• Title/Summary/Keyword: Potential radionuclides

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Assessment of Radiological Hazards in Some Foods Products Consumed by the Malian Population Using Gamma Spectrometry

  • Adama Coulibaly;David O. Kpeglo;Emmanuel O. Darko
    • Journal of Radiation Protection and Research
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    • v.48 no.2
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    • pp.84-89
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    • 2023
  • Background: Food consumption is one of the most important routes for radionuclide intake for the public; therefore, there is the need to have a comprehensive understanding of the amount of radioactivity in food products. Consumption of radionuclide-contaminated food could increase potential health risks associated with exposure to radiation such as cancers. The present study aims to determine radioactivity levels in some food products (milk, rice, sugar, and wheat flour) consumed in Mali and to evaluate the radiological effect on the public health from these radionuclides. Materials and Methods: The health impact due to ingestion of radionuclides from these foods was evaluated by the determination of activity concentration of radionuclides 238U, 232Th, 40K, and 137Cs using gamma spectrometry system with high-purity germanium detector and radiological hazards index in 16 samples collected in some markets, mall, and shops of Bamako-Mali. Results and Discussion: The average activity concentrations were 9.8±0.6 Bq/kg for 238U, 8.7±0.5 Bq/kg for 232Th, 162.9±7.9 Bq/kg for 40K, and 0.0035±0.0005 Bq/kg for 137Cs. The mean values of radiological hazard parameters such as annual committed effective dose, internal hazard index, and risk assessment from this work were within the dose criteria limits given by international organizations (International Commission on Radiological Protection and United Nations Scientific Committee on the Effects of Atomic Radiation) and national standards. Conclusion: The results show low public exposure to radioactivity and associated radiological impact on public health. Nevertheless, this study stipulates vital data for future research and regulatory authorities in Mali.

A Conservative Safety Study on Low-Level Radioactive Waste Repository Using Radionuclide Release Source Term Model (선원항 모델을 사용한 저준위 방사성폐기물 처분장의 보수적인 안전성고찰)

  • Kim, Chang-Lak;Lee, Myung-Chan;Cho, Chan-Hee
    • Nuclear Engineering and Technology
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    • v.25 no.1
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    • pp.63-70
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    • 1993
  • A simplified safety assessment is carried out on rock-cavern type disposal of LLW using the analytical repository source term (REPS) model. For reliable prediction of the leach rates for various radionuclides, degradation of concrete structures, corrosion rate of waste container, degree of corrosion on the container surface, and the characteristics of radionuclides are considered in the REPS model. The results of preliminary assessment show that Cs-137, Ni-63, and Sr-90 are dominant. For the parametric uncertainty and sensitivity analysis, Latin hypercube sampling technique and rank correlation technique are applied. The results of the potential public health impacts show that radiological dose to intruder in the worst case scenario will be negligible and that more attention should be given to near-field performance.

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Three-dimensional MXene (Ti3C2Tx) Film for Radionuclide Removal From Aqueous Solution

  • Jang, Jiseon;Lee, Dae Sung
    • Proceedings of the Korean Radioactive Waste Society Conference
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    • 2018.11a
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    • pp.379-379
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    • 2018
  • MXenes are a new family of 2D transition metal carbide nanosheets analogous to graphene (Lv et al., 2017; Sun et al., 2018). Due to the easy availability, hydrophilic behavior, and tunable chemistry of MXenes, their use in applications for environmental pollution remediation such as heavy metal adsorption has recently been explored (Li et al., 2017). In this study, three-dimensional (3D) MXene ($Ti_3C_2T_x$) films with high adsorption capacity, good mechanical strength, and high selectivity for specific radionuclide from aquose solution were successfully fabricated by a polymeric precursor method using vacuum-assisted filtration. The highest removal efficiency on the films was 99.54%, 95.61%, and 82.79% for $Sr^{2+}$, $Co^{2+}$, and $Cs^+$, respectively, using a film dosage of 0.06 g/ L in the initial radionuclide solution (each radionuclide concentration = 1 mg/L and pH = 7.0). Especially, the adsorption process reached an equilibrium within 30 min. The expanded interlayer spacing of $Ti_3C_2T_x$ sheets in MXene films showed excellent radionuclide selectivity ($Cs^+$ and/or $Sr^{2+}/Co^{2+}$) (Simon, 2017). Besides, the MXene films was not only able to be easily retrieved from an aqueous solution by filtration after decontamination processes, but also to selectively separate desired target radionuclides in the solutions. Therefore, the newly developed MXene ($Ti_3C_2T_x$) films has a great potential for radionuclide removal from aqueous solution.

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Assessment of Potential Radiation Dose Rates to Marine Organisms Around the Korean Peninsula

  • Lee, Dong-Myung;Lee, Jun-ho
    • Journal of Radiation Protection and Research
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    • v.41 no.1
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    • pp.1-6
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    • 2016
  • Background: It is very difficult to set a regulatory guidance or criteria for the protection of non-human species from the ionizing radiation, because there are no generally or internationally accepted methods for demonstrating the compliance with such criteria. It is needed that Korea develop the primary dose rate standards for the protection of both aquatic and terrestrial biota in the near future. Materials and Methods: The potential dose rates due to both external and internal radiation exposures to marine organisms such as plaice/flounder, gray mullet, and brown seaweed collected within territorial seas around the Korean Peninsula were estimated. Results and Discussion: The total dose rates to plaice/flounder, gray mullet and brown seaweed due to $^{40}K$, a primordial radionuclide in marine environment, were found to be 0.2%, 0.08% and 0.3% of approximately the values of the Derived Consideration Reference Levels (DCRLs, i.e. $1-10mGy{\cdot}d^{-1}$), respectively, as suggested by the International Commission on Radiological Protection (ICRP) publication 124. The total dose rates to marine fishes and brown seaweed due to anthropogenic radionuclides such as $^{90}Sr$, $^{137}Cs$ and $^{239+240}Pu$ were considered to be negligible compared to the total dose rate due to $^{40}K$. The external exposure to benthic fish due to all radionuclides was much higher than that of pelagic fish. Conclusion: From this study, it is recommended that the further study is required to develop a national regulatory guidance for the evaluation of doses to non-human species.

Desorption Characteristics of Cobalt, Strontium, and Cesium in Natural Soil and Kaolin Using CMCD (CMCD를 이용한 자연토양 및 카올린에서의 코발트, 스트론튬, 세슘의 탈착 특성)

  • Choi, Jeonghak;Cheon, Kyeongho
    • Journal of the Korean GEO-environmental Society
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    • v.15 no.12
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    • pp.61-69
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    • 2014
  • Carboxymethyl-${\beta}$-cyclodextrin (${\beta}$-CMCD), as a biodegradable surfactant with hydrophobic and hydrophilic properties, has potential advantages of being applicable to the simultaneous treatment of multiple contaminated soils. In this study, the desorption behaviors of r adionuclides such as cobalt (Co), strontium (Sr), and cesium (Cs) from the soil contaminated with them were experimentally investigated and the effectiveness of CMCD as a desorbent was evaluated. The desorption equilibrium of used radionuclides could be achieved within 1~3 hr and the desorption ratio from kaolin was higher than that from natural soil. The addition of CMCD of 2 g/L increased the desorption ratio by 5~20 % and the desorption ratio of used r adionuclides was shown in the order of Co > Cs > Sr. The experimental desorption data were fitted successfully by pseudo-second order kinetic model and the desorption rate of the r adionuclides was shown in the order of Cs > Co > Sr. Hysteresis between adsorption and desorption of the r adionuclides, as shown in the order of Sr > Co > Cs, increased as the desorption rate decreased. Consequently, it could be considered that the desorption rate was one of the significant factors of the hysteresis. The addition of CMCD as desorbent increased the amount of desorbed radionuclides and decreased the hysteresis. However, the CMCD could not completely desorb the radionuclides from soils even though the excess of CMCD was added.

Electrosorption and Separation of $Co^{2+}$ and $Sr^{2+}$ Ions from Decontaminated Liquid Wastes

  • Kim, Jun-Soo;Jung, Chong-Hun;Oh, Won-Zin;Ryu, Seung-Kon
    • Carbon letters
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    • v.3 no.1
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    • pp.6-12
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    • 2002
  • A study on the electrosorption of $Co^{2+}$ and $Sr^{2+}$ ions onto a porous activated carbon fiber (ACF) was performed to treat radioactive liquid wastes resulting from chemical or electrochemical decontamination and to regenerate the spent carbon electrode. The result of batch electrosorption experiments showed that applied negative potential increased adsorption kinetics and capacity in comparison with open-circuit potential (OCP) adsorption for $Co^{2+}$ and $Sr^{2+}$ ions. The adsorbed $Co^{2+}$ and $Sr^{2+}$ ions are released from the carbon fiber by applying a positive potential on the electrode, showing the reversibility of the sorption process. The possibility of application of the electrosorption technique to the separation of radionuclides was examined. The result of a selective removal experiments of a single component from a mixed solution showed that perfect separation of $Co^{2+}$ and $Sr^{2+}$ ions was possible by the electrosorption process.

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Numerical Estimates of Seasonal Changes of Possible Radionuclide Dispersion at the Kori Nuclear Power Plants (고리 원자력 발전 단지 사고 발생에 따른 방사능 물질 확산 가능성의 계절적 특성 연구)

  • Kim, Ji-Seon;Lee, Soon-Hwan;Park, Kang-Won;Lee, Sung-Gwang;Choi, Se-Young;Cho, Kyu-Chan;Lee, Hyeuk-Woo
    • Journal of Environmental Science International
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    • v.27 no.6
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    • pp.425-436
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    • 2018
  • To establish initial response scenarios for nuclear accidents around the Kori nuclear power plants, the potential for radionuclide diffusion was estimated using numerical experiments and statistical techniques. This study used the numerical model WRF (Weather Research and Forecasting) and FLEXPART (Flexible Particle dispersion model) to calculate the three-dimensional wind field and radionuclide dispersion, respectively. The wind patterns observed at Gijang, near the plants, and at meteorological sites in Busan, were reproduced and applied to estimates of seasonally averaged wind fields. The distribution of emitted radionuclides are strongly associated with characteristics of topography and synoptic wind patterns over nuclear power plants. Since the terrain around the power plants is complex, estimates of radionuclide distribution often produce unexpected results when wind data from different sites are used in statistical calculations. It is highly probable that in the summer and autumn, radionuclides move south-west, towards the downtown metropolitan area. This study has clear limitations in that it uses the seasonal wind field rather than the daily wind field.

Application of In Situ Measurement for Site Remediation and Final Status Survey of Decommissioning KRR Site

  • Hong, Sang Bum;Nam, Jong Soo;Choi, Yong Suk;Seo, Bum Kyoung;Moon, Jei Kwon
    • Journal of Radiation Protection and Research
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    • v.41 no.2
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    • pp.173-178
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    • 2016
  • Background: In situ gamma spectrometry has been used to measure environmental radiation, assumptions are usually made about the depth distribution of the radionuclides of interest in the soil. The main limitation of in situ gamma spectrometry lies in determining the depth distribution of radionuclides. The objective of this study is to develop a method for subsurface characterization by in situ measurement. Materials and Methods: The peak to valley method based on the ratio of counting rate between the photoelectric peak and Compton region was applied to identify the depth distribution. The peak to valley method could be applied to establish the relation between the spectrally derived coefficients (Q) with relaxation mass per unit area (${\beta}$) for various depth distribution in soil. The in situ measurement results were verified by MCNP simulation and calculated correlation equation. In order to compare the depth distributions and contamination levels in decommissioning KRR site, in situ measurement and sampling results were compared. Results and Discussion: The in situ measurement results and MCNP simulation results show a good correlation for laboratory measurement. The simulation relationship between Q and source burial for the source layers have exponential relationship for a variety depth distributions. We applied the peak to valley method to contaminated decommissioning KRR site to determine a depth distribution and initial activity without sampling. The observed results has a good correlation, relative error between in situ measurement with sampling result is around 7% for depth distribution and 4% for initial activity. Conclusion: In this study, the vertical activity distribution and initial activity of $^{137}Cs$ could be identifying directly through in situ measurement. Therefore, the peak to valley method demonstrated good potential for assessment of the residual radioactivity for site remediation in decommissioning and contaminated site.

Nuclide Release from Penetrations in Radioactive Waste Container (방사성 폐기물 저장용기 표면의 결함으로부터 핵종유출 연구)

  • Kim, Chang-Lak
    • Nuclear Engineering and Technology
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    • v.21 no.4
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    • pp.302-307
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    • 1989
  • Nuclide release through penetrations in radioactive waste container is analyzed. Penetrations may result from corrosion or cracking and may be through the container material or through deposits of corrosion products. The analysis deals with the resultant nuclide release, but not with the way these penetrations occur. Numerical illustrations show that mass transport from multiple holes can be significant and may approach the mass transfer rate calculated from bare waste forms. Although partially-failed containers may present an important long-term barrier to release of radionuclides, numerous small holes on a container surface have the potential of bypassing the effectiveness of these barriers.

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