DOI QR코드

DOI QR Code

A Comparative Study on Gamma-ray Measurement and MCNP Simulation for Precise Measurement of Spent Nuclear Fuel Burnup

  • Sohee Cha (Kyung Hee University) ;
  • Kwangheon Park (Kyung Hee University)
  • 투고 : 2024.01.12
  • 심사 : 2024.04.18
  • 발행 : 2024.06.30

초록

To non-destructively determine the burnup of a spent nuclear fuel assembly, it is essential to analyze the nuclear isotopes present in the assembly and detect the neutrons and gamma rays emitted from these isotopes. Specifically, gamma-ray measurement methods can utilize a single radiation measurement value of 137Cs or measure based on the energy peak ratio of Cs isotopes such as 134Cs/137Cs and 154Eu/137Cs. In this study, we validated the extent to which the results of gamma-ray measurements using cadmium zinc telluride (CZT) sensors based on 137Cs could be accurately simulated by implementing identical conditions on MCNP. To simulate measurement scenarios using a lead collimator, we propose equations that represent radiation behavior that reaches the detector by assuming "Direct hit" and "Penetration with attenuation" situations. The results obtained from MCNP confirmed an increase in measurement efficiency by 0.47 times when using the CZT detector, demonstrating the efficacy of the measurement system.

키워드

과제정보

This work was partly supported by Korea Institute of Energy Technology Evaluation and Planning (KETEP) grant funded by the Korea government (MOTIE) (20222B10100060, Development of On-site Burn-up Detection System for the Spent Fuel).

참고문헌

  1. S.H. Cha and K.H. Park, "An Analysis of Neutron Sources and Gamma-Ray in Spent Fuels Using SCALE-ORIGEN-ARP", J. Surf. Sci. Eng., 56(1), 84-93 (in Korean) (2023). 
  2. H. Trellue, G. McMath, A. Trahan, A. Favalli, T. Burr, A. Sjoland, and U. Backstrom, "Spent Fuel Nondestructive Assay Integrated Characterization From Active Neutron, Passive Neutron, and Passive Gamma", Nucl. Instrum. Methods Phys. Res. A, 988, 164937 (2021). 
  3. C.A. Miller, W.A. Peters, F.Y. Odeh, T.H. Shin, M. Mamtimin, S.D. Clarke, T.L. Grimm, and S.A. Pozzi, "Sub-Critical Assembly Die-Away Analysis With Organic Scintillators", Nucl. Instrum. Methods Phys. Res. A, 959, 163598 (2020). 
  4. S.M. Bowman and I.C. Gauld, OrigenArp Primer: How to Perform Isotopic Depletion and Decay Calculations With SCALE/ORIGEN, Oak Ridge National Laboratory, ORNL/TM-2010/43 (2010). 
  5. J. Hu, R. McElroy Jr., A.D. Nicholson, and S. Croft. Fork Experiments in the Hot Cell Using Spent Fuel Rods for International Nuclear Safeguards, Oak Ridge National Laboratory Technical Report, ORNL/SPR-2020/1774 (2021). 
  6. S. Vaccaro, I.C. Gauld, J. Hu, P. de Baere, J. Peterson, P. Schwalbach, A. Smejkal, A. Tomanin, A. Sjoland, S. Tobin, and D. Wiarda, "Advancing the Fork Detector for Quantitative Spent Nuclear Fuel Verification", Nucl. Instrum. Methods Phys. Res. A, 888, 202-217 (2018). 
  7. T.W. Doering and G.A. Cordes, "Status of the MultiDetector Analysis System (MDAS) and the Fork Detector Research Programs", Proc. of Technical Committee Meeting on Implementation of Burnup Credit in Spent Fuel Management Systems, IAEA-TECDOC-1241, 286-297, IAEA, Vienna (2000). 
  8. H.M. Park, T.Y. Kim, Y.S. Song, U.J. Lee, and C.M. Ham, "Spectroscopic Properties of Gamma-Ray Detector to Measure the Burnup of Spent Nuclear Fuel", J. Radiat. Ind., 17(1), 119-125 (in Korean) (2023). 
  9. S. Cha, K. Park, M.O. Kim, J.H. Ko, and J.H. Sung, "A Method to Estimate the Burnup Using Initial Enrichment, Cooling Time, Total Neutron Source Intensity and Gamma Source Activities in Spent Fuels", J. Nucl. Fuel Cycle Waste Technol., 21(3), 303-313 (2023).