• Title/Summary/Keyword: Weathering Half-Life

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Mass Interception Fractions and Weathering Half-lives of Iodine-131 and Radiocesium in Leafy Vegetables Observed after the Fukushima Daiichi Nuclear Power Plant Accident

  • Tagami, Keiko;Uchida, Shigeo
    • Journal of Radiation Protection and Research
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    • v.46 no.4
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    • pp.178-183
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    • 2021
  • Background: This study was carried out to provide environmental transfer parameter values to estimate activity concentrations of these radionuclides in agricultural crops when direct contamination occurred. Materials and Methods: Mass interception fractions (FBs) and weathering half-lives (Tws) of 131I and radiocesium were calculated using openly available monitoring data obtained after the Fukushima Daiichi Nuclear Power Plant accident. FB is the ratio between the initial radioactivity concentration of a radionuclide retained by the edible part of the plant (Bq·kg-1 fresh weight [FW]) and the amount of deposited radionuclide in that area (Bq·m-2). Tw values can be calculated using activity concentrations of crops decreased with time after the initial contamination. Results and Discussion: Calculated FB and Tw values for 131I and radiocesium were mostly obtained for leafy vegetables. The analytical results showed that there was no difference of FBs between 131I and radiocesium by t-test; geometric mean values for leafy vegetables cultivated under outdoor conditions were 0.058 and 0.12 m2·kg-1 FW, respectively. Geometric mean Tw value of 131I in leafy vegetables grown under outdoor conditions was 8.6 days, and that of radiocesium was 6.6 days; there was no significant difference between Tw values of these radionuclides by Wilcoxon rank sum test. Conclusion: There was no difference between 131I and radiocesium for FBs and Tws. By using these factors, we would be able to carry out a rough estimation of the activity concentrations of 131I and radiocesium in the edible part of leafy crops when a nuclear accident occurred.

Study on the Illite Modification for Removal of Radioactive Cesium in Water Environment near Nuclear Facilities (원자력 시설 인근 수계에서 방사성 세슘 제거를 위한 일라이트 개질 연구)

  • Hwang, Jeonghwan;Choung, Sungwook;Shin, Woosik;Han, Weon Shik
    • Economic and Environmental Geology
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    • v.51 no.2
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    • pp.113-120
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    • 2018
  • Radioactive cesium($^{137}Cs$) can be released into the environment through severe nuclear accidents such as the Chernobyl and Fukushima, The $^{137}Cs$ is one of major monitoring radionuclides due to its chemical toxicity, ${\gamma}$ radiation and long half-life($t_{1/2}=30.2yrs$). It has been known well that illite adsorb selectively and strongly the cesium due to frayed edge sites. The quantity of the FES in the illite could be controlled by weathering processes. Therefore, this study was modified illite samples through artificial weathering in the laboratory to increase sorption efficiency for cesium. Abundant interlayer cations(i.e., K, Ca) were eluted within 1 day, while Si and Al were gradually released from the crystal structure. In addition, broad peaks of XRD indicated the occurrence of chemical weathering. The cesium sorption distribution coefficients increased up to approximately 2 times after the weathering. These results suggested that sorption capacity of illite could be enhanced for cesium through artificial weathering under low temperature.

Sensitivity Analysis for Input Parameters of a Radiological Dose Assessment Model (U. S. NRC Model) for Ingestion Pathways (오염 음식물에 의한 피폭선량 평가모델 (U. S. NRC 모델)의 입력변수에 대한 민감도분석)

  • Hwang, Won-Tae;Suh, Kyung-Suk;Kim, Eun-Han;Choi, Young-Gil;Han, Moon-Hee
    • Journal of Radiation Protection and Research
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    • v.25 no.4
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    • pp.233-239
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    • 2000
  • The sensitivity analysis of input parameters was Performed fer an ingestion dose assessment model (U. S. NRC's Regulatory Guide 1.109 model) from routine releases of radionuclides. In this study, three kinds of typical Korean foodstuffs (rice, leaff vegetables, milk) and two kinds of radionuclides $(^{l37}Cs,\;^{131}I)$ were considered. The values of input parameters were sampled using a Latin hypercube sampling technique based on Monte Carlo approach. Sensitivity indices, which represent the influence or the importance of input parameters for predictive results, were quantitatively expressed by the partial rank correlation coefficients. As the results, the ratio of the interception fraction to the yield of agricultural plants and the human consumption rate were sensitive input parameters for the considered foodstuffs and radionuclides. Additionally, in case of milk, the transfer factor of radionuclides from animal intake to milk and the daily intake rate of feedstuffs were sensitive input parameters. The weathering removal half-life and the delay time from food production to human consumption were relatively sensitive for $^{137}Cs$ and $^{131}I$ depositions, respectively.

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