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Development of a Cost-Effective 20K Hydrogen BET Measurement for Nanoporous Materials

나노다공체 물성 측정을 위한 극저온(20K) 수소 BET 개발 및 응용

  • Park, Jaewoo (Department of Energy Engineering, Gyeongnam National University of Science and Technology) ;
  • Oh, Hyunchul (Department of Energy Engineering, Gyeongnam National University of Science and Technology)
  • 박재우 (국립경남과학기술대학교 에너지공학과) ;
  • 오현철 (국립경남과학기술대학교 에너지공학과)
  • Received : 2017.07.25
  • Accepted : 2017.08.14
  • Published : 2017.09.27

Abstract

With the matters of climate change, energy security and resource depletion, a growing pressure exists to search for replacements for fossil fuels. Among various sustainable energy sources, hydrogen is thought of as a clean energy, and thus efficient hydrogen storage is a major issue. In order to realize efficient and safe hydrogen storage, various porous materials are being explored as solid-states materials for hydrogen storage. For those purposes, it is a prerequisite to characterize a material's textural properties to evaluate its hydrogen storage performance. In general, the textural properties of porous materials are analyzed by the Brunauer-Emmett-Teller (BET) measurement using nitrogen gas as a probe molecule. However, nitrogen BET analysis is sometimes not suitable for materials possessing small pores and surfaces with high curvatures like MOFs because the nitrogen molecule may sometimes be too large to reach the entire porous framework, resulting in an erroneous value. Hence, a smaller probe molecule for BET measurements (such as hydrogen) may be required. In this study, we describe a cost-effective novel cryostat for BET measurement that can reach temperatures below the liquefaction of hydrogen gas. Temperature and cold volume of the cryostat are corrected, and all measurements are validated using a commercial device. In this way, direct observation of the hydrogen adsorption properties is possible, which can translate directly into the determination of textural properties.

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References

  1. M. A. de la Casa-Lillo, F. Lamari-Darkrim, D. Cazorla-Amoros, A. Linares-Solano, J. Phys. Chem. B, 106, 10930 (2002). https://doi.org/10.1021/jp014543m
  2. A. Zuttel, Naturwissenschaften, 91, 157 (2004). https://doi.org/10.1007/s00114-004-0516-x
  3. B. Sakintuna, F. Lamari-Darkrim and M. Hirscher, Int. J. Hydrogen Energy, 32, 1121 (2007). https://doi.org/10.1016/j.ijhydene.2006.11.022
  4. G. Leofanti, M. Padovan, G. Tozzola and B. Venturelli, Catal. Today, 41, 207 (1998). https://doi.org/10.1016/S0920-5861(98)00050-9
  5. T. Duren, F. Millange, G. Ferey, K. S. Walton and R. Q. Snurr, J. Phys. Chem. C, 111, 15350 (2007). https://doi.org/10.1021/jp074723h
  6. K. Sing, Colloids Surf. A, 187-188, 3 (2001). https://doi.org/10.1016/S0927-7757(01)00612-4
  7. NIST Standard Reference Data, Thermophysical Properties of Fluid Systems, Retrieved May 15, 2017 from http://webbook.nist.gov/chemistry/fluid
  8. H. Oh, KHNES, 27, 349 (2016) (in Korean).
  9. S. Brunauer, P. H. Emmett, E. Teller J. Am. Chem. Soc., 60, 309 (1938). https://doi.org/10.1021/ja01269a023
  10. P. Llewellyn, F. Rodriquez-Reinoso, J. Rouqerol and N. Seaton, Stud. Surf. Sci. Catal., 160, 49 (2007).
  11. D. Denysenko, M. Grzywa, J. Jelic, K. Reuter and D. Volkmer, Angew. Chem., Int. Ed., 53, 5832 (2014). https://doi.org/10.1002/anie.201310004