• 제목/요약/키워드: Isotope Production

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13C 추적자를 이용한 팔당호 수변역 부유 및 부착조류의 일차생산력과 광합성 색소 생산속도 연구 (Primary Productivity and Photosynthetic Pigment Production Rates of Periphyton and Phytoplankton in Lake Paldang using 13C Tracer)

  • 민준오;하선용;허진;신경훈
    • 생태와환경
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    • 제52권3호
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    • pp.202-209
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    • 2019
  • 팔당호 수변지역 내 부유조류와 부착조류의 일차생산력은 부착조류의 일차생산력이 더 높게 나타났다. 따라서 수변 지역이나 하천에서는 부착조류에 의한 유기물 생성이 주요한 수생태계 에너지 공급원이 될 것으로 판단된다. 본 연구를 통해 국내에서 처음으로 지표색소의 생산속도 분석결과가 제시되었는데 향후 일차생산력을 측정하는 데 있어서 조류의 총 일차생산력으로 국한된 측정 방법을 좀 더 세분화하여 특정 조류의 기여도 및 개별 생산력을 판단하는 데 유용하게 사용될 것으로 사료된다.

COMPUTATIONAL INVESTIGATION OF 99Mo, 89Sr, AND 131I PRODUCTION RATES IN A SUBCRITICAL UO2(NO3)2 AQUEOUS SOLUTION REACTOR DRIVEN BY A 30-MEV PROTON ACCELERATOR

  • GHOLAMZADEH, Z.;FEGHHI, S.A.H.;MIRVAKILI, S.M.;JOZE-VAZIRI, A.;ALIZADEH, M.
    • Nuclear Engineering and Technology
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    • 제47권7호
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    • pp.875-883
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    • 2015
  • The use of subcritical aqueous homogenous reactors driven by accelerators presents an attractive alternative for producing $^{99}Mo$. In this method, the medical isotope production system itself is used to extract $^{99}Mo$ or other radioisotopes so that there is no need to irradiate common targets. In addition, it can operate at much lower power compared to a traditional reactor to produce the same amount of $^{99}Mo$ by irradiating targets. In this study, the neutronic performance and $^{99}Mo$, $^{89}Sr$, and $^{131}I$ production capacity of a subcritical aqueous homogenous reactor fueled with low-enriched uranyl nitrate was evaluated using the MCNPX code. A proton accelerator with a maximum 30-MeV accelerating power was used to run the subcritical core. The computational results indicate a good potential for the modeled system to produce the radioisotopes under completely safe conditions because of the high negative reactivity coefficients of the modeled core. The results show that application of an optimized beam window material can increase the fission power of the aqueous nitrate fuel up to 80%. This accelerator-based procedure using low enriched uranium nitrate fuel to produce radioisotopes presents a potentially competitive alternative in comparison with the reactor-based or other accelerator-based methods. This system produces ~1,500 Ci/wk (~325 6-day Ci) of $^{99}Mo$ at the end of a cycle.

Recent Developments in Nuclear Forensic and Nuclear Safeguards Analysis Using Mass Spectrometry

  • Song, Kyuseok;Park, Jong-Ho;Lee, Chi-Gyu;Han, Sun-Ho
    • Mass Spectrometry Letters
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    • 제7권2호
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    • pp.31-40
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    • 2016
  • The analysis of nuclear materials and environmental samples is an important issue in nuclear safeguards and nuclear forensics. An analysis technique for safeguard samples has been developed for the detection of undeclared nuclear activities and verification of declared nuclear activities, while nuclear forensics has been developed to trace the origins and intended use of illicitly trafficked nuclear or radioactive materials. In these two analytical techniques, mass spectrometry has played an important role in determining the isotope ratio of various nuclides, contents of trace elements, and production dates. These two techniques typically use similar analytical instruments, but the analytical procedure and the interpretation of analytical results differ depending on the analytical purpose. The isotopic ratio of the samples is considered the most important result in an environmental sample analysis, while age dating and impurity analysis may also be important for nuclear forensics. In this review, important aspects of these techniques are compared and the role of mass spectrometry, along with recent progress in related technologies, are discussed.

남서태평양 리코후 드리프트 퇴적층의 쇄설성 실트입자 크기의 수직적 변화를 이용한 플라이스토세 후기 심해서안경계해류의 세기 변화 (Late Pleistocene Variation in Intensity of Deep Western Boundary Current from Vertical Change in Size of Terrigenous Silt in the Rekohu Sediment Drift, SW Pacific)

  • 김부근;이영주;박유현;박장준
    • Ocean and Polar Research
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    • 제28권4호
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    • pp.451-457
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    • 2006
  • Hole 1124 of ODP Leg 181 was located in the Rekohu sediment drift off eastern New Zealand in the southwest Pacific Ocean. Mean gain sizes of sortable silt were measured in two drilled cores (1124A and l124B). Chronostratigraphy of core 1124 was correlated with the well-dated nearby core S931, resulting that the age of core 1124 covers the late Pleistocene spanning about MIS (Marine Isotope Stage) 5. Mean grain size of sortable silt seemed to be relatively large during the glacial period, whereas that of the interglacial period was smaller, although several tephra layers contain some coarse-grained pyroclatic particles. The variation in mean grain size of sortable silt in Rekohu sediment drift during the late Pleistocene indicates that the intensity of Deep Western Boundary Current (DWBC) might have been enhanced during the glacial period as a result of increased production of Antarctic Bottom Water (AABW).

Neutronics analysis of TRIGA Mark II research reactor

  • Rehman, Haseebur;Ahmad, Siraj-ul-Islam
    • Nuclear Engineering and Technology
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    • 제50권1호
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    • pp.35-42
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    • 2018
  • This article presents clean core criticality calculations and control rod worth calculations for TRIGA (Training, Research, Isotope production-General Atomics) Mark II research reactor benchmark cores using Winfrith Improved Multi-group Scheme-D/4 (WIMS-D/4) and Program for Reactor In-core Analysis using Diffusion Equation (PRIDE) codes. Cores 133 and 134 were analyzed in 2-D (r, ${\theta}$) and 3-D (r, ${\theta}$, z), using WIMS-D/4 and PRIDE codes. Moreover, the influence of cross-section data was also studied using various libraries based on Evaluated Nuclear Data File (ENDF/B-VI.8 and VII.0), Joint Evaluated Fission and Fusion File (JEFF-3.1), Japanese Evaluated Nuclear Data Library (JENDL-3.2), and Joint Evaluated File (JEF-2.2) nuclear data. The simulation results showed that the multiplication factor calculated for all these data libraries is within 1% of the experimental results. The reactivity worth of the control rods of core 134 was also calculated with different homogenization approaches. A comparison was made with experimental and reported Monte Carlo results, and it was found that, using proper homogenization of absorber regions and surrounding fuel regions, the results obtained with PRIDE code are significantly improved.

Expression and Purification of a Cathelicidin-Derived Antimicrobial Peptide, CRAMP

  • Park Eu-Jin;Chae Young-Kee;Lee Jee-Young;Lee Byoung-Jae;Kim Yang-Mee
    • Journal of Microbiology and Biotechnology
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    • 제16권9호
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    • pp.1429-1433
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    • 2006
  • Application of recombinant protein production and particularly their isotopic enrichment has stimulated development of a range of novel multidimensional heteronuclear NMR techniques. Peptides in most cases are amenable to assignment and structure determination without the need for isotopic labeling. However, there are many cases where the availability of $^{15}N$ and/or $^{13}C$ labeled peptides is useful to study the structure of peptides with more than 30 residues and the interaction between peptides and membrane. CRAMP (Cathelicidin-Related AntiMicrobial Peptide) was identified from a cDNA clone derived from mouse femoral marrow cells as a member of cathelicidin-derived antimicrobial peptides. CRAMP was successfully expressed as a GST-fused form in E. coli and purified using affinity chromatography and reverse-phase chromatography. The yield of the CRAMP was 1.5 mg/l 1. According to CD spectra, CRAMP adopted ${\alpha}$-helical conformation in membrane-mimetic environments. Isotope labeling of CRAMP is expected to make it possible to study the structure and dynamic properties of CRAMP in various membrane systems.

DESIGN OF LSDS FOR ISOTOPIC FISSILE ASSAY IN SPENT FUEL

  • Lee, Yongdeok;Park, Chang Je;Kim, Ho-Dong;Song, Kee Chan
    • Nuclear Engineering and Technology
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    • 제45권7호
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    • pp.921-928
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    • 2013
  • A future nuclear energy system is being developed at Korea Atomic Energy Research Institute (KAERI), the system involves a Sodium Fast Reactor (SFR) linked with the pyro-process. The pyro-process produces a source material to fabricate a SFR fuel rod. Therefore, an isotopic fissile content assay is very important for fuel rod safety and SFR economics. A new technology for an analysis of isotopic fissile content has been proposed using a lead slowing down spectrometer (LSDS). The new technology has several features for a fissile analysis from spent fuel: direct isotopic fissile assay, no background interference, and no requirement from burnup history information. Several calculations were done on the designed spectrometer geometry: detection sensitivity, neutron energy spectrum analysis, neutron fission characteristics, self shielding analysis, and neutron production mechanism. The spectrum was well organized even at low neutron energy and the threshold fission chamber was a proper choice to get prompt fast fission neutrons. The characteristic fission signature was obtained in slowing down neutron energy from each fissile isotope. Another application of LSDS is for an optimum design of the spent fuel storage, maximization of the burnup credit and provision of the burnup code correction factor. Additionally, an isotopic fissile content assay will contribute to an increase in transparency and credibility for the utilization of spent fuel nuclear material, as internationally demanded.

Identification of 1H-NMR characteristics for black ginger specimens from different places of origin

  • Kwon, Hyeok;Lee, Sojung;Hong, Sukyung;Kiyonga, Alice Nguvoko;Yi, Jong-Jae;Jung, Kiwon;Son, Woo Sung
    • 한국자기공명학회논문지
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    • 제23권4호
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    • pp.93-97
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    • 2019
  • Black ginger (Kaempferia parviflora) is a short-lived ginger plant with dark purple colored root and is known to be effective in treating diabetes and obesity. To find out the difference in the characteristics of the black ginger according to the variety of production, 1D proton NMR experiments were performed on 4 types of black gingers from different regions. The NMR spectra of all black ginger showed the characteristic peaks of the polymethoxy flavone compounds, and the chemical shifts and intensity of peaks showed slight differences depending of the type of black ginger implying the difference in molecular environment. These initial NMR experiments can be applied to the identification of the diversity of black ginger in physiological function according to the climate of regions using SNIF-NMR (Site-specific Natural Isotope Fractionation studied by NMR).

Molybdenum isotopes separation using squared-off optimized cascades

  • Mahdi Aghaie;Valiyollah Ghazanfari
    • Nuclear Engineering and Technology
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    • 제55권9호
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    • pp.3291-3300
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    • 2023
  • Recently molybdenum alloys have been introduced as accident tolerating materials for cladding of fuel rods. Molybdenum element has seven stable isotopes with different neutron absorption cross section used in various fields, including nuclear physics and radioisotope production. This study presents separation approaches for all intermediate isotopes of molybdenum element by squared-off cascades using a newly developed numerical code with Salp Swarm Algorithm (SSA) optimization algorithm. The parameters of cascade including feed flow rate, feed entry stage, cascade cut, input feed flow rate to gas centrifuges (GCs), and cut of the first stage are optimized to maximize both isotope recovery and cascade capacity. The squared off and squared cascades are studied, and the efficiencies are compared. The results obtained from the optimization showed that for the selected squared off cascade, Mo94 in four separation steps, Mo95 in five steps, Mo96 in six steps, Mo97 in seven steps, and Mo98 in two steps are separated to the desired concentrations. The highest recovery factor is obtained 63% for Mo94 separation and lowest recovery factor is found 45% for Mo95.

Assessment of neutron-induced activation of irradiated samples in a research reactor

  • Ildiko Harsanyi;Andras Horvath;Zoltan Kis;Katalin Gmeling;Daria Jozwiak-Niedzwiedzka;Michal A. Glinicki;Laszlo Szentmiklosi
    • Nuclear Engineering and Technology
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    • 제55권3호
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    • pp.1036-1044
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    • 2023
  • The combination of MCNP6 and the FISPACT codes was used to predict inventories of radioisotopes produced by neutron exposure of a sample in a research reactor. The detailed MCNP6 model of the Budapest Research Reactor and the specific irradiation geometry of the NAA channel was established, while realistic material cards were specified based on concentrations measured by PGAA and NAA, considering the precursor elements of all significant radioisotopes. The energy- and spatial distributions of the neutron field calculated by MCNP6 were transferred to FISPACT, and the resulting activities were validated against those measured using neutron-irradiated small and bulky targets. This approach is general enough to handle different target materials, shapes, and irradiation conditions. A general agreement within 10% has been achieved. Moreover, the method can also be made applicable to predict the activation properties of the near-vessel concrete of existing nuclear installations or assist in the optimal construction of new nuclear power plant units.