• Title/Summary/Keyword: Deep Geological Disposal

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Surface Modification of Bentonite for the Improvement of Radionuclide Sorption

  • Hong, Seokju;Kim, Jueun;Um, Wooyong
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.20 no.1
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    • pp.1-12
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    • 2022
  • Bentonite is the most probable candidate to be used as a buffer in a deep geological repository with high swelling properties, hydraulic conductivity, thermal conductivity, and radionuclide sorption ability. Among them, the radionuclide sorption ability prevents or delays the transport of radionuclides into the nearby environment when an accident occurs and the radionuclide leaks from the canister, so it needs to be strengthened in terms of long-term disposal safety. Here, we proposed a surface modification method in which some inorganic additives were added to form NaP zeolite on the surface of the bentonite yielded at Yeonil, South Korea. We confirmed that the NaP zeolite was well-formed on the bentonite surface, which also increased the sorption efficiency of Cs and Sr from groundwater conditions. Both NaP and NaX zeolite can be produced and we have demonstrated that the generation mechanism of NaX and NaP is due to the number of homogeneous/heterogeneous nucleation sites and the number of nutrients supplied from an aluminosilicate gel during the surface modification process. This study showed the potential of surface modification on bentonite to enhance the safety of deep geological radioactive waste repository by improving the radionuclide sorption ability of bentonite.

Cross-verified Measurement of Sulfide Concentration in Anaerobic Conditions Using Spectroscopic, Electrochemical, and Mass Spectrometric Methods

  • Nakkyu Chae;Samuel Park;Sungyeol Choi
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.21 no.1
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    • pp.43-53
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    • 2023
  • Sulfide concentrations critically affect worker safety and the integrities of underground facilities, such as deep geological repositories for spent nuclear fuel. Sulfide is highly sensitive to oxygen, which can oxidize sulfide to sulfate. This can hinder precise measurement of the sulfide concentration. Hence, a literature review was conducted, which revealed that two methods are commonly used: the methylene blue and sulfide ion-selective electrode (ISE) methods. Inductively coupled plasma optical emission spectroscopy (ICP-OES) was used for comparison with the two methods. The sulfide ISE method was found to be superior as it yielded results with a higher degree of accuracy and involved fewer procedures for quantification of the sulfide concentration in solution. ICP-OES results can be distorted significantly when sulfide is present in solution owing to the formation of H2S gas in the ICP-OES nebulizer. Therefore, the ICP-OES must be used with caution when quantifying underground water to prevent any distortion in the measured results. The results also suggest important measures to avoid problems when using ICP-OES for site selection. Furthermore, the sulfide ISE method is useful in determining sulfide concentrations in the field to predict the lifetime of disposal canisters of spent nuclear fuel in deep geological repositories and other industries.

Preliminary Selection of Safety-Relevant Radionuclides for Long-Term Safety Assessment of Deep Geological Disposal of Spent Nuclear Fuel in South Korea

  • Kyu Jung Choi;Shin Sung Oh;Ser Gi Hong
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.21 no.4
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    • pp.451-463
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    • 2023
  • With South Korea increasingly focusing on nuclear energy, the management of spent nuclear fuel has attracted considerable attention in South Korea. This study established a novel procedure for selecting safety-relevant radionuclides for long-term safety assessments of a deep geological repository in South Korea. Statistical evaluations were performed to identify the design basis reference spent nuclear fuels and evaluate the source term for up to one million years. Safety-relevant radionuclides were determined based on the half-life criteria, the projected activities for the design basis reference spent nuclear fuel, and the annual limit of ingestion set by the Nuclear Safety and Security Commission Notification No. 2019-10 without considering their chemical and hydrogeological properties. The proposed process was used to select 56 radionuclides, comprising 27 fission and activation products and 29 actinide nuclides. This study explains first the determination of the design basis reference spent nuclear fuels, followed by a comprehensive discussion on the selection criteria and methodology for safety-relevant radionuclides.

Review of In-situ Installation of Buffer and Backfill and Their Water Saturation Management for a Deep Geological Disposal System of Spent Nuclear Fuel (국외 사례를 통한 사용후핵연료 심층처분시스템 완충재 및 뒤채움재의 현장시공 및 포화도 관리 기술 분석)

  • Ju-Won Yun;Won-Jin Cho;Hyung-Mok Kim
    • Tunnel and Underground Space
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    • v.34 no.2
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    • pp.104-126
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    • 2024
  • Buffer and backfill play an essential role in isolating high-level radioactive waste and retard the migration of leaked radionuclides in deep geological disposal system. A bentonite mixture, which exhibits a swelling property, is considered for buffer and backfill materials, and excessive groundwater inflow from surrounding rock mass may affect stability and efficiency of their role as an engineered barrier. Therefore, stringent quality control as well as in-situ installation management and inflow water constrol for buffer and backfill are required to ensure the safety of deep disposal facilities. In this study, we analyzed the design requirements of buffer and backfill by examining various laboratory tests and a field study of the Steel Tunnel Test at the Äspö Hard Rock Laboratory in Sweden. We introduced how to control the quality of buffer and backfill construction in-field, and also presented how to handle excessive groundwater inflow into disposal caverns, validating the groundwater retention capacity of bentonite pellets and the effectiveness of geotexile use.

Suggestion on Screening Concept of Radionuclides to be Considered for the Radiological Safety Assessment of the Domestic KBS-3 Type Geological Disposal Facility of High-level Radioactive Waste(HLW) (국내 KBS-3 방식 고준위방사성폐기물 심층처분시설 방사선학적 안전성 평가 대상 방사성핵종 목록 선정개념(안) 제언)

  • Sukhoon Kim;Donghyun Lee;Dong-Keuk Park
    • Journal of Radiation Industry
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    • v.17 no.1
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    • pp.45-59
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    • 2023
  • The transport calculation for a wide variety of radionuclides contained in high-level radioactive waste, especially spent nuclear fuel, is computationally difficult, and input data collection for this also take a considerable amount of time. Accordingly, considering limited resources, it is possible to reduce the calculation time while minimizing impact on accuracy by including only radionuclides important to calculation result through applying some criteria among potential radiation source terms that may release into environment. In this paper, therefore, we reviewed and analyzed the screening process performed to select radionuclides to be considered in the safety assessment for the KBS-3 type repository in Sweden and Finland. In both countries, it was confirmed that a list of radionuclides was selected by comprehensively considering screening criteria such as radioactivity inventory, half-life, radiotoxicity, risk quotient, and transport properties, and etc. A comparison of radionuclides included in the radiological safety assessment in both countries suggests that most of nuclides are considered in common, and a few nuclides considered only in one country are due to differences in decay chain treatment or spent fuel types. As of now, since most of information on the disposal facility in Korea has not been determined, it is necessary to comprehensively model release and transport of all radionuclides considered in Sweden and Finland when performing the radiological safety assessment. Based on these results, we derived the screening concept of selecting a list of radionuclides to be considered in the radiological safety assessment for the domestic KBS-3 type geological disposal facility, and this result is expected to be used as technical basis for confirming conformity with the safety objective. In a more detailed evaluation reflecting domestic characteristics in the future, it would be desirable to consider only radionuclides selected in accordance with the screening procedure. However, further research should be conducted to determine the quantitative limit for each criteria.

Review of International Cases for Managing Input Data in Safety Assessment for High-Level Radioactive Waste Deep Disposal Facilities (고준위방사성폐기물 심층처분시설 안전성평가 입력자료 관리를 위한 해외사례 분석)

  • Mi Kyung Kang;Hana Park;Sunju Park;Hae Sik Jeong;Woon Sang Yoon;Jeonghwan Lee
    • Economic and Environmental Geology
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    • v.56 no.6
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    • pp.887-897
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    • 2023
  • Leading waste disposal countries, such as Sweden, Switzerland, and the United Kingdom, conduct safety assessments across all stages of High-Level Radioactive Waste Deep Geological Disposal Facilities-from planning and site selection to construction, operation, closure, and post-closure management. As safety assessments are repeatedly performed at each stage, generating vast amounts of diverse data over extended periods, it is essential to construct a database for safety assessment and establish a data management system. In this study, the safety assessment data management systems of leading countries, were analyzed, categorizing them into 1) input and reference data for safety assessments, 2) guidelines for data management, 3) organizational structures for data management, and 4) computer systems for data management. While each country exhibited differences in specific aspects, commonalities included the classification of safety assessment input data based on disposal system components, the establishment of organizations to supply, use, and manage this data, and the implementation of quality management systems guided by instructions and manuals. These cases highlight the importance of data management systems and document management systems for securing the safety and enhancing the reliability of High-Level Radioactive Waste Disposal Facilities. To achieve this, the classification of input data that can be flexibly and effectively utilized, ensuring the consistency and traceability of input data, and establishing a quality management system for input data and document management are necessary.

Analysis on Design Change for Backfilling Solution of the Disposal Tunnel in the Deep Geological Repository for High-Level Radioactive Waste in Finland (핀란드 고준위방사성폐기물 심층처분시설 처분터널 뒤채움 설계 변경을 위한 연구사례 분석)

  • Heekwon Ku;Sukhoon Kim;Jeong-Hwan Lee
    • Tunnel and Underground Space
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    • v.33 no.6
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    • pp.435-444
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    • 2023
  • In the licensing application for the deep geological disposal system of high-level radioactive waste in Finland, the disposal tunnel backfilling has been changed from the block/pellet (for the construction) to the granular type (for the operation). Accordingly, for establishing the design concept for backfilling, it is necessary to examine applicability to the domestic facility through analyzing problems of the existing method and improvements in the alternative design. In this paper, we first reviewed the principal studies conducted for changing the backfill method in the licensing process of the Finnish facility, and identified the expected problems in applying the block/pellet backfill method. In addition, we derived the evaluation factors to be considered in terms of technical and operational aspects for the backfilling solution, and then conducted a comparative analysis for two types of backfill methods. This analysis confirmed the overall superiority of the design change. It is expected that these results could be utilized as the technical basis for deriving the optimum design plan in development process of the Korean-specific deep disposal facility. However, applicability should be reviewed in advance based on the latest technical data for the detailed evaluation factors that must be considered for selecting the backfilling method.

Nuclear Criticality Analyses of Two Different Disposal Canisters for Deep Geological Repository Considering Burnup Credit

  • Hyungju Yun;Manho Han;Seo-Yeon Cho
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.20 no.4
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    • pp.501-510
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    • 2022
  • The nuclear criticality analyses considering burnup credit were performed for a spent nuclear fuel (SNF) disposal cell consisting of bentonite buffer and two different types of SNF disposal canister: the KBS-3 canister and small standardized transportation, aging and disposal (STAD) canister. Firstly, the KBS-3 & STAD canister containing four SNFs of the initial enrichment of 4.0wt% 235U and discharge burnup of 45,000 MWD/MTU were modelled. The keff values for the cooling times of 40, 50, and 60 years of SNFs were calculated to be 0.79108, 0.78803, and 0.78484 & 0.76149, 0.75683, and 0.75444, respectively. Secondly, the KBS-3 & STAD canister with four SNFs of 4.5wt% and 55,000 MWD/MTU were modelled. The keff values for the cooling times of 40, 50, and 60 years were 0.78067, 0.77581, and 0.77335 & 0.75024, 0.74647, and 0.74420, respectively. Therefore, all cases met the performance criterion with respect to the keff value, 0.95. The STAD canister had the lower keff values than KBS-3. The neutron absorber plates in the STAD canister significantly affected the reduction in keff values although the distance among the SNFs in the STAD canister was considerably shorter than that in the KBS-3 canister.

Preliminary Analyses of the Deep Geoenvironmental Characteristics for the Deep Borehole Disposal of High-level Radioactive Waste in Korea (고준위 방사성폐기물 심부시추공 처분을 위한 국내 심부지질 환경특성 예비분석)

  • LEE, Jongyoul;LEE, Minsoo;CHOI, Heuijoo;KIM, Geonyoung;KIM, Kyungsu
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.14 no.2
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    • pp.179-188
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    • 2016
  • Spent fuels from nuclear power plants, as well as high-level radioactive waste from the recycling of spent fuels, should be safely isolated from human environment for an extremely long time. Recently, meaningful studies on the development of deep borehole radioactive waste disposal system in 3-5 km depth have been carried out in USA and some countries in Europe, due to great advance in deep borehole drilling technology. In this paper, domestic deep geoenvironmental characteristics are preliminarily investigated to analyze the applicability of deep borehole disposal technology in Korea. To do this, state-of-the art technologies in USA and some countries in Europe are reviewed, and geological and geothermal data from the deep boreholes for geothermal usage are analyzed. Based on the results on the crystalline rock depth, the geothermal gradient and the spent fuel types generated in Korea, a preliminary deep borehole concept including disposal canister and sealing system, is suggested.

Thermal Analyses of Deep Geological Disposal Cell With Heterogeneous Modeling of PLUS7 Spent Nuclear Fuel

  • Hyungju Yun;Min-Seok Kim;Manho Han;Seo-Yeon Cho
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.21 no.4
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    • pp.517-529
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    • 2023
  • The objectives of this paper are: (1) to conduct the thermal analyses of the disposal cell using COMSOL Multiphysics; (2) to determine whether the design of the disposal cell satisfies the thermal design requirement; and (3) to evaluate the effect of design modifications on the temperature of the disposal cell. Specifically, the analysis incorporated a heterogeneous model of 236 fuel rod heat sources of spent nuclear fuel (SNF) to improve the reality of the modeling. In the reference case, the design, featuring 8 m between deposition holes and 30 m between deposition tunnels for 40 years of the SNF cooling time, did not meet the design requirement. For the first modified case, the designs with 9 m and 10 m between the deposition holes for the cooling time of 40 years and five spacings for 50 and 60 years were found to meet the requirement. For the second modified case, the designs with 35 m and 40 m between the deposition tunnels for 40 years, 25 m to 40 m for 50 years and five spacings for 60 years also met the requirement. This study contributes to the advancement of the thermal analysis technique of a disposal cell.