• Title/Summary/Keyword: Pyrochemical reprocessing

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Criticality analysis of pyrochemical reprocessing apparatuses for mixed uranium-plutonium nitride spent nuclear fuel using the MCU-FR and MCNP program codes

  • P.A. Kizub ;A.I. Blokhin ;P.A. Blokhin ;E.F. Mitenkova;N.A. Mosunova ;V.A. Kovrov ;A.V. Shishkin ;Yu.P. Zaikov ;O.R. Rakhmanova
    • Nuclear Engineering and Technology
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    • v.55 no.3
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    • pp.1097-1104
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    • 2023
  • A preliminary criticality analysis for novel pyrochemical apparatuses for the reprocessing of mixed uranium-plutonium nitride spent nuclear fuel from the BREST-OD-300 reactor was performed. High-temperature processing apparatuses, "metallization" electrolyzer, refinery remelting apparatus, refining electrolyzer, and "soft" chlorination apparatus are considered in this work. Computational models of apparatuses for two neutron radiation transport codes (MCU-FR and MCNP) were developed and calculations for criticality were completed using the Monte Carlo method. The criticality analysis was performed for different loads of fissile material into the apparatuses including overloading conditions. Various emergency situations were considered, in particular, those associated with water ingress into the chamber of the refinery remelting apparatus. It was revealed that for all the considered computational models nuclear safety rules are satisfied.

PYROPROCESSING FLOWSHEETS FOR RECYCLING USED NUCLEAR FUEL

  • Williamson, M.A.;Willit, J.L.
    • Nuclear Engineering and Technology
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    • v.43 no.4
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    • pp.329-334
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    • 2011
  • Two conceptual flowsheets were developed for recycling used nuclear fuel. One flowsheet was developed for recycling used oxide nuclear fuel from light water reactors while the other was developed for recycling used metal fuel from fast spectrum reactors. Both flowsheets were developed from a set of design principles including efficient actinide recovery, nonproliferation, waste minimization and commercial viability. Process chemistry is discussed for each unit operation in the flowsheet.