Journal of Electrochemical Science and Technology

The Korean Electrochemical Society (한국전기화학회)
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Free-standing Three Dimensional Graphene Incorporated with Gold Nanoparticles as Novel Binder-free Electrochemical Sensor for Enhanced Glucose Detection

  • Bui, Quoc Bao (Sustainable Developments in Civil Engineering Research Group, Faculty of Civil Engineering, Ton Duc Thang University) ;
  • Nguyen, Dang Mao (Department of Polymer and Composite Materials, Faculty of Material Science, University of Science, Vietnam National University Ho Chi Minh city (VNU)) ;
  • Nguyen, Thi Mai Loan (The National Centre of Drug Information and Adverse Drug Reaction Monitoring, Hanoi University of Pharmacy) ;
  • Lee, Ku Kwac (Institute of Carbon Technology, Jeonju University) ;
  • Kim, Hong Gun (Institute of Carbon Technology, Jeonju University) ;
  • Ko, Sang Cheol (Institute of Carbon Technology, Jeonju University) ;
  • Jeong, Hun (Institute of Carbon Technology, Jeonju University)
  • Received : 2018.05.16
  • Accepted : 2018.07.04
  • Published : 2018.09.30
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Abstract

The electrochemical sensing performance of metal-graphene hybrid based sensor may be significantly decreased due to the dissolution and aggregation of metal catalyst during operation. For the first time, we developed a novel large-area high quality three dimensional graphene foam-incorporated gold nanoparticles (3D-GF@Au) via chemical vapor deposition method and employed as free-standing electrocatalysis for non-enzymatic electrochemical glucose detection. 3D-GF@Au based sensor is capable to detect glucose with a wide linear detection range of $2.5{\mu}M$ to 11.6 mM, remarkable low detection limit of $1{\mu}M$, high selectivity, and good stability. This was resulted from enhanced electrochemical active sites and charge transfer possibility due to the stable and uniform distribution of Au NPs along with the enhanced interactions between Au and GF. The obtained results indicated that 3D-GF@Au hybrid can be expected as a high quality candidate for non-enzymatic glucose sensor application.

Keywords

References

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