• Title/Summary/Keyword: Atomic configuration

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Analysis of Key Parameters for Designing the Spent Nuclear Fuel Disposal Container in Korea (사용후핵연료 처분용기 설계를 위한 주요인자 분석)

  • Choi, Jong-Won;Cho, Dong-Keun;Choi, Hui-Ju
    • Journal of Radiation Protection and Research
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    • v.31 no.1
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    • pp.37-46
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    • 2006
  • For the first step to develop a reference disposal container of spent fuel to be used in a deep geological repository, this paper examined safe dimensions of the disposal container on the points of nuclear criticality and radiation safety and mechanical structural safety and provided basic information for dimensioning the container and configuration of the container components, and establishing the favorable and safe disposal conditions. When the safety factor for stress due to the external loads (hydrostatic and swelling pressure) is taken as 2.0, the safe diameter of the filler material to provide enough container strength under the assumed external loads is found to be 112cm with 13cm spacing between inner baskets in PWR container. Also the thickness of the thinner section between the fuel basket and the surface of the cast insert is determined to be 150 mm. Regarding these dimensions of the container, the PWR fuel container is sketched to accommodate 4 square assemblies or 297 CANDU fuel 297 bundles (33 circle tubes x 9 stacks). However the top and bottom parts need to be checked again through the detail radiation shielding analysis with respects to the emplacement position and handling processes of the disposal container.

ANALYSIS OF THE TRANSPORTATION LOGISTICS FOR SPENT NUCLEAR FUEL IN KOREA

  • Lee, Hyo-Jik;Ko, Won-Il;Seo, Ki-Seok
    • Nuclear Engineering and Technology
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    • v.42 no.5
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    • pp.582-589
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    • 2010
  • As a part of the back-end fuel cycle, transportation of spent nuclear fuel (SNF) from nuclear power plants (NPPs) to a fuel storage facility is very important in establishing a nuclear fuel cycle. In Korea, the accumulated amount of SNF in the NPP pools is troublesome since the temporary storage facilities at these NPP pools are expected to be full of SNF within ten years. Therefore, Korea cannot help but plan for the construction of an interim storage facility to solve this problem in the near future. Especially, a decision on several factors, such as where the interim storage facility should be located, how many casks a transport ship can carry at a time and how many casks are initially required, affect the configuration of the transportation system. In order to analyze the various possible candidate scenarios, we assumed four cases for the interim storage facility location, three cases for the load capacity that a transport ship can carry and two cases for the total amount of casks used for transportation. First, this study considered the currently accumulated amount of SNF in Korea, and the amount of SNF generated from NPPs until all NPPs are shut down. Then, how much SNF per year must be transported from the NPPs to an interim storage facility was calculated during an assumed transportation period. Second, 24 candidate transportation scenarios were constructed by a combination of the decision factors. To construct viable yearly transportation schedules for the selected 24 scenarios, we created a spreadsheet program named TranScenario, which was developed by using MS EXCEL. TranScenario can help schedulers input shipping routes and allocate transportation casks. Also, TranScenario provides information on the cask distribution in the NPPs and in the interim storage facility automatically, by displaying it in real time according to the shipping routes, cask types and cask numbers that the user generates. Once a yearly transportation schedule is established, TranScenario provides some statistical information, such as the voyage time, the availability of the interim storage facility, the number of transported casks sent from the NPPs, and the number of transported casks received at the interim storage facility. By using this information, users can verify and validate a yearly transportation schedule. In this way, the 24 candidate scenarios could be constructed easily. Finally, these 24 scenarios were compared in terms of their operation cost.

Shielding Design Optimization of the HANARO Cold Neutron Triple-Axis Spectrometer and Radiation Dose Measurement (냉중성자 삼축분광장치의 차폐능 최적화 설계 및 선량 측정)

  • Ryu, Ji Myung;Hong, Kwang Pyo;Park, J.M. Sungil;Choi, Young Hyeon;Lee, Kye Hong
    • Journal of Radiation Protection and Research
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    • v.39 no.1
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    • pp.21-29
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    • 2014
  • A new cold neutron triple-axis spectrometer (Cold-TAS) was recently constructed at the 30 MWth research reactor, HANARO. The spectrometer, which is composed of neutron optical components and radiation shield, required a redesign of the segmented monochromator shield due to the lack of adequate support of its weight. To shed some weight, lowering the height of the segmented shield was suggested while adding more radiation shield to the top cover of the monochromator chamber. To investigate the radiological effect of such change, we performed MCNPX simulations of a few different configurations of the Cold-TAS monochromator shield and obtained neutron and photon intensities at 5 reference points just outside the shield. Reducing the 35% of the height of the segmented shield and locating lead 10 cm from the bottom of the top cover made of polyethylene was shown to perform just as well as the original configuration as radiation shield excepting gamma flux at two points. Using gamma map by MCNPX, it was checked that is distribution of gamma. Increased flux had direction to the top and it had longer distance from top of segmented shield. However, because of reducing the 35% of the height, height of dissipated gamma was lower than original geometry. Reducing the 35% of the height of the segmented shield and locating lead 10cm from the bottom of the top cover was selected. After changing geometry, radiation dose was measured by TLD for confirming tester's safety at any condition. Neutron(0.21 ${\mu}Svhr^{-1}$) and gamma(3.69 ${\mu}Svhr^{-1}$) radiation dose were satisfied standard(6.25 ${\mu}Svhr^{-1}$).

Synthesis of Novel Platinum Precursor and Its Application to Metal Organic Chemical Vapor Deposition of Platinum Thin Films

  • Lee, Sun-Sook;Lee, Ho-Min;Park, Min-Jung;An, Ki-Seok;Kim, Jin-Kwon;Lee, Jong-Heun;Chung, Taek-Mo;Kim, Chang-Gyoun
    • Bulletin of the Korean Chemical Society
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    • v.29 no.8
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    • pp.1491-1494
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    • 2008
  • A novel platinum aminoalkoxide complex, Pt$(dmamp)_2$ has been prepared by the reaction of cis-$(py)_2PtI_2$ with two equivalents of Na(dmamp) (dmamp = 1-dimethylamino-2-methyl-2-propanolate). Single-crystal X-ray crystallographic analysis shows that the Pt(dmamp)2 complex keeps a square planar geometry with each two nitrogen atoms and two oxygen atoms having trans configuration. Platinum films have been deposited on TaN/ Ta/Si substrates by metal organic chemical vapor deposition (MOCVD) using Pt$(dmamp)_2$. As-deposited platinum thin films did not contain any appreciable amounts of impurities except a little carbon. As the deposition temperature was increased, the films resistivity and deposition rate increased. The electrical resistivity (13.6 $\mu\Omega$cm) of Pt film deposited at 400 ${^{\circ}C}$ is a little higher than the bulk value (10.5 $\mu\Omega$cm) at 293 K. The chemical composition, crystalline structure, and morphology of the deposited films were investigated by X-ray photoelectron spectroscopy, X-ray diffraction, and atomic force microscopy.

Preliminary Study of Performance Evaluation of a Dual-mode Compton Camera by Using Geant4 (Geant4 몬테칼로 전산모사 툴킷을 이용한 이중모드 컴프턴 카메라 최적화 설계 및 성능평가)

  • Park, Jin Hyung;Seo, Hee;Kim, Seoung Hoon;Kim, Young Soo;Kim, Chan Hyeong
    • Journal of Radiation Protection and Research
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    • v.37 no.4
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    • pp.191-196
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    • 2012
  • A double-scattering type Compton camera which is appropriate to imaging a high-energy gamma source has been developed for nuclear material surveillance at Hanyang University. The double-scattering type Compton camera can provide high imaging resolution; however, it has disadvantage of relatively low imaging sensitivity than existing single-scattering type Compton camera. In this study, we introduce a novel concept of a dual-mode Compton camera which incorporates two different types of Compton camera, i.e., single- and double-scattering type. The dual-mode Compton camera can operate high-resolution mode and high-sensitivity mode in a single system. To maximize its performance, the geometrical configuration was optimized by using Geant4 Monte Carlo simulation toolkit. In terms of imaging sensitivity, high-sensitivity mode had higher sensitivity than high-resolution mode up to 100 times while high imaging resolution of the double-scattering Compton camera was maintained.

RAMAN SPECTROSCOPY IN SYMBIOTIC STARS (공생별에서 라만 산란선의 형성)

  • LEE HEE-WON
    • Publications of The Korean Astronomical Society
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    • v.15 no.spc1
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    • pp.103-112
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    • 2000
  • Symbiotic stars are known as binary systems of a giant with heavy mass loss and a white dwarf accompanied by an emission nebula. They often show bipolar nebulae, and are believed to form an accretion disk around the white dwarf component by attracting the slow but heavy stellar wind around the giant companion. However, the existence and physical properties of the accretion disk in these systems still remain controversial. Unique to the spectra of symbiotic stars is the existence of the symbiotic bands around $6830{\AA}$ and $7088{\AA}$, which have been identified by Schmid (1989) as the Raman scattered features of the O VI $1032{\AA}$ and $1038{\AA}$ doublet by atomic hydrogen. Due to the incoherency of the Raman scattering, these features have very broad profiles and they are also strongly polarized. In the accretion disk emission model, it is expected that the Raman features are polarized perpendicular to the binary axis and show multiple peak structures in the profile, because the neutral scatterers located near the giant component views the accretion disk in the edge-on direction. Assuming the presence of scattering regions outflowing in the polar directions, we may explain the additional red wing or red peak structure, which is polarized parallel to the binary axis. We argue that in the accretion disk emission model it is predicted that the profile of the Raman feature around $6830{\AA}$ is different from the profile of the $7088{\AA}$ because the O VI line optical depth varies locally around the white dwarf component. We conclude that the Raman scattered features are an important tool to investigate the physical conditions and geometrical configuration of the accretion disk in a symbiotic star.

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The characteristics of nonlinear magneto-optical effect based on coherent population trapping in the D1 line of Rh atoms (87Rb D1 전이선에서 원자결맞음을 이용한 비선형 광자기 효과 신호의 특성)

  • Lee, L.;Moon, H.S.;Kim, J.B.
    • Korean Journal of Optics and Photonics
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    • v.17 no.1
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    • pp.1-6
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    • 2006
  • We investigated the characteristics of the nonlinear magneto-optic effect (NMOE) depend on the transitions, the laser intensity and the temperature of the vapor cell, in the $D_1$ transition of $^{87}Rb$ atoms by using the Rb vapor cell contained with buffer gas of Ne 6.7 kPa. The size and the width of NMOE signal were increased according to the light intensity and temperature in the transition of F=2$\to$F'=2. However, In the case of using the F=2$\to$F'=1 transition, the size of the signal could be increased according to the light intensity without additional broadening of the width. We confirmed that the sensitivity of detecting small magnetic flux improved in this transition, and explained these effects by the different of the CPT configuration between Zeeman sublevels. At the optimal condition in experiment, the sensitivity of this system was evaluated less then $70pT/\sqrt{Hz}$.

Magnetic properties of micro-patterned array of anti-dots in Co/Ni bilayer

  • Deshpande, N.G.;Seo, M.S.;Zheng, H.Y.;Lee, S.J.;Rhee, J.Y.;Kim, K.W.;Lee, Y.P.
    • Proceedings of the Korean Vacuum Society Conference
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    • 2010.08a
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    • pp.276-276
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    • 2010
  • Large-area micropatterned array of Co/Ni bilayer anti-dots was fabricated using photolithography and wet etching process. The surface morphology as well as the surface topography was checked by scanning electron microscopy and atomic force microscopy, whereas the magnetic properties were studied by magneto-optical Kerr effect (MOKE) and magnetic force microscopy (MFM). Systematic studies of the magnetic-reversal mechanism, the in-plane anisotropy and the switching field properties were carried out. To get a comprehensive knowledge about the domain configuration, we also employed OOMMF simulations. It was found from the MOKE measurements that a combined effect of configurational and the magneto-crystalline anisotropy simultaneously works in such micropatterned bilayer structures. In addition, the inclusion of holes in the uniform magnetic film drastically affected the switching field. The MFM images show well-defined domain structures which are periodic in nature. The micromagnetic simulations indicate that the magnetization reversal of such a structure proceeds by formation and annihilation of domain walls, which were equally manifested by the field-dependent MFM images. The observed changes in the magnetic properties are strongly related to both the patterning that hinders the domain-wall motion and to the magneto-anisotropic bilayered structure.

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Growth and characterization of periodically polarity-inverted ZnO structures grown on Cr-compound buffer layers

  • Park, J.S.;Goto, T.;Hong, S.K.;Chang, J.H.;Yoon, E.;Yao, T.
    • Proceedings of the Korean Vacuum Society Conference
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    • 2010.08a
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    • pp.259-259
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    • 2010
  • Periodically polarity inverted (PPI) ZnO structures on (0001) Al2O3 substrates are demonstrated by plasmas assisted molecular beam epitaxy. The patterning and re-growth methods are used to realize the PPI ZnO by employing the polarity controlling method. For the in-situ polarity controlling of ZnO films, Cr-compound buffer layers are used.[1, 2] The region with the CrN intermediate layer and the region with the Cr2O3 and Al2O3 substrate were used to grow the Zn- and O-polar ZnO films, respectively. The growth behaviors with anisotropic properties of PPI ZnO heterostructures are investigated. The periodical polarity inversion is evaluated by contrast images of piezo-response microscopy. Structural and optical interface properties of PPI ZnO are investigated by the transmission electron microcopy (TEM) and micro photoluminescence ($\mu$-PL). The inversion domain boundaries (IDBs) between the Zn and the O-polar ZnO regions were clearly observed by TEM. Moreover, the investigation of spatially resolved local photoluminescence characteristics of PPI ZnO revealed stronger excitonic emission at the interfacial region with the IDBs compared to the Zn-polar or the O-polar ZnO region. The possible mechanisms will be discussed with the consideration of the atomic configuration, carrier life time, and geometrical effects. The successful realization of PPI structures with nanometer scale period indicates the possibility for the application to the photonic band-gap structures or waveguide fabrication. The details of application and results will be discussed.

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Characterization of Basal Plane Dislocations in PVT-Grown SiC by Transmission Electron Microscopy

  • Jeong, Myoungho;Kim, Dong-Yeob;Hong, Soon-Ku;Lee, Jeong Yong;Yeo, Im Gyu;Eun, Tai-Hee;Chun, Myoung-Chuel
    • Korean Journal of Materials Research
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    • v.26 no.11
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    • pp.656-661
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    • 2016
  • 4H- and 6H-SiC grown by physical vapor transport method were investigated by transmission electron microscopy (TEM). From the TEM diffraction patterns observed along the [11-20] zone axis, 4H- and 6H-SiC were identified due to their additional diffraction spots, indicating atomic stacking sequences. However, identification was not possible in the [10-10] zone axis due to the absence of additional diffraction spots. Basal plane dislocations (BPDs) were investigated in the TEM specimen prepared along the [10-10] zone axis using the two-beam technique. BPDs were two Shockley partial dislocations with a stacking fault (SF) between them. Shockley partial BPDs arrayed along the [0001] growth direction were observed in the investigated 4H-SiC. This arrayed configuration of Shockley partial BPDs cannot be recognized from the plan view TEM with the [0001] zone axis. The evaluated distances between the two Shockley partial dislocations for the investigated samples were similar to the equilibrium distance, with values of several hundreds of nanometers or even values as large as over a few micrometers.