• Title/Summary/Keyword: Radioactive nuclides

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Occupational Dose Analysis of Spent Resin Handling Accident During NPP Decommissioning

  • Hyunjin Lee;Chang-Lak Kim;Sang-Rae Moon;Sun-Kee Lee
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.21 no.2
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    • pp.247-253
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    • 2023
  • According to NSSC Notice No. 2021-10, safety analysis needs to be introduced in the decommissioning plan. Public and occupational dose analyses should be conducted, specifically for unexpected radiological accidents. Herein, based on the risk matrix and analytic hierarchy process, the method of selecting accident scenarios during the decommissioning of nuclear power plants has been proposed. During decommissioning, the generated spent resin exhibits relatively higher activity than other generated wastes. When accidents occur, the release fraction varies depending on the conditioning method of radioactive waste and type of radioactive nuclides or accidents. Occupational dose analyses for 2 (fire and drop) among 11 accident scenarios have been performed. The radiation doses of the additional exposures caused by the fire and drop accidents are 1.67 and 4.77 mSv, respectively.

A study on the effect of material impurity concentration on radioactive waste levels for plans for decommissioning of nuclear power plant

  • Gilyong Cha;Minhye Lee;Soonyoung Kim;Minchul Kim;Hyunmin Kim
    • Nuclear Engineering and Technology
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    • v.55 no.7
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    • pp.2489-2497
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    • 2023
  • Co and Eu impurities in the SSCs are nuclides that dominantly influence the neutron-induced radioactive inventory in metal and concrete radwastes (radioactive wastes) during NPP decommission. The impurity concentrations provided by NUREG/CR-3474 were used for the practical range of Co and Eu impurity concentrations to be applied to the code calculations. Metal structures near the core were evaluated to be ILW (intermediate-level waste) for the whole range of Co impurity concentration, so the boundary line between ILW and LLW (low-level waste) has no change for the whole concentration range provided by NUREG/CR-3474. Also, the boundary line between VLLW (very low-level waste) and CW (clearance waste) in the concrete shield could alter a little depending on the Eu impurity concentration within the range provided by NUREG/CR-3474. From this work, it is found that the concentration of material impurities of SSCs gives no critical impact on determining radwaste levels.

Modeling Study on Nuclide Transport in Ocean - an Ocean Compartment Model (해양에서의 핵종이동 모델링 - 해양구획 모델)

  • Lee, Youn-Myoung;Suh, Kyung-Suk;Han, Kyong-Won
    • Nuclear Engineering and Technology
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    • v.23 no.4
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    • pp.387-400
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    • 1991
  • An ocean compartment model simulating transport of nuclides by advection due to ocean circulation and intertaction with suspended sediments is developed, by which concentration breakthrough curves of nuclides can be calculated as a function of time. Dividing ocean into arbitrary number of characteristic compartments and performing a balance of mass of nuclides in each ocean compartment, the governing equation for the concentration in the ocean is obtained and a solution by the numerical integration is obtained. The integration method is specially useful for general stiff systems. For transfer coefficients describing advective transport between adjacent compartments by ocean circulation, the ocean turnover time is calculated by a two-dimensional numerical ocean model. To exemplify the compartment model, a reference case calculation for breakthrough curves of three nuclides in low-level radioactive wastes, Tc-99, Cs-137, and Pu-238 released from hypothetical repository under the seabed is carried out with five ocean compartments. Sensitivity analysis studies for some parameters to the concentration breakthrough curves are also made, which indicates that parameters such as ocean turnover time and ocean water volume of compartments have an important effect on the breakthrough curves.

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Chinese buffer material for high-level radiawaste disposal --Basic features of GMZ-l

  • WEN Zhijian
    • Proceedings of the Korean Radioactive Waste Society Conference
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    • 2005.11b
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    • pp.236-244
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    • 2005
  • Radioactive wastes arising from a wide range of human activities are in many different physical and chemical forms, contaminated with varying radioactivity. Their common feature is the potential hazard associated with their radioactivity and the need to manage them in such a way as to protect the human environment. The geological disposal is regarded as the most reasonable and effective way to safely disposal high-level radioactive wastes in the world. The conceptual model of geological disposal in China is based on a multi-barrier system that combines an isolating geological environment with an engineered barrier system. The buffer is one of the main engineered barriers for HLW repository. The buffer material is expected to maintain its low water permeability, self-sealing property, radio nuclides adsorption and retardation property, thermal conductivity, chemical buffering property, overpack supporting property, stress buffering property over a long period of time. Benotite is selected as the main content of buffer material that can satisfy above. GMZ deposit is selected as the candidate supplier for Chinese buffer material of High Level Radioactive waste repository. This paper presents geological features of GMZ deposit and basic property of GMZ Na bentonite. GMZ bentonite deposit is a super large scale deposits with high content of Montmorillonite (about $75\%$) and GMZ-l, which is Na-bentonite produced from GMZ deposit is selected as reference material for Chinese buffer material study.

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Sorption Characteristics of Strontium and Nickel on Mackinawite According to pH Variations in Alkaline Conditions (염기 환경에서 pH 변화에 따른 맥키나와이트 광물에 스트론튬과 니켈의 수착 특성)

  • Park, Chung-Kyun;Park, Tae-Jin;Lee, Seung-Yup;Lee, Jae-Kwang
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.18 no.1
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    • pp.73-81
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    • 2020
  • Strontium (90Sr) and nickel (59Ni) have been considered as key radionuclides in the safety assessment of radioactive waste disposal. Through various efforts to impede the migration of radioactive nuclides underground, it has been established that some minerals generated from the corrosion of the waste containers have a positive chemical interaction with these radionuclides. Among these minerals we selected mackinawite (FeS), an iron and sulfur compound, and performed a sorption experiment for the Sr and Ni in FeS under anoxic and alkaline conditions by reflecting deep underground environments. The effects of pH on sorption were likewise investigated in the pH range of 8 ~ 12. As a result, it was found that strontium failed to exhibit a good sorption capacity in a weak alkaline range, while nickel showed a noticeably higher sorption affinity over the entire experimental pH range. Moreover, we determined that as the pH increased in the solution, the distribution coefficients (Kd) were increased for both nuclides, which reflects when an alkalinity increses, the surface of the mineral charges much negatively by detaching the hydrogen or cations on the mineral surface. Thus, it can be concluded that the cationic nuclides of Sr and Ni can attach easily to the mineral under strong alkalinity.

The Measurement of Unsaturated Hydraulic Conductivity from One-Step Outflow Method (One-Step Outflow Method를 이용한 불포화 수리전도도 측정)

  • 이수홍;황주호;이재민;김창락
    • Proceedings of the Korean Radioactive Waste Society Conference
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    • 2003.11a
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    • pp.300-305
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    • 2003
  • One of the most important parts in constructing radioactive waste repository may be its safety aspect. The fundamental function of the repository is to isolate completely and forever the radioactive wastes disposed of in it. However, since either normally or abnormally nuclides are to be released from the repository with a certain causes. The hydraulic conductivity is related to transportation of nuclide in soil. However, hydraulic characteristics research in unsaturated soil is not enough at present time. A fast and easy procedure for estimating unsaturated flow parameters is presented. The estimation is based on direct measurement of the retention characteristics combined with inverse estimation of the hydraulic conductivity characteristics from one-step outflow experiment.

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Near-Field Transport of Radionuclide Decay Chains (방사성 핵종 붕괴 사슬의 Near-Field 이동)

  • Kang, Chul-Hyung
    • Nuclear Engineering and Technology
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    • v.26 no.2
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    • pp.277-284
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    • 1994
  • Much attention has been given to predict the near-field mass transfer of a single radioactive species from a waste solid into surrounding porous medium. But only limited considerations have been given to predict the coupled mass transfer of species with a radioactive decay chain. In this study we present an analysis assuming that the members of a decay chain dissolve congruently with a solubility-limited matrix. We give general, non-recursive analytic solutions for the transport of a radioactive decay chain in a finite porous medium when nuclides are released congruently with the matrix. As an illustration we consider the decay chain $^{234}$ Ulongrightarrow$^{230}$ Thlongrightarrow$^{226}$ Ra from spent fuel. These solutions may be useful and potentially important in performance assessment of radioactive waste repositories.

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The Study on the Fixation of Cs-137 Radionuclide in Clinoptillolite - The Fixation of Cesium in Clinoptillolite - (Clinoptillolite에 의(依)한 Cs-137 핵종(核種) 흡착(吸着)에 관(關)한 연구(硏究))

  • Lee, Sang-Hoon;Sung, Nak-June;Park, Won-Jong
    • Journal of Radiation Protection and Research
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    • v.3 no.1
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    • pp.1-5
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    • 1978
  • Investigation is carried out that low-level liquid radioactive wastes which is consisted of long half-life nuclides such as cesium can be treated by Korean clinoptillolite as a kind of zeolites. Column operation using a activated clinoptillolite shows good results in terms of break-through curves and comparing to clinoptillolite classified at WARD in U.S, Korean clinoptillolite shows a tailing phenomena longer than that of WARD. The fixation quantity of radioactivity in Korea clinoptillolite is to be about $75{\mu}Ci/100g$ using a $2.5{\times}10^{-3}{\mu}Ci/ml$ solution.

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Current status of disposal and measurement analysis of radioactive components in linear accelerators in Korea

  • Kwon, Na Hye;Shin, Dong Oh;Kim, Jinsung;Yoo, Jaeryong;Park, Min Seok;Kim, Kum Bae;Kim, Dong Wook;Choi, Sang Hyoun
    • Nuclear Engineering and Technology
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    • v.54 no.2
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    • pp.507-513
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    • 2022
  • When X-ray energy above 8 MV is used, photoneutrons are generated by the photonuclear reaction, which activates the components of linear accelerator (linac). Safely managing the radioactive material, when disposing linac or replacing components, is difficult, as the standards for the radioactive material management are not clear in Korea. We surveyed the management status of radioactive components occurred from medical linacs in Korea. And we also measured the activation of each part of the discarded Elekta linac using a survey meter and portable High Purity Germanium (HPGe) detector. We found that most medical institutions did not perform radiation measurements when disposing of radioactive components. The radioactive material was either stored within the institution or collected by the manufacturer. The surface dose rate measurements showed that the parts with high surface dose rates were target, primary collimator, and multileaf collimator (MLC). 60Co nuclide was detected in most parts, whereas for the target, 60Co and 184Re nuclides were detected. Results suggest that most institutions in Korea did not have the regulations for disposing radioactive waste from linac or the management procedures and standards were unclear. Further studies are underway to evaluate short-lived radionuclides and to lay the foundation for radioactive waste management from medical linacs.