• Title/Summary/Keyword: Aerosol sources

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Characterization of Atmospheric Dispersion Pattern from Large Sources in Chungnam, Korea (충남지역 대형사업장의 대기오염물질 확산 특성 파악)

  • Choi, Woo Yeong;Park, Min Ha;Jung, Chang Hoon;Kim, Yong Pyo;Lee, Ji Yi
    • Particle and aerosol research
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    • v.17 no.3
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    • pp.55-69
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    • 2021
  • Chungnam region accounts for the largest SOX (22.8%) emission with the second-largest NOX (10.8%) emission in Korea due to the integration of many large industrial sources including a steel mill, coal-fired power plants, and petrochemical complex. Air pollutants emitted by large industrial sources can cause harmful problems to humans and the environment. Thus, it is necessary to understand dispersion patterns of air pollutants from large industrial sources in Chungnam to characterize atmospheric contamination in Chungnam and the surrounding area. In this study, seasonal atmospheric dispersion characteristics for SOX, NOX, and PM2.5 from ten major point sources in Chungnam were evaluated using HYSPLIT 4 model, and their contributions to SO2, NO2 concentrations in the regions near the source areas were estimated. The predictions of the HYSPLIT 4 model show a seasonal different dispersion pattern, in which air pollutants were dispersed toward the southeast in winter while, northeast in summer. In summer, due to weaker wind speed, air pollutants concentrations were higher than in winter, and they were dispersed to the metropolitan area. The local emissions of air pollutants in Taean area had a greater influence on the ambient SO2 and NO2 concentrations at Taean, whereas SOX and NOX emissions from large sources located at Seosan showed relatevely little effect on the ambient ambient SO2 and NO2 concentrations at Seosan.

Aerosol Size Distribution and Composition at Kosan, Cheju Island : Measurements in April 1998 (제주도 고산에서의 에어로솔 입경분포별 조성: 1998년 4월 측정 연구)

  • 김용표;배귀남;지준호;진현철;문길주
    • Journal of Korean Society for Atmospheric Environment
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    • v.15 no.5
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    • pp.677-685
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    • 1999
  • Aerosol mass size distributions were measured at Kosan, Cheju Island in April 1998 and their compositions were analyzed. Microorifice Uniform Deposit Impactor(MOUDI) was used to collect aerosols. Sulfate and ammonium ions were predominatly present at fine mode of the aerosols while nitrate, chloride, and metal ions were mostly at coarse mode. Based on the size distribution of nitrate, it is suggested that most nitrate were from gas to particle conversion on coarse particles. Non-sea salt(nss) fraction of sulfate accounted for more than 90% of total sulfate mass concentration. In general, ion concentrations in this study are lower than those measured at the same site from the previous studies. Ion balance and chloride ion levels indicates that there had been anthropogenic chloride emission sources near to the site during the measurements.

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Dilution methods for combustion aerosol measurement from stationary emission sources: A review (고정 오염원의 연소과정에서 발생하는 먼지를 측정하기 위한 희석방법 연구동향)

  • Woo, Chang Gyu;Kim, Hak-Joon;Kim, Yong-Jin;Han, Bangwoo;Kang, Su Ji;Chun, Sung-Nam
    • Particle and aerosol research
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    • v.13 no.4
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    • pp.165-172
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    • 2017
  • For precise particle measurements in combustion environments, various dilution sampling methods were compared. Dilution equipments using dilution tunnels and hot/cold dilution with porous tube dilutors were most frequently used so far. The combination of porous tube dilutor and ejector diluter has relatively small footprint, and it results in lower particle losses compared to other methods. To determine the portion of condensable particulate matter, proper temperature control and flow control is required.

Estimation of the major sources for organic aerosols at the Anmyeon Island GAW station (안면도에서의 초미세먼지 유기성분 주요 영향원 평가)

  • Han, Sanghee;Lee, Ji Yi;Lee, Jongsik;Heo, Jongbae;Jung, Chang Hoon;Kim, Eun-Sill;Kim, Yong Pyo
    • Particle and aerosol research
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    • v.14 no.4
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    • pp.135-144
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    • 2018
  • Based on a two-year measurement data, major sources for the ambient carbonaceous aerosols at the Anmyeon Global Atmosphere Watch (GAW) station were identified by using the Positive Matrix Factorization (PMF) model. The particulate matter less than or equal to $2.5{\mu}m$ in aerodynamic diameter (PM2.5) aerosols were sampled between June 2015 to May 2017 and carbonaceous species including ~80 organic compounds were analyzed. When the number of factors was 5 or 6, the performance evaluation parameters showed the best results, With 6 factor case, the characteristics of transported factors were clearer. The 6 factors were identified with various analyses including chemical characteristics and air parcel movement analysis. The 6 factors with their relative contributions were (1) anthropogenic Secondary Organic Aerosols (SOA) (10.3%), (2) biogenic sources (24.8%), (3) local biomass burning (26.4%), (4) transported biomass burning (7.3%), (5) combustion related sources (12.0%), and (6) transported sources (19.2%). The air parcel movement analysis result and seasonal variation of the contribution of these factors also supported the identification of these factors. Thus, the Anmyeon Island GAW station has been affected by both regional and local sources for the carbonaceous aerosols.

Estimation of nighttime aerosol optical thickness from Suomi-NPP DNB observations over small cities in Korea (Suomi-NPP위성 DNB관측을 이용한 우리나라 소도시에서의 야간 에어로졸 광학두께 추정)

  • Choo, Gyo-Hwang;Jeong, Myeong-Jae
    • Korean Journal of Remote Sensing
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    • v.32 no.2
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    • pp.73-86
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    • 2016
  • In this study, an algorithm to estimate Aerosol Optical Thickness (AOT) over small cities during nighttime has been developed by using the radiance from artificial light sources in small cities measured from Visible Infrared Imaging Radiometer Suite (VIIRS) sensor's Day/Night Band (DNB) aboard the Suomi-National Polar Partnership (Suomi-NPP) satellite. The algorithm is based on Beer's extinction law with the light sources from the artificial lights over small cities. AOT is retrieved for cloud-free pixels over individual cities, and cloud-screening was conducted by using the measurements from M-bands of VIIRS at infrared wavelengths. The retrieved nighttime AOT is compared with the aerosol products from MODerate resolution Imaging Spectroradiometer (MODIS) aboard Terra and Aqua satellites. As a result, the correlation coefficients over individual cities range from around 0.6 and 0.7 between the retrieved nighttime AOT and MODIS AOT with Root-Mean-Squared Difference (RMSD) ranged from 0.14 to 0.18. In addition, sensitivity tests were conducted for the factors affecting the nighttime AOT to estimate the range of uncertainty in the nighttime AOT retrievals. The results of this study indicate that it is promising to infer AOT using the DNB measaurements over small cities in Korea at night. After further development and refinement in the future, the developed retrieval algorithm is expected to produce nighttime aerosol information which is not operationally available over Korea.

Spatial Analysis of Major Atmospheric Aerosol Species Using Earth Observing Satellite Data (지구관측 위성자료를 이용한 주요 대기 에어러솔 성분의 공간분포 분석)

  • Lee, Kwon-Ho
    • Journal of the Korean Association of Geographic Information Studies
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    • v.14 no.2
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    • pp.109-127
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    • 2011
  • Atmospheric aerosols, small particles in the atmosphere, are one of the important parameters in climate change and human health. Additionally, accurate estimates of aerosol species are increasingly important in environmental impact assessment studies. Recent advances in global satellite remote sensing provide powerful tool for air quality monitoring. This study explores the potential usage of satellite derived data such as atmospheric aerosols for air quality monitoring as well as climate change study. The objectives of this study is to understand the general features of the global distribution of type dependent aerosols. A detailed spatio-temporal variability of the each different satellite dataset shows the variation of the global zonal average and specific geographical regions where the strong emission sources are located. Especially, significantly large aerosol amounts are observed in Asia and Africa because of the desert dust storm, anthropogenic and biomass burning emissions.

The Influence of Yellow Sand Phenomena on the Concentration Variation of Polycyclic Aromatic Hydrocarbons in Ambient Air of Seoul (황사가 서울시 대기 중 PAHs 농도에 미치는 영향)

  • 박찬구;어수미;기원주;김기현;모세영
    • Journal of Korean Society for Atmospheric Environment
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    • v.17 no.2
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    • pp.179-192
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    • 2001
  • In order to characterize the distribution patterns of PAHs between Yellow Sand (YS) and non-Yellow Sand(NYS) periods, we collected and analyzed aerosol samples for PAHs for the periods covering 28 March through 24 April 2000. The concentrations of TSP measured during the YS periods were approximately two times higher than the NYS periods. By contrast, the concentrations of PAHs during YS were higher than those of NYS by 140%. In ad-dition, their concentrations in PM 10 were larger than those TSP by 120% . Detailed inspections of our data indi-catd that three species including chrysene. benzo(b)fluoranthene, and benzo(k)fluoranthene were effeciently ad-sorbed by particles less than 10${\mu}{\textrm}{m}$ diameter and that there were dominating the distribution characterstics of PAHs during the YS periods. Results of correlation analysis also indicated that PAHs exhibited strong correlations with those pollutants originating from combustion sources. It is thus concluded that pollutants such as toxic PAHs that originate from diverse anthropogenic sources of China should be contributing to the degradation of the ambient air quality in Seoul.

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Source Apportionment and the Origin of Asian Dust Observed in Korea by Receptor Modelling (CMB) (수용모델(CMB)을 이용한 한반도에서 관측된 황사의 발원지 추정과 기여도에 대한 연구)

  • Shin S.A.;Han J.S.;Kim S.D.
    • Journal of Korean Society for Atmospheric Environment
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    • v.22 no.2
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    • pp.157-166
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    • 2006
  • Ambient TSP at four sites in Korea and soil samples from the source regions of Asian Dust in northern China were collected and analyzed for 15 metal components and 6 water-soluble ions to conduct a chemical mass balance (CMB). CMB receptor model was used to estimate the source contribution of TSP during the Asian Dust period, and the model results showed that China soil was the largest source contributor, accounting for 81% of TSP ($458.2{\mu}g/m^3$). Vehicle emission and geological sources contributed to about 8.8% and 4.4% of aerosol mass, followed by sea salt (1.5%) and secondary aerosol (2.9%). Fuel combustion and industrial process sources were found to be relatively minor contributors to TSP (${\leq}1%$). In addition to source contribution estimates, this study tried to identify the origin of Asian Dust observed in Korea. Among all 13 China soil profiles presented in this study, the most adoptable profile which can project the case well was selected and considered as the origin of the applied case.

Sensitivity Analysis of the CMB Modeling Results by Considering Photochemical Degradation of Polycyclic Aromatic Hydrocarbons (PAHs) in the Seoul atmosphere (서울 대기에서 PAHs 광화학반응을 고려한 CMB 수용모델 결과 검토)

  • Cho, Ye Seul;Jung, Da Bin;Kim, In Sun;Lee, Ji Yi;Kim, Yong Pyo
    • Particle and aerosol research
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    • v.10 no.1
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    • pp.9-17
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    • 2014
  • Several studies have been carried out on the source contribution of the particulate Polycyclic Aromatic Hydrocarbons (PAHs) over Seoul by using the Chemical Mass Balance Model (CMB)(Lee and Kim, 2007; Kim et al., 2013). To confirm the validity of the modeling results, the modified model employing a photochemical loss rate along with varying residence times and the standard model that considers no loss were compared. It was found that by considering the photochemical loss rate, a better performance was obtained as compared to those obtained from the standard model in the CMB calculation. The modified model estimated higher contributions from coke oven, transportation, and biomass burning by 4 to 8%. However, the order of the relative importance of major sources was not changed, coke oven followed by transportation and biomass burning. Thus, it was concluded that the standard CMB model results are reliable for identifying the relative importance of major sources.

An improvement of Simplified Atmospheric Correction : MODIS Visible Channel

  • Lee, Chang-Suk;Han, Kyung-Soo
    • Korean Journal of Remote Sensing
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    • v.25 no.6
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    • pp.487-499
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    • 2009
  • Atmospheric correction of satellite measurements is a major step to estimate accurate surface reflectance of solar spectrum channels. In this study, Simplified Method for the Atmospheric Correction (SMAC) radiative transfer model used to retrieve surface reflectance from MODIS (MODerate resolution Imaging Spectrometer) top of atmosphere (TOA) reflectance. It is fast and simple atmospheric correction method, so it uses for work site operation in various satellite. This study attempts a test of accuracy of SMAC through a sensitivity test to detected error sources and to improve accuracy of surface reflectance using SMAC. The results of SMAC as compared with MODIS surface reflectance (MOD09) was represented that low accuracy ($R^2\;=\;0.6196$, Root Means Square Error (RMSE) = 0.00031, bias = - 0.0859). Thus sensitivity analysis of input parameters and coefficients was conducted to searching error sources. Among the input parameters, Aerosol Optical Depth (AOD) is the most influence input parameter. In order to modify AOD term in SMAC code, Stepwise multiple regression was performed with testing and remove variable in three stages with independent variables of AOD at 550nm, solar zenith angle, viewing zenith angle. Surface reflectance estimation by using Newly proposed AOD term in the study showed that improve accuracy ($R^2\;=\;0.827$, RMSE = 0.00672, bias = - 0.000762).