• Title/Summary/Keyword: Radioactive concentration

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Alarm Setpoint Determination Method of Gaseous Effluent Radiation Monitoring Systems Using Dose Factors Based on ICRP-60 Recommendations (선량환산인자를 이용한 기체유출물 RMS 경보설정 개선방안)

  • 박규준;김희근;하각현;엄희문
    • Proceedings of the Korean Radioactive Waste Society Conference
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    • 2003.11a
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    • pp.491-496
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    • 2003
  • In Korea, the dose limits to the public were reduced according to ICRP-60 recommendations. The secondary quantities, Effluent Concentration Limits (ECLs) were derived and enacted to Korean Atomic Laws based on ICRP-60 recommendations. The Korea atomic laws require assurance that radioactive materials within gaseous effluents do not exceed dose limits and ECLs. This simply means that any effluent that would possibly contain radioactivity must be monitored. There are various methods to monitor the radioactivity of effluent monitor to satisfy the dose limits and the ECLs for gaseous effluents. The many factors (safety margin) should be considered in determining of the setpoint of effluent monitor, following these limits. In this study, we studied the determination method of alarm setpoint for gaseous effluent Radiation Monitoring Systems using dose factors considered the main pathway of radionuclides to compare the preceding determination method of alarm setpoint for gaseous effluent RMSs using dose assessment program considered all the practicable pathways of radionuclides.

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Characteristics of regional scale atmospheric dispersion around Ki-Jang research reactor using the Lagrangian Gaussian puff dispersion model

  • Choi, Geun-Sik;Lim, Jong-Myoung;Lim, Kyo-Sun Sunny;Kim, Ki-Hyun;Lee, Jin-Hong
    • Nuclear Engineering and Technology
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    • v.50 no.1
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    • pp.68-79
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    • 2018
  • The Ki-Jang research reactor (KJRR), a new research reactor in Korea, is being planned to fulfill multiple purposes. In this study, as an assessment of the environmental radiological impact, we characterized the atmospheric dispersion and deposition of radioactive materials released by an unexpected incident at KJRR using the weather research and forecasting-mesoscale model interface program-California Puff (WRF-MMIF-CALPUFF) model system. Based on the reproduced three-dimensional gridded meteorological data obtained during a 1-year period using WRF, the overall meteorological data predicted by WRF were in agreement with the observed data, while the predicted wind speed data were slightly overestimated at all stations. Based on the CALPUFF simulation of atmospheric dispersion (${\chi}/Q$) and deposition (D/Q) factors, relatively heavier contamination in the vicinity of KJRR was observed, and the prevailing land breeze wind in the study area resulted in relatively higher concentration and deposition in the off-shore area sectors. We also compared the dispersion characteristics between the PAVAN (atmospheric dispersion of radioactive release from nuclear power plants) and CALPUFF models. Finally, the meteorological conditions and possibility of high doses of radiation for relatively higher hourly ${\chi}/Q$ cases were examined at specific discrete receptors.

Development of Internal Dose Assessment Procedure for Workers in Industries Using Raw Materials Containing Naturally Occurring Radioactive Materials

  • Choi, Cheol Kyu;Kim, Yong Geon;Ji, Seung Woo;Koo, Boncheol;Chang, Byung Uck;Kim, Kwang Pyo
    • Journal of Radiation Protection and Research
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    • v.41 no.3
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    • pp.291-300
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    • 2016
  • Background: It is necessary to assess radiation dose to workers due to inhalation of airborne particulates containing naturally occurring radioactive materials (NORM) to ensure radiological safety required by the Natural Radiation Safety Management Act. The objective of this study is to develop an internal dose assessment procedure for workers at industries using raw materials containing natural radionuclides. Materials and Methods: The dose assessment procedure was developed based on harmonization, accuracy, and proportionality. The procedure includes determination of dose assessment necessity, preliminary dose estimation, airborne particulate sampling and characterization, and detailed assessment of radiation dose. Results and Discussion: The developed dose assessment procedure is as follows. Radioactivity concentration criteria to determine dose assessment necessity are $10Bq{\cdot}g^{-1}$ for $^{40}K$ and $1Bq{\cdot}g^{-1}$ for the other natural radionuclides. The preliminary dose estimation is performed using annual limit on intake (ALI). The estimated doses are classified into 3 groups ( < 0.1 mSv, 0.1-0.3 mSv, and > 0.3 mSv). Air sampling methods are determined based on the dose estimates. Detailed dose assessment is performed using air sampling and particulate characterization. The final dose results are classified into 4 different levels ( < 0.1 mSv, 0.1-0.3 mSv, 0.3-1 mSv, and > 1 mSv). Proper radiation protection measures are suggested according to the dose level. The developed dose assessment procedure was applied for NORM industries in Korea, including coal combustion, phosphate processing, and monazite handing facilities. Conclusion: The developed procedure provides consistent dose assessment results and contributes to the establishment of optimization of radiological protection in NORM industries.

Ions Removal of Contaminated Water with Radioactive Ions by Reverse Osmosis Membrane Process (방사성이온으로 오염된 물의 역삼투막공정을 이용한 이온제거)

  • Shin, Do Hyoung;Cheong, Seong Ihl;Rhim, Ji Won
    • Membrane Journal
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    • v.26 no.5
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    • pp.401-406
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    • 2016
  • In this study, we have investigated the removal of the low level radioactive ions of Cs and I in water by the reverse osmosis (RO) process. The two RO modules produced in domestic region and the waste RO module after the cleaning process were selected. Then we compared removal performance of both Cs and I. The experiments are conducted by varying the concentration of feed, the pressure. As a results, it was confirmed that all three modules are higher I decontamination factor than Cs. And particularly, for the cleaned RO module, its decontamination factor of I was 1140. Since the results at low pressure condition were better than that at high pressure conditions, the use of the direct installation of RO modules on the tap water might be possible. In addition, it was confirmed that the waste RO module after cleaning process using EDTA, SBS and NaOH, increased the decontamination performance better than before cleaning, in particular, the recovery ratio after cleaning was 6.3% higher.

Radiochemical Analysis of Filters Used During the Decommissioning of Research Reactors for Disposal

  • Kyungwon Suh;Jung Bo Yoo;Kwang-Soon Choi;Gi Yong Kim;Simon Oh;Kanghyun Yoo;Kwang Eun Lee;Shinkyoung Lee;Young Sang Lee;Hyeju Lee;Junhyuck Kim;Kyunghun Jung;Sora Choi;Tae-Hong Park
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.20 no.4
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    • pp.489-500
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    • 2022
  • The decommissioning of nuclear facilities produces various types of radiologically contaminated waste. In addition, dismantlement activities, including cutting, packing, and clean-up at the facility site, result in secondary radioactive waste such as filters, resin, plastic, and clothing. Determining of the radionuclide content of this waste is an important step for the determination of a suitable management strategy including classification and disposal. In this work, we radiochemically characterized the radionuclide activities of filters used during the decommissioning of Korea Research Reactors (KRRs) 1 and 2. The results indicate that the filter samples contained mainly 3H (500-3,600 Bq·g-1), 14C (7.5-29 Bq·g-1), 55Fe (1.1- 7.1 Bq·g-1), 59Ni (0.60-1.0 Bq·g-1), 60Co (0.74-70 Bq·g-1), 63Ni (0.60-94 Bq·g-1), 90Sr (0.25-5.0 Bq·g-1), 137Cs (0.64-8.7 Bq·g-1), and 152Eu (0.19-2.9) Bq·g-1. In addition, the gross alpha radioactivity of the samples was measured to be between 0.32-1.1 Bq·g-1. The radionuclide concentrations were below the concentration limit stated in the low- and intermediatelevel waste acceptance criteria of the Nuclear Safety and Security Commission, and used for the disposal of the KRRs waste drums to a repository site.

Key Parameters Analysis of Important Radionuclides in Dose Evaluation Model of Decommissioning Site (해체 부지 선량평가모텔의 주요 핵종에 대한 Key parameter 분석)

  • 임용규;김학수;손중권;박경록;강기두;김경덕;정찬우
    • Proceedings of the Korean Radioactive Waste Society Conference
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    • 2004.06a
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    • pp.52-57
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    • 2004
  • In order to analyze key parameters of important radionuclides in dose evaluation model of decommissioning site, a sensitivity analysis was performed. This analysis assumed a resident farmer for an exposure scenario and 0.037Bq/g for the concentration of radionuclides. As a result of sensitivity analysis, the key parameters of radionuclides considered were the area of contaminated zone, external gamma shielding factor and indoor time fraction for Cs-137 and Co-60. The key parameters for C-14 were the environmental parameters and hydrological parameters of unsaturated zone. Also, the key parameter for Sr-90 was the density of contaminated zone.

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Soil Samples in 134Cs of the 604, 795 keV Spectrum Analysis (토양시료 속 134Cs의 604, 795 keV 에너지 스펙트럼 분석)

  • Jang, Eunsung
    • Journal of the Korean Society of Radiology
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    • v.8 no.7
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    • pp.443-447
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    • 2014
  • $^{134}Cs$ radioactive concentration among soil samples is difficult to classify due to the background impact on crust originated natural radioactive nuclide, and overlapping and interfering between peaks. The ways to identify true peaks in gamma-ray spectroscopy are as follows to reduce statistical fluctuation by smoothing based on the fact that the shapes of peak are mostly Gaussian, to inspect the levels of width and height of peaks, to add functions on low-energy trailing phenomena, or 4) to check the peaks after modifying Gaussian function itself. Therefore, it is considered that information and knowledge for spectrum analysis are necessary.

Dissolution of Tc(IV) Oxides in Aqueous Solutions

  • LIU De-jun;FAN Xian-hua
    • Proceedings of the Korean Radioactive Waste Society Conference
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    • 2005.11b
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    • pp.51-59
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    • 2005
  • The long-lived fission product $^{99}Tc$ is present in large quantities in nuclear wastes and its chemical behavior in aqueous solution is of considerable interest. Under oxidizing conditions technetium exists as the anionic species $TcO_4^-$ whereas under the reducing conditions it is generally predicted that technetium will be present as $TcO_2{\cdot}nH_2O$. Technetium oxide was prepared by reduction of a technetate solution with $Sn^{2+}$. The concentration of total technetium and Tc(IV) species in the solutions were periodically determined by separating the oxidized and reduced technetium species using a solvent extraction procedure and counting the beta activity of the $^{99}Tc$ with a liquid scintillation counter. The experimental results show that the rate of oxidation of Tc(IV) in simulated groundwater and redistilled water is about $(1.49{\~}1.86){\times}10^{-9} mol/(L{\cdot}d$) under aerobic conditions, but Tc(IV) in simulated groundwater and redistilled water is not oxidized under anaerobic conditions. Under aerobic or anaerobic conditions the solubility of Tc(IV) oxide in simulated groundwater and redistilled water is equal on the whole.

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Evaluation of the Demineralizer Performance and $^{65}Zn$ Activity on Spent Resin for a Zinc Addition Operation

  • Kim, Kwang-Rag;Sung, Ki-Woung;Na, Jung-Won;Kim, Uh-Chul
    • Proceedings of the Korean Radioactive Waste Society Conference
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    • 2003.11a
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    • pp.191-195
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    • 2003
  • Zinc acetate has been proposed and used to evaluate ionic zinc as a means to reduce reactor radiation buildup at several nuclear plants. Thermodynamic analysis of the aqueous zinc system using reliable data shows that the stability of the hydrolyzed zinc species increases with pH and temperature. Adsorption kinetics and isotherm studies were carried out to investigate the mixed resin performance of the zinc adsorption. The equilibrium isotherms of the zinc adsorption onto nuclear grade resin indicate that the data correlate well with the Langmuir model and that the adsorption is physical in nature. The maximum capacity according to the Langrnuir model is about 0.6meq/g for an initial zinc concentration of 100ppm at $50^{\circ}C$. The use of natural zinc could result in the generation of a $^{65}Zn$ activity with about $500{\mu}Ci/mL$ of resin after 12 months of operation.

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Effect of a Hydrothermal Reaction on the Expandibility, Layer Charge, and CEC of Smectite Clay (스멕타이트 점토의 팽창도, 층전하, 양이온 교환능에 대한 열수반응의 영향)

  • Lee, Jae-Owan;Cho, Won-Jin
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.8 no.3
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    • pp.173-179
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    • 2010
  • In a HLW repository, the buffer is exposed to an elevated temperature due to a radioactive decay and geochemical conditions for a long time and such a hydrothermal condition may cause a significant loss of its barrier function. This study carried out hydrothermal tests with a domestic smectite clay to investigate the changes in the expandibility, layer charge, and cation exchange capacity of the smectite. When the temperature and potassium concentration in solution was increased for the hydrothermal treatments, the expandibility decreased, the layer charge negatively increased, and the CEC also decreased.