DOI QR코드

DOI QR Code

A Numerical Study of the Performance Assessment of Coupled Thermo-Hydro-Mechanical (THM) Processes in Improved Korean Reference Disposal System (KRS+) for High-Level Radioactive Waste

수치해석을 활용한 향상된 한국형 기준 고준위방사성폐기물 처분시스템의 열-수리-역학적 복합거동 성능평가

  • Received : 2021.07.22
  • Accepted : 2021.08.06
  • Published : 2021.08.31

Abstract

A numerical study of the performance assesment of coupled thermo-hydro-mechanical (THM) processes in improved Korean reference disposal system (KRS+) for high-level radioactive waste is conducted using TOUGH2-MP/FLAC3D simulator. Decay heat from high-level radioactive waste increases the temperature of the repository, and it decreases as decay heat is reduced. The maximum temperature of the repository is below a maximum temperature criterion of 100℃. Saturation of bentonite buffer adjacent to the canister is initially reduced due to pore water evaporation induced by temperature increase. Bentonite buffer is saturated 250 years after the disposal of high-level radioactive waste by inflow of groundwater from the surrounding rock mass. Initial saturation of rock mass decreases as groundwater in rock mass is moved to bentnonite buffer by suction, but rock mass is saturated after inflow of groundwater from the far-field area. Stress changes at rock mass are compared to the Mohr-Coulomb failure criterion and the spalling strength in order to investigate the potential rock failure by thermal stress and swelling pressure. Additional simulations are conducted with the reduced spacing of deposition holes. The maximum temperature of bentonite buffer exceeds 100℃ as deposition hole spacing is smaller than 5.5 m. However, temperature of about 56.1% volume of bentonite buffer is below 90℃. The methodology of numerical modeling used in this study can be applied to the performance assessment of coupled THM processes for high-level radioactive waste repositories with various input parameters and geological conditions such as site-specific stress models and geothermal gradients.

기존의 한국형 기준 처분시스템의 처분 효율을 높인 향상된 한국형 기준 처분시스템(Improved Korean Reference Disposal System, KRS+)의 열-수리-역학적 복합거동 성능평가를 위해 TOUGH2-MP/FLAC3D를 이용한 수치모델링 연구가 수행되었다. 사용후핵연료 처분 이후 방사성 붕괴열에 의해 처분시스템의 온도가 상승하고, 방사성 붕괴열이 빠르게 감소함에 따라 온도가 감소하여 최대 온도가 설계기준 온도인 100℃를 넘지 않는 것으로 나타났다. 완충재의 초기 포화도는 온도 상승으로 인한 공극수의 증발로 인해 감소하였다가 주변 암반으로부터 지하수가 유입되어 처분 약 250년 후 포화 상태에 이르렀다. 암반에서는 완충재와 암반의 흡입력의 차이로 인해 암반에서 완충재로 지하수가 유입되어 처분 직후 포화도가 감소하다가 이후 원계 암반으로부터 지하수가 유입되어 포화 상태에 도달했다. 처분시스템 내 열응력과 팽윤압 발생에 의한 주변 암반의 파괴 가능성을 평가하고자 모어-쿨롱 파괴기준식과 스폴링 강도를 사용하였다. KRS+ 처분시스템의 처분공의 간격을 감소시키면서 처분시스템의 열적 거동 변화를 확인하였는데, 처분공 간격이 5.5 m 이하에서는 완충재의 설계 기준 온도를 초과하게 된다. 다만, 벤토나이트 완충재 부피의 56.1%의 온도는 90℃ 이하로 유지되었다. 본 연구에서 사용한 수치해석 기법은 향후 응력 모델, 지온 경사 및 입력 물성을 변화시킨 다양한 조건에서의 처분시스템의 THM 복합거동 성능평가에 활용할 수 있을 것으로 판단된다.

Keywords

Acknowledgement

이 논문은 2021년도 정부(과학기술정보통신부)의 재원으로 사용후핵연료관리핵심기술개발사업단 및 한국연구재단의 지원(2021M2E1A1085193)과 고준위폐기물관리차세대혁신기술개발사업의 지원(2021M2E3A2041312)을 받아 수행된 연구사업입니다.

References

  1. 김형찬, 황재홍, 박승균, 2019, 2019 한국의 지열주제도감, 한국지질자원연구원, 41p.
  2. Aydan, O. and Kawamoto, T., 2001, The stability assessment of a large underground opening at great depth, In: Proceedings of the 17th International Mining Congress and Exhibition of Turkey (IMCET2001), Ankara ,Turkey, June 2001, 277-288.
  3. Aydan, O., Akagi, T., and Kawamoto, T., 1993, The squeezing potential of rocks around tunnels; theory and prediction, Rock Mechanics and Rock Engineering, 26(2), 137-163. https://doi.org/10.1007/BF01023620
  4. Bieniawski, Z.T., 1989, Engineering rock mass classifications, New York, Wiley.
  5. Birkholzer, J., Rutqvist, J., Sonnenthal, E., and Barr D., 2007, DECOVALEX-THMC project. Task D. Long-term permeability/porosity changes in the EDZ and near field due to THM and THC processes in volcanic and crystalline-bentonite systems, Phase 1 report, SKI technical report 2007-10, Swedish Nuclear Power Inspectorate, Stockholm, Sweden.
  6. Cho, W.J., Chun, K.S., and Lee, J.O., 1999, Effect of dry density and temperature on the hydraulic conductivity of domestic compacted bentonite as a buffer material in the high-level waste repository, KAERI Technical Report, KAERI/TR-1223/1999, Korea Atomic Energy Research Institute.
  7. Cho, W.J., Lee, J.O., Kwon, S., 2010, Analysis of Thermo-hydro-mechanical Behavior of the Engineered Barrier System of a High-level Waste Repository. KAERI Technical Report KAERI/TR-4142/2010. Korea Atomic Energy Research Institute.
  8. Choi, H.J., Lee, J.Y., Kim, S.S., Kim, S.K., Cho, D.G., Kim, K.Y., Jeong, J.T., Jeon, K.S., Choi, J.W., Lee, J.O., Lee, M.S., and Kim, P.O., 2008, Korean reference HLW disposal system. KAERI technical report, KAERI/TR-3563/2008, Korea Atomic Energy Research Institute.
  9. Cui, Y.J., 2017, On the hydro-mechanical behaviour of MX80 bentonite-based materials, Journal of Rock Mechanics and Geotechnical Engineering, 9, 565-574. https://doi.org/10.1016/j.jrmge.2016.09.003
  10. ENRESA, 2000, FEBEX project: full-scale engineered barrieres experiment for a deep geological repository for high level radioactive waste in crystaline host rock, Final report, ENRESA, Madrid, Spain.
  11. Garitte, B., Nguyen, T.S., Barnichon, J.D., Graupner, B.J., Lee C., Maekawa, K., Manepally, C., Ofoegbu, G., Dasgupta, B., Fedors, R., Pan, P.Z., Feng, X.T., Rutqivst, J., Chen, F., Birkholzer, J., Wang, Q., Kolditz, O., and Shao, H., 2017, Modelling the Mont Terri HE-D experiment for the thermal-hydraulic-mechanical response of a bedded argillaceous formation to heating, Environmental Earth Sciences, 76, 345. https://doi.org/10.1007/s12665-017-6662-1
  12. Gens, A., 2017, DECOVALEX 2019 Task D: HM and THM interactions in bentonite engineered barrieres (INBEB), Stage 2: Post-dismantling period of the EB experiment, Task description of Task D.
  13. Gens, A., Sanchez, M., Guimaraes, L.D.N., Alonso, E.E., Lloret, A., Olivella, S., Villar, M.V., and Huertas, F., 2009, A full-scale in situ heating test for high-level nuclear waste disposal: Observations, analysis and interpretation, Geotechnique, 59(4), 377-399. https://doi.org/10.1680/geot.2009.59.4.377
  14. Genuchten, M.T.V., 1980, A closed-form equation for predicting the hydraulic conductivity of unsaturated soils, Soil Science Society of America Journal, 44(5), 892-898. https://doi.org/10.2136/sssaj1980.03615995004400050002x
  15. Guo, R., Xu, H., Plua, C., and Armand, G., 2020, Prediction of the thermal-hydraulic-mechanical response of a geological repository at large scale and sensitivity analyses, International Journal of Rock Mechanics and Mining Sciences, 136, 104484. https://doi.org/10.1016/j.ijrmms.2020.104484
  16. Itasca, 2012, FLAC3D, Fast Lagrangian Analysis of Continua in 3 Dimensions, Version 5.0. Itasca Consulting Group, Minneapolis, Minnesota, Itasca.
  17. Jeanne, P., Rutqivst, J., Dobson, P.F., Walters, M., Hartline, C., and Garcia, J., 2014, The impacts of mechanical stress transfers caused by hydromechanical and thermal processes on fault stability during hydraulic stimulation in a deep geothermal reservoir, International Journal of Rock Mechanics and Mining Sciences, 72, 149-163. https://doi.org/10.1016/j.ijrmms.2014.09.005
  18. Kim, G.W., 1993, Revaluation of geomechanics classifications of rock masses, In: Geotechnical Engineering and Tunneling Technology, Korean Geotechnical Society Spring 93 National Conference, Seoul Korea.
  19. Kim, H.C. and Lee, Y., 2007, Heat flow in the republic of Korea, Journal of Geophysical Research, 112, B05413. https://doi.org/10.1029/2006JB004266
  20. Kim, I.Y., Kim, H.A., and Choi, H.J., 2013, Evaluation on thermal performance and thermal dimensioning of direct deep geolocial disposal systeme for high burn-up spent nuclear fuel, KAERI technical report, KAERI/TR-5230/2013, Korea Atomic Energy Research Institute.
  21. Kim, H., Synn, J.H., Park, C., Song, W.K., Park, E.S., Jung, Y.B., Cheon, D.S., Base, S., Choi, S.O., Chang, C., and Min, K.B., 2021, Korea stress map 2020 using hydraulic fracturing and overcoring data, Tunnel and Underground Space, 31(3), 145-166. https://doi.org/10.7474/TUS.2021.31.3.145
  22. Kwon, S. and Min, K.B., 2020, An introduction to the DECOVALEX-2019 task G: EDZ evolution - reliability, feasibility, and significance of measurements of conductivity and transmissivity of the rock mass, Tunnel and Underground Space, 30(4), 306-319. https://doi.org/10.7474/TUS.2020.30.4.306
  23. Lee, C., 2012, Characterization of thermal-mechanical behavior of rock mass in the excavation damaged zone at KURT, Ph.D. dissertation, Seoul National University, Korea.
  24. Lee, C., Cho, W.J., Lee, J. and Kim, G.Y., 2019a, Numerical analysis of coupled thermo-hydro-mechanical (THM) behavior at Korean reference disposal system (KRS) using TOUGH2-MP/FLAC3D simulator, Journal of Nuclear Fuel Cycle and Waste Technology, 17(2), 183-202. https://doi.org/10.7733/jnfcwt.2019.17.2.183
  25. Lee, C., Choi, H.J., and Kim, G.Y., 2020a, Numerical modelling of coupled thermo-hydro-mechanical behavior of heater experiment-D (HE-D) at Mont Terri rock laboratory in Switzerland, Tunnel and Underground Space, 30(3), 242-255. https://doi.org/10.7474/TUS.2020.30.3.242
  26. Lee, C., Lee, J., and Kim, G.Y., 2020b, Numerical analysis of FEBEX at Grimsel test site in Switzerland, Tunnel and Underground Space, 30(4), 359-381. https://doi.org/10.7474/TUS.2020.30.4.359
  27. Lee, C., Lee, J., Park, S., Kwon, S., Cho, W.J., and Kim, G.Y., 2020c, Numerical analysis of coupled thermo-hydro-mechanical behavior in single- and multi-layer repository concepts for high-level radioactive waste disposal, Tunnelling and Underground Space Technology, 103, 103452. https://doi.org/10.1016/j.tust.2020.103452
  28. Lee, C., Yoon, S., Cho, W.J., Jo, Y., Lee, S., Jeon, S., and Kim, G.Y., 2019b, Study on thermal, hydraulic, and mechanical properties of KURT granite and Gyeongju bentonite, Journal of Nuclear Fuel Cycle and Waste Technology, 17, 65-80. https://doi.org/10.7733/jnfcwt.2019.17.S.65
  29. Lee, J. and Cho, W.J., 2009, Thermal-hydro-mechanical properties of reference bentonite buffer for a Korean HLW repository. KAERI Technical Report, KAERI/TR-3729/2009, Korea Atomic Energy Research Institute.
  30. Lee, J., Cho, D., Choi, H., and Choi, J., 2007, Concept of a Korean reference disposal system for spent fuels, Journal of Nuclear Science and Technology, 44(12), 1565-1573. https://doi.org/10.3327/jnst.44.1565
  31. Lee, J., Kim, H., Kim, Y., Choi, H., and Cho, D., 2020e, Analyses on thermal stability and structural integrity of the improved disposal systems for spent nuclear fuels in Korea, Journal of Nuclear Fuel Cycle and Waste Technology, 18, 21-36. https://doi.org/10.7733/jnfcwt.2020.18.S.21
  32. Lee, J., Kim, I., Ju, H.J., Choi, H., and Cho, D., 2020d, Proposal of an improved concept design for the deep geological disposal system of spent nuclear fuel in Korea. Journal of Nuclear Fuel Cycle and Waste Technology, 18, 1-19.
  33. Lee, J., Lee, C. and Kim, G.Y., 2016, Development of TOUGH2-MP/FLAC3D simulator for the coupled thermal-hydraulic-mechanical analysis in porous media, KAERI Technical Report, KAERI/TR-6737/2016, Korea Atomic Energy Research Institute.
  34. Meier, T., Backers, T, Eberhardt, E., Fisher, B., Geier, J., Kwon, S., Min, K.-B., Blaheta, R., Hancilova, I., Hasal, M., Riha, J., and Lanaro, F., 2021, Reliability, feasibility and significance of measurements of conductivity and transmissivity of the rock mass for the understanding of the evolution of a repository of radioactive waste, Swedish Radiation Safety Authority Report SSM 2021:14, Stockholm, Sweden.
  35. Nguyen, T.S., Selvadurai, A.P.S., and Armand, G., 2005, Modelling the FEBEX THM experiment using a state surface approach, International Journal of Rock Mechanics and Mining Sciences, 42, 639-651. https://doi.org/10.1016/j.ijrmms.2005.03.005
  36. Plua, C., Vu, M.N., Armand, G., Rutqivst, J., Birkholzer, J., Xu, H., Guo, R., Thatcher, K.E., Bond, A.E., Wang, W., Nagel, T., Shao, H., and Kolditz, O., 2021, A reliable numerical analysis for large-sacle modelling of a high-level radioactive waste repository in the Callovo-Oxfordian claystone, International Journal of Rock Mechanics and Mining Sciences, 140, 104574. https://doi.org/10.1016/j.ijrmms.2020.104574
  37. Pruess, K., Oldenburg, C., and Moridis, G., 2011, TOUGH2 user's guide, version 2, Lawrence Berkeley National Laboratory Report LBNL-43134, Berkeley, CA, USA.
  38. Pusch, R., 2001, The microstructure of MX-80 clay with respect to its bulk physical properties under different environmental conditions, Technical Report TR-01-08, Stockholm, Sweden: Swedish Nuclear Fuel and Waste Management Co.
  39. Rutqvist, J. and Tsang, C.F., 2002, A study of caprock hydromechanical changes associated with CO2-injection into a brine formation, Environmental Geology, 42, 296-305. https://doi.org/10.1007/s00254-001-0499-2
  40. Rutqvist, J. and Tsang, C.F., 2004, A fully coupled three-dimensional THM analysis of the Febex in situ test with the Rockmas code: Prediction of THM behavior in a bentonite barrier, Elsevier Geo-Engineering Book Series 2, 143-148. https://doi.org/10.1016/S1571-9960(04)80032-6
  41. Rutqvist, J., 2020, Thermal management associated with geologic disposal of large spent nuclear fuel canisters in tunnels with thermally engineered backfill, Tunnelling and Underground Space Technology, 102, 103454. https://doi.org/10.1016/j.tust.2020.103454
  42. Rutqvist, J., Rinaldi, A.P., Cappa, F., and Moridis, G.J., 2013, Modeling of fault reactivation and induced seismicity during hydraulic fracturing of shale-gas reservoirs, Journal of Petroleum Science and Engineering, 107, 31-44. https://doi.org/10.1016/j.petrol.2013.04.023
  43. Rutqvist, J., Wu, Y.S., Tsang, C.F., and Bodvarsson, G., 2002, A modeling approach for analysis of coupled multiphase fluid flow, heat transfer, and deformation in fractured porous rock, International Journal of Rock Mechanics and Mining Sciences 39, 429-442. https://doi.org/10.1016/S1365-1609(02)00022-9
  44. Sanchez, M., Gens, A., and Guimaraes, L., 2012, Thermal-hydraulic mechanical (THM) behaviour of a large-sacle in situ heating experiment during cooling and dismantling, Canadian Geotechnical Journal, 49, 1169-1195. https://doi.org/10.1139/t2012-076
  45. SKB, 2010, Design and production of the KBS-3 repository, Technical Report TR-10-12, Stockholm, Sweden: Swedish Nuclear Fuel and Waste Management Co.
  46. Song, Y., Kim, H.C., and Lee, S.K., 2006, Geothermal research and development in Korea, Economic and Engivronmental Geology, 39(4), 485-494.
  47. Synn, J.H., Park, C., and Lee, B.J., 2013, Regional distribution pattern and geo-historical transition of in-situ stress fields in the Korean Peninsula, Tunnel and Underground Space 23(6),457-469. https://doi.org/10.7474/TUS.2013.23.6.457
  48. Trueman, R., 1988, An evaluation of strata support techniques in dual life gateroads, Ph.D. Thesis, University of Wales, Cardiff, UK.
  49. Urpi, L., Rinaldi, A.P., Rutqvist, J., and Wiemer, S., 2019, Fault stability perturbation by thermal pressurization and stress transfer around a deep geological repository in a caly formation, Journal of Geophysical Research: Solid Earth, 124, 8506-8518. https://doi.org/10.1029/2019JB017694
  50. Vargaftik, N.B., 1975, Tables on the thermophysical properties of liquids and gases, second ed. John Wiley & Sons, New York.
  51. Villar, M.V., 2005, MX-80 bentonite. Thermo-hydro-mechanical characterisation performed at CIEMAT in the context of the prototype project, CIEMAT/DIAE/54540/2/04, Centro de Invstigaciones Energeticas, MedioAmbientales y Tecnologicas.
  52. Walker, W.R., Sabey, J.D., and Hamption, D.R., 1981, Studies of heat transfer and water migration in soils, Final report, Department of Agricultural and Chemical Engineering, Colorado State University, Fort Collins, CO, pp. 80523.
  53. Yoo, H., Park, S., Xie, L., Kim, K.I., Min, K.B., Rutqvist, J., and Rinaldi, A.P., 2021, Hydro-mechanical modeling of the first and second hydraulic stimulations in a fractured geothermal reservoir in Pohang, South Korea, Geothermics, 89, 101982. https://doi.org/10.1016/j.geothermics.2020.101982
  54. Yoon, S., Cho, W.H., Lee, C., and Kim, G.Y., 2018, Thermal conductivity of Korean compacted bentonite buffer materials for a nuclear waste repository, Energies (11), 2269. https://doi.org/10.3390/en11092269
  55. Zhang, K., Wu, Y.S., and Pruess, K., 2008, User's guide for TOUGH2-MP - A massively parallel version of the TOUGH2 code, Lawrence Berkeley National Laboratory Report LBNL-315E, Berkeley, CA, USA.