• Title/Summary/Keyword: Thermal neutron

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Upgrade of Neutron Energy Spectrometer with Single Multilayer Bonner Sphere Using Onion-like Structure

  • Mizukoshi, Tomoaki;Watanabe, Kenichi;Yamazaki, Atsushi;Uritan, Akira;Iguchi, Tetsuo;Ogata, Tomohiro;Muramatsu, Takashi
    • Journal of Radiation Protection and Research
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    • v.41 no.3
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    • pp.185-190
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    • 2016
  • Background: In order to measure neutron energy spectra, the conventional Bonner Sphere Spectrometers (BSS) are widely used. In this spectrometer, several measurements with different size Bonner spheres are required. Operators should, therefore, place these spheres in several times to a measurement point where radiation dose might be relatively high. In order to reduce this effort, novel neutron energy spectrometer using an onion-like single Bonner sphere was proposed in our group. This Bonner sphere has multiple sensitive spherical shell layers in the single sphere. In this spectrometer, a band-shaped thermal neutron detection medium, which consists of a LiF-ZnS mixed powder scintillator sheet and a wavelength-shifting (WLS) fiber readout, was looped to each sphere at equal angular intervals. Amount of LiF neutron converter is reduced near polar region, where the band-shaped detectors are concentrated, in order to uniform the directional sensitivity. The LiF-ZnS mixed powder has an advantage of extremely high light yield. However, since it is opaque, scintillation photons cannot be collect uniformly. This type of detector shows no characteristic shape in the pulse height spectrum. Subsequently, it is difficult to set the pulse height discrimination level. This issue causes sensitivity fluctuation due to gain instability of photodetectors and/or electric modules. Materials and Methods: In order to solve this problem, we propose to replace the LiF-ZnS mixed powder into a flexible and Transparent RUbber SheeT type $LiCaAlF_6$ (TRUST LiCAF) scintillator. TRUST LiCAF scintillator can show a peak shape corresponding to neutron absorption events in the pulse height spectrum. Results and Discussion: We fabricated the prototype detector with five sensitive layers using TRUST LiCAF scintillator and conducted basic experiments to evaluate the directional uniformity of the sensitivity. Conclusion: The fabricated detector shows excellent directional uniformity of the neutron sensitivity.

Optimization of target, moderator, and collimator in the accelerator-based boron neutron capture therapy system: A Monte Carlo study

  • Cheon, Bo-Wi;Yoo, Dohyeon;Park, Hyojun;Lee, Hyun Cheol;Shin, Wook-Geun;Choi, Hyun Joon;Hong, Bong Hwan;Chung, Heejun;Min, Chul Hee
    • Nuclear Engineering and Technology
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    • v.53 no.6
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    • pp.1970-1978
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    • 2021
  • The aim of this study was to optimize the target, moderator, and collimator (TMC) in a neutron beam generator for the accelerator-based BNCT (A-BNCT) system. The optimization employed the Monte Carlo Neutron and Photon (MCNP) simulation. The optimal geometry for the target was decided as the one with the highest neutron flux among nominates, which were called as angled, rib, and tube in this study. The moderator was optimized in terms of consisting material to produce appropriate neutron energy distribution for the treatment. The optimization of the collimator, which wrapped around the target, was carried out by deciding the material to effectively prevent the leakage radiations. As results, characteristic of the neutron beam from the optimized TMC was compared to the recommendation by the International Atomic Energy Agent (IAEA). The tube type target showed the highest neutron flux among nominates. The optimal material for the moderator and collimator were combination of Fluental (Al203+AlF3) with 60Ni filter and lead, respectively. The optimized TMC satisfied the IAEA recommendations such as the minimum production rate of epithermal neutrons from thermal neutrons: that was 2.5 times higher. The results can be used as source terms for shielding designs of treatment rooms.

Neutron-irradiated effect on the thermoelectric properties of Bi2Te3-based thermoelectric leg

  • Huanyu Zhao;Kai Liu;Zhiheng Xu;Yunpeng Liu;Xiaobin Tang
    • Nuclear Engineering and Technology
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    • v.55 no.8
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    • pp.3080-3087
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    • 2023
  • Thermoelectric (TE) materials working in radioisotope thermoelectric generators are irradiated by neutrons throughout its service; thus, investigating the neutron irradiation stability of TE devices is necessary. Herein, the influence of neutron irradiation with fluences of 4.56 × 1010 and 1 × 1013 n/cm2 by pulsed neutron reactor on the electrical and thermal transport properties of n-type Bi2Te2.7Se0.3 and p-type Bi0.5Sb1.5Te3 thermoelectric alloys prepared by cold-pressing and molding is investigated. After neutron irradiation, the properties of thermoelectric materials fluctuate, which is related to the material type and irradiation fluence. Different from p-type thermoelectric materials, neutron irradiation has a positive effect on n-type Bi2Te2.7Se0.3 materials. This result might be due to the increase of carrier mobility and the optimization of electrical conductivity. Afterward, the effects of p-type and n-type TE devices with different treatments on the output performance of TE devices are further discussed. The positive and negative effects caused by irradiation can cancel each other to a certain extent. For TE devices paired with p-type Bi0.5Sb1.5Te3 and n-type Bi2Te2.7Se0.3 thermoelectric legs, the generated power and conversion efficiency are stable after neutron irradiation.

A Numerical Technique for Predicting Deformation due to Neutron Irradiation for Integrity Assessment of Research Reactors (연구용 원자로의 건전성 평가를 위한 수치해석적 중성자 조사 재료변형 예측기법 개발)

  • Jun-Geun Park;Tae-Hyeon Seok;Nam-Su Huh
    • Transactions of the Korean Society of Pressure Vessels and Piping
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    • v.20 no.1
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    • pp.39-48
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    • 2024
  • Research reactors are operated under ambient temperature and atmospheric pressure, which is much less severe conditions compared to those in typical nuclear power plants. Due to the high temperature, heat resistant materials such as austenite stainless steel should be used for the reactors in typical nuclear power plants. Whereas, as the effect of temperature is low for research reactors, materials with high resistance to neutron irradiation, such as zircaloy and beryllium, are used. Therefore, these conditions should be considered when performing integrity assessment for research reactors. In this study, a computational technique through finite element (FE) analysis was developed considering the operating conditions and materials of research reactor when conducting integrity assessment. Neutron irradiation analysis techniques using thermal expansion analysis were proposed to consider neutron irradiation growth and swelling in zirconium alloys and beryllium. A user subroutine program that can calculate the strain rate induced by neutron irradiation creep was developed for use in the commercial analysis program Abaqus. To validate the proposed technique and the user subroutine, FE analysis results were compared with hand-calculation results, and showed good agreement. Consequently, developed technique and user subroutine are suitable for evaluating structural integrity of research reactors.

Development and application analysis of high-energy neutron radiation shielding materials from tungsten boron polyethylene

  • Qiankun Shao;Qingjun Zhu;Yuling Wang;Shaobao Kuang;Jie Bao;Songlin Liu
    • Nuclear Engineering and Technology
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    • v.56 no.6
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    • pp.2153-2162
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    • 2024
  • The purpose of this study is to develop a high-energy neutron shielding material applied in proton therapy environment. Composite shielding material consisting of 10.00 wt% boron carbide particles (B4C), 13.64 wt% surface-modified cross-linked polyethylene (PE), and 76.36 wt% tungsten particles were fabricated by hot-pressure sintering method, where the optimal ratio of the composite is determined by the shielding effect under the neutron field generated in typical proton therapy environment. The results of Differential Scanning Calorimetry measurements (DSC) and tensile experiment show that the composite has good thermal and mechanical properties. In addition, the high energy-neutron shielding performance of the developed material was evaluated using cyclotron proton accelerator with 100 MeV proton. The simulation shows a 99.99% decrease in fast neutron injection after 44 cm shielding, and the experiment result show a 99.70% decrease. Finally, the shielding effect of replacing part of the shielding material of the proton therapy hall with the developed material was simulated, and the results showed that the total neutron injection decreased to 0.99‰ and the neutron dose reduced to 1.10‰ before the enhanced shielding. In summary, the developed material is expected to serve as a shielding enhancement material in the proton therapy environment.

Sensing changes in tumor during boron neutron capture therapy using PET with a collimator: Simulation study

  • Yang, Hye Jeong;Yoon, Do-Kun;Suh, Tae Suk
    • Nuclear Engineering and Technology
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    • v.52 no.9
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    • pp.2072-2077
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    • 2020
  • The purpose of this study was to demonstrate the feasibility of sensing changes in a tumor during boron neutron capture therapy (BNCT) using a Monte Carlo simulation tool. In the simulation, an epi-thermal neutron source and a water phantom including boron uptake regions (BURs) were simulated. Moreover, this simulation also included a detector for positron emission tomography (PET) scanning and an adaptively-designed collimator (ADC) for PET. After the PET scanning of the water phantom, including the 511 keV source in the BUR, the ADC was positioned in the PET's gantry. Single prompt gamma rays were collected through the ADC during neutron irradiation. Then, single prompt gamma ray-based tomography images of different sized tumors were acquired by a four-step process. Both the signal-to-noise ratio (SNR) and tumor size were analyzed from each step image. From this analysis, we identified a decreasing trend of both the SNR and signal intensity as the tumor size decreased, which was confirmed in all images. In conclusion, we confirmed the feasibility of sensing changes in a tumor during BNCT using PET and an ADC through Monte Carlo simulation.

Visualization of Crust in Metallic Piping Through Real-Time Neutron Radiography Obtained with Low Intensity Thermal Neutron Flux

  • Luiz, Leandro C.;Ferreira, Francisco J.O.;Crispim, Verginia R.
    • Nuclear Engineering and Technology
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    • v.49 no.4
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    • pp.781-786
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    • 2017
  • The presence of crust on the inner walls of metallic ducts impairs transportation because crust completely or partially hinders the passage of fluid to the processing unit and causes damage to equipment connected to the production line. Its localization is crucial. With the development of the electronic imaging system installed at the Argonauta/Nuclear Engineering Institute (IEN)/National Nuclear Energy Commission (CNEN) reactor, it became possible to visualize crust in the interior of metallic piping of small diameter using real-time neutron radiography images obtained with a low neutron flux. The obtained images showed the resistance offered by crust on the passage of water inside the pipe. No discrepancy of the flow profile at the bottom of the pipe, before the crust region, was registered. However, after the passage of liquid through the pipe, images of the disturbances of the flow were clear and discrepancies in the flow profile were steep. This shows that this technique added the assembled apparatus was efficient for the visualization of the crust and of the two-phase flows.

An investigative study of enrichment reduction impact on the neutron flux in the in-core flux-trap facility of MTR research reactors

  • Xoubi, Ned;Darda, Sharif Abu;Soliman, Abdelfattah Y.;Abulfaraj, Tareq
    • Nuclear Engineering and Technology
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    • v.52 no.3
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    • pp.469-476
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    • 2020
  • Research reactors in-core experimental facilities are designed to provide the highest steady state flux for user's irradiation requirements. However, fuel conversion from highly enriched uranium (HEU) to low enriched uranium (LEU) driven by the ongoing effort to diminish proliferation risk, will impact reactor physics parameters. Preserving the reactor capability to produce the needed flux to perform its intended research functions, determines the conversion feasibility. This study investigates the neutron flux in the central experimental facility of two material test reactors (MTR), the IAEA generic10 MW benchmark reactor and the 22 MW s Egyptian Test and Research Reactor (ETRR-2). A 3D full core model with three uranium enrichment of 93%, 45%, and 20% was constructed utilizing the OpenMC particle transport Monte Carlo code. Neutronics calculations were performed for fresh fuel, the beginning of life cycle (BOL) and end of life cycle (EOL) for each of the three enrichments for both the IAEA 10 MW generic reactor and core 1/98 of the ETRR-2 reactor. Criticality calculations of the effective multiplication factor (Keff) were executed for each of the twelve cases; results show a reasonable agreement with published benchmark values for both reactors. The thermal, epithermal and fast neutron fluxes were tallied across the core, utilizing the mesh tally capability of the code and are presented here. The axial flux in the central experimental facility was tallied at 1 cm intervals, for each of the cases; results for IAEA 10 MW show a maximum reduction of 14.32% in the thermal flux of LEU to that of the HEU, at EOL. The reduction of the thermal flux for fresh fuel was between 5.81% and 9.62%, with an average drop of 8.1%. At the BOL the thermal flux showed a larger reduction range of 6.92%-13.58% with an average drop of 10.73%. Furthermore, the fission reaction rate was calculated, results showed an increase in the peak fission rate of the LEU case compared to the HEU case. Results for the ETRR-2 reactor show an average increase of 62.31% in the thermal flux of LEU to that of the HEU due to the effect of spectrum hardening. The fission rate density increased with enrichment, resulting in 34% maximum increase in the HEU case compared to the LEU case at the assemblies surrounding the flux trap.

Probabilistic Fracture Analysis of Nuclear Reactor Vessel under Pressurized Thermal Shock (가압열충격을 받는 원자로의 확률론적 파괴해석)

  • 김지호;김종욱;김종인;박근배
    • Proceedings of the Computational Structural Engineering Institute Conference
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    • 2004.04a
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    • pp.309-316
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    • 2004
  • A probabilistic structural integrity assessment is performed for a reactor pressure vessel under PTS(Pressurized Thermal Shock). A semi-elliptical finite axial crack is assumed to he in the beltline region(either base metal or weld meta)1 of the reactor vessel inside surface. The selected random variables are initial crack depth, neutron fluence on the vessel inside surface, copper, nickel, and phosphorus content of the vessel material, and RT/sub NDT/. The probabilities of crack initiation or vessel failure where the crack is propagated through vessel wall are calculated. The probabilities obtained with random crack size are compared to these obtained with deterministic us. Since the failure function cannot to explicitly by selected by selected random variables, Monte Carlo Simulation is applied to perform probabilistic analysis The influence of the amount of neutron fluence is also examined to assess the structural reliability for vessel life time.

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Study on Core Debris Recriticality During Hypothetical Severe Accidents in Three Element Core Design of The Advanced Neutron Source Reactor

  • Shin, Sung-Tack
    • Proceedings of the Korean Nuclear Society Conference
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    • 1996.05b
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    • pp.467-472
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    • 1996
  • This study discusses special aspects of severe accident related recriticality modeling and analysis in the Advanced Neutron Source (ANS) reactor.$^{1, 2)}$ The analytical comparison of three elements core to former two elements case is conducted including evaluation of suitable nuclear cross-section sets to account for the effects of system configulation, fuel and moderator mixture temperature, material dispersion and the other thermal-hydraulics. Three elements core ANS reactor is the alternative core design which was proposed as a modified core design, with three fuel elements instead of two, that would allow operation with only 50% enriched uranium (former uranium fuel is the baseline design value of 93%) A comprehensive test matrix of calculations to evaluate the threat of a criticality event in the ANS is described. Strong dependencies still on geometry, material constituents, and thermal-hydraulic conditions are verified. Therefore, the concepts of mitigative design features are qualified.d.

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