• Title/Summary/Keyword: Uranium and radon

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Measurement and Spatial Analysis of Uranium-238 and Radon-222 of Soil in Seoul

  • Oh, Dal-Young;Shin, Kyu-Jin;Jeon, Jae-Sik
    • Journal of Soil and Groundwater Environment
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    • v.22 no.1
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    • pp.33-40
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    • 2017
  • Identification of radon in soil provides information on the areas at risk for high radon exposure. In this study, we measured uranium-238 and radon-222 concentrations in soil to assess their approximate levels in Seoul. A total of 246 soil samples were taken to analyze uranium with ICP-MS, and 120 measurements of radon in soil were conducted with an in-situ radon detector, Rad7 at a depth of 1-1.5 m. The data were statistically analyzed and mapped, layered with geological classification. The range of uranium in soil was from 0.0 to 8.5 mg/kg with a mean value of 2.2 mg/kg, and the range of radon in soil was from 1,887 to $87,320Bq/m^3$ with a mean value of $18,271Bq/m^3$. The geology had a distinctive relationship to the uranium and radon levels in soil, with the uranium and radon concentrations in soils overlying granite more than double those of soils overlying metamorphic rocks.

Distribution Characteristics of Uranium and Radon Concentration in Groundwaters of Provinces in Korea (지역별 지하수중 우라늄과 라돈의 함량 분포 특성)

  • Jeong, Do-Hwan;Kim, Moon-Su;Ju, Byoung-Kyu;Kim, Tae-Seung
    • Journal of Soil and Groundwater Environment
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    • v.16 no.6
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    • pp.143-149
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    • 2011
  • In order to figure out the characteristics of radionuclides concentrations of nine provinces, we analyzed uranium and radon in 681 samples of groundwater. Most of uranium concentrations in each province were less than $10{\mu}g/L$, and Gyeongnam, Jeonnam, Jeju provinces did not have groundwaters exceeding the US EPA drinking water MCL ($30{\mu}g/L$) of uranium. The ratio of radon values exceeding US EPA drinking water AMCL (4,000 pCi/L) was 22.6% (154/681) and Gyeongnam and Jeju provinces had no groundwaters exceeding the AMCL (alternative maximum contaminant level). Uranium and radon concentrations in groundwaters of Gyeonggi, Chungbuk, Jeonbuk, Chungnam mainly composed of the Mesozoic granite and the Precambrian gneiss were relatively high, but the concentrations of Gyeongnam and Jeju widely comprised of the sedimentary rock and the volcanic rock were relatively low. A week correlation between uranium and radon values showed in Gangwon, Chungbuk, Gyeonggi provinces.

Distribution Characteristics of Uranium and Radon Concentrations of Groundwater in Gwangju Area (광주지역 지하수 중 우라늄과 라돈의 함량 분포 특성)

  • Seo, Heejeong;Min, Kyoungwoo;Park, Jiyoung;Park, Juhyun;Hwang, Hoyeon;Park, Seil;Kim, Seonjeong;Jeong, Sukkyung;Bae, Seokjin;Kim, Seongjun
    • Journal of Environmental Health Sciences
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    • v.48 no.2
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    • pp.86-95
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    • 2022
  • Background: As high concentrations of uranium and radon have been detected in some areas in Korea, it is considered necessary to investigate natural radioactive materials in the Gwangju area. Objectives: This study aimed to identify the hydrochemical characteristics of groundwater in Gwangju and investigate the distribution characteristics of uranium and radon, which are naturally radioactive substances. Methods: To determine the uranium and radon concentrations in groundwater according to the geology of the Gwangju area, we measured 62 groundwater wells. A geological distribution map of uranium and radon content was prepared for this study. Results: The groundwater type, defined using a Piper diagram, was mainly Ca-HCO3. The concentration of uranium in the groundwater ranged from 0 to 29.3 ㎍/L, with a mean of 3.3 ㎍/L and a median of 0.9 ㎍/L. The median concentration of uranium in groundwater was highest in alluvium, granitic gneiss, and biotite granite (classified by geological unit), in that order. The concentration of radon in the groundwater ranged from 4.8 to 313.2 Bq/L, with a mean of 75.6 Bq/L and a median of 59.6 Bq/L. The median concentration of radon in groundwater was highest in biotite granite, alluvium, and granitic gneiss, in that order. As a result of the correlation analysis of groundwater in the study area, there was no significant correlation between uranium and radon. Conclusions: In this study area, uranium was shown to be far below the concentrations allowed by drinking water quality standards, but radon concentrations exceeded drinking water quality monitoring standards in 11% of the samples. It was judged that appropriate measures, such as the installation of radon reduction facilities, will be required after a thorough review of high-concentration radon detection sites of in the research area.

Hydrogeochemistry and Occurrences of Uranium and Radon in Groundwater of in Chungwon, Korea (청원지역 지하수의 우라늄과 라돈의 산출 특성과 수리지화학)

  • Lee, Byeongdae
    • Journal of Environmental Science International
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    • v.27 no.8
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    • pp.651-663
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    • 2018
  • The hydrochemistry of groundwater from 47 wells in the Chungwon area, Korea was analyzed to examine the occurrence of natural radionuclides like uranium and radon. The range of Electrical Conductivity (EC) value in the study area was $67{\sim}1,404{\mu}S/cm$. In addition to the high EC value, the content of cations and anions also tends to increase. Uranium concentrations ranged from $ND{\sim}178{\mu}g/L$ (median value, $0.8{\mu}g/L$) and radon concentrations ranged from 80~12,900 pCi/L (median value, 1,250 pCi/L). Uranium concentrations in one well, that is 2.8% of the samples, exceeded $30{\mu}g/L$, which is the Maximum Contaminant Level (MCL) proposed by the US Environmental Protection Agency (EPA), based on the chemical toxicity of uranium. Radon concentrations in three wells, that is 6% of the samples, and one well, that is 2.8% of the samples, exceeded 4,000 pCi/L (AMCL of the US EPA) and 8,100 pCi/L (Finland's guideline level), respectively. Concentrations of uranium and radon related to geology of the study area show the highest values in the groundwater of the granite area. The uranium and radon contents in the groundwater were found to be low compared to those of other countries with similar geological settings. It is likely that the measured value was lower than the actual content due to the inflow of shallow groundwater by the lack of casing and grouting.

Hydrogeochemical Characterization of Natural Radionuclides Uranium and Radon in Groundwater, Jeonnam Province (전라남도 일대 지하수 중에서 산출하는 자연방사성물질 우라늄과 라돈의 수리지구화학적 거동특징)

  • Cho, Byong Wook;Kim, Moon Su;Kim, Hyun Gu;Hwang, Jae Hong;Cho, Soo Young;Choo, Chang Oh
    • The Journal of Engineering Geology
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    • v.27 no.4
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    • pp.501-511
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    • 2017
  • Natural radionuclides such as uranium and radon from 170 groundwater wells in Jeonnam Province were investigated, together with hydrogeochemical properties, and concentration maps of uranium and radon were also constructed in this study. Characteristics of their concentrations and occurrence were discussed using hydrogeochemical factors and geostatistical methods based on individual geological units. Though uranium and radon in groundwater show a wide range in the concentration, most of which occur as low levels except a few sites. Based on factor analysis, correlation coefficients between uranium and radon are very low. Such results verify that these radionuclides behave independently, well consistent with most previous results investigated nationwide in groundwater. Besides uranium and radon, most hydrochemical components in groundwater show a close relation to indicate the water-rock interaction taken place actively in aquifer.

Analysis of queuing mine-cars affecting shaft station radon concentrations in Quzhou uranium mine, eastern China

  • Hong, Changshou;Zhao, Guoyan;Li, Xiangyang
    • Nuclear Engineering and Technology
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    • v.50 no.3
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    • pp.453-461
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    • 2018
  • Shaft stations of underground uranium mines in China are not only utilized as waiting space for loaded mine-cars queuing to be hoisted but also as the principal channel for fresh air taken to working places. Therefore, assessment of how mine-car queuing processes affect shaft station radon concentration was carried out. Queuing network of mine-cars has been analyzed in an underground uranium mine, located in Quzhou, Zhejiang province of Eastern China. On the basis of mathematical analysis of the queue network, a MATLAB-based quasi-random number generating program utilizing Monte-Carlo methods was worked out. Extensive simulations were then implemented via MATALB operating on a DELL PC. Thereafter, theoretical calculations and field measurements of shaft station radon concentrations for several working conditions were performed. The queuing performance measures of interest, like average queuing length and waiting time, were found to be significantly affected by the utilization rate (positively correlated). However, even with respect to the "worst case", the shaft station radon concentration was always lower than $200Bq/m^3$. The model predictions were compared with the measuring results, and a satisfactory agreement was noted. Under current working conditions, queuing-induced variations of shaft station radon concentration of the study mine are not remarkable.

Characteristics of Groundwater Environment in Highly Enriched Areas of Natural Radionuclides (고함량 자연방사성물질 우려지역에 대한 지하수 환경 특성 연구)

  • Jeong, Do-Hwan;Eom, Ig-Chun;Yoon, Jeong-Ki;Kim, Moon-Su;Kim, Yeong-Kyoo;Kim, Tae-Seung
    • Journal of Soil and Groundwater Environment
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    • v.15 no.6
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    • pp.9-16
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    • 2010
  • Groundwater sampling was performed at 38 wells where they are located in the areas with high uranium and radon (marked as A and B, respectively) concentrations, which were based on the previous research results. In-situ parameters (temperature, pH, EC, Eh, DO) and natural radionuclides (uranium and radon) were analyzed to figure out the characteristics of groundwater environments. In-situ data did not show any relations to natural radionuclide data, which could be caused by groundwater mixing, depths of wells, and geological settings, etc. But the highest radon well presented relatively low temperature value and the highest uranium well presented relatively low pH values The highest uranium concentration ranging $1.14{\sim}188.19{\mu}g/L$ showed in the area of A region consisted of Jurassic two-mica granite. The areas of Jurassic biotite granite and Cretaceous granite in the A region have the uranium concentrations ranging $0.10{\sim}49.78{\mu}g/L$ and $0.36{\sim}3.01{\mu}g/L$, respectively. The uranium values from between wells of community water systems (CWSs) penetrating fractured bed-rock aquifers and personal boreholes settled in shallow aquifers near the wells of CWSs show big differences. It implies that the groundwaters of the two areas have evolved from different water-rock interaction paths that may caused by various types of wells having different aquifers. High radon activities in the area of B region composed of Precambrian gneiss showed ranging from 6,770 to 64,688 pCi/L. Even though the wells are located in the same geological settings, their rodon concentration presented different according to depth and distance.

Environmental Characteristics of Naturally Occurring Radioactive Materials (238U, 222Rn) Concentration in Drinking Groundwaters of Metamorphic Rock Areas: Korea (국내 변성암 지역 음용지하수 중 자연방사성물질(238U, 222Rn)의 환경 특성 연구)

  • Ju, Byoung Kyu;Kim, Moon Su;Jeong, Do Hwan;Hong, Jung Ki;Kim, Dong Su;Noh, Hoe Jung;Yoon, Jeong Ki;Kim, Tae Seung
    • Journal of Soil and Groundwater Environment
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    • v.18 no.3
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    • pp.82-92
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    • 2013
  • This study has investigated naturally occurring radioactive materials (N.O.R.M; $^{238}U$, $^{222}Rn$) for 353 drinking groundwater wells in metamorphic rock areas in Korea. Uranium concentrations ranged from N.D (not detected) to 563.56 ${\mu}g/L$ (median value, 0.68 ${\mu}g/L$) and radon concentrations ranged from 108 to 11,612 pCi/L (median value, 1,400 pCi/L). Uranium and radon concentrations in the groundwater generally are similar to USA with similar geological setting. Uranium concentrations in 9 wells (2.6%) exceeded 30 ${\mu}g/L$, which is the maximum contaminant level (MCL) by the US environmental protection agency (EPA), radon concentrations in 46 wells (13%) exceeded 4,000 pCi/L, which is the Alternative MCL (AMCL) by the US.EPA. The log-log correlation coefficient between uranium and radon was 0.32. The correlation coefficient between uranium and pH was 0.12 and the correlation coefficient between radon and temperature was -0.01. The correlation coefficient between uranium and $HCO_3$ was 0.09 and the correlation coefficient between uranium and Ca was 0.11. The median value of uranium was high Chung-Buk (1.78 ${\mu}g/L$), Gyeong-Buk (1.37 ${\mu}g/L$), In-Cheon (1.06 ${\mu}g/L$) for each province. On the other hand, the median value of radon was high In-Cheon (2,962 pCi/L), Chung-Buk (2,339 pCi/L), Jeon-Buk (2,165 pCi/L) for each province. Jeon-Buk for log-log correlation coefficient is the highest (0.63) among provinces.

Occurrence Characteristics of Uranium and Radon-222 in Groundwater at ○○ Village, Yongin Area (용인 ○○마을 지하수내 우라늄 및 라돈-222의 산출특성)

  • Jeong, Chan Ho;Yang, Jae Ha;Lee, Yong Cheon;Lee, Yu Jin;Cho, Hyeon Young;Kim, Moon Su;Kim, Hyun Koo;Kim, Tae Seong;Jo, Byung Uk
    • The Journal of Engineering Geology
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    • v.26 no.2
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    • pp.261-276
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    • 2016
  • The occurrence of natural radioactive materials such as uranium and radon-222 in groundwater was examined with hydrogeochemistry and geology at ○○ village in the Yongin area. Two rounds of 19 groundwater and 5 surface water sampling were collected for analysis. The range of pH value in groundwaters was 5.81 to 7.79 and the geochemical types of the groundwater were mostly Ca(Na)-HCO3 and Ca(Na)-NO3(Cl)-HCO3. Uranium and radon-222 concentrations in the groundwater ranged from 0.06 to 411 μg/L and from 5.56 to 903 Bq/L, respectively. Two deep groundwaters used as common potable well-water sources exceeded the maximum contaminant levels of the uranium and radon-222 proposed by the United States Environmental Protection Agency (US EPA). Three groundwater samples from residential areas contained unsuitable levels of uranium, and 12 groundwater samples were unsuitable due to radon-222 concentrations. Radioactive materials in the unsuitable groundwater are naturally occurring in a Jurassic amphibole- and biotite-bearing granitic gneiss. High uranium and radon-222 groundwater concentrations were only observed in two common wells; the others showed no relationship between bedrock geology and groundwater geochemical constituents. With such high concentrations of naturally occurring radioactive materials in groundwater, the affected areas may extend tens of meters for uranium and even farther for radon-222. Therefore, we suggest the radon-222 and the uranium did not originate from the same source. Based on the distribution of radon-222 in the study area, zones of higher radon-222 concentrations may be the result of diffusion through cracks, joint, or faults. Surface radioactivity and uranium concentrations in the groundwater show a positive relationship, and the impact areas may extend for ~200m beyond the well in the case of wells containing high concentrations of uranium. The highest uranium and thorium concentrations in rock samples were detected in thorite and monazite.

Application of advanced spectral-ratio radon background correction in the UAV-borne gamma-ray spectrometry

  • Jigen Xia;Baolin Song;Yi Gu;Zhiqiang Li;Jie Xu;Liangquan Ge;Qingxian Zhang;Guoqiang Zeng;Qiushi Liu;Xiaofeng Yang
    • Nuclear Engineering and Technology
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    • v.55 no.8
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    • pp.2927-2934
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    • 2023
  • The influence of the atmospheric radon background on the airborne gamma spectrum can seriously affect researchers' judgement of ground radiation information. However, due to load and endurance, unmanned aerial vehicle (UAV)-borne gamma-ray spectrometry is difficulty installing upward-looking detectors to monitor atmospheric radon background. In this paper, an advanced spectral-ratio method was used to correct the atmospheric radon background for a UAV-borne gamma-ray spectrometry in Inner Mongolia, China. By correcting atmospheric radon background, the ratio of the average count rate of U window in the anomalous radon zone (S5) to that in other survey zone decreased from 1.91 to 1.03, and the average uranium content in S5 decreased from 4.65 mg/kg to 3.37 mg/kg. The results show that the advanced spectral-ratio method efficiently eliminated the influence of the atmospheric radon background on the UAV-borne gamma-ray spectrometry to accurately obtain ground radiation information in uranium exploration. It can also be used for uranium tailings monitoring, and environmental radiation background surveys.