• Title/Summary/Keyword: Wet deposition

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Measurement of Nitrogen and Sulfur Deposition to Lake Paldang (팔당호로의 질소와 황성분 침적 측정)

  • Ghim Young Sung;Jin Hyoun Cheol
    • Journal of Korean Society for Atmospheric Environment
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    • v.21 no.1
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    • pp.39-48
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    • 2005
  • Nitrogen and sulfur deposition was measured on Lake Pal dang from March 2002 to October 2003. Wet and dry depositions were separately measured using wet- and dry-only samplers, respectively. In order to measure the dry deposition to the water body, a dry deposition sampler composed of three pans filled with pure water, called the deposition water, was used. Since ammonium was generally in excess in ambient air, more than half of ammonium was present in the gaseous form. Ammonium concentration was also generally higher than the sum of major anion concentrations in the deposition water because gaseous species were much easily deposited than the species in fine particles. Nevertheless, the contribution of gaseous ammonia to the deposition of ammonium was not high as well as that of particulate ammonium while the contribution of gaseous nitric acid was much higher than that of particulate nitrate. Annual wet deposition fluxes of nitrogen and sulfur were five and six times higher than their dry deposition fluxes, respectively. Except for ammonium, the dry deposition flux estimated in the present work was a half of the previous results. This was mainly caused by much smaller dry deposition velocities over the water than over the ground.

Measurement of Dry deposition at Seoul, Chunchon and Anmyon-do by Using Filter pack Method (필터팩을 이용한 서울과 춘천, 안면도의 건성 강하량 측정)

  • Kim, Man-Goo;Kang, Mi-Hee;Hong, Young-Min;Park, Ki-Jun;Lee, Bo-Kyung;Lee, Dong-Soo;Kim, San
    • Journal of Korean Society for Atmospheric Environment
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    • v.17 no.1
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    • pp.19-29
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    • 2001
  • Atmospheric concentrations of acidic pollutant were measured by the 4 stage filter pak method at Chunchon and by the 3 stage filter pack method at Seoul and Anmyon-do from January to December 1998. The sample was collected for 24 hours on every Wednesday. Concentrations of particulate matters were highest at Anmyon-do. The particulate concentration was much higher during the warm season than other seasons. While the particulate concentration was higher during the warm season, the concentration of gaseous matter was higher in winter. Dry deposition flux was calculated by using reported deposition velocities and concentration of pollutants measured in this study. The dry deposition velocities used in this study for SO$_2$, SO$_{4}^{2}$, HNO$_3$,NO$_{3}^{-}$ and NH$_3$ were 0.29, 0.15, 2.08( 2.13 only for Anmyon-do), 0.20 and 1.00cm/sec, respectively. At Chunchon, annual sulfur flux originated from dry deposition was 384 kg/$textrm{km}^2$, and the flux from wet deposition was 782kg/$textrm{km}^2$. Dry deposition of sulfur was 33% of total sulfur deposition. The annual nitrogen flux originated from dry deposition was 1,892kg/$textrm{km}^2$. And the flux from wet deposition was 1,066kg/$textrm{km}^2$. Dry deposition of nitrogen was 64% of total nitrogen deposition. Dry deposition as well as wet deposition have to be considerd in the study on acidification of environment such as soil or watershed.

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Studies on the Transportation and Wet Deposition of Air Pollutant($SO_2$) by Modeling and Precipitation Analysis in Wonju City (강우분석과 모델링에 의한 원주시 대기오염물질($SO_2$) 이동과 침적에 관한 연구)

  • Kwon, Young Sik;Song, Dong Woong;Kang, Kyung Ho
    • Analytical Science and Technology
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    • v.9 no.1
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    • pp.98-106
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    • 1996
  • The concentration of sulfur dioxide in Wonju City was predicted using TCM (Texas Climatological Model). We have studied the transportation and wet deposition of $SO_2$ using the TCM and the analysis of rainfalls. The results are as follows : At the Hak-Sung Dong site in Wonju city, the correlation coefficient between the measured and calculated concentrations were 0.904. Sulfur dioxide was washed out by wet deposition. The wet deposition ratio to total amount of emitted sulfur dioxide was higher in summer than in autumn and winter seasons due to heavy rainfall in summer. The correlation coefficient between the precipitation and wet deposition of sulfur dioxide was 0.68. The months with greater rainfall showed that the measured concentrations of sulfur dioxide were much lower than the predicted ones. Although the amount of precipitation in April was smaller than in summer, the wet deposition ratio in April was much higher than any other months, due to the sulfur dioxide that was adsorbed on particulate matter and moisture was transported during the period of yellow sand phenomena from China.

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Wet Deposition Fluxes of Ions Contributed by Cyclone-, Stationary Front- and Typhoon-associated Rains at the Southwestern Japan Coast

  • Toyonaga, Satoshi;Zhang, Daizhou
    • Asian Journal of Atmospheric Environment
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    • v.10 no.2
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    • pp.57-66
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    • 2016
  • Wet deposition fluxes of ions at a coastal site in southwestern Japan in the period 1996-2003 were investigated to quantify the respective contributions of cyclone-, stationary front- and typhoon-associated rains. On average, the deposition fluxes of terrigenous-origin ions, nss-$SO_4{^{2-}}$, $NO_3{^-}$, $NH_4{^+}$ and nss-$Ca^{2+}$ were $37.6{\pm}7.3$, $16.3{\pm}4.2$, $19.0{\pm}3.4$ and $9.6{\pm}4.8meq\;m^{-2}yr^{-1}$, and those of $Na^+$ and $Cl^-$, the major ions in sea water, were $97.0{\pm}38.2$ and $115.2{\pm}48.2meq\;m^{-2}yr^{-1}$, respectively. Cyclone-associated rain constituted more than 50% of the fluxes of the terrigenous ions in almost all years. Stationary front-associated rain also contributed significantly, although the contribution was lower than the contribution by Cyclone-associated rain in almost all years. In particular, the wet deposition flux of nitrogen compounds of $NO_3{^-}$ and $NH_4{^+}$, which are important nutrients for micro-bioactivities in sea surface water, was dominated by cyclone-associated rain. Due to the extreme abundance of $Na^+$ and $Cl^-$ in the rainwater of typhoons, the fluxes of $Na^+$ and $Cl^-$ were contributed substantially by typhoons in years with typhoons' passage although cyclones were still the largest contributor to the fluxes. These results indicate the dominance of cyclones in the wet deposition to the East China Sea areas and the necessity to take rain types into account for a more accurate elucidation of the temporal and spatial variation of the wet deposition.

Influence of Radioactive Contamination to Agricultural Products Due to Dry and Wet Deposition Processes During a Nuclear Emergency (원자력 사고 중 핵종의 건. 습침적에 따른 농작물 오염 영향)

  • Hwang, Won-Tae;Kim, Eun-Han;Suh, Kyung-Suk;Han, Moon-Hee;Choi, Pong-Ho;Lee, Chang-Woo
    • Journal of Radiation Protection and Research
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    • v.27 no.3
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    • pp.165-170
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    • 2002
  • Combined with deposition model onto the ground of radionuclides, the influence of radioactive contamination to agricultural products was analyzed due to wet deposition as well as dry deposition from radioactive air concentration during a nuclear emergency. The previous dynamic food chain model, in which initial input parameter is only radionuclide concentrations on the ground, was improved for the evaluating of radioactive contamination to agricultural products from either radionuclide concentrations in air or radionuclide concentrations on the ground. As the results, in case of deposition onto the ground, wet deposition was more dominant process than thy deposition. While the contamination levels of agricultural products were dependent on the a variety of factors such as radionuclides and rainfall rate. It means that the contamination levels of agricultural products are determined from which is more dominant process between deposition on the ground and interception onto agricultural plants.

Current Wet Deposition of Pu Isotopes in the mid-Yellow Sea Coast of Korea (최근 한반도 중부 황해안의 Pu 핵종 습식 침착)

  • 이상한;정창수;김석현;이광우
    • Journal of Korean Society for Atmospheric Environment
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    • v.15 no.2
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    • pp.79-87
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    • 1999
  • $^{239+240}Pu$ concentrations in precipitation were determined for the period of May 1994 to August 1996 in oder to describe current $^{239+240}Pu$ deposition at the mid-western coat of Korea (Ansan, 37$^{\circ}$17'N, $126^{\circ}$50'E). $^{239+240}Pu$ concentration in daily precipitation varied from 0.05 to 131$\mu$Bq $kg^{-1}$ with a geometric mean of $1.26\mu$Bq $kg^{-1}$. The concentration was high in the period of Yellow Sand Storm in spring and low in wet summer monsoon. The specific $^{239+240}Pu$ concentration in daily precipitation appears to be controlled by the $^{239+240}Pu$ input to the atmosphere in spring and washout effects by precipitation in the wet summer monsoon. Wet depositional flux of $^{239+240}Pu$ varied from 4 to 123$\mu$Bq $m^{-2}d^{-1}$ with a geometric mean of $33.8\mu$Bq $m^{-2}d^{-1}$ and with a maximum in the period of Yellow Sand Storm and a minimum in the period of wet summer monsoon. $^{238}Pu$/$^{239+240}Pu$ activity raios(0.04~0.31) in precipitation for March-June period suggested that one of the major sources of Pu isotopes falling in Ansan area is the arid region of the Chinese continent.

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A Study on Estimation of Wet Deposition Flux using ADOM (ADOM을 이용한 습성침적 플럭스 산정에 관한 연구)

  • 이화운;문난경;임주연
    • Proceedings of the Korea Air Pollution Research Association Conference
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    • 2001.11a
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    • pp.87-88
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    • 2001
  • 대기오염물질 제거에 중요한 역할을 하는 침적 현상은 크게 건성침적(dry deposition)과 습성침적(wet deposition)으로 구분된다. 건성침적은 오염물질이 중력이나 분자 확산에 의해 지면이나 그 부근에 침강ㆍ흡착하는 현상이며, 습성침적은 구름 속의 에어로졸이 응결핵으로 제거되는 성우제거(rainout)와 구름 이하의 고도에서 강수에 의해 제거되는 세척제거(washout)와 같은 현상을 일컫는다. 습성침적은 강수 및 구름 물리와 관련하여 대기 중 오염물질 제거에 큰 비중을 차지함에도 불구하고 건성침적에 비해 그 연구가 미흡한 실정이며, 침적 모형을 이용한 연구는 더욱 찾아보기 어렵다. (중략)

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Pattern of Nutrient Fluxes in Deciduous Forest Ecosystem Imparted by Acidic Deposition (산성강하물 조건하에서 활엽수림 생태계의 양료순환 양상)

  • Chang, Kwan-Soon
    • Korean Journal of Environment and Ecology
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    • v.15 no.3
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    • pp.230-236
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    • 2001
  • The fluxes of wet deposition(WD), throughfall(TF), stemflow(SF) and soil leachates were measured to understand base cation budgets on deciduous ecosystem impacted by acidic deposition in the north-western part of Tomakomai in Hokkaido, Japan. The flux of $H^{+}$ for wet deposition was $0.34kmo1_{c}$ $ha^{2+}$ and the flux of base cation, $K^{+}$ /, Na$^{ + }$, $Ca^{2+}$ and $Mg^{2+}$ far throughfall plus stemflow wart 1.6 kmolc $ha^{-1}$ , 3 times higher level than that for wet deposition. The flux of base cation for canopy leaching(LI) was 0.95 kmolc ha$^{-1}$ , 2.8 times higher level than $H^{+}$ sources in wet deposition. The major mechanism of $^{+}$ consumption closely related to acidic neutralizing capacity of canopy. The ionic flux for soil leachates from Boil reservoir and proton consumption in soil was dependent on soil chemical states and exchangeable Ca in soil had a major factor of H$^{+ }$ consumption. The base cation budgets on deciduous ecosystem showed positive balance fur Na, Ca and Mg, while K was the negative value.

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Characteristics of Atmosphere-rice Paddy Exchange of Gaseous and Particulate Reactive Nitrogen in Terms of Nitrogen Input to a Single-cropping Rice Paddy Area in Central Japan

  • Hayashi, Kentaro;Ono, Keisuke;Matsuda, Kazuhide;Tokida, Takeshi;Hasegawa, Toshihiro
    • Asian Journal of Atmospheric Environment
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    • v.11 no.3
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    • pp.202-216
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    • 2017
  • Nitrogen (N) is an essential macronutrient. Thus, evaluating its flows and stocks in rice paddy ecosystems provides important insights into the sustainability and environmental loads of rice production. Among the N sources of paddy fields, atmospheric deposition and irrigation inputs remain poorly understood. In particular, insufficient information is available for atmosphere-rice paddy exchange of gaseous and particulate reactive N (Nr, all N species other than molecular N) which represents the net input or output through dry deposition and emission. In this study, we assessed the N inputs via atmospheric deposition and irrigation to a Japanese rice paddy area by weekly monitoring for 2 years with special emphasis on gas and particle exchange. The rice paddy during the cropping season acted as a net emitter of ammonia ($NH_3$) to the atmosphere regardless of the N fertilizer applications, which reduced the effects of dry deposition to the N input. Dry N deposition was quantitatively similar to wet N deposition, when subtracting the rice paddy $NH_3$ emissions from N exchange. The annual N inputs to the rice paddy were 3.2 to $3.6\;kg\;N\;ha^{-1}\;yr^{-1}$ for exchange, 8.1 to $9.8\;kg\;N\;ha^{-1}\;yr^{-1}$ for wet deposition, and 11.1 to $14.5\;kg\;N\;ha^{-1}\;yr^{-1}$ for irrigation. The total N input, 22.8 to $27.5\;kg\;N\;ha^{-1}\;yr^{-1}$, corresponded to 38% to 55% of the N fertilizer application rate and 53% to 67% of the brown rice N uptake. Monitoring of atmospheric deposition and irrigation as N sources for rice paddies will therefore be necessary for adequate N management.

Source-Receptor Relationships of Transboundary Air Pollutants in East Asia Region Simulated by On-Line Transport Model

  • Jang, Eun-Suk;Itsushi Uno
    • Environmental Sciences Bulletin of The Korean Environmental Sciences Society
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    • v.4 no.2
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    • pp.111-116
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    • 2000
  • Transboundary air pollution has recently become an area of increasing scientific interest and political concern as countries are receiving air pollutants from their neighbors. In order to gain a better understanding of the long-range transport processes of air pollutants and the source-receptor relationships among neighboring countries, an atmospheric transport model coupled with a RAMS(Regional Atmospheric Modeling System) model was applied to the East Asia region during the entire month of January 1993. The scalar transport option of the RAMS model was used to calculate special atmospheric constituents such as trace gases or aerosols. The sulfate production in clouds and rainwater and its removal processes by dry and wet deposition were considered. The sulfate budget from source regions to receptor regions was estimated by analysing the source-receptor relationships. When a specific receptor site revealed a sulfate value higher than the sulfate concentration based on its own source origin, this was taken to indicate long-range transport from another source region. The contribution ratio from various source region was calculated. The contribution ratio of dry and wet deposition was higher on the main continent of the East region. Furthermore, the high deposition amounts were identified on the west coast of Korea and the East China Sea.

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