• Title/Summary/Keyword: nuclear waste disposal

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Radiation effect on the corrosion of disposal canister materials

  • Minsoo Lee;Junhyuk Jang;Jin Seop Kim
    • Nuclear Engineering and Technology
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    • v.56 no.3
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    • pp.941-948
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    • 2024
  • The effects of radiation on the corrosion of canister materials were investigated for the reliable disposal of high-level radioactive waste. The test specimens were gamma-irradiated at a very low dose rate of approximately 0.1 Gy/h for six and twelve months. The copper and cast iron species were less corroded when irradiated. It is hypothesized that gamma rays suppress the formation of lower-enthalpy species like metal oxides and activate reductive reactions. In contrast, it was difficult to evaluate the effect of radiation on the corrosion of titanium and stainless steel.

Review of Instant Release Fractions of Long-lived Radionuclides in CANDU and PWR Spent Nuclear Fuels Under the Geological Disposal Conditions

  • Choi, Heui Joo;Koo, Yang-Hyun;Cho, Dong-Keun
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.20 no.2
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    • pp.231-241
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    • 2022
  • Several countries, including Korea, are considering the direct disposal of spent nuclear fuels. The radiological safety assessment results published after a geological repository closure indicate that the instant release is the main radiation source rather than the congruent release. Three Safety Case reports recently published were reviewed and the IRF values of seven long-lived radionuclides, including relevant experimental results, were compared. According to the literature review, the IRF values of both the CANDU and low burnup PWR spent fuel have been experimentally measured and used reasonably. In particular, the IRF values of volatile long-lived nuclides, such as 129I and 135Cs, were estimated from the FGR value. Because experimental leaching data regarding high burnup spent nuclear fuels are extremely scarce, a mathematical modelling approach proposed by Johnson and McGinnes was successfully applied to the domestic high burnup PWR spent nuclear fuel to derive the IRF values of iodine and cesium. The best estimate of the IRF was 5.5% at a discharge burnup of 55 GWd tHM-1.

Radiochemical Analysis of Filters Used During the Decommissioning of Research Reactors for Disposal

  • Kyungwon Suh;Jung Bo Yoo;Kwang-Soon Choi;Gi Yong Kim;Simon Oh;Kanghyun Yoo;Kwang Eun Lee;Shinkyoung Lee;Young Sang Lee;Hyeju Lee;Junhyuck Kim;Kyunghun Jung;Sora Choi;Tae-Hong Park
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.20 no.4
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    • pp.489-500
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    • 2022
  • The decommissioning of nuclear facilities produces various types of radiologically contaminated waste. In addition, dismantlement activities, including cutting, packing, and clean-up at the facility site, result in secondary radioactive waste such as filters, resin, plastic, and clothing. Determining of the radionuclide content of this waste is an important step for the determination of a suitable management strategy including classification and disposal. In this work, we radiochemically characterized the radionuclide activities of filters used during the decommissioning of Korea Research Reactors (KRRs) 1 and 2. The results indicate that the filter samples contained mainly 3H (500-3,600 Bq·g-1), 14C (7.5-29 Bq·g-1), 55Fe (1.1- 7.1 Bq·g-1), 59Ni (0.60-1.0 Bq·g-1), 60Co (0.74-70 Bq·g-1), 63Ni (0.60-94 Bq·g-1), 90Sr (0.25-5.0 Bq·g-1), 137Cs (0.64-8.7 Bq·g-1), and 152Eu (0.19-2.9) Bq·g-1. In addition, the gross alpha radioactivity of the samples was measured to be between 0.32-1.1 Bq·g-1. The radionuclide concentrations were below the concentration limit stated in the low- and intermediatelevel waste acceptance criteria of the Nuclear Safety and Security Commission, and used for the disposal of the KRRs waste drums to a repository site.

Analyses of the Double-Layered Repository Concepts for Spent Nuclear Fuels (사용후핵연료 심지층 처분장 복층개념 분석)

  • Lee, Jongyoul;Kim, Hyeona;Lee, Minsoo;Choi, Heui-Joo;Kim, Kyungsu
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.15 no.2
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    • pp.151-159
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    • 2017
  • A deep geological disposal at a depth of 500 m in stable host rock is considered to be the safest method with current technologies for disposal of spent fuels classified as high-level radioactive waste. The most important requirement is that the temperature of the bentonite buffer, which is a component of the engineered barrier, should not exceed $100^{\circ}C$. In Korea, the amount of spent fuel generated by nuclear power generation, which accounts for about 30% of the total electricity, is continuously increasing and accumulating. Accordingly, the area required to dispose of it is also increasing. In this study, various duplex disposal concepts were derived for the purpose of improving the disposal efficiency by reducing the disposal area. Based on these concepts, thermal analyses were carried out to confirm whether the critical disposal system requirements were met, and the thermal stability of the disposal system was evaluated by analyzing the results. The results showed that upward 75 m or downward 75 m apart from the reference disposal system location of 500 m depth would qualify for the double layered disposal concept. The results of this study can be applied to the establishment of spent fuel management policy and the design of practical commercial disposal system. Detailed analyses with data of a real disposal site are necessary.

Preliminary Analysis on Decommissioning Strategies for Fukushima Daiichi Nuclear Power Station From Waste Management Perspective

  • Watanabe, Naoko;Yanagihara, Satoshi
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.19 no.3
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    • pp.297-306
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    • 2021
  • In this study, basic strategies for the decommissioning and site remediation of the Fukushima Daiichi Nuclear Power Station (FDNPS) were investigated. Six scenarios were formulated based on two of the three decommissioning strategies of nuclear power plants defined by the International Atomic Energy Agency (IAEA): immediate dismantling and deferred dismantling. A multicriteria decision analysis was performed to analyze the preferences of the options from the viewpoints of the timeframe to complete decommissioning, the resulting waste, the site usability, and the availability of the radioactive waste disposal route. The same six scenarios were applied to both the FDNPS and the nuclear power plants that ceased operation after a normal plant life cycle for comparison. For the FDNPS, the decommissioning project involved fuel debris retrieval, dismantling, and site remediation. The analysis results suggest that the balance between the amount of waste and the time to achieve the end state may be one of the most critical factors to consider when planning the decommissioning and site remediation of the FDNPS.

The Establishment and Improvement of Full Cycle History Management System for Low- and Intermediate-level Radioactive Waste (중저준위 방사성폐기물 전주기 이력관리체계 구축 및 개선)

  • Jin-Woo Lee;Jun Lee;Hee-Chul Eun;Ji-Young Jeong
    • Journal of Radiation Industry
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    • v.18 no.1
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    • pp.95-100
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    • 2024
  • To establish a radioactive waste life cycle history management system, a series of processes including waste generation, classification, packaging, storage, transportation, and disposal were reflected in the information management system. A preliminary review process was introduced to reduce the amount of radioactive waste generated and manage it efficiently. Through this, the amount of radioactive waste generated must be checked from the beginning of the research, and the generated radioactive waste must be thoroughly managed from the stage of generation to final disposal. In particular, in the case of radioactive waste data generated during nuclear facility operation and each experiment, a radioactive waste information management system must be operated to receive information from the waste generator and integrate it with processing information at the management stage. The application process for small-package containers was reflected so that information such as the generation facility of radioactive waste, generation facility, project information, types of radioactive waste, major radionuclides, etc. In the radioactive waste management process, the preceding steps are to receive waste history from the waste generators. This includes an application for a specified container with a QR label, pre-inspection, and management request. Next, the succeeding steps consist of repackaging, treatment, characterization, and evaluating the suitability of disposal, for a process to transparently manage radioactive wastes.

A SYSTEMS ASSESSMENT FOR THE KOREAN ADVANCED NUCLEAR FUEL CYCLE CONCEPT FROM THE PERSPECTIVE OF RADIOLOGICAL IMPACT

  • Yoon, Ji-Hae;Ahn, Joon-Hong
    • Nuclear Engineering and Technology
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    • v.42 no.1
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    • pp.17-36
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    • 2010
  • In this study, we compare the mass release rates of radionuclides(1) from waste forms arising from the KIEP-21 pyroprocessing system with (2) those from the directly-disposed pressurized-water reactor spent fuel, to investigate the potential radiological and environmental impacts. In both cases, most actinides and their daughters have been observed to remain in the vicinity of waste packages as precipitates because of their low solubility. The effects of the waste-form alteration rate on the release of radionuclides from the engineered-barrier boundary have been found to be significant, especially for congruently released radionuclides. the total mass release rate of radionuclides from direct disposal concept is similar to those from the pyroprocessing disposal concept. While the mass release rates for most radionuclides would decrease to negligible levels due to radioactive decay while in the engineered barriers and the surrounding host rock in both cases even without assuming any dilution or dispersal mechanisms during their transport, significant mass release rates for three fission-product radionuclides, $^{129}I$, $^{79}Se$, and $^{36}Cl$, are observed at the 1,000-m location in the host rock. For these three radionuclides, we need to account for dilution/dispersal in the geosphere and the biosphere to confirm finally that the repository would achieve sufficient level of radiological safety. This can be done only after we have known where the repository site would by sited. the footprint of repository for the KIEP-21 system is about one tenth of those for the direct disposal.

Assessment of Corrosion Lifetime of a Copper Disposal Canister Based on the Finnish Posiva Methodology

  • Choi, Heui-Joo;Lee, Jongyoul;Cho, Dongkeun
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.18 no.spc
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    • pp.51-62
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    • 2020
  • In this paper, an approach developed by the Finnish nuclear waste management organization, Posiva, for the construction license of a geological repository was reviewed. Furthermore, a computer program based on the approach was developed. By using the computer program, the lifetime of a copper disposal canister, which was a key engineered barrier of the geological repository, was predicted under the KAERI Underground Research Tunnel (KURT) geologic conditions. The computer program was developed considering the mass transport of corroding agents, such as oxygen and sulfide, through the buffer and backfill. Shortly after the closure of the repository, the corrosion depths of a copper canister due to oxygen in the pores of the buffer and backfill were calculated. Additionally, the long-term corrosion of a copper canister due to sulfide was analyzed in two cases: intact buffer and eroded buffer. Under various conditions of the engineered barrier, the corrosion lifetimes of the copper canister due to sulfide significantly exceeded one million years. Finally, this study shows that it is necessary to carefully characterize the transmissivity of rock and sulfide concentration during site characterization to accurately predict the canister lifetime.

Important Radionuclides and Their Sensitivity for Ground water Pathway of a Hypothetical Near-Surface Disposal Facility

  • Park, J. W.;K. Chang;Kim, C. L.
    • Nuclear Engineering and Technology
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    • v.33 no.2
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    • pp.156-165
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    • 2001
  • A radiological safety assessment was performed for a hypothetical near-surface radioactive waste repository as a simple screening calculation to identify important nuclides and to provide insights on the data needs for a successful demonstration of compliance. Individual effective doses were calculated for a conservative ground water pathway scenario considering well drilling near the site boundary. Sensitivity of resulting ingestion dose to input parameter values was also analyzed using Monte Carlo sampling. Considering peak dose rate and assessment time scale, C-14 and T-129 were identified as important nuclides and U-235 and U-238 as potentially important nuclides. For C-14, the dose was most sensitive to Darcy velocity in aquifer The distribution coefficient showed high degree of sensitivity for I-129 release.

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Comprehensive Development Plans for the Low- and Intermediate-Level Radioactive Waste Disposal Facility in Korea and Preliminary Safety Assessment (우리나라 중·저준위 방사성폐기물 처분시설 종합개발계획(안)과 예비안전성평가)

  • Jung, Kang Il;Kim, Jin Hyeong;Kwon, Mi Jin;Jeong, Mi Seon;Hong, Sung Wook;Park, Jin Beak
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.14 no.4
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    • pp.385-410
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    • 2016
  • The disposal facility in Gyeongju is planning to dispose of 800,000 packages of low- and intermediate- level radioactive waste. This facility will be developed as a complex disposal facility that has various types of disposal facilities and accompanying management. In this study, based on the comprehensive development plan of the disposal facility, a preliminary post-closure safety assessment is performed to predict the phase development of the total capacity for the 800,000 packages to be disposed of at the site. The results for each scenario meet the performance target of the disposal facility. The assessment revealed that there is a significant impact of the inventory of intermediate-level radionuclide waste on the safety evaluation. Due to this finding, we introduce a disposal limit value for intermediate-level radioactive waste. With stepwise development of safety case, this development plan will increase the safety of disposal facilities by reducing uncertainties within the future development of the underground silo disposal facilities.