996 and the fall and winter of 1997. PM25 particles were collected on the prefired quartz filters for 24 hours and analyzed by the selective thermal oxidation method. The concentrations of OC at the sites were higher than those commonly observed from clean areas around the world, but those of EC at both sites were lower than, or comparable to, other clean areas in the world. Both the OC and EC levels at Kangwha were higher than those at Kosan. According to backward trajectory analysis, most air pollutants collected at the two sites were from China. It was found that the OC and EC concentrations in air masses from southern China were higher than those from northern China.

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COASTAL ENVIRONMENT MONITORING USING ADJACENT EFFECT OF RADIATION

  • Takashima, Tsutomu;Jung, Sung-Chul;Yi, San-Oh;Kim, Tu-Hwan
    • 대한원격탐사학회:학술대회논문집
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    • 대한원격탐사학회 2006년도 Proceedings of ISRS 2006 PORSEC Volume I
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    • pp.430-431
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    • 2006
  • KOMPSAT-2 was successively launched on July 28,06. She carries Fine Spatial Resolution Sensor with three channels. It is 4m monochromatic and 1m panchromatic. The main purposes would derive fine urban map and digital elevation model(DEM).Therefore we extend to coastal environment monitoring using the adjacent effect of radiation due to an interaction of radiation between heterogeneous surface and atmosphere. With data analysis of ASTER on TERA, which is 15m resolution in visible and near infrared wavelengths, we found atmospheric aerosols were always large. Note that data analysis was limited in Nagoya bay, Lake Tahoe, California & La Pozuelos, La Picasa, Argentina. Thus this time we expect data analyses around isolated island and peninsula in west and south coast of Korea.

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1993년 8월의 서울지역 시정 연구 (Visibility study in Seoul in Aug., 1993.)

  • 이종훈;백남준;김용표;문길주
    • 한국대기환경학회지
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    • 제11권3호
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    • pp.291-298
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    • 1995
  • An intensive field study was carried out during Aug. 1993 in Seoul to study the characteristics of summertime visibility and diurnal trend of ionic composition of ambient particles. A transmissometer, nephelometer with heated and unheated inlets, PM3 fine particle sampler, and cascade impactor were used to measure optical and particle properties of ambient air. During this study period, a weak smog episode has occurred. Light scattering by particles is the most dominant factor on total light extinction. The effect of light absorption by particles in Seoul is much higher than other major cities in U.S.A. throughout the summer and fall with relatively constant values. The effect of water on $b_{sp}$ was small during the period. The particle size distribution shows a typical bimodal one. Sulfate, ammonium, chloride, and nitrate are the major chemical species in fine fraction aerosols, about 30% of toral mass concentration. Concentraion of sulfate is higher during the daytime while those of nitrate and chloride are higher during the nighttime. Ammonium concentration is constant through the daytime.

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대기에어로졸중 음이온성분에 대한 입경분포의 변화특성 (Characterization of Size distribution of Anion Species in Atmospheric Aerosols)

  • 최금찬;박정호;임경택
    • 한국대기환경학회지
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    • 제10권2호
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    • pp.124-129
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    • 1994
  • Aerosol size distribution was determined using Anderson sampler for the anions( sulfate nitrate and chloride ) and TSP. Ionic species concentration and size distribution have been investigated in the daytime and nightime individually. Size classified samples were extracted with distilled water and analyzed for C $l^{[-10]}$ , N $O_3$$^{[-10]}$ and S $O_4$$^{2-}$, by ion chromatography. The size distribution of these ions and TSP was analyzed to investigate the seasonal and diurnal variation of concentrations as follows: (1)Size distribution of TSP showed bi- modal type in the daytime, but indicated tri-mode distribution in the nightime without any seasonal variation. (2)Sulfate concentrations were higher in fine- mode both in the daytime and nightime but fraction of sulfate was higher in coarse-mode during the Yellow Sand Period. (3)Nitrate and Chloride ions are dominant in fine-mode in winter while dominant in coarse-mode in the summer.

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Variation in chemical composition of Asian dusts on Jeju Island related to their inflow pathways during 2010-2015

  • Song, Jung-Min;Bu, Jun-Oh;Ko, Hee-Jung;Kim, Won-Hyung;Kang, Chang-Hee
    • 분석과학
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    • 제30권4호
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    • pp.182-193
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    • 2017
  • In order to examine the variation characteristics of chemical compositions in relation to the inflow pathways of Asian dust, $PM_{10}$ and $PM_{2.5}$ aerosols were collected at Gosan site of Jeju Island during the Asian dust days between 2010 and 2015, and their chemical compositions were analyzed. The mean mass concentrations of $PM_{10}$ and $PM_{2.5}$ during Asian dust days were $130.0{\pm}90.2$ and $38.2{\pm}24.7{\mu}g/m^3$, respectively. The composition ratios of major secondary pollutants ($nss-SO_4{^{2-}}$, $NH_4{^+}$, $NO_3{^-}$) were high as 53.7 % for $PM_{10-2.5}$ and 90.6 % for $PM_{2.5}$. When the Asian dusts had been transported to the Korean Peninsula via Loess Plateau of central China, the concentrations of $nss-Ca^{2+}$, $NH_4{^+}$, $nss-SO_4{^{2-}}$, and $NO_3{^-}$ increased more noticeably. Whereas in case when the inflow pathways of Asian dust had been through the Bohai bay, the concentrations of the crustal species such as Al, Fe, and Ca were relatively high in coarse particles. The atmospheric aerosols were acidified largely by sulfuric and nitric acids. They were neutralized mainly by calcium carbonate in coarse particle mode passed through Manchuria area, but by ammonia in fine particle mode passed through Loess plateau and Bohai bay. Ammonium salts are assumed to exist as ammonium sulfate and ammonium nitrate in coarse particles, but mostly as ammonium sulfate in fine particles.

GOCI 자료를 이용한 서울 지역 고농도 미세먼지와 옅은 황사 시 에어로졸 광학적 특성 분석 (Analysis of Aerosol Optical Properties for High Particulate Matters and Light Asian Dust in Seoul Using GOCI)

  • 김덕래;최원준;최명제;김지영;조아라;김상균;김준;문경정
    • 한국대기환경학회지
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    • 제33권3호
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    • pp.233-240
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    • 2017
  • To distinguish between high particulate matter (HPM) and light Asian dust (LAD) events, aerosol optical properties from GOCI were investigated in Seoul from 2014 to 2016. The poor air quality case caused by fine atmospheric particulate matter (i.e., 80<$PM_{10}$<$400{\mu}g/m^3$) is clearly separated from the case of heavy Asian dust that generally shows the $PM_{10}$ concentration more than $400{\mu}g/m^3$. In this study, we have found eight cases for the poor air quality and divided them into the two events(i.e., HPM and LAD). In case of aerosol optical depth (AOD), there was no big difference between two events. However, Angstrom exponent (AE) for HPM events was greater than 1, while that for LAD events less than 1. As a result of comparing aerosol type, non-absorbing fine mode aerosols were dominant for HPM events, but coarse and absorbing coarse mode aerosols for LAD events. Therefore, AE and aerosol type from GOCI can be used to distinguish between two events effectively.