• Title/Summary/Keyword: Mass aerosol

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Numerical Computation of the Mass Transfer between Gaseous and Particulate Materials Considering the Hysteresis Phenomena of Atmospheric Aerosol (에어로솔의 이력현상을 고려한 대기 중 기체상/입자상 간의 물질전달 수치모사)

  • Kim, Du-Eil;Yoo, Kee-Youn
    • Journal of Korean Society for Atmospheric Environment
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    • v.26 no.2
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    • pp.202-218
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    • 2010
  • It is well known that the atmospheric inorganic aerosol has the hysteresis phenomena depending on the history of relative humidity. However, the current computational researches have assumed that the physical/chemical state of atmospheric aerosol is only determined by a branch of hysteresis, efflorescence or deliquescence. In this work, we applied the MATLAB-based UHAEROm thermodynamics module to simulate the dynamic interaction between gaseous species $NH_3$ and $HNO_3$, and the two mono-disperse particulate populations in the course of efflorescence and deliquescence, respectively. We conducted the 10 case studies considering the particulate phase with the atmospherically prevailing chemical composition and found that the final states of the particles are determined through the qualitatively five different trajectories by the dynamic interaction between gaseous and two different kinds of particulates. As a result, we show that the coexistence of meta-stable and stable particles drives the different physical/chemical destination comparing with the ones generated from the solitary efflorescence or deliquescence branch.

Change of the Size-Resolved Aerosol Concentration Due to Relative Humidity (습도 변화에 따른 에어로졸의 농도 및 크기의 변화경향 파악)

  • Jung, Chang Hoon;Park, Jin Hee;Kim, Yong Pyo
    • Particle and aerosol research
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    • v.9 no.2
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    • pp.69-78
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    • 2013
  • In this study, the atmospheric aerosol concentration measured at different relative humidity levels was analyzed. Using an optical particle counter, PM10 and PM2.5 concentration as well as particle size distribution were measured and the relation between these size resolved data and relative humidity was studied. The results showed that mass concentration increases as relative humidity increases. The comparison between PM1, PM2.5 and PM10 showed that the fine particles grow more than coarse particles as relative humidity increases. The results also showed that PM10-2.5 and relative humidity do not show close correlation, which means that the mass increase of PM10 at high relative humidity is mainly due to the growth of PM2.5.

Characteristics of Incheon Aerosol during Asian Dust Period in 2004 using Optical Particle Counter (OPC) (광학적 입자계수기를 이용한 2004년 황사기간 인천지역 에어로졸 특성)

  • Jung Chang-Hoon;Cho Yong-Sung;Lee Jong-Tae
    • Journal of Environmental Science International
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    • v.14 no.6
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    • pp.565-575
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    • 2005
  • The characteristics for the aerosol number distribution was studied during spring, 2004 in Incheon. Optical Particle Counter (OPC, HIAC/ROYCO 5230) was used in order to measure the number concentration of aerosol in the range of $0.3\~25{\mu}m.$. The obtained results were compared with $PM_{2.5}\;and\;PM_{10}$ data during Asian dust events. The results show that the size resolved aerosol number concentration from OPC measurement has a similar tendency with $PM_{10}\;and\;PM_{2.5}$ mass concentration. During Asian dust periods, the number concentrations in large particle $(CH5\~CH8)$ increase more than small particles which diameter is less than $2.23{\mu}m(CH5)$ and the same results were shown when $PM_{10}$ was compared with $PM_{2.5}$ data compared with non-dust days, Consequently, this study shows that size resolved aerosol number concentration from OPC measurement can be used as a useful tool in comparison of mass concentration data.

A Modeling Study on Aerosol Property Changes due to Sea-Salts (해염성분에 의한 에어로솔 물성변화 모사연구)

  • 김용표
    • Journal of Korean Society for Atmospheric Environment
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    • v.16 no.2
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    • pp.113-120
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    • 2000
  • Effects of sea-salts on the properties of aerosol collected in a coastal region were studied by applying a gas-particle equilibrium model SCAPE to the measurement data from Korea Cheju Island in summer 1994. It was found that the observed higher ammonium concentrations in fine particles (PM2.5) than in TSP were caused by forced evaporation of ammonium in coarse fraction of aerosol by sea-salts and the degree of evaporation was quantified through an application of SCAPE. By subtracting the sea-salt fraction from the measured concentra-tions the changes of aerosol property were also studied. The concentrations of nitrate at both TSP and PM2.5 decreased when alkaline sea-salt fraction was removed from the measured data. Estimates of aerosol acidity increased for most samples with sea salt loadings, However in some cases with high mass fractions of sea-salt components the aerosol acidity of PM2.5 decreased slightly. This is though to be related with the formation of solid salt with the removal of sea-salts.

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Analysis of Aerosol Dynamics, Heat and Mass Transfer in the Modified Chemical Vapor Deposition (수정된 화학증착공정에서 에어로졸 역학, 열전달 및 물질전달 해석)

  • Park, Kyong Soon;Lee, Bang Weon;Choi, Mansoo
    • Transactions of the Korean Society of Mechanical Engineers B
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    • v.23 no.2
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    • pp.262-271
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    • 1999
  • A study of aerosol dynamics has been done to obtain axially and radially varying size distributions of particles generated in the Modified Chemical Vapor Deposition process. Heat and mass transfer have also been studied since particle generation and deposition strongly depend on the temperature field in a tube. Bimodal size distributions of particles have been obtained both in the particulate flow and in the deposited particle layer for the first time using the sectional method to solve aerosol dynamics. Variations of geometric mean diameter, geometric standard deviation have been studied for various parameters; flow rates and maximum wall temperature. The comparison between one-dimensional and two-dimensional approaches has also been made.

Detection of Asian Dust Air-mass based on Short Wavelength Observation of SeaWiFS

  • Fukushima, H.;Hagihara, Y.;Hoshikuma, Y.;Ohta, S.;Uno, I.
    • Proceedings of the KSRS Conference
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    • 2003.11a
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    • pp.1203-1205
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    • 2003
  • To detect dust-loaded air-mass over land and ocean, we propose an index, which is essentially the difference in Rayleigh-corrected reflectance between 412 and 443 nm bands of SeaWiFS. Radiative transfer simulations are conducted to show that the index is linearly related to the optical thickness of modeled dust-contaminated aerosol while showing insensitivity against non-absorbing model aerosols. Asian SeaWiFS data set of 2001 spring is used to produce daily composite imagery of the index, which compares well with TOMS Aerosol Index and with predicted aerosol optical thickness predicted by CFORS chemical weather forecast.

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Performance Evaluation of Gas Cleaning Industrial Filters using a Bi-Modal Test Aerosol for Dust Loading Studies

  • Lee, Jae-Keun;Kim, Seong-Chan;Benjamin Y.H. Liu
    • Journal of Energy Engineering
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    • v.5 no.2
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    • pp.131-137
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    • 1996
  • Typical size distribution of emission particulates is bi-modal in shape with particles in the fine mode (< 2.0 $\mu\textrm{m}$) and the coarse mode. An experimental study of pressure drop across the industrial gas cleaning filters has been conducted using particle mixture of fine alumina and coarse Arizona dusts with a rotating aerosol disperser to generate the bi-modal test aerosol. Pressure drop increased linearly with increasing mass loading. The pressure drop was found to be strongly dependent upon the mass ratio of fine to coarse particles. The smaller the mass ratio of fine to coarse particles and the higher face velocity are, the faster pressure drop rises. The fine particles and the greater inertia of the particle moving fast would cause a denser cake formation on the filter surface, resulting in a greater specific resistance to the gas flow.

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A case study of aerosol features of Asian dust, fog, clear sky, and cloud at Anmyeon Island in April 2006 (2006년 4월 안면도에서 발생한 황사, 안개, 청명, 구름 사례에 대한 에어러솔 특성 분석)

  • Goo, Tae-Young;Hong, Gi-Man;Kim, Sang-Beak;Gong, Jong-Ung;Kim, Myoung-Soo
    • Atmosphere
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    • v.18 no.2
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    • pp.97-109
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    • 2008
  • The aerosol characteristics in terms of 4 different cases (Asian dust, fog, clear sky and cloud) which had happened at Anmyeon Island in April 2006 were studied using various measurements such as the Micro Pulse Lidar (MPL), sunphotometer, $\beta$-ray $PM_{10}$ Analyzer, anemoscope and anemometer. In addition, synoptic charts, back trajectory analyses and satellite images were also used to help characterize the aerosol events. The aerosol optical properties were featured by the Aerosol Optical Depth (AOD) and ${\AA}ngstr\ddot{o}m$ exponent which were estimated by the sunphotometer. When Anmyeon Island was dominated by the Asian dust, the AOD was sharply increased as seven times as a yearly average of it (0.35). As compared with a yearly average of the ${\AA}ngstr\ddot{o}m$ exponent of 0.97, the ${\AA}ngstr\ddot{o}m$ exponent of a dust day was significantly low (0.099). In addition, $PM_{10}$ mass concentration showed an extremely high record. The maximum concentration reached $1790.5{\mu}gm^{-3}$ on 8 April 2006. The maximum mass concentration was shown with delay when the wind speed of $0ms^{-1}$ was observed. It was also found that a satellite image of the MODIS-RGB had a good agreement with the results of those measurements. It was shown that the MPL was able to describe effectively the vertical distribution of aerosol for all the cases. In particular, the MPL evidently captured the aerosol layer before the cloud observation. The aerosol layer was similarly described by the AOD. On a clear sky day, the AOD had not only a very low value (0.054) but also a feature of homogeneity.

Characteristics of long-range transported PM2.5 at a coastal city using the single particle aerosol mass spectrometry

  • Cai, Qiuliang;Tong, Lei;Zhang, Jingjing;Zheng, Jie;He, Mengmeng;Lin, Jiamei;Chen, Xiaoqiu;Xiao, Hang
    • Environmental Engineering Research
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    • v.24 no.4
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    • pp.690-698
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    • 2019
  • Air pollution has attracted ever-increasing attention because of its substantial influence on air quality and human health. To better understand the characteristics of long-range transported pollution, the single particle chemical composition and size were investigated by the single particle aerosol mass spectrometry in Fuzhou, China from 17th to 22nd January, 2016. The results showed that the haze was mainly caused by the transport of cold air mass under higher wind speed (10 m·s-1) from the Yangtze River Delta region to Fuzhou. The number concentration elevated from 1,000 to 4,500 #·h-1, and the composition of mobile source and secondary aerosol increased from 24.3% to 30.9% and from 16.0% to 22.5%, respectively. Then, the haze was eliminated by the clean air mass from the sea as indicated by a sharp decrease of particle number concentration from 4,500 to 1,000 #·h-1. The composition of secondary aerosol and mobile sources decreased from 29.3% to 23.5% and from 30.9% to 23.1%, respectively. The particles with the size ranging from 0.5 to 1.5 ㎛ were mainly in the accumulation mode. The stationary source, mobile source, and secondary aerosol contributed to over 70% of the potential sources. These results will help to understand the physical and chemical characteristics of long- range transported pollutants.

Opto-Chemical Characteristics of Visibility Impairment Using Semi-Continuous Aerosol Monitoring in an Urban Area during Summertime (에어로졸의 준실시간 관측에 의한 여름철 도시지역 시정 감쇄 현상의 광ㆍ화학적인 특성 분석)

  • 김경원;김영준
    • Journal of Korean Society for Atmospheric Environment
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    • v.19 no.6
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    • pp.647-661
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    • 2003
  • For continuous monitoring of atmospheric visibility in the city of Kwanaju, Korea, a transmissometer system consisting of a transmitter and a receiver was installed at a distance of 1.91 km across the downtown Kwanaju. At the transmitter site an integrating nephelometer and an aethalometer were also installed to measure the scattering and absorption coefficients of the atmosphere, respectively. At the receiver site. an URG PM$_{2.5}$ cyclone sampler and an URG-VAPS (Versatile Air Pollutant Sampler) with three filter packs and two denuders were used to collect both PM$_{2.5}$ and PM$_{10}$ samples at a 2-hour or 12-hour sampling interval for aerosol chemical analysis. Sulfate, organic mass by carbon (OMC), nitrate, elemental carbon (EC) components of fine aerosol were the major contributors to visibility impairment. Diurnal variation of visibility during best-case days showed rapid improvement in the morning hours, while it was delayed until afternoon during the worst-case days. Aerosol mass concentration of each aerosol component for the worst-case was calculated to be 11.2 times larger than the best-case for (NH$_4$)$_2$SO$_4$(NHSO), 19.0 times for NH$_4$NO$_3$ (NHNO), 2.2 times for OMC, respectively. Also result shows that elemental carbon and fine soil (FS) were 3.7 and 2.2 times more than those of best-case. respectively- Sum of total contributions of wet NHSO and NHNO to light extinction was calculated to be 301 Mm$^{-1}$ for the worst-case. However, sum of contributions by dry NHSO and NHNO was calculated to be 123 Mm$^{-1}$ for the best case. Mass extinction efficiencies of fine and coarse particles were calculated to be 5.8$\pm$0.3 $m^2$/g and 1.8$\pm$0.1 $m^2$/g, respectively.ely.