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제주지역 도로변 대기 중 에어로졸의 입경별 조성특성

Composition of Size-Segregated Atmospheric Aerosol Collected at an Urban Roadside Environment in Jeju Area

  • 허철구 (제주대학교 환경공학과) ;
  • 김수미 (제주특별자치도 보건환경연구원 대기환경과) ;
  • 이기호 (제주대학교 환경공학과)
  • Hu, Chul-Goo (Department of Environmental Engineering, Jeju National University) ;
  • Kim, Su-Mi (Air Environmental Division, Jeju Special Self-Governing Province Research Institute of Health & Environment) ;
  • Lee, Ki-Ho (Department of Environmental Engineering, Jeju National University)
  • 투고 : 2019.11.19
  • 심사 : 2019.12.17
  • 발행 : 2020.01.31

초록

To determine the size distributions of water-soluble inorganic ionic species (WSIS) in roadside aerosols, sampling experiments were carried out in the urban roadside area of Jeju City on August 2018 and January 2019 by using the eight-stage cascade impactor sampler. The mass of roadside aerosols were partitioned at 57% in fine fraction, 36-37% in coarse fraction, and 6-7% in giant fraction, regardless of summer and winter. The mass concentrations of WSIS except for Na+ and SO42- in roadside aerosols were higher in winter than in summer. The size distributions of Na+, Mg2+, Ca2+ and Cl- were characterized by bimodal types with coarse particle mode peaking around 3.3-4.7 ㎛ and 5.8-9.0 ㎛. The size distributions of NO3- and K+ shifted from a single fine mode peaking around 0.7-1.1 ㎛ in winter to bimodal and/or trimodal types with peaks around coarse mode in summer. SO42- and NH4+ showed a single fine mode peaking around 0.7-1.1 ㎛. The MMAD of roadside aerosols was lower than that of Na+, Mg2+, Ca2+ and Cl-. Based on the marine enrichment factors and the ratio values of WSIS and the corresponding value for sea water, the composition of roadside aerosols in Jeju City may be practically affected by terrestrial sources rather than marine source.

키워드

참고문헌

  1. Bathmanabhan, S., Madanayak, S. N. S., 2010, Analysis and interpretation of particulate matter-$PM_{10}$, $PM_{2.5}$ and -$PM_{1}$ emissions from the heterogeneous traffic near an urban roadway, Atmospheric Pollution Research, 1, 184-194. https://doi.org/10.5094/APR.2010.024
  2. Cacciola, R. R., Sarva, M., Polosa, R., 2002, Adverse respiratory effects and allergic susceptibility in relation to particulate air pollution: flirting with disaster, Allergy, 57, 281-286. https://doi.org/10.1034/j.1398-9995.2002.1r3315.x
  3. Calvo, A. I., Alves, C., Castro, A., Pont, V., Vicente, A. M., Fraile, R., 2013, Research on aerosol sources and chemical composition: Past, current and emerging issues, Atmospheric Research, 120-121, 1-28. https://doi.org/10.1016/j.atmosres.2012.09.021
  4. Cho, B. Y., Shin, S. H., Jung, C. S., Ju, M. H., Yoon, M. H., Ahn, J. E., Bae,, G. S., 2019, Characteristics of particle size distribution at the roadside of Daegu. J. Korean Society for Atmospheric Environment, 35, 16-26. https://doi.org/10.5572/KOSAE.2019.35.1.016
  5. Custodio, D., Cerqueira, M., Alves, C., Nunes, T., Pio, C., Esteves, V., Frosini, D., Lucarelli, F., Querol, X., 2016, A One-year record of carbonaceous components and major ions in aerosols from an urban kerbside location in Oporto, Portugal, Science of the Total Environment, 562, 822-833. https://doi.org/10.1016/j.scitotenv.2016.04.012
  6. DoT (Department of Transport) (UK), 2002, Sources of Particulate Matter in Urban Areas: TRAMAQ Project UG 250.
  7. Duan, J., Li, X., Tan, J., Chai, F., 2009, Size distribution and source apportionment of atmospheric particle number concentration in winter in Beijing, Research of Environmental Sciences, 22, 1134-1140.
  8. Economopoulou, A. A, Economopoulos, A. P., 2002, Air pollution in Athens Basin and health risk assessment, Environmental Monitoring and Assessment, 80, 277-299. https://doi.org/10.1023/A:1021124404645
  9. Espinosa, A. J. F., Ternero Rodriguez, M., Barragan de la Rosa, F. J., Jimnez Sanchez, J. C., 2001, Size distribution of metals in urban aerosols in Seville (Spain), Atmospheric Enveironment, 35, 2595-2601. https://doi.org/10.1016/S1352-2310(00)00403-9
  10. Ha, H. J., 2011, Comparative evaluation of the air quality at the center lane and roadside in the exclusive median bus lane, Ph. D. Dissertation, University of Seoul, Seoul.
  11. Han, X., Naeher, L. P., 2006, A Review of traffic-related air pollution exposure assessment studies in the developing world, Environmental International, 32, 106-120. https://doi.org/10.1016/j.envint.2005.05.020
  12. Hu, C. G., Lee, K. H., 2018, Chemical composition of fine particulate matter in the downtown Area of Jeju City, J. of Environmental Science International, 27, 597-610. https://doi.org/10.5322/JESI.2018.27.7.597
  13. Hu, H., Lia, T., Chen, X., 2017, The concentration distribution of exposures to particulate air pollution on different road sections, Transportation Research Procedia, 25, 3343-3353. https://doi.org/10.1016/j.trpro.2017.05.199
  14. Jiang, F., Liu, F., Lin, Q., Fu, Y., Yang, Y., Peng, L., Lian, X., Zhang, G., Bi, X., Wang, X., Sheng, G., 2019, Characteristics and formation mechanisms of sulfate and nitrate in size-segregated atmospheric particles from urban Guangzhou, China, Aerosol and Air Quality Research, 19, 1284-1293. https://doi.org/10.4209/aaqr.2018.07.0251
  15. Karagulian, F., Belis, C. A., Dora, C. F. C., Prüss-Ustün, A. M., Bonjour, S., Adair-Rohani, H., Amann, M., 2015, Contributions to cities' ambient particulate matter (PM): A systematic review of local source contributions at global level, Atmospheric Environment, 120, 475-483. https://doi.org/10.1016/j.atmosenv.2015.08.087
  16. Kerminen, V. M., Pakkanen, T. A., Hillamo, R. E., 1997, Interactions between inorganic trace gases and super -micrometer particles at a coastal site, Atmospheric Environment, 31, 2753-2765. https://doi.org/10.1016/S1352-2310(97)00092-7
  17. Kim, S. M., Kim, K. S., Hyun, S. S., Kim, J. H., Kim, M. C., Kim, B. J., Lee, K. H., 2018, Chemical composition and source apportionment of $PM_{2.5}$ in Jeju City in 2017, J. of the Korean Society for Environmental Analysis, 21, 61-70.
  18. Kim, Y. P., Bae, G. N., Ji, J. H., Jin, H. C., Moon, K. C., 1999, Aerosol size distribution and composition at Kosan, Cheju Island: Measurements in April 1998. J. Korean Society for Atmospheric Environment, 15, 677-685.
  19. Kulshrestha, U. C., Sarkar, A. K., Srivastava, S. S., Parashar, D. C., 1995, Wet-only and bulk deposition studies at New Delhi(India), Water, Air and Soil Pollution, 85, 2137-2142. https://doi.org/10.1007/BF01186150
  20. Lee, D. E., Kim, W. H., Jo, E. K., Han, J. H., Kang, C. H., Kim, K. H., 2011, Acidification and neutralization characteristics of atmospheric fine particles at Gosan Site of Jeju Island in 2008, J. Korean Society for Atmospheric Environment, 27, 603-613. https://doi.org/10.5572/KOSAE.2011.27.5.603
  21. Lee, J. H., Kim, Y. P., Moon, K. C., Kim, H. K., Lee, C. B., 2001, Fine particle measurements at two background sites in Korea between 1996 and 1997, Atmospheric Environment, 35, 635-643. https://doi.org/10.1016/S1352-2310(00)00378-2
  22. Lee, K. H., Yang, H. J., Hu, C. G., 2003, Size distribution of ambient aerosol measured at a coastal site in Jeju Island, J. of the Environmental Sciences, 12, 1043-1054. https://doi.org/10.5322/JES.2003.12.10.1043
  23. Lee, K. H., Hu, C. G., 2018, Elemental composition and source identification of $PM_{2.5}$ in Jeju City, J. of Environmental Science International, 27, 543-554. https://doi.org/10.5322/JESI.2018.27.7.543
  24. Lee, K. H., Kim, S. M., Hu, C. G., 2017, Ionic compositions of fine particulate matter during summer and winter in the downtown area of Jeju City in Jeju Island, J. of Environmental Science International, 26, 591-600. https://doi.org/10.5322/JESI.2017.26.5.591
  25. MOLIT (Ministry of Land, Instructure and Transport) and LH, 2019, 2018 Statistics of urban planning; http://upis.go.kr/upispweb/statsmgmt/viewListdown.do.
  26. Moon, K. J., Han, J. S., Kong, B. J., Lee, M. D., Jung, I. R., 2005, Characteristics of chemical species in gaseous and aerosol phase measured at Gosan, Korea During ABC- EAREX2005, J. Korean Society for Atmospheric Environment, 21, 675-687.
  27. Oh, M. S., Lee, T. J., Kim, D. S., 2009, Characteristics of ionic components in size-resolved particulate matters in Suwon area, J. Korean Society for Atmospheric Environment, 25, 46-56. https://doi.org/10.5572/KOSAE.2009.25.1.046
  28. Pakkanen, T. A., Loukkola, K., Korhonen, C. H., Aurela, M., Makela, T., Hillamo, R. E., Maenhaut, W., 2001, Sources and chemical composition of atmospheric fine and coarse particles in the Helsinki area. Atmospheric Environment, 35, 5381-5391. https://doi.org/10.1016/S1352-2310(01)00307-7
  29. Park, J. Y., Lim, H. J., 2006, Characteristics of water soluble ions in fine particles during the winter and spring in Daegu, J. Korean Society for Atmospheric Environment, 22, 627-641.
  30. Parmar, R. S., Satsangi, G. S., Kumari, M., Lakhani, A., Srivastava, S. S., Prakash, S., 2001, Study of size distribution of atmospheric aerosol at Agra. Atmospheric Environment, 35, 693-702. https://doi.org/10.1016/S1352-2310(00)00317-4
  31. Pey, J., Querol, X., Alastuey, A., Rodriguez, S., Putaud, J. P., Van Dingenen, R., 2009, Source apportionment of urban fine and ultra-fine particle number concentration in a Western Mediterranean city, Atmospheric Environment, 43, 4407-4415. https://doi.org/10.1016/j.atmosenv.2009.05.024
  32. Samara, C., Voutsa, D., 2005, Size distribution of airborne particulate matter and associated heavy metals in the roadside environment, Chemosphere, 59, 1197-1206. https://doi.org/10.1016/j.chemosphere.2004.11.061
  33. Shields, L. G., Suess, D. T., Prather, K. A., 2007, Determination of single particle mass spectral signatures from heavy-duty diesel vehicle emissions for $PM_{2.5}$ source apportionment. Atmospheric Environment, 41, 3841-3852. https://doi.org/10.1016/j.atmosenv.2007.01.025
  34. Thorpe, A., Harrison, R. M., 2008, Sources and properties of non-exhaust particulate matter from road traffic a review. Science of the Total Environment, 400, 270-282. https://doi.org/10.1016/j.scitotenv.2008.06.007
  35. UN, 2018, World urbanization prospects; https://esa.un.org/unpd/wup/Download/.
  36. Wrobel, A., Rokita, E., Maenhaut, W., 2000, Transport of traffic-related aerosols in urban areas. The Science of the Total Environment, 257, 199-211. https://doi.org/10.1016/S0048-9697(00)00519-2
  37. Yoo, E. C., Dou, W. G.,Cho, J. G., 2009, Study for the control of re-suspended dust from paved poad, The Annual Report of Busan Metropolitan City Institute of Health & Environment, 19, 177-186.
  38. Zavala, M., Herndon, S. C., Wood, E. C., Onasch, T. B., Knighton, W. B., Marr, L. C., Kolb, C. E., Molina, L. T., 2009, Evaluation of mobile emissions contributions to Mexico City's emissions inventory using on-road and cross-road emission measurements and ambient data. Atmospheric Chemistry and Physics, 9, 6305-6317. https://doi.org/10.5194/acp-9-6305-2009
  39. Zhang, K., Chai, F., Zhang, X., Duan, N., Ma, X., 2008, Mass Concentration Characters of PM2.5 in Autumn in Jiaxing, Research of Environmental Sciences, 3, 1-6.