• Title/Summary/Keyword: $^{232}Th$

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Acute oral toxicity and bioavailability of uranium and thorium in contaminated soil

  • Nur Shahidah Abdul Rashid;Wooyong Um ;Ibrahim Ijang ;Kok Siong Khoo ;Bhupendra Kumar Singh;Nurul Syiffa Mahzan ;Syazwani Mohd Fadzil ;Nur Syamimi Diyana Rodzi ;Aina Shafinas Mohamad Nasir
    • Nuclear Engineering and Technology
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    • v.55 no.4
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    • pp.1460-1467
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    • 2023
  • A robust approach was conducted to determining the absolute oral bioavailable (fab) fractions of 238U and 232Th in rats exposed to contaminated soil along with their hematotoxicity and nephrotoxicity. The soil sample is the International Atomic Energy Agency-312 (IAEA-312) certified reference material, whereas blood, bones, and kidneys of in vivo female Sprague-Dawley (SD) rats estimate 238U- and 232Th-fab fractions post-exposure. We predict the bioavailable concentration (Cab) and fab values of 238U and 232Th after acute soil ingestion. The blood 238U (0.750%) and 232Th (0.028%) reach their maximum fab values after 48 h. The 238U (fab: 0.169-0.652%) accumulates mostly in the kidney, whereas the 232Th (fab: 0.004-0.021%) accumulates primarily in the bone. Additionally, 238U is more bioavailable than 232Th. Post 48 h acute ingestion demonstrates noticeable histopathological and hematological alterations, implying that intake of 238U in co-contaminated soil can lead to erythrocytes and proximal tubules damage, whereas, 232Th intake can harm erythrocytes. Our study provides new directions for future research into the health implications of acute oral exposures to 238U and 232Th in co-contaminated soils. The findings offer significant insight into the utilization of in vivo SD rat testing to estimate 238U and 232Th bioavailability and toxicity in exposure assessment.

Evaluation of Daily Intake of $^{238} U$ and $^{232} Th$ in a Korean Mixed Diet Sample Using RNAA

  • Chung, Yong-Sam;Moon, Jong-Hwa;Kim, Sun-Ha;Park, Kwang-Won;Kang, Sang-Hoon;Cho, Seung-Yeon
    • Nuclear Engineering and Technology
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    • v.32 no.5
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    • pp.477-484
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    • 2000
  • To estimate the degree of intake of $^{238}$ U and $^{232}$ Th through daily diet, a Korean mixed diet sample was prepared after the investigation of the amount of consumption of the daily diet which corresponds to the age of 20 to 60 years. For the analysis of U and Th, the RNAA method was applied. Two standard reference materials were used for quality control and assurance and the analytical results were compared with a certified value. The determination of U and Th in the Korean mixed diet sample was carried out under the same analytical conditions and procedures with SRM. It is found that the concentration of U and Th in a Korean mixed diet was about 35.4 ppb and 3.4 ppb. From these results, the daily intake of $^{238}$ U and $^{232}$ Th by diet is evaluated to be 6.98 and 0.67 $\mu\textrm{g}$ per day, respectively. Radioactivities related to the intake of $^{238}$ U and $^{232}$ Th were estimated to be about 86 mBq and 27 mBq per person per day and the annual dose equivalents from $^{238}$ U and $^{232}$ Th revealed as 3.18 $\mu$Sv and 0.29 $\mu$Sv per person, respectively.

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Determination of the exposure conversion coefficient for 3" X 3" NaI spectrum (3" X 3" NaI 스펙트럼의 조사선량 변환계수 결정)

  • Lee, M.S.
    • Journal of Radiation Protection and Research
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    • v.26 no.2
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    • pp.73-78
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    • 2001
  • In order to find the exposure conversion coefficients for 3"X3" NaI spectrum, we measured the exposure rates with the pressurized ion chamber at 29 different areas in the range of $4{\sim}23{\mu}R\;h^{-1}$, and also measured the gamma spectra with 3"X3" and 4"X4" NaI detectors, simultaneously. The exposure conversion coefficient of the total energy method was determined using the linear relation between the measured exposure rate and the gamma spectrum energy. In order to find the exposure conversion coefficients of the energy band method, we applied the exposure conversion coefficients recommended by NCRP to the 4"X4" NaI spectra, and calculated the exposure rates due to $^{40}K,\;^{238}U$, and $^{232}Th$ series respectively. Using the linearly proportional relation between the obtained $^{232}Th$ series exposure rate and peak area of 2614 keV that represents the $^{232}Th$ series, we obtained the exposure conversion coefficients for $^{232}Th$ series. We also determined the conversion coefficients for $^{238}U$ series and $^{40}K$ using a similar method.

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Evaluation of Radiation effective dose by Naturally Radionuclides in the Soil of Busan (부산지역 토양 내 천연방사성핵종 분석 및 유효선량율 평가)

  • Kim, Jung-Hoon;Kim, Chang-Soo;Lim, Chang-Seon
    • Journal of the Korea Academia-Industrial cooperation Society
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    • v.15 no.6
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    • pp.3658-3666
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    • 2014
  • The presence of $^{238}U$, $^{232}Th$ and $^{40}K$, which are naturally residing radionuclides, in the ordinary soil of Busan, the 2nd largest city in Korea, was anlayzed and the residents' radiation exposure to ordinary soil was evaluated. Regarding the measurement methods, to conduct a detailed analysis of the naturally residing radionuclides in the soil of Busan, this study divided the 16 administrative districts into a lattice structure with 3 spots, and collected a total of 48 soil samples (July 2012 and April 2013). ICP-MS was used to analyze the concentration of the radioactivity of $^{238}U$ and $^{232}Th$ in the soil, and a HpGe detector, a gamma ray detector, was used to analyze the radioactivity of $^{40}K$. The measurement values of this study were compared with the concentration of radioactivity of East Asian regions. The concentration of $^{238}U$ nuclides in Korea was lower than the mean, whereas the concentration of $^{232}Th$ and $^{40}K$ nuclides was higher than the mean. The higher mean concentrations of $^{232}Th$ and $^{40}K$ than the mean were attributed to the many granite areas that contain a great deal of naturally occurring radionuclides.

Evaluation of elemental concentrations of uranium, thorium and potassium in top soils from Kuwait

  • Bajoga, A.D.;Al-Dabbous, A.N.;Abdullahi, A.S.;Alazemi, N.A.;Bachama, Y.D.;Alaswad, S.O.
    • Nuclear Engineering and Technology
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    • v.51 no.6
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    • pp.1638-1649
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    • 2019
  • Top soil samples across the state of Kuwait numering ninety were collected and analysed using gamma-ray spectrometry, to evaluate the elemental concentration of $^{238}U$, $^{232}Th$ and $^{40}K$ and their depletion/enrichment. Results of elemental concentration ranges from 0.48 to 2.61 mg/kg, 0.87-5.23 mg/kg, and 0.24-2.23%, with a mean values of 1.39 mg/kg, 3.47 mg/kg, and 1.18%, for the $^{238}U$, $^{232}Th$ and $^{40}K$, respectively. Further analysis was conducted amongst the five identified soil types, i.e. Aquisalids (S1), Calcigypsids (S2), Petrocalcids (S3), Petrogypsids (S4), and torripsamment (S5). The highest radioactivity concentrations from both uranium and thorium were recorded in the S2 (Calcigypsids) soil, with a value of 1.71 (mg/kg) and 4.45 (mg/kg), respectively. Minimum and maximum values of $^{40}K$ are 1.1(%) and 1.27(%) and is prevalent in Aquisalids (S1) and Petrocalcids (S3) soil types, respectively. Ratios of elemental concentration for $^{232}Th/^{238}U$, $^{40}K/^{238}U$, $^{40}K/^{232}Th$ across the soil types are 2.53, 0.09 and 0.03, with a correlation coefficient of 0.92, 0.34, and 0.38, respectively. A progressively higher $^{232}Th/^{238}U$ ratio is observed moving south-wards, indicating lower $^{238}U$ content in soils from the south relative to the northern part. Overall results indicate Kuwait to be relatively an area with low level of natural radioactivity.

Activity concentrations and radiological hazard assessments of 226Ra, 232Th, 40K, and 137Cs in soil samples obtained from the Dongnam Institute of Radiological & Medical Science, Korea

  • Jieun Lee;HyoJin Kim;Yong Uk Kye; Dong Yeon Lee;Wol Soon Jo;Chang Geun Lee;Jeung Kee Kim;Jeong-Hwa Baek;Yeong-Rok Kang
    • Nuclear Engineering and Technology
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    • v.55 no.7
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    • pp.2388-2394
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    • 2023
  • The radioactivity concentration of environmental radionuclides was analyzed for soil and sand at eight locations within a radius of 255 m centered on the Dongnam Institute of Radiological & Medical Science (DIRAMS), Korea. The average activity concentrations of 40K, 137Cs, 226Ra, and 232Th were 661.1 Bq/kg-dry, 0.9 Bq/kg-dry, 21.9 Bq/kg-dry, and 11.1 Bq/kg-dry, respectively. The activity of 40K and 137Cs was lower than the 3-year (2017-2019) average reported by the Korea Institute of Nuclear Safety, respectively. Due to the nature of granite-rich soil, the radioactivity of 40K was 0.6-fold higher than in other countries, while 137Cs was in the normal fluctuation range (15-30 Bq/kg-dry) of the concentration of radioactive fallout from nuclear tests. The activity of 226Ra and 232Th was lower than in Korean soils reported by the United Nations Scientific Committee on the Effects of Atomic Radiation (UNSCEAR). The average activity concentrations of 232Th and 40K for the soil and sand samples from DIRAMS were within the range specified by UNSCEAR in 2000. The radium equivalent activity and internal and external hazard index values were below the recommended limits (1 mSv/y). These radionuclide concentration (226Ra, 232Th, 40K, and 137Cs) data can be used for regional environmental monitoring and ecological impact assessments of nuclear power plant accidents.

Review of the Current Status of the U-238, NP-237 and Th-232 Fission Cross Sections

  • Bak, H.I.;Lorenz, A.
    • Nuclear Engineering and Technology
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    • v.3 no.2
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    • pp.77-97
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    • 1971
  • The experimental fission cross-section data of U-238, Np-237 and Th-232, published up to the end of 1970, are reviewed and analyzed between their respective thresholds and 20.0 MeV. The results of a statistical analysis of the available data, performed with a weighted Least-squares Orthogonal Polynomial Pitting computer programme are presented in the form of point-wise cross-section values together with their uncertainties, and in the form of graphs of the fitted curves with an indication of a region of 95% statistical confidence level. An estimate of the fission spectrum weighted average cross-sections and their respective uncertainties is also given.

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Assessment of the terrestrial gamma radiation dose in Korea

  • Choi, Seok-Won;Yun, Ju-Yong;Kim, Chang-Kyu;Rho, Byung-Hwan;Lee, Jong-Seong
    • Journal of Radiation Protection and Research
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    • v.30 no.4
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    • pp.161-165
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    • 2005
  • The gamma-ray dose rates in air at 233 locations in Korea have been determined. The contribution to the gamma-ray dose rates in air due to the presence of $^{232}Th-series,\;^{238}U-series\;and\;^{40}K$ is as follows: 47.3% $(36\;nGyh^{-1})\;^{232}Th-series$ 14.5% $(11\;nGyh^{-1})\;^{238}U-series$ and 38.2% $(29\;nGyh^{-1})\;^{40}K$. The mean gamma-ray dose rate theoretically derived from $^{232}Th-series,\;^{238}U-series\;and\;^{40}K\;was\;76{\pm}17\;nGyh^{-1}$. This corresponds to an annual effective dose of $410\;{\mu}Sv$ and an annual collective dose of 18900 person-Sv for all provinces under study. The results have been compared with other global radiation dose.

Radioactivity concentrations of natural radionuclides in fine dust of Jeju, Korea

  • Chung-Hun Han;Sohyeon Lim;Hee-Jung Im
    • Analytical Science and Technology
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    • v.36 no.4
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    • pp.191-197
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    • 2023
  • Radioactivity concentrations for natural radionuclides were determined from fine dust samples collected in Jeju, Korea according to atmospheric events (Asian dust, haze, fog-mist, and non-event), and radium equivalent activity was calculated. The mean atmospheric radioactivity concentrations for 238U, 232Th, and 40K in 127 fine dust samples were 0.49, 0.24, and 7.23 µBq m-3, respectively, and the radium equivalent activity was 33.25 Bq kg-1. The mean concentrations of 238U and 232Th in the fine dust during the Asian dust period were 1.31 and 1.60 µBq m-3, respectively, above the global average, while the values for the other three atmospheric events were lower. The ratio of 232Th/238U radioactivity during the Asian dust period was 1.22, higher than the ratio for the other three atmospheric events.