• Title/Summary/Keyword: Radioactive source

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A Study on the Radiation Shielding Analysis for Reinforcing the Hot Cell Regular Concrete Shield Wall (핫셀의 일반 콘크리트 보강을 위한 방사선 차폐해석 연구)

  • 조일제;황용화
    • Proceedings of the Korea Concrete Institute Conference
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    • 2003.05a
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    • pp.985-990
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    • 2003
  • In order to demonstrate Advanced Spent Fuel Conditioning Process (ACP), shielding facilities such as hot cell suitable to handling radionuclides and process property will be necessary. But the construction of new facilities needs much money, man-power and time, it is now scheduled to remodel the hot cell, which has already been installed and maintained at Irradiated Material Experiment Facility (IMEF) in the Korea Atomic Energy Research Institute (KAERI). The basic structure and concrete shield wall of hot cell partly have been constructed on the base floor in IMEF building in current status. And hot cell after remodeling will be used for carrying out the lab-scale experiment of ACP. The hot cell was built in accordance with 35 curies of fe-59(1.2 MeV) as design criteria of radiation dose limit. But the radioactive source of ACP is expected to be much higher than design criteria of IMEF, shielding ability of the hot cell in the current status is unsatisfactory to the hot test of ACP. Therefore shield wall shall be reinforced with heavy concrete, steel or lead. In this paper, dose rates are calculated according to ACP source, shielding materials, etc., and reinforcement structures are determined considering the current situation of hot cells, installation of shield windows and the easiness of work.

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A Conservative Safety Study on Low-Level Radioactive Waste Repository Using Radionuclide Release Source Term Model (선원항 모델을 사용한 저준위 방사성폐기물 처분장의 보수적인 안전성고찰)

  • Kim, Chang-Lak;Lee, Myung-Chan;Cho, Chan-Hee
    • Nuclear Engineering and Technology
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    • v.25 no.1
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    • pp.63-70
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    • 1993
  • A simplified safety assessment is carried out on rock-cavern type disposal of LLW using the analytical repository source term (REPS) model. For reliable prediction of the leach rates for various radionuclides, degradation of concrete structures, corrosion rate of waste container, degree of corrosion on the container surface, and the characteristics of radionuclides are considered in the REPS model. The results of preliminary assessment show that Cs-137, Ni-63, and Sr-90 are dominant. For the parametric uncertainty and sensitivity analysis, Latin hypercube sampling technique and rank correlation technique are applied. The results of the potential public health impacts show that radiological dose to intruder in the worst case scenario will be negligible and that more attention should be given to near-field performance.

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Estimation of nuclear heating by delayed gamma rays from radioactive structural materials of HANARO

  • Noh, Tae-yang;Park, Byung-Gun;Kim, Myong-Seop
    • Nuclear Engineering and Technology
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    • v.50 no.3
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    • pp.446-452
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    • 2018
  • To improve the accuracy and safety of irradiation tests in High flux Advanced Neutron Application ReactOr (HANARO), the nuclear energy deposition rate, which is called nuclear heating, was estimated for an irradiation capsule with an iridium sample in the irradiation hole in order. The gamma rays emitted from the radioisotopes (RIs) of the structural materials such as flow tubes of fuel assemblies and heavy water reflector tank were considered as radiation source. Using the ORIGEN2.1 code, emission rates of delayed gamma rays were calculated in consideration of the activation procedure for 8 years and 2 months of HANARO operation. Calculated emission rates were used as a source term of delayed gamma rays in the MCNP6 code. By using the MCNP code, the nuclear heating rates of the irradiation capsules in the inner core, outer core, and heavy water reflector tank were estimated. Calculated nuclear heating in the inner core, outer core, and heavy water reflector tank were 200-260 mW, 80-100 mW, and 10 mW, respectively.

Design and Fabrication of CLYC-Based Rotational Modulation Collimator (RMC) System for Gamma-Ray/Neutron Dual-Particle Imager

  • Kim, Hyun Suk;Lee, Jooyub;Choi, Sanghun;Bang, Young-bong;Ye, Sung-Joon;Kim, Geehyun
    • Journal of Radiation Protection and Research
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    • v.46 no.3
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    • pp.112-119
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    • 2021
  • Background: This work aims to develop a new imaging system based on a pulse shape discrimination-capable Cs2LiYCl6:Ce (CLYC) scintillation detector combined with the rotational modulation collimator (RMC) technique for dual-particle imaging. Materials and Methods: In this study, a CLYC-based RMC system was designed based on Monte Carlo simulations, and a prototype was fabricated. Therein, a rotation control system was developed to rotate the RMC unit precisely, and a graphical user interface-based software was also developed to operate the data acquisition with RMC rotation. The RMC system was developed to allow combining various types of collimator masks and detectors interchangeably, making the imaging system more versatile for various applications and conditions. Results and Discussion: Operational performance of the fabricated system was studied by checking the accuracy and precision of the collimator rotation and obtaining modulation patterns from a gamma-ray source repeatedly. Conclusion: The prototype RMC system showed reliability in its mechanical properties and reproducibility in the acquisition of modulation patterns, and it will be further investigated for its dual-particle imaging capability with various complex radioactive source conditions.

Ignition and flame propagation in hydrogen-air layers from a geological nuclear waste repository: A preliminary study

  • Ryu, Je Ir;Woo, Seung Min;Lee, Manseok;Yoon, Hyun Chul
    • Nuclear Engineering and Technology
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    • v.54 no.1
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    • pp.130-137
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    • 2022
  • In the geological repository of radioactive nuclear waste, anaerobic corrosion can generate hydrogen, and may conservatively lead to the production of hydrogen-air layer. The accumulated hydrogen may cause a hazardous flame propagation resulting from any potential ignition sources. This study numerically investigates the processes of ignition and flame propagation in the layered mixture. Simple geometry was chosen to represent the geological repository, and reactive flow simulations were performed with different ignition power, energy, and locations. The simulation results revealed the effects of power and energy of ignition source, which were also analyzed theoretically. The mechanism of layered flame propagation was suggested, which includes three stages: propagation into the hydrogen area, downward propagation due to the product gas, and horizontal propagation along the top wall. To investigate the effect of the ignition source location, simulations with eight different positions were performed, and the boundary of hazardous ignition area was identified. The simulation results were also explained through scaling analysis. This study evaluates the potential risk of the accumulated hydrogen in geological repository, and illustrates the layered flame propagation in related ignition scenarios.

An analysis of neutron sources and gamma-ray in spent fuels using SCALE-ORIGEN-ARP (SCALE-ORIGEN-ARP를 이용한 사용후핵연료 내 중성자 및 감마선원 분석)

  • So-Hee Cha;Kwang-Heon Park
    • Journal of the Korean institute of surface engineering
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    • v.56 no.1
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    • pp.84-93
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    • 2023
  • The spent nuclear fuel is burned during the planned cycle in the plant and then generates elements such as actinide series, fission products, and plutonium with a long half-life. An 'interim storage' step is needed to manage the high radioactivity and heat emitted by nuclides until permanent-disposal. In the case of Korea, there is no space to dispose of high-level radioactive waste after use, so there is a need for a period of time using interim storage. Therefore, the intensity of neutrons and gamma-ray must be determined to ensure the integrity of spent nuclear fuel during interim storage. In particular, the most important thing in spent nuclear fuel is burnup evaluation, estimation of the source term of neutrons and gamma-ray is regarded as a reference measurement of the burnup evaluation. In this study, an analysis of spent nuclear fuel was conducted by setting up a virtual fuel burnup case based on CE16×16 fuel to check the total amount and spectrum of neutron, gamma radiation produced. The correlation between BU (burnup), IE (enrichment), and CT (cooling time) will be identified through spent nuclear fuel burnup calculation. In addition, the composition of nuclide inventory, actinide and fission products can be identified.

Preliminary Selection of Safety-Relevant Radionuclides for Long-Term Safety Assessment of Deep Geological Disposal of Spent Nuclear Fuel in South Korea

  • Kyu Jung Choi;Shin Sung Oh;Ser Gi Hong
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.21 no.4
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    • pp.451-463
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    • 2023
  • With South Korea increasingly focusing on nuclear energy, the management of spent nuclear fuel has attracted considerable attention in South Korea. This study established a novel procedure for selecting safety-relevant radionuclides for long-term safety assessments of a deep geological repository in South Korea. Statistical evaluations were performed to identify the design basis reference spent nuclear fuels and evaluate the source term for up to one million years. Safety-relevant radionuclides were determined based on the half-life criteria, the projected activities for the design basis reference spent nuclear fuel, and the annual limit of ingestion set by the Nuclear Safety and Security Commission Notification No. 2019-10 without considering their chemical and hydrogeological properties. The proposed process was used to select 56 radionuclides, comprising 27 fission and activation products and 29 actinide nuclides. This study explains first the determination of the design basis reference spent nuclear fuels, followed by a comprehensive discussion on the selection criteria and methodology for safety-relevant radionuclides.

Verification of MCNP/ORIGEN-2 Model and Preliminary Radiation Source Term Evaluation of Wolsung Unit 1 (월성 1호기 MCNP/ORIGEN-2 모델 검증 및 예비 선원항 계산)

  • Noh, Kyoungho;Hah, Chang Joo
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.13 no.1
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    • pp.21-34
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    • 2015
  • Source term analysis should be carried out to prepare the decommissioning of the nuclear power plant. In the planning phase of decommissioning, the classification of decommissioning wastes and the cost evaluation are performed based on the results of source term analysis. In this study, the verification of MCNP/ORIGEN-2 model is carried out for preliminary source term calculation for Wolsung Unit 1. The inventories of actinide nuclides and fission products in fuel bundles with different burn-up were obtained by the depletion calculation of MCNPX code modelling the single channel. Two factors affecting the accuracy of source terms were investigated. First, the neutron spectrum effect on neutron induced activation calculation was reflected in one-group microscopic cross-sections of relevant radio-isotopes using the results of MCNP simulation, and the activation source terms calculated by ORIGEN-2 using the neutron spectrum corrected library were compared with the results of the original ORIGEN-2 library (CANDUNAU.LIB) in ORIGEN-2 code package. Second, operation history effect on activation calculation was also investigated. The source terms on both pressure tubes and calandria tubes replaced in 2010 and calandria tank were evaluated using MCNP/ORIGEN-2 with the neutron spectrum corrected library if the decommissioning wastes can be classified as a low level waste.

Preliminary Post-closure Safety Assessment of Disposal Options for Disused Sealed Radioactive Source (폐밀봉선원 처분방식별 폐쇄후 예비안전성평가)

  • Lee, Seunghee;Kim, Juyoul;Kim, Sukhoon
    • Economic and Environmental Geology
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    • v.49 no.4
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    • pp.301-314
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    • 2016
  • Disused Sealed Radioactive Sources (DSRSs) are stored temporally in the centralized storage facility of Korea Radioactive Waste Agency (KORAD) and planned to be disposed in the low- and intermediate-level radioactive waste (LILW) disposal facility in Gyeongju city. In this study, preliminary post-closure safety assessment was performed for DSRSs in order to draw up an optimum disposal plan. Two types of disposal options were considered, i.e. engineered vault type disposal and rock cavern type disposal which were planned to be constructed and operated respectively in LILW disposal facility in Gyeongju city. Assessment end-point was individual effective dose of critical group and calculated by using GoldSim code. In normal scenario, the maximum dose was estimated to be approximately $1{\times}10^{-7}mSv/yr$ for both disposal options. It meant that both options had sufficient safety margin when compared with regulatory limit (0.1 mSv/yr). Otherwise, in well scenario, the maximum dose exceeded regulatory limit of 1 mSv/yr in engineered vault type disposal and the exposure dose was mainly contributed by $^{226}Ra$, $^{210}Pb$ (daughter nuclide of $^{226}Ra$) and $^{237}Np$ (daughter nuclide of $^{241}Am$). For rock cavern type disposal, even though the peak dose satisfied regulatory limit, the exposure doses by $^{14}C$ and $^{237}Np$ were relatively high above 10% of regulatory limit. Therefore, it is necessary to exclude $^{14}C$, $^{226}Ra$ and $^{241}Am$ for two type of disposal options and additional management such as long-term storage and development of disposal container for those radionuclides should be performed before permanent disposal for conservative safety and security.

Separation for the Determination of $^{59/63}Ni$ in Radioactive Wastes (방사성 폐기물 내 $^{59/63}Ni$ 정량을 위한 분리)

  • Lee, Chang-Heon;Jung, Kie-Chul;Choi, Kwang-Soon;Jee, Kwang-Young;Kim, Won-Ho
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.3 no.4
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    • pp.309-317
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    • 2005
  • A study on the separation of $^{99}Tc,\;^{94}Nb,\;^{55}Fe,\;^{90}Sr\;and\;^{59/63}Ni$ in various radioactive wastes discharged from nuclear power plants has been performed for a use in their quantification which is indispensible for the evaluation of the radionuclide inventory Ni was recovered along with Ca, Mg, Al, Cr, Ti, Mn, Ce, Na, K, and Cu through the sequential separation procedure of Re(as a surrogate of $^{99}Tc$), Nb, Fe and Sr by anion exchange and Sr-Spec extraction chromatography. In this research, chemical separation of Ni from the co-existing elements was investigated by cation exchange and Ni-Spec extraction chromatography. Precipitation behaviour of Ni and the co-existing elements with dimethylglyoxime(DMG) was investigated in ammonium $citrate/ethanol-H_2O$ and tartaric $acid/acetone-H_2O$ in order to purify separated Ni fractions and to prepare $^{59/63}Ni$ source for the radioactivity measurement using a gas proportional counter. Recovery of Ni separated through ion exchange chromatographic separation procedure was $92.1\%$ with relative standard deviation of $0.9\%$. In addition, recovery of Ni with DMG in the tartaric $acid/acetone-H_2O$ was $85.6\%$ with relative standard deviation of $1.9\%$.

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