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Radon Concentrations in Groundwater of the Goesan Area, Korea

괴산지역 지하수의 라돈 함량

  • Cho, Byong-Wook (Groundwater and Ecohydrology Research Center, Korea Institute of Geoscience and Mineral Resources)
  • 조병욱 (한국지질자원연구원 지하수생태연구센터)
  • Received : 2017.08.03
  • Accepted : 2017.09.19
  • Published : 2017.10.31

Abstract

Radon concentrations were measured in 250 groundwater samples collected from the Goesan area where uraniferous black slate and granites abundantly occur in the formations. The measured radon levels ranged from 0.90 to 7,218.7 Bq/L with the median value of 54.3 Bq/L, similar to the value measured in the nationwide survey in 4,853 wells (52.1 Bq/L). The median value was highest in the Cretaceous granite area (390.0 Bq/L) while it was as low as 20.0~58.8 Bq/L in the Ogcheon meta-sedimentary rock areas. About 23.6% of the total samples exceeded the WHO guideline value of 100 Bq/L established in 2011. The exceeding rate was 69.0, 39.4, and 7.0~13.7% in the Cretaceous granite area, Jurassic granite area, and Ogcheon meta-sedimentary rock areas, respectively.

Keywords

References

  1. Abdallah, S.M., Habib, R.R., Nuwayhid, R.Y., Chatila, M., and Katul, G., 2007, Radon measurements in well and spring water in Lebanon, Radia. Meas., 42(2), 298-303. https://doi.org/10.1016/j.radmeas.2006.11.004
  2. Alabdula'aly, A.I., 1999, Occurrence of radon in the central region groundwater of Saudi Arabia, J. Environ. Radioact., 44, 85-95. https://doi.org/10.1016/S0265-931X(98)00063-0
  3. Althoyaib, S.S. and El-Taher, A., 2015, Natural radioactivity measurements in groundwater from Al-Jawa, Saudi Arabia, J. Radioanal. Nucl., Chem., 304, 547-552. https://doi.org/10.1007/s10967-014-3874-7
  4. Atkins, M.L., Santos, I.R., Perkins, A., and Maher, D.T., 2016, Dissolved radon and uranium in groundwater in a potential coal seam gas development region (Richmond River Catchment, Australia), J. Environ. Radioact., 154, 83-92. https://doi.org/10.1016/j.jenvrad.2016.01.014
  5. Banks, D., Royset, O., Strand, T., and Skarphagen, H., 1995, Radioelement (U, Th, Rn) concentrations in Norwegian bedrock groundwaters, Environ. Geol., 25, 165-180. https://doi.org/10.1007/BF00768546
  6. Banks, D., Frengstad, B., Midtgard, A.K., Krog, J.R., and Strand, T., 1998, The chemistry of Norwegian groundwaters: I The distribution of radon, major and minor elements in 1,604 crystalline bedrock groundwaters. Total Environ., 222, 71-91. https://doi.org/10.1016/S0048-9697(98)00291-5
  7. Barcelona, M.J., Gibb, J.P., Helfrich, J.A., and Garske, E.E., 1985, Practical guide for groundwater sampling, SWS Contract Report, 374 p.
  8. Cho, B.W., Sung, I.H., Cho, S.Y., and Park, S.K., 2007, A preliminary investigation of radon concentrations in groundwater of South Korea, J. Korea Soc. Groundw. Environ., 12(4), 98-104.
  9. Cho, B.W., Choo, C.O., Kim, M.S., Lee, Y.J., Yun, U., and Lee, B.D., 2011, Uranium and radon concentrations in groundwater near the Icheon granite, J. Eng. Geol., 21(3), 259-269. https://doi.org/10.9720/kseg.2011.21.3.259
  10. Cho, B.W., Kim, M.S., Kim, T.S., Yun, U., Lee, B.D., Hwang, J.H., and Choo C.O., 2013, Characteristics of occurrence and distribution of natural radioactive materials, uranium and radon in groundwater of the Danyang area, J. Eng. Geol., 23(4), 477-491. https://doi.org/10.9720/kseg.2013.4.477
  11. Cho, J.S., Ahn, J.K., Jim, H.Ch., and Lee, D.W., 2004, Radon concentrations in groundwater in Busan measured with a liquid scintillation counter method, J. Environ. Radioact., 78, 105-112. https://doi.org/10.1016/j.jenvrad.2004.02.007
  12. Godoy, J.M. and Godoy, M.L., 2006, Natural radioactivity in Brazilian groundwater, J. Environ. Radioact., 85, 71-83. https://doi.org/10.1016/j.jenvrad.2005.05.009
  13. Han, Y.L., Tom Kuo, M.C., Fan, K.C., Chiang, C.J., and Lee, Y.P., 2004, Radon distribution in groundwater of Taiwan, Hydrog. J., 14, 173-179.
  14. Hess, C.T., Michel, T.R., Horton T.R., Orichard, H.M., and Coniglo, W.A., 1985, The occurrence of radiocativity in public water supplies in the United States, Health Physics, 48(5), 553-586. https://doi.org/10.1097/00004032-198505000-00002
  15. Kim, J.H., 1989, Geochemistry and genesis of the Guryongsan (Ogcheon) uraniferous black slate, J. Kor. Inst. Min. Geol., 22(1), 35-63.
  16. Kim, M.S., Yang J.H., Geong, C.H., Kim, H.K., Kim, D.W., and Cho, B.W., 2014, Geochemical origins and occurrences of Natural radioactive materials in borehole groundwater in the Goesan area, J. Eng. Geol., 24(4), 535-550. https://doi.org/10.9720/kseg.2014.4.535
  17. King, P.T., Michel, J., and Moore, W.S., 1982, Ground water geochemistry of $^{228}Ra,\;^{226}Ra\;and\;^{220}Rn$, Geochim. et Cosmoche. Acta, 46, 1173-1182. https://doi.org/10.1016/0016-7037(82)90003-5
  18. Lee, B.J., Kim, D.H., Choi, H.I., Kee, W.S., and Park, K.H., 1996, The geological map of the Daejeon sheet (1:250,000), Korea Institute of Geology, Mining and Materials.
  19. Lee, C.H. and Kim, J.H., 1972, The geological map of Goesan sheet, Geological survey of Korea.
  20. Loomis, D.P., 1987, Radon-222 concentration and aquifer lithology in North Carolina, Ground Water Monit. Rev., 7(2), 33-39.
  21. Morland, G., Reimann, C., Strand, T., Skarphagen, H., Banks, D., Bjorvatn, K., Hall, E.M., and Siewers, U., 1997, The hydrogeochemistry of Norwegian bedrock groundwater-selected parameters (pH, F, Th, U, Th, Na, Ca) in samples from Vestfold and Hordaland, Norway, NGU Bull, 432, 103-117.
  22. National Research Council, 1999, Risk assessment of radon in drinking water, National Academies press, Washington.
  23. NIER, 2008, Studies on the naturally occurring radionuclides in groundwater of Korea (I) KIGAM report, 293 p.
  24. NIER, 2010, Occurrences of radionuclides in groundwater of the 4 high potential areas (10), KIGAM Report, 251 p.
  25. NIER, 2011, Study on the naturally occurring radionuclides in groundwater of the two high potential areas (11), KIGAM report, 253 p.
  26. NIER, 2012, Study on the naturally occurring radionuclides in groundwater of high potential area, NIER-SP2012-373, 245 p.
  27. NIER, 2013, Studies on the naturally occurring radionuclides in groundwater of the Youngin high potential area, NIER-SP2013-416, 220 p.
  28. NIER, 2015, Studies on the naturally occurring radionuclides in groundwater in the multi-geologic areas (15), NIER-SP2015-386, 203 p.
  29. Pinti, D.L., Retailleau, S., Barnetche, D., Moreira, F., Mortiz, A.M., Larocque, M., Gelinas, Y., Lefebvre, R., Helie, J.F., and Valadez, A., 2014, $^{222}Rn$ activity in groundwater of the St. Lawrence Lowlands, Quebec, eastern Canada: relation with local geology and health hazard, J. Environ. Radioact., 136, 206-217. https://doi.org/10.1016/j.jenvrad.2014.05.021
  30. Prasad, Y., Prasad, G., Choubey, V.M., and Ramola, R.C., 2009, Geohydrological control on radon availability in groundwater, Radia. Meas., 44, 122-126. https://doi.org/10.1016/j.radmeas.2008.10.006
  31. Przylibski, T.A., Mamont-Ciesla, K., Kusyk, M., Dorda, J., and Kozlowska, B., 2004, Radon concentrations in groundwaters of the Polish part of the Sudety Mountains (SW Poland), Environ. Radioact., 75, 193-209. https://doi.org/10.1016/j.jenvrad.2003.12.004
  32. Salonen, L. and Hukkanen, H., 1997, Advantages of low-background liquid scintillation alpha-spectrometry and pulse shape analysis in measuring radon, uranium, and radium-226 in groundwater samples, J. Radioanal. Nucl., Chem., 226(1), 67-74. https://doi.org/10.1007/BF02063626
  33. Shin, D.B. and Kim, S.J., 2011, Geochemical characteristics of black slate and coaly slate from the uranium deposit in Deokpyeong area, Econo. Environm. Geol., 44(5), 373-386. https://doi.org/10.9719/EEG.2011.44.5.373
  34. Skeppstrom, K. and Olofsson, B., 2007, Uranium and radon in groundwater, European Water, 17/18, 51-62.
  35. SSI, 1999, Radon legislation and national guidelines, Swedish Radiation Protection Institute.
  36. USEPA, 1999, Proposed radon in drinking water rule, Office of Water, EPA 815-F-99-006.
  37. Vesterbacka, P., Mkelinen, I. and Arvela, H., 2005, Natural radioactivity in drinking water in private wells in Finland, J. Radia. Prot. Dosim., 113(2), 223-232. https://doi.org/10.1093/rpd/nch446
  38. Voutilainen, A., Mkelinen, I., Huikuri, P., and Salonen, L., 2000, Radon atlas of wells drilled into bedrock in Finland, STUKA171, Helsinki: Steilyturvakeskus.
  39. WHO, 2011, Guidelines for drinking water quality. Chapter 9. Radiological aspects, 4th edition. World Health Organization, Geneva.
  40. Wu, Y.Y., Ma, Y.Z., Cui, H.X., Liu J.X., Sun Y.R., Shang, B., and Su, X., 2014, Radon concentrations in drinking water in Beijing City, China and contribution to radiation dose, Inter. J. Environ. Res. Pub. Health., 11, 11121-11131. https://doi.org/10.3390/ijerph111111121