• Title/Summary/Keyword: Radionuclide Transport

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AN ANALYSIS OF THE EFFECT OF HYDRAULIC PARAMETERS ON RADIONUCLIDE MIGRATION IN AN UNSATURATED ZONE

  • Kim, Gye-Nam;Moon, Jei-Kwon;Lee, Kune-Woo
    • Nuclear Engineering and Technology
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    • v.42 no.5
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    • pp.562-567
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    • 2010
  • A One-Dimensional Water Flow and Contaminant Transport in Unsaturated Zone (FTUNS) code has been developed in order to interpret radionuclide migration in an unsaturated zone. The pore-size distribution index (n) and the inverse of the air-entry value ($\alpha$) for an unsaturated zone were measured by KS M ISO 11275 method. The hydraulic parameters of the unsaturated soil are investigated by using soil from around a nuclear facility in Korea. The effect of hydraulic parameters on radionuclide migration in an unsaturated zone has been analyzed. The higher the value of the n-factor, the more the cobalt concentration was condensed. The larger the value of $\alpha$-factor, the faster the migration of cobalt was and the more aggregative the cobalt concentration was. Also, it was found that an effect on contaminant migration due to the pore-size distribution index (n) and the inverse of the air-entry value ($\alpha$) was minute. Meanwhile, migrations of cobalt and cesium are in inverse proportion to the Freundich isotherm coefficient. That is to say, the migration velocity of cobalt was about 8.35 times that of cesium. It was conclusively demonstrated that the Freundich isotherm coefficient was the most important factor for contaminant migration.

Interpretation of Migration of Radionuclides in a Rock Fracture Using a Particle Tracking Method (입자추적법을 사용한 암반균열에서 핵종이동 해석)

  • Chung Kyun Park;Pil Soo Hahn;Douglas J. Drew
    • Nuclear Engineering and Technology
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    • v.27 no.2
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    • pp.176-188
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    • 1995
  • A particle tracking scheme was developed in order to model radionuclide transport through a tortuous flow Held in a rock fracture. The particle tacking method may be used effectively in a heterogeneous flow field such as rock fracture. The parallel plate representation of the single fracture fails to recognize the spatial heterogeneity in the fracture aperture and thus seems inadequate in describing fluid movement through a real fracture. The heterogeneous flow field une modeled by a variable aperture channel model after characterizing aperture distribution by a hydraulic test. To support the validation of radionuclide transport models, a radionuclide migration experiment was performed in a natural fracture of granite. $^3$$H_2O$ and $^{131}$ I are used as tracers. Simulated results were in agreement with experimental result and therefore support the validity of the transport model. Residence time distributions display multipeak curves caused by the fast arrival of solutes traveling along preferential fracture channels and by the much slower arrival of solutes following tortous routes through the fracture. Results from the modelling of the transport of nonsorbing tracer through the fracture show that diffusion into the interconnected pore space in the rock mass has a significant effect on retardation.

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Containment Evaluation of the KN-12 Transport Cask

  • Chung, Sung-Hwan;Choi, Byung-Il;Lee, Heung-Young;Song, Myung-Jae
    • Journal of Radiation Protection and Research
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    • v.28 no.4
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    • pp.291-298
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    • 2003
  • The KN-12 transport cask has been designed to transport 12 PWR spent nuclear fuel assemblies and to comply with the regulatory requirements for a Type B(U) package. The containment boundary of the cask is defined by a cask body, a cask lid, lid bolts with nuts, O-ring seals and a bolted closure lid. The containment vessel for the cask consists of a forged thick-walled carbon steel cylindrical body with an integrally-welded carbon steel bottom and is closed by a lid made of stainless steel, which is fastened to the cask body by lid bolts with nuts and sealed by double elastomer O-rings. In the cask lid an opening is closed by a plug with an O-ring seal and covered by the bolted closure lid sealed with an O-ring. The cask must maintain a radioactivity release rate of not more than the regulatory limit for normal transport conditions and for hypothetical accident conditions, as required by the related regulations. The containment requirements of the cask are satisfied by maintaining a maximum air reference leak rate of $2.7{\times}10^{-4}ref.cm^3s^{-1}$ or a helium leak rate of $3.3{\times}10^{-4}cm^3s^{-1}$ for normal transport conditions and for hypothetical accident conditions.

Development of Radionuclide Inventory Declaration Methods Using Scaling Factors for the Korean NPPs - Scope and Activity Determination Method - (국내 원전 대상의 척도인자를 활용한 핵종재고량 규명 방법의 개발 - 범위 및 방사능 결정 방법-)

  • Hwang, Ki-ha;Lee, Sang-chul;Kang, Sang-hee;Lee, Kun-Jai;Jeong, Chan-woo;Ahn, Sang-myeon;Kim, Tae-wook;Kim, Kyoung-doek;Herr, Young-hoi
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.2 no.1
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    • pp.77-85
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    • 2004
  • Regulations and guidelines for radioactive waste disposal require detailed information about the characteristics of radioactive waste drums prior to transport to the disposal sites. However, estimation of radionuclide concentrations in the drummed radioactive waste is difficult and unreliable. In order to overcome this difficulty, scaling factor (SF) method has been used to assess the activities of radionuclides, which could not be directly analyzed. A radioactive waste assay system has been operated at Korean nuclear power plant (KORI site) since 1996 and consolidated SF concept has played a dominant role in the determination of radionuclide concentrations. However, SFs are somewhat dispersive and limited in KORI site. Therefore establishment of the assay system using more improved SFs is planned and progressed. In this paper, the scope of research is briefly introduced. For the selection of more reliable activity determination method, the accuracy of predicted SF values for each activity determination method is compared. From the comparison of each activity determination method, it is recommended that SF determination method should be changed from the arithmetic mean to the geometrical mean for more reliable estimation of radionuclide activity. Arithmetic mean method and geometric mean method are compared based on the data set in KORI system. And, this change of SF determination method will prevent an inordinate over-estimation of radionuclide inventory in radwaste drum.

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Radionuclide Diffusion in Compacted Domestic Bentonite (압축 국산 벤토나이트 내에서 방사성 핵종의 확산이동)

  • Choi, Jong-Won;Lee, Byung-Hun
    • Journal of Radiation Protection and Research
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    • v.16 no.2
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    • pp.27-39
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    • 1991
  • The diffusion of Sr-85, Cs-137, Co-60 and Am-241 in compacted domestic bentonite was studied, using a diffusion cell unit in which diffusion took place axially from the center of cylindrical bentonite sample body. The effects of compaction density and heat-treated bentonite on diffusion were analysed. And the diffusion mechanism of radionuclide was also analysed by evaluating the measured diffusivity of anion Cl-36. The apparent diffusivities obtained for Sr-85, Cs-137, Co-60 and Am-241 were $l.07{\times}10^{-11},\;6.705{\times}10^{-13},\;l.226{\times}10^{-13}\;and\; l.310{\times}10^{-14}m^2/sec$, respectively. When the as-pressed density of bentonite increased from $1.8\;to\;2.0g/cm^3$, the apparent diffusivity of Cs-137 decreased by quarter. In the case of bentonite heat-treated to $150^{\circ}C$, no significant change in diffusivity was observed, which showed the possibility that the domestic bentonite could be used as a chemical barrier to retard the radionuclide migration at below $150^{\circ}C$. From the calculated pore and surface diffusivity, the surface diffusion due to the concentration gradient of radionuclide sorbed on the solid phase was found to dominate greatly in total transport process.

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Evaluation of Internal Dosimetry according to Various Radionuclides Conditions in Nuclear Medicine Myocardial Scan: Monte Carlo Simulation (심근 핵의학 검사에서 다양한 방사성핵종 조건에 따른 내부피폭선량 평가: 몬테카를로 시뮬레이션)

  • Min-Gwan Lee;Chanrok Park
    • Journal of radiological science and technology
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    • v.47 no.3
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    • pp.213-218
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    • 2024
  • The myocardial nuclear medicine examination is widely performed to diagnose myocardium disease using various radionuclides. Although image quality according to radionuclides has improved, the radiation exposure for target organ as well as peripheral organs should be considered. Here, the aim of this study was to evaluate absorbed dose (Gy) for peripheral organs in myocardial nuclear medicine scan from myocardium according to various scan environments based on Monte Carlo simulation. The simulation environment was modeled 5 cases, which were considered by radionuclides, number of injections, and radiodosage. In addition, the each radionuclide simulation such as distribution fraction was considered by recommended standard protocol, and the mesh computational female phantom, which is provided by International Commission on Radiological Protection (ICRP) 145, was used using the particle and heavy ion transport code system (PHITS) version 3.33. Based on the results, the closer to the myocardium, the higher the absorbed dose values. In addition, application for dual injection for radionuclides leaded to high absorbed dose compared with single injection for radionuclide. Consequently, there is difference for absorbed dose according to radionuclides, number of injections, and radiodosage. To detect the accurate diseased area, acquisition for improved image quality is crucial process by injecting radionuclides, however, we need to consider absorbed dose both target and peripheral inner organs from radionuclides in terms radiation protection for patient.

AN INTEGRATED APPROACH TO RISK-BASED POST-CLOSURE SAFETY EVALUATION OF COMPLEX RADIATION EXPOSURE SITUATIONS IN RADIOACTIVE WASTE DISPOSAL

  • Seo, Eun-Jin;Jeong, Chan-Woo;Sato, Seichi
    • Journal of Radiation Protection and Research
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    • v.35 no.1
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    • pp.6-11
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    • 2010
  • Embodying the safety of radioactive waste disposal requires the relevant safety criteria and the corresponding stylized methods to demonstrate its compliance with the criteria. This paper proposes a conceptual model of risk-based safety evaluation for integrating complex potential radiation exposure situations in radioactive waste disposal. For demonstrating compliance with a risk constraint, the approach deals with important exposure scenarios from the viewpoint of the receptor to estimate the resulting risk. For respective exposure situations, it considers the occurrence probabilities of the relevant exposure scenarios as their probability of giving rise to doses to estimate the total risk to a representative person by aggregating the respective risks. In this model, an exposure scenario is simply constructed with three components:radionuclide release, radionuclide migration and environment contamination, and interaction between the contaminated media and the receptor. A set of exposure scenarios and the representative person are established from reasonable combinations of the components, based on a balance of their occurrence probabilities and the consequences. In addition, the probability of an exposure scenario is estimated on the assumption that the initiating external factors influence release mechanisms and transport pathways, and its effect on the interaction between the environment and the receptor may be covered in terms of the representative person. This integrated approach enables a systematic risk assessment for complex exposure situations of radioactive waste disposal and facilitates the evaluation of compliance with risk constraints.

Effect of Exchangeable Cation on Radionuclide Diffusion In Compacted Bentonite

  • Park, Jong-Won;Park, Hyun-Soo;Dennis W. Oscarson
    • Nuclear Engineering and Technology
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    • v.28 no.3
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    • pp.274-279
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    • 1996
  • Diffusion coefficient is a critical parameter for predicting radiological source term(migration rate and flux of radionuclide) through given near field conditions in spent fuel or high level waste repository. The effect of exchangeable cation-$Na^+$ and $Ca^{2+} - on the diffusion of $I^- \;and^3H$ (as HTO) in compacted bentonite was examined using a through-diffusion method. Bentonite material used here was compacted to a density of 1.3 Mg/m$^3$, and Na-bentonite was saturated with a solution of 100 mol NaCl/m$^3$ and Ca-bentonite with 50 $mol\;CaCl_2$/m$^3$. The results show that effective diffusion coefficients are generally higher by a factor of two to five in Ca-than Na-clay. This is attributed to the larger particle size of Ca-compared to Na-bentonite; hence, Ca-bentonite has a greater proportion of relatively large pores, which make a greater contribution to mass transport than small pores. Although the nature of the exchangeable cation affects mass diffusion in compacted bentonite, the effect is small and not likely to influence performance assessment modeling of compacted bentonite-based barriers.

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The Assessment of The Collective Dose Resulting from Airborne Releases of Radionuclides (방사성핵종(放射性核種)의 대기방출(大氣放出)로 인한 집단선량(集團線量) 평가(評價))

  • Lee, Tea-Young;Yook, Chong-Chul;Lee, Byung-Ki
    • Journal of Radiation Protection and Research
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    • v.8 no.2
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    • pp.41-46
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    • 1983
  • Annual collective dose within 50 miles radius of Ko-ri I reactor site due to normal airborne effluent discharges in 1979 has been estimated by AIRDOS-EPA computer code. Gaussian plume equation is used for estimation of both horizontal and vertical dispersion of radionuclide release into the atmosphere. Also, radionuclide concentrations in meat, milk, and fresh produce consumed by near-by population are estimated by coupling the output of the atmospheric transport models with the USNRC terrestrial food chain models. Annual collective doses are found to be $3.348{\times}10^{-1}$ whole body manrem and 84.95 thyroid manrem. Whole body manrem calculated by AIRDOS-EPA computer code do not differ greatly from that calculated by GASPAR computer code, but value for thyroid manrem have been estimated lower than that calculated by GASPAR computer code.

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A modularized numerical framework for the process-based total system performance assessment of geological disposal systems

  • Kim, Jung-Woo;Jang, Hong;Lee, Dong Hyuk;Cho, Hyun Ho;Lee, Jaewon;Kim, Minjeong;Ju, Heejae
    • Nuclear Engineering and Technology
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    • v.54 no.8
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    • pp.2828-2839
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    • 2022
  • This study developed a safety assessment tool for geological disposal systems called APro, a systemically integrated modeling system based on modularizing and coupling the processes which need to be considered in a geological disposal system. Thermal, hydraulic, chemical, canister failure, radionuclide release and transport processes were considered in the current version of APro. Each of the unit processes in APro consists of a single Default Module, and several Alternative Modules which can increase the flexibility of the model. As an initial stage of developing the modularization concept and modeling interface, the Default Modules of each unit process were described, with one Alternative Module of chemical process. The computation part of APro is mainly a MATLAB workspace controlling COMSOL and PHREEQC, which are coupled by an operator splitting scheme. The APro model domain is a stylized geological disposal system employing the Swedish disposal concept (KBS-3 type), but the repository layout can be freely adjusted. In order to show the applicability of APro to the total system performance assessment of geological disposal system, some sample simulations were conducted. From the results, it was confirmed that coupling of the thermal and hydraulic processes and coupling of the canister failure and the radionuclide release processes were well reflected in APro. In addition, the technical connectivity between COMSOL and PHREEQC was also confirmed.