• Proceedings of the Optical Society of Korea Conference
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• 2000.02a
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• pp.18-19
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• 2000

Recently, coherent control of exciton populations has been demonstrated through terahertz, reflection, and four-wave-mixing experiments. However, the most direct probe of exciton population control is the absorption, which has been lacking in previous studies. In this report, we probe the time evolution of exciton population directly through a transmission experiment. In particular, using upconversion technique with both narrow (spectrally broad) and long (spectrally narrow) pulses, we can obtain both the temporal and the spectral information. The main thrust of our report is that when phase controlled, the second pulse can be either greatly enhanced or completely destroyed by gaining energy from exciton (thus destroying the exciton population) or giving all of its energy to the system (thus greatly increasing the exciton population), respectively. (omitted)

• Journal of the Optical Society of Korea
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• v.2 no.1
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• pp.22-25
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• 1998

We present a spectrum broadening technique to improve the signal-to-noise ratio of spectrum sliced incoherent light sources using the fiber four-wave mixing effect which occurs in a nonlinear loop mirror located at the receiver. The initial transmission channel bandwidth of 0.92 nm was increased to 1.62 nm in the nonlinear loop mirror at the optical receiver, which enhances the signal-to-noise ratio to a desired value. Using this technique, we have demonstrated the transmission of a 2.5 Gb/s NRZ signal with the 0.92 nm bandwidth through a 80 km dispersion-shifted fiber. The measured transmission penalty was less than 0.2 dB at $1{\imes}10^{-10}$ BER.

• Bulletin of the Korean Chemical Society
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• v.16 no.2
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• pp.126-129
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• 1995

Linear and nonlinear optical properties of CuCl nanocrystals in silica glass have been studied using low temperature absorption, degenerate four wave mixing (DFWM), and time-resolved photoluminescence spectroscopy. Assuming a spherical shape, effective radius of the CuCl quantum dots was estimated to be 2.5 nm, which is obtained from low temperature absorption data. The DFWM experiment was performed in 380-386 nm wavelength region, and the diffracted signal was measured as a function of wavelength with 1.0 nm interval. Time-resolved photoluminescence measurement was also carried out at 77 K to obtain the time response of CuCl nanocrystals. The experimental results on the large third order nonlinear optical of CuCl quantum dots are explained in terms of crystal size and oscillator strength of quantum spheres.

• Bulletin of the Korean Chemical Society
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• v.17 no.7
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• pp.607-612
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• 1996

A series of new NLO-active poly(4-nitrophenylallylamine) derivatives was synthesized by the nucleophilic substitution reaction of several substituted 4-nitrohalobenzenes and poly(allylamine hydrochloride). All polymers obtained were amorphous and their glass transition temperatures (Tg) were observed around 148-160 ℃. For each of these polymers, their specific Tg values were dependent on characteristic electronic structures. UV-visible absorption spectra showed maximum absorption intensity at 355-393 nm for π-π* transition of alkylaminonitrophenyl groups. The χ(2)value of poly(4-nitrophenylallylamine), as determined by the second harmonic generation at 1064 nm, for a thin polymer film poled at an elevated temperature, was 1.4x10-8esu. The third-order NLO properties of poly(4-nitrophenylallylamine) derivatives were evaluated through measurement of degenerate four-wave mixing technique and χ(3) coefficient in the range of 2.7~3.2x10-12 esu at 602 nm was found with 400 fs laser pulses.

• Macromolecular Research
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• v.17 no.11
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• pp.874-878
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• 2009

Photorefractive polymer composites were synthesized based on poly (N-vinylcazbazole) (PVK) doped with liquid nonlinear optical chromophores and a sensitizer $C_{60}$. PVK/liquid NLO chromophores/$C_{60}$ devices showed no signs of phase separation and did not require a plasticizer, such as ethylcarbazole. The composites showed 69% diffraction efficiency (C3) and a rapid response time of 46 ms (C1) in four-wave mixing experiments at a light intensity of $60\;mW/cm^2$ and a wavelength of 633 nm.

• Korean Journal of Optics and Photonics
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• v.9 no.1
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• pp.20-24
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• 1998

Fiber four-wave mixing(FWM) in zero-dispersion wavelength region is studied. FWM efficiency of -26 dBm and bandwidth of 2nm are measured. The linear dispersion slope in zero-dispersion wavelength region is calculated from the modulation behavior of FWM efficiency.

• Electronics and Telecommunications Trends
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• v.34 no.5
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• pp.91-98
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• 2019

Optical frequency comb generators have been investigated as a signal source capable of generating highly stabilized ultrafast pulse lasers. The precise control of the optical frequency comb spacing by RF clock signals has led to a revolutionary paradigm shift in the precise measurement of time and frequency. Optical frequency combs also have advantages such as stable frequency spacing, stable number of lines, and robustness. Owing to these characteristics, optical frequency combs have been applied to the fields of high precision optical clock, communication, spectroscopy, waveform generation, and astronomy. In this article, we introduce the properties (i.e., generation methods, advantages, and so on) of various optical frequency combs, and discuss the expected future technological trends and applications.

• Journal of the Korea Institute of Information and Communication Engineering
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• v.12 no.2
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• pp.328-335
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• 2008

The system performance of NRZ format in WDM transmission system with lumped dispersion management(DM) and optical phase conjugator(OPC) is compared with that of RZ format. It is confirmed that eye opening penalty(EOP) of both NRZ and RZ format in WDM transmission system having lumped DM combined with OPC are greatly improved than those in WDM system with only OPC. The optimal net residual dispersion(NRD) in the case of RZ format is decided to so small value that path-averaged dispersion coefficient become almost zero, while that in the case of NRZ format is decided to larger value, for the best improvement of overall WDM channels. It is also confirmed that EOP in the case of RZ format is more improved than that in the case of NRZ format in lumped DM with optimal NRD. This is resulted from that lumped DM combined with OPC suppress the signal distortion due to intrachannel four-wave mixing(IFWM) and intrachannel cross phase modulation(IXPM). Consequently, lumped DM combined with OPC proposed in this paper is effective technique to mitigate intrachannel nonlinearities in WDM transmitting RZ format.

• Bulletin of the Korean Chemical Society
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• v.29 no.1
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• pp.177-180
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• 2008

Laser induced fluorescence studies of hydrogen atom using four wave mixing technique are reported for the photodissociation of CH4 and its isotopomers at Lya (121.6 nm). The source of dissociating and probe radiation is one and the same (delay time??20 nsec). The average translational energy of ejected hydrogen atoms (50 Kcal/mol) reveals that CH4 + hn??CH3 + H(2S) and CH4 + hn??CH2(a1A1) + H2(1Sg) are the main dissociation processes. The absolute quantum yield for CH4 and CD4 are the same, FH(CH4) = FD(CD4) = 0.31 0.05. If one divides the experimental H/D ratios from the isotopomers CH3D, CH2D2, CHD3 by the isotopic H/D ratios, a value 2 is obtained in all three cases. Overall, the heavier D atoms are more likely than the H atoms to remain attached to the carbon atom.

• Macromolecular Research
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• v.11 no.4
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• pp.250-255
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• 2003

We prepared the photorefractive sol-gel glass based on organic-inorganic hybrid materials containing a charge transporting molecule, second-order nonlinear optical (NLO) chromophore, photosensitizer, and plasticizer. Carbazole and 2-{ 4-[(2-hydroxy-ethyl)-methyl-amino]-benzylidene}-malononitrile were reacted with isocyanato-triethoxy silane and the functionalized silanes were employed to fabricate the efficient photorefractive media induding 2,4,7-trinitrot1uorenone (TNF) to form a charge transfer complex. The prepared sol-gel glass samples showed a large net gain coefficient and high diffraction efficiency at a certain composition. As the concentration of photosensitizer increased, the photorefractive properties were enhanced due to an increment of charge carrier density. Dynamic behavior of the diffraction efficiency was also investigated with the concentration of the photosensitizer.