• Particle and aerosol research
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• v.5 no.2
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• pp.45-52
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• 2009

Black carbon, which is a by-product of combustion of fossil fuel and biomass burning, is the component that imposes the largest uncertainty on quantifying aerosol climate effect. The direct, indirect and semi-direct climate effects of black carbon depend on its state of the mixing with other water-soluble aerosol components. The process that transforms hydrophobic externally mixed black carbon particles into hygroscopic internally mixed ones is called "aging". In most climate models, simple parameterizations for the aging time scale are used instead of solving detailed dynamics equations on the aging process due to the computation cost. In this study, a new parameterization for the black carbon aging time scale due to condensation and coagulation is presented as a function of the concentration of hygroscopic atmospheric components and the black carbon particle size. It is shown that the black carbon aging time scale due to condensation of sulfuric acid vapors varies to a large extent depending on the sulfuric acid concentration and the black carbon particle size. This result indicates that the constant aging time scale values suggested in the literature cannot be directly applied to a global scale modeling. The aging time scale due to coagulation with internally mixed aerosol particles shows an even stronger dependency on particle size, which implies that the use of a particle-size-independent aging time scale may lead to a large error when the aging is dominated by coagulation.

• Particle and aerosol research
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• v.7 no.3
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• pp.99-108
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• 2011

To establish area specific control strategies for the reduction of the ozone concentration, the Ozone Isopleth Plotting Package for Research(OZIPR) model has been widely used. However, the model results tend to changed by various input parameters such as the background concentration, emission amount of NOx and volatile organic compounds (VOCs), and meteorological condition. Thus, sensitivity analysis should be required to ensure the reliability of the result. The OZIPR modeling results for five local government districts in the Seoul Metropolitan Area (SMA) in June 2000 were used for the sensitivity analysis. The sensitivity analysis result showed that the modeling result of the SMA being VOC-limited region be still valid for a wide range of input parameters' variation. The estimated ozone concentrations were positively related with the initial VOCs concentrations while were negatively related with the initial NOx concentrations. But, the degree of the variations at each local district was different suggesting area specific characteristics being also important. Among the five local governments, Suwon was chosen to identify other variance through the period from April to September in 2000. The monthly modeling results show different ozone values, but still showing the characteristics of VOCs-limited region. Limitations due to not considering long range transport and transfer from neighbor area, limitation of input data, error between observed data and estimated data are all discussed.

• Proceedings of the Korean Environmental Sciences Society Conference
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• 2019.10a
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• pp.87-87
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• 2019

• Nuclear Engineering and Technology
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• v.56 no.9
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• pp.3483-3490
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• 2024

The initial size distribution and morphological parameters of sodium aerosols are critical in evaluating the accidental suspended aerosol behaviour in Sodium-cooled Fast Reactor (SFR) containment. Mass-based measurements were more familiar in characterizing the sodium aerosols. Real-time number size distribution measurements are carried out in this study. The sensitivity analysis of sodium aerosol effective density (ρ_e) in deriving the actual number size distributions from the measured Aerodynamic Particle Size Distributions (APSD) and predicting suspended aerosol dynamics is presented. Tests are conducted in a 1 m³ chamber at 47 ± 3% RH for different initial mass concentrations (M₀) of 0.1, 1, and 2.9 g/m³. The initial APSDs measured just after the generation completions are observed to be polydisperse with the count median aerodynamic diameter (CMAD) < 1 ㎛. The literature reported ρ_e values of sodium aerosols, 2.27, 1.362, and 0.61 g/cm³ are used to derive mobility equivalent PSDs from APSD in each test. The real-time number concentration decay and size growth for four different PSDs are measured and compared with the estimate using nodal method-based code to ascertain the actual parameters. The validated parameters CMD = 0.66 ㎛, σ_g = 1.96, ρ_e = 1 g/cm³ and χ = 1 are used for improved estimation of sodium aerosol dynamics in Indian SFR containment with M₀ = 4 g/m³ for severe accident scenarios.

• Proceedings of the Korean Radioactive Waste Society Conference
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• 2019.05a
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• pp.303-304
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• 2019

• Asian Journal of Atmospheric Environment
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• v.5 no.2
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• pp.97-104
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• 2011

Recent studies have indicated that the observed nitric acid ($HNO_3$) uptake rates ($R_{HNO_3}$) onto dust particles are much slower than $R_{HNO_3}$ used in the previous modeling studies. Three factors that possibly affect $R_{HNO_3}$ onto dust particles are discussed in this study: (1) the magnitude of reaction probability of $HNO_3$ (${\gamma}_{HNO_3}$), (2) aerosol surface areas, and (3) gas-phase $HNO_3$ mixing ratio. Through the discussion presented here, it is shown that the use of accurate ${\gamma}_{HNO_3}$ is of primary importance. We suggest that the use of ${\gamma}_{HNO_3}$ values between $\sim10^{-3}$ and $\sim10^{-5}$ produces more realistic results than the use of ${\gamma}_{HNO_3}$ values between $\sim10^{-1}$ and $\sim10^{-2}$ does, more accurately modeling the nitrate formation characteristics on/in dust particles. We also discuss two different types of aerosol surface area, active and geometric, since the use of different aerosol surface areas often leads to an erroneous result in $R_{HNO_3}$. In addition, the levels of the gas-phase $HNO_3$ are investigated with the example cases of TRACE-P DC-8 flights in East Asia. The $HNO_3$ levels were found to be relatively high, indicating that they can not limit nitrate formation in dust particles.

• Atmosphere
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• v.20 no.1
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• pp.49-61
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• 2010

Atmospheric aerosols play a crucial role for changing climate, resulting in a wide range of uncertainty for future climate prediction. In this paper we review current international research status and trend of climate-related aerosol science. There have been carried out a number of campaigns (including ACE-Asia, TRACE-P, ABC, and so on) and special experiments with some modeling studies over Korea, East Asia, and the Northwestern Pacific to characterize the various properties (physical, chemical, optical, and radiative) of Asian aerosols and evaluate their climate forcing impacts. But some parts of the aerosol research may need to be improved, advanced, or newly launched. Especially, a chemical transport model (CTM) embedded by a general circulation model (GCM) should be developed by the national scientific community with a high research priority, actively collaborating with international community in order to estimate direct and indirect global radiative forcing due to anthropogenic and natural aerosols.

• Journal of Environmental Science International
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• v.28 no.1
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• pp.107-123
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• 2019

The aerosol chemical components in $PM_{2.5}$ in several regions (Seoul, Busan, Daejeon, and Jeju Island) were investigated with regard to their concentration characteristics and optical properties. The optical properties of the various aerosol components (e.g., water-soluble, insoluble, Black Carbon (BC), and sea-salt) were estimated using hourly and daily aerosol sampling data from the study area via a modeling approach. Overall, the water-soluble component was predominant over all other components in terms of concentration and impact on optical properties (except for the absorption coefficient of BC). The annual mean concentration and Aerosol Optical Ddepth (AOD) of the water-soluble component were highest in Seoul (at the Gwangjin site) ($26{\mu}g/m^3$ and 0.29 in 2013, respectively). Further, despite relatively moderate BC concentrations, the annual mean absorption coefficient of BC ($21.7Mm^{-1}$) was highest in Busan (at the Yeonsan site) in 2013, due to the strong light absorbing ability of BC. In addition, high AODs for the water-soluble component were observed most frequently in spring and/or winter at most of the study sites, while low values were noted in summer and/or early fall. The diurnal variation in the AOD of each component in Seoul (at the Gwangjin site) was slightly high in the morning and low in the afternoon during the study period; however, such distinctions were not apparent in Jeju Island (at the Aweol site), except for a slightly high AOD of the water-soluble component in the morning (08:00 LST). The monthly and diurnal differences in the AOD values for each component could be attributed to the differences in their mass concentrations and Relative Humidities (RH). In a sensitivity test, the AODs estimated under RH conditions of 80 and 90% were factors of 1.2 and 1.7 higher, respectively, than the values estimated using the observed RH.

• 제어로봇시스템학회:학술대회논문집
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• 2002.10a
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• pp.60.3-60
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• 2002

1. Introduction 2. The Localized Aerosol Hyperthermia 3. Hardware Development of a Heated Vapor Inhalator 4. Modeling of the Control System 5. The Design of LQG/LTR Controller 6. Conclusion

• Particle and aerosol research
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• v.10 no.1
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• pp.9-17
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• 2014

Several studies have been carried out on the source contribution of the particulate Polycyclic Aromatic Hydrocarbons (PAHs) over Seoul by using the Chemical Mass Balance Model (CMB)(Lee and Kim, 2007; Kim et al., 2013). To confirm the validity of the modeling results, the modified model employing a photochemical loss rate along with varying residence times and the standard model that considers no loss were compared. It was found that by considering the photochemical loss rate, a better performance was obtained as compared to those obtained from the standard model in the CMB calculation. The modified model estimated higher contributions from coke oven, transportation, and biomass burning by 4 to 8%. However, the order of the relative importance of major sources was not changed, coke oven followed by transportation and biomass burning. Thus, it was concluded that the standard CMB model results are reliable for identifying the relative importance of major sources.