DOI QR코드

DOI QR Code

Fundamental study on volume reduction of cesium contaminated soil using cyclone-type magnetic separator

  • Hina Miura (Graduate School of Engineering, Osaka University) ;
  • Yoko Akiyama (Graduate School of Engineering, Osaka University) ;
  • Yuichiro Manabe (Graduate School of Engineering, Osaka University) ;
  • Fuminobu Sato (Graduate School of Engineering, Osaka University)
  • 투고 : 2024.05.23
  • 심사 : 2024.09.28
  • 발행 : 2024.09.30

초록

A large amount of cesium-contaminated soil was generated as a result of the decontamination work following the accident at the Fukushima Daiichi Nuclear Power Plant. To reduce the final disposal volume of contaminated soil, it is necessary to separate the contaminated soil into low- and high-dose soil components and reuse the low-dose soil under 8000 Bq/kg. We have investigated a magnetic separation technique to reduce the volume of the contaminated soil. Magnetic separation is a volume reduction technology that utilizes these differences in magnetic properties. However, the high-gradient magnetic separation technique (HGMS) we have been studied has problems such as clogging of filters and low separation accuracy due to the passage of 2:1 type clay minerals with small particle diameters. In this study, we propose a new separation method using a cyclone-type magnetic separator that focuses not only on magnetic susceptibility but also on differences in particle size. The cyclone-type magnetic separator can separate 2:1 type clay minerals from 1:1 type clay minerals by inducing 1:1 type clay minerals with large particle diameters to the outside of the cylinder and 2:1 type clay minerals with small and large particle diameters to the inside of the cylinder through the difference in the combined magnetic and centrifugal forces acting on soil particles. Separation accuracy was evaluated using simulated soil consisting of vermiculite and kaolinite. Based on these results, the reduction rate of the radioactivity concentration was estimated, and the design guidelines of the device for practical use were discussed.

키워드

참고문헌

  1. Ministry of the Environment, Japan, "Efforts toward final disposal outside the prefecture, Amount of soil removed and radioactivity concentration" Interim storage facility information site, http://josen.env.go.jp/chukanchozou/facility/effort/
  2. Ministry of the Environment, Japan, "Strategy for the Development of Technology for Volume Reduction and Recycling of Soil Removed from Interim Storage, etc.", p. 5, April 2016.
  3. Y. Nishimoto, Y. Akiyama, H. Tsujimoto, M. Kawano, K. Miura, "Study on Volume Reduction of Cesium Contaminated Soil by High Gradient Magnetic Separation: Design of Magnetic Filters" IEEE Transactions on Applied Superconductivity, vol. 31, No. 5, pp. 1-5, Aug. 2021.
  4. K. Yukumatsu, N. Nomura, F. Mishima, Y. Akiyama, S. Nishijima. "Study on Volume Reduction of Cesium Contaminated Soil by Magnetic Separation", IEEE Transactions on Applied Superconductivity, vol.26, No.4, pp. 1-4, June 2016.
  5. A. Nakao, S. Funakawa, T. Kosaki, "Characterization of the frayed edge site of micaceous minerals in soil clays influenced by different pedogenetic conditions in Japan and northern Thailand", Soi Science and Plant Nutrition, vol.54, No.4, pp. 479-489, July 2008.
  6. M. Yoshida, "Properties of mineral composition of Soma Ohori clay in Fukushima prefecture" Journal of the Ceramic Society of Japan, vol.79, No.907, pp.75-81, April 1971.
  7. Soil formation classification laboratory, Environmental resources department, National Institute of Agro-Environmental Sciences "Typology and Regional Characteristics of Clay Mineral Composition in Lowland Soils in Japan" https://www.naro.affrc.go.jp/archive/niaes/sinfo/result/result13/result13_02.html
  8. M. Kawano and H. Watarai,"Brownian motion-magnetophoresis of nano/micro-particles" Analyst, vol. 137, pp.4123-4126, 2012.
  9. Y. Akemoto, M. Kan, S. Tanaka, "Static Adsorption of Cesium Ions on Kaolin/Vermiculite and Dynamic Adsorption/Desorption Using the Electrokinetic Process", Journal of Chemical Engineering of Japan, vol.52, No.7, pp.662-669, 2019.
  10. Ministry of the Environment, Japan, "The 10th Meeting of the Committee on the Development Strategy for Volume Reduction and Recycling of Soil Removed from Interim Storage, Strategy for Volume Reduction and Recycling of Soil Removed from Interim Storage", March 19, 2019. http://josen.env.go.jp/chukanchozou/facility/effort/investigative_commission/pdf/proceedings_190319_04_03.pdf
  11. H. Horie, K. Yukumatsu, F. Mishima, Y. Akiyama, S. Nishijima, T. Sekiyama, S. Mitsui, and M. Kato, "Volume reduction of cesium contaminated soil by magnetic separation - Pretreatment of organic matters -", Journal of Physics: Conference Series, 871, 012102, 2017.