• Title/Summary/Keyword: Radioactive Effluent

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CURRENT RESEARCH AND DEVELOPMENT ACTIVITIES ON FISSION PRODUCTS AND HYDROGEN RISK AFTER THE ACCIDENT AT FUKUSHIMA DAIICHI NUCLEAR POWER STATION

  • NISHIMURA, TAKESHI;HOSHI, HARUTAKA;HOTTA, AKITOSHI
    • Nuclear Engineering and Technology
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    • v.47 no.1
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    • pp.1-10
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    • 2015
  • After the Fukushima Daiichi nuclear power plant (NPP) accident, new regulatory requirements were enforced in July 2013 and a backfit was required for all existing nuclear power plants. It is required to take measures to prevent severe accidents and mitigate their radiological consequences. The Regulatory Standard and Research Department, Secretariat of Nuclear Regulation Authority (S/NRA/R) has been conducting numerical studies and experimental studies on relevant severe accident phenomena and countermeasures. This article highlights fission product (FP) release and hydrogen risk as two major areas. Relevant activities in the S/NRA/R are briefly introduced, as follows: 1. For FP release: Identifying the source terms and leak mechanisms is a key issue from the viewpoint of understanding the progression of accident phenomena and planning effective countermeasures that take into account vulnerabilities of containment under severe accident conditions. To resolve these issues, the activities focus on wet well venting, pool scrubbing, iodine chemistry (in-vessel and ex-vessel), containment failure mode, and treatment of radioactive liquid effluent. 2. For hydrogen risk: because of three incidents of hydrogen explosion in reactor buildings, a comprehensive reinforcement of the hydrogen risk management has been a high priority topic. Therefore, the activities in evaluation methods focus on hydrogen generation, hydrogen distribution, and hydrogen combustion.

Special monitoring results for determination of radionuclide composition of Russian NPP atmospheric releases

  • Vasyanovich, Maxim;Vasilyev, Aleksey;Ekidin, Aleksey;Kapustin, Ivan;Kryshev, Alexander
    • Nuclear Engineering and Technology
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    • v.51 no.4
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    • pp.1176-1179
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    • 2019
  • Measurements of activity concentrations of radionuclides in atmospheric releases were performed in 2017-2018 at vent stacks of seven Russian nuclear power plants. The selected instruments and research methods, with detection limits significantly lower than the existing detection limit of Russian NPPs routine control, allowed to reliably determine up to 26 radionuclides. Analysis of experimental data allows to determine the list of radionuclides for calculation the effective dose rates to public and the permissible annual discharge levels for each Russian NPP. Radiocarbon is determined as major contributor for the dose from the atmospheric releases of LWGR reactors - up to 98% for EGP-6 and RBMK-1000 (Smolensk NPP) reactors. For PWR reactors (VVER) radionuclides contribution to the annual dose from atmospheric releases is more complicated, but, in general, dose is formed by tritium, $^{14}C$ and noble gases. The special monitoring results with ranking of measured radionuclides according to their contribution to the effective dose makes it possible to optimize the list of controlled radionuclides in airborne releases of Russian NPPs from 94 to 8-16 for different NPPs.

An Assessment of Air Sampling Location for Stack Monitoring in Nuclear Facility (원자력시설 굴뚝 내 공기시료채취 위치의 적절성 평가)

  • Lee, JungBok;Kim, TaeHyoung;Lee, JongIl;Kim, BongHwan
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.15 no.2
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    • pp.173-180
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    • 2017
  • In this study, air sampling locations in the stack of the Advanced Fuel Science Building (AFSB) at the Korea Atomic Energy Research Institute (KAERI) were assessed according to the ANSI/HPS N13.1-1999 specification. The velocity profile, flow angle and $10{\mu}m$ aerosol particle profile at the cross-section as functions of stack height L and stack diameter D (L/D) were assessed according to the sampling location criteria using COMSOL. The criteria for the velocity profile were found to be met at 5 L/D or more for the height, and the criteria for the average flow angle were met at all locations through this assessment. The criteria for the particle profile were met at 5 L/D and 9 L/D. However, the particle profile at the cross-section of each sampling location was found to be non-uniform. In order to establish uniformity of the particle profile, a static mixer and a perimeter ring were modeled, after which the degrees of effectiveness of these components were compared. Modeling using the static mixer indicated that the sampling locations that met the criteria for the particle profile were 5-10 L/D. When modeling using the perimeter ring, the sampling locations that met the criteria for particle profile were 5 L/D and 7-10 L/D. The criteria for the velocity profile and the average flow angle were also met at the sampling locations that met the criteria for the particle profile. The methodologies used in this study can also be applied during assessments of air sampling locations when monitoring stacks at new nuclear facilities as well as existing nuclear facilities.

WASHING-ELECTROKINETIC DECONTAMINATION FOR CONCRETE CONTAMINATED WITH COBALT AND CESIUM

  • Kim, Gye-Nam;Yang, Byeong-Il;Choi, Wang-Kyu;Lee, Kune-Woo;Hyeon, Jay-Hyeok
    • Nuclear Engineering and Technology
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    • v.41 no.8
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    • pp.1079-1086
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    • 2009
  • A great volume of radioactive concrete is generated during the operation and the decommissioning of nuclear facilities. The washing-electrokinetic technology in this study, which combined an electrokinetic method and a washing method, was developed to decontaminate the concrete generated in nuclear facilities. The results of only an electrokinetic decontamination for the concrete showed that cobalt was removed to below 1% from the concrete due to its high pH. Therefore, the washing-electrokinetic technology was applied to lower the pH of the concrete. Namely, when the concrete was washed with 3 M of hydrochloric acid for 4 hours (0.17 day), the $CaCO_3$ in the concrete was decomposed into $CO_2$ and the pH of the concrete was reduced to 3.7, and the cobalt and cesium in the concrete were removed by up to 85.0% and 76.3% respectively. Next, when the washed concrete was decontaminated by the electrokinetic method with 0.01M of acetic acid in the 1L electrokinetic equipment for 14.83 days, the cobalt and the cesium in the concrete were both removed by up to 99.7% and 99.6% respectively. The removal efficiencies of the cobalt and cesium by 0.01M of acetic acid were increased more than those by 0.05M of acetic acid due to the increase of the concrete zeta potential. The total effluent volume generated from the washing-electrokinetic decontamination was 11.55L (7.2ml/g).

Establishment of Release Limits for Airborne Effluent into the Environment Based on ALARA Concept (ALARA 개념(槪念)에 의한 기체상방사성물질(氣體狀放射性物質)의 환경방출한도(環境放出限度) 설정(設定))

  • Lee, Byung-Ki;Cha, Moon-Hoe;Nam, Soon-Kwon;Chang, Si-Young;Ha, Chung-Woo
    • Journal of Radiation Protection and Research
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    • v.10 no.1
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    • pp.50-63
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    • 1985
  • A derivation of new release limit, named Derived Release Limit(DRL), into the atomsphere from a reference nuclear power plant has been performed on the basis of the new system of dose limitation recommended by the ICRP, instead of the (MPC)a limit which has been currently used until now as a general standard for radioactive effluents in Korea. In DRL Calculation, a Concentration Factor Method was applied, in which the concentrations of long-term routinely released radionuclides were in equilibrium with dose in environment under the steady state condition. The analytical model used in the exposure pathway analysis was the one which has been suggested by the USNRC and the exposure limits applied in this analysis were those recommended by the USEPA lately. In the exposure pathway analysis, all of the pathways are not considered and some may be excluded either because they are not applicable or their contribution to the exposure is insignificant compared with other pathways. In case, the environmental model developed in this study was applied to the Kori nuclear power plant as the reference power plant, the highest DRL value was calculated to be as $9.10{\times}10^6Ci/yr$ for Kr-85 in external whole body exposure from the semi-infinite radioactive cloud, while the lowest DRL value was observed 3.64Ci/yr for Co-60 in external whole body exposure from the contaminated ground, by the radioactive particulates. The most critical exposure pathway to an individual in the unrestricted area of interest (Kilchun-Ri, 1.3 km to the north of the release point) seems to be the exposure pathway from the contaminated ground and the most critical radionuclide in all pathways appears to be Co-60 in the same pathway. When comparing the actual release rate from KNU-l in 1982 with the DRL's obtained here the release of radionuclides from KNU-1 were much lower than the DRL's and it could be conclued that the exposure to an individual had been kept below the exposure limits recommended by the USEPA.

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Status of a national monitoring program for environmental radioactivity and investigation of artificial radionuclide concentrations (134Cs, 137Cs, 131I) in rivers and lakes (방사성물질 측정망 현황 및 하천·호소 내 인공방사성물질 (134Cs, 137Cs, 131I) 조사)

  • Kim, Jiyu;Jung, Hyun-ji;An, Mijeong;Hong, Jung-Ki;Kang, Taegu;Kang, Tae-Woo;Cho, Yoon-Hae;Han, Yeong-Un;Seol, Bitna;Kim, Wansuk;Kim, Kyunghyun
    • Analytical Science and Technology
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    • v.28 no.6
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    • pp.377-384
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    • 2015
  • A survey of the artificial radionuclides in rivers and lakes was conducted to investigate their levels in surface water. Water samples were collected at 60 points and analyzed by gamma-ray spectrometry with a measurement time of 10,000 seconds for 134Cs, 137Cs, and 131I. The obained values were lower than MDA for all points, except one point for 131I that was 0.533±0.058 Bq/L. 131I is known as a radioactive material that occurs frequently in sewage treatment plants. Because it is often used for medical treatments and subject to spreading into the environment due to the excretion from the patients. For the point where 131I was detected, we conducted additional investigation on the upstream river point and the effluent points of nearby sewage treatment plant to find the source of 131I. 131I was not detected at the upstream points of one of the upstream sewage treatment plants but found at the downstream points with the level being 0.257±0.034 to 0.799±0.051 Bq/L, proving the sewage treatment plant was the 131Isource.

The Cesium Removal Using a Polysulfone Carrier Containing Nitric Acid-treated Bamboo Charcoal (질산으로 표면처리한 대나무 활성탄을 첨가한 폴리술폰 담체의 세슘제거 효율 규명)

  • Rahayu, Ni Wayan Sukma Taraning;Kim, Seonhee;Tak, Hyunji;Kim, Kyeongtae;Lee, Minhee
    • Economic and Environmental Geology
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    • v.53 no.5
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    • pp.529-542
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    • 2020
  • The cesium (Cs) sorption characteristics of a bead-type polysulfone carrier contained HNO3-treated bamboo charcoal (3 - 5 mm in diameter) in water system were investigated and its Cs removal efficiency as an adsorbent from water was also identified by various laboratory experiments. From the results of batch sorption experiments, the bead-type polysulfone carrier with only 5% HNO3-treated bamboo charcoal (P-5NBC) represented the high Cs removal efficiency of 57.8% for 1 hour sorption time. The Cs removal efficiency of P-5NBC in water after 24 hours reaction maintained > 69% at a wide range of pH and temperature conditions, attesting to its applicability under various water systems. Batch sorption experiments were repeated for P-5NBC coated with two cultivated microorganisms (Pseudomonas fluorescens and Bacillus drentensis), which were typical indigenous species inhabited in soil and groundwater. The Cs removal efficiency for two microorganisms coated polysulfone carrier (BP-5NBC) additionally increased by 19% and 18%, respectively, compared to that of only P-5NBC without microorganisms coated. The average Cs desorption rate of P-5NBC for 24 h was lower than 16%, showing the Cs was stably attached on HNO3-treated bamboo charcoal in so much as its long-term use. The maximum Cs sorption capacity (qm) of P-5NBC calculated from the Langmuir isotherm model study was 60.9 mg/g, which was much higher than those of other adsorbents from previous studies for 1 h sorption time. The results of continuous column experiments showed that the P-5NBC coated with microorganisms packed in the column maintained > 80% of the Cs removal efficiency during 100 pore volumes flushing. It suggested that only 14.7 g of P-5NBC (only 0.75 g of HNO3 treated bamboo charcoal included) can successfully clean-up 7.2 L of Cs contaminated water (the initial Cs concentration: 1 mg/L; the effluent concentration: < 0.2 mg/L). The present results suggested that the Cs contaminated water can be successfully cleaned up by using a small amount of the polysulfone carrier with HNO3-treated bamboo charcoal.