• Title/Summary/Keyword: transboundary flux

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Aircraft Measurement of SO$_2$, NO$_{x}$ over Yellow Sea Area (항공기를 이용한 서해안에서의 SO$_2$ 및 NO$_{x}$의 측정)

  • 김병곤;차준석;한진석;박일수;김정수;나진균;최덕일;안준영;강창국
    • Journal of Korean Society for Atmospheric Environment
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    • v.13 no.5
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    • pp.361-369
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    • 1997
  • In order to investigate the abundance and transboundary fluxes of air pollutants over the Yellow Sea, airborne measurements were made aboard the SF-600 aircraft (Pan-Asia Engineering) in March, 1996. The data presented in this paper are preliminary results and airborne experiment will be carried out until 1999. The vertical profile of relevant meteorological parameters such as temperature, water vapor, wind direction and wind speed were also observed at Taean. Mixing layer height was about 1000~1100m during the flights. The SO$_2$ and NO$_{x}$ concentrations were 3~6 ppb and 5~7 ppb below 1000 m, within 1 ppb and 3~5 ppb at 1000~2000m, respectively. Backward trajectory analyses were also carried out. A mathematical method by Lelieveld et al.(1989) was used to estimate the flux of air pollutants through the planetary boundary layer of Yellow Sea area. Transboundary fluxes were calculated using the measurement results with respect to the pollutants concentration, depth of the planetary boundary layer, wind speed and wind direction. The estimated transboundary flux of SO$_2$through the western boundary of Korea was about 39~42 tons/hour.r.

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Spatial Distribution and Variation of Long-range Transboundary Air Pollutants Flux during 1997~2004 (장거리이동 대기오염물질 이동량의 공간적 분포와 변화 추이(1997~2004))

  • Han J. S.;Kim Y. M.;Ahn J. Y.;Kong B. J.;Choi J. S.;Lee S. U.;Lee S. J.
    • Journal of Korean Society for Atmospheric Environment
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    • v.22 no.1
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    • pp.99-106
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    • 2006
  • Aircraft measurements have been executed for the purpose of monitoring the long range transported air pollution and estimation of air pollutant in/out-flux over the Yellow sea. Total 74 missions of measurements have been done since 1997, mainly in spring and fall. The main study domain was over $124^{\circ}$E $/sim$ $124^{\circ}$E, $35^{\circ}$N $/sim$ $37^{\circ}$N below 3,000m. In long-term trends, mixing ratios of $SO_{2}$N were around 2 ppbv expect in summer ( < 1 ppbv). NOx exhibited 24 ppbv and have no clear annual trends over the Yellow Sea. The concentrations of 03 were 51, 58, 41 ppbv in spring, summer and fall-winter, respectively. Backward trajectory was performed for three days to investigate the source regions of the air mass. Six regions were divided around Korea peninsular centering at $36^{\circ}$N, $126^{\circ}$E. I, II, III, IV and V regions represents in sequence northeast China and Siberia, Sandong peninsula and Balhae gulf, Sanghi and southern China, the south Pacific included Jeju island and the East sea included Japan. L region correspond to the airmass from Korea peninsula. Influx of $SO_{2}$N was approximately five times higher than outflux in yearly flux variation and showed a decreasing long-term trend since 1998. NOx outflux was average 0.095 ton/km/hr and three times higher than $SO_{2}$ outflux. In/out flux of 03 showed even distribution in yearly basis except 2002 (influx 5.45 ton/km/hr). The transported amounts from I, II, III regions were much higher than those from other region. In seasonal flux variation, influx levels of gas phases were the lowest in summer and the levels gradually increased from fall toward spring. As a result, transport of pollutants begins from fall and prevails in winter and spring.

Studies on the Behavior of SO2 and NOx over Yellow Sea Area during Long Term Aircraft Measurements(1997~2007) (장기간(1997~2007) 창공관측을 이용한 서해상 SO2 및 NOx의 거동 연구)

  • Song, Hyung-Do;Choi, Jin-Soo;Jang, Im-Suk;Kim, Jeong-Soo;Lee, Suk-Jo
    • Journal of Environmental Science International
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    • v.18 no.5
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    • pp.569-578
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    • 2009
  • Aircraft Measurements of gaseous pollutants($SO_2$, NOx and $O_3$) in the Yellow Sea area, were carried out on 1997-2007. Main measurement site in 124$^{\circ}$-127$^{\circ}$E, 35$^{\circ}$-37$^{\circ}$N (in the Yellow Sea), have been done along the paths classified vertically and zonally. To understand how the air stream affects Long-range transboundary pollutants in Northease Asia (LTP), the tracks of pollutants in northeast Asia have been analyzed by dividing into 6 different regions(regions I-V and L). Compared with Korea's local sources and western north Pacific influenced by the Yellow Sea, when the air stream from region II is dominant, the $SO_2$ concentrations are 3-6times higher. In region II and III, $SO_2$ concentrations are represented highest at 25.0 and 14.7 ppb, respectively. However, in other regions, $SO_2$ concentration was recorderd the highest at 1.1-3.8 ppb, which is 7-15% higher then the highest one over the region II and III. During 1997-2007, the mean amount of incoming pollutants is 0.162 $ton/km{\cdot}hr$ exceeding about 5-times mean amount of outgoing pollutants over the West Sea. During the observed period, the amount of incoming and outgoing $SO_2$ over the Yellow Sea is the highest in winter, at 0.224 $ton/(km{\cdot}hr)$ and 0.120 $ton/(km{\cdot}hr)$, respectively.