• Title/Summary/Keyword: Particle extinction

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Classification of Dust/Non-dust Particle from the Asian Dust Plumes and Retrieval of Microphysical Properties using Raman Lidar System (다파장 라만 라이다 시스템을 이용한 황사/비황사입자 구분 및 비황사입자의 미세물리적 특성 연구)

  • Shin, Sungkyun;Shin, Dongho;Lee, Kwonho;Noh, Youngmin
    • Journal of Korean Society for Atmospheric Environment
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    • v.28 no.6
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    • pp.688-696
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    • 2012
  • The particle depolarization ratios were retrieved from the observation with a multi-wavelength Raman lidar at Gwangju, Korea ($35.11^{\circ}N$, $126.54^{\circ}E$). The measurements were carried out on 24 February and 9 March 2004. Using the particle depolarization ratios, the non-dust aerosol particles were distinguished from the Asian dust plume, and the proportion of the non-dust particle to total dust plume was retrieved. The calculated proportion of the non-dust particle was used for the retrieval of backscatter coefficients at 355, 532, and 1064 nm and extinction coefficients at 355 and 532 nm of non-dust particles in the dust plume. Microphysical parameters of non-dust particles including single-scattering albedo at 532 nm were retrieved using retrieved optical values. The retrieved single-scattering albedo of non-dust particles was 0.92~0.95 below 1 km height and 0.82~0.91 above 1 km height on 24 February 2004 and $0.81{\pm}0.03$ on 9 March 2004.

A Study on the Soot Particle Measurement in Co-Flow Diffusion Flame Using a Laser Diagnostics and a Thermocouple (레이저 및 열전대를 이용한 동축류 확산화염에서의 매연입자 측정에 관한 연구)

  • Han, Yong-Taek;Lee, Ki-Hyng;Lee, Won-Nam
    • Transactions of the Korean Society of Mechanical Engineers B
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    • v.28 no.7
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    • pp.863-870
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    • 2004
  • The temperature and soot particle measurement technique in a laminar diffusion flame has been studied to investigate the characteristics of soot particle with temperature using a co-flow burner. The temperature distribution in the flame were measured by rapid insertion of a R-type thermocouple and the soot particles by LEM/LIS techniques. In these measurement, soot volume fraction, number density and soot diameters were analyzed experimentally. As a results, the spacial distributions of particle volume fraction, soot diameter, and number density are mapped throughout the flame using the Rayleigh theory for the scattering of light by particles. A laser extinction method was used to measure the soot volume fraction and laser induced scattering method was used to measure the soot particle diameter and number density. Also, we measured temperature without the effect of soot particles attached to the thermocouple junction, which is close to the nozzle. In this result, we found that upstream zone has a unstable flowing in co-flow diffusion flame and the y-axis temperature of flame has a uniform temperature distribution in the most soot volume fraction zone.

A Study on the Soot Particle Measurement in Co-flow Diffusion Flame Using a Laser Diagnostics and a Thermocouple (레이저 및 열전대를 이용한 동축류 확산화염에서의 매연입자 측정에 관한 연구)

  • Han, Yong-Taek;Lee, Ki-Hyung;Lee, Won-Nam
    • Proceedings of the KSME Conference
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    • 2004.04a
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    • pp.1267-1273
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    • 2004
  • The temperature and soot particle measurement technique in a laminar diffusion flame have been studied to investigate the characteristics of soot particle with temperature using a co-flow burner. The temperature distributions in the flame were measured by rapid insertion of a R-type thermocouple and the soot particles were detected were detected by LEM/LIS techniques. In these measurement, soot volume fraction, number density and soot diameters were analyzed experimentally. As a results, the spacial distributions of particle volume fraction, soot diameter, and number density are mapped throughout the flame using the Rayleigh theory for the scattering of light by absorbing particles. A laser extinction method was used to measure the soot volume fraction and Laser induced scattering method was used to measure the soot particle diameter and number density. Also, we measured temperature without the effect of soot particles attached to the thermocouple junction, which is close to the nozzle. In this result, we found that upstream zone has a unstable flowing in co-flow diffusion flame and the y-axis temperature of flame has a uniform temperature distribution in the most soot volume fraction zone.

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Fabrication of 50 to 1000 nm Monodisperse ZnS Colloids

  • Chae, Weon-Sik;Kershner, Ryan J.;Braun, Paul V.
    • Bulletin of the Korean Chemical Society
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    • v.30 no.1
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    • pp.129-132
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    • 2009
  • Monodisperse ZnS colloidal particles with precisely specified diameters over a broad size range were synthesized by controlled aggregation. Sub-10nm ZnS seed crystals were first nucleated at ambient temperature and then grown at an elevated temperature, which produced large polydisperse colloidal particles. Subsequent rapid thermal quenching and heating processes induced a number of secondary nucleations in addition to growing the large polydisperse microparticles which were finally removed by centrifugation and discarded at the completion of the reaction. The secondary nuclei were then aggregated further at elevated temperatures, resulting in colloidal particles which exhibited a nearly monodisperse size distribution. Particle diameters were controlled over a wide size range from 50 nm to 1 μm. Mie simulations of the experiment extinction spectra determined that the volume fraction of the ZnS is 0.66 in an aggregated colloidal particle and the colloidal particle effective refractive index is approximately 2.0 at 590 nm in water. The surface of the colloidal particles was subsequently coated with silica to produce ZnS@silica core-shell particles.

Measurement of soot concentration in flames using laser-induced incandescence method (레이저 가열 측정법을 이용한 화염 내 매연 농도 측정)

  • Jurng, Jong-Soo
    • Journal of the Korean Society of Combustion
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    • v.1 no.1
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    • pp.75-82
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    • 1996
  • Laser induced incandescence, LII, recently developed technique for measuring soot concentration in flames, can overcome most of limitations of conventional laser extinction measurement. In this study, experiments were performed to investigate the effect of laser intensity, detection wavelength, and also laser beam quality on both LII signal at a particular position and peak-to-centerline LII signal ratio. The results of LII signal with increasing laser intensity shows its near-independence of laser intensity once threshold level of laser intensity has been reached. However, this near-independence depends on laser beam quality and the incident optical setup. The peak-to-centerline LII signal ratio slowly but continuously increases with laser power. This fact is due to the dependence of LII signal on particle mean diameter. LII signal is attenuated during it passes through the flame containing soot particles. The attenuation rate is inversely proportional to detection wavelength. In this study, LII signal at 680 nm band is 10% greater than the signal at 400 nm band.

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The Measurement of the LIDAR Ratio by Using the Rotational Raman LIDAR

  • Choi, Sung-Chul;Baik, Sung-Hoon;Park, Seung-Kyu;Cha, Hyung-Ki;Song, Im-Kang;Kim, Duk-Hyeon
    • Journal of the Optical Society of Korea
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    • v.14 no.3
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    • pp.174-177
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    • 2010
  • The rotational Raman LIDAR technique has been used to accurately measure aerosol optical properties such as backscatter coefficient, extinction coefficient, and LIDAR ratio. In the case of the vibrational Raman technique, the ${\AA}$ngstr$\ddot{o}$om exponent, which has wavelength dependence on the particle properties, is assumed to obtain the extinction coefficient. However, this assumed ${\AA}$ngstr$\ddot{o}$m exponent can cause systematic errors in retrieving aerosol optical properties. In the case of the rotational Raman technique, the aerosol optical properties can be measured without any assumptions about the ${\AA}$ngstr$\ddot{o}$m exponent. In this paper, the LIDAR ratio was measured by using the rotational Raman LIDAR and vibrational Raman LIDAR in the troposphere. And, the LIDAR ratios measured by these two methods were compared.

Behavior Analysis of Particle Crushing about Sabkha Layer under Hydrotest (Sabkha층의 Hydrotest 시 입자파쇄 거동분석)

  • Kim, Seokju;Han, Heuisoo
    • Journal of the Korean GEO-environmental Society
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    • v.14 no.9
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    • pp.57-65
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    • 2013
  • Carbonate sands can be crushed under low confining pressure to achieve high compressibility. So particle crushing has significant influence on characteristics of strength and deformation. Trial embankment and hydrotest are conducted on Sabkha layer, consisting of carbonate sand to build tank structure. In this paper the settlement behavior was analyzed from each test. Particle crushing happened from 80 to 170kPa stress under compression test, and calcium was detected from chemical test. The test result came out Sabkha soil was very weak and easy to be crushing. About trial embankment test, particle crushing was not happen, and then extinction of pore water pressure and settlements were finished just during 2 days. On the other hand, the long-term settlement was happened in hydrotest. So the two test results did not correspond to each other. If loading stress is higher than yielding stress, instant settlement and secondary compression settlement are happened as a result of the particle crushing.

An Experimental Study on Optical and Physical Properties of Particulate Matter produced from F-76 Marine Diesel and JP-8 Aviation Fuels (F-76 선박용 디젤유 및 JP-8 항공유 입자상물질의 광학 및 물리적 특성에 대한 실험적 연구)

  • Choi, Jae-Hyuk;Choi, Seuk-Cheun;Kim, Dae-Yong;Lee, Joo-Hee;Park, Seul-Hyun
    • Journal of the Korean Society of Marine Environment & Safety
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    • v.20 no.6
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    • pp.781-787
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    • 2014
  • The dimensionless extinction constants of particulate matter for F-76 diesel and JP-8 aviation fuels were measured at both 633 nm and 853 nm in the transmission cell where the simultaneous gravimetric measurement of PM concentration is compared to the light extinction measurement. For the F-76 diesel PM, the average value of the dimensionless extinction constants at 633 nm was 8.8 whereas that of the dimensionless extinction constants for JP-8 was 9.8 at the same wavelength. As the wavelength is increased to 853 nm, the average value for the F-76 diesel was reduced to 8.2 whereas that for JP-8 was decreased to 8.9.

Opto-Chemical Characteristics of Visibility Impairment Using Semi-Continuous Aerosol Monitoring in an Urban Area during Summertime (에어로졸의 준실시간 관측에 의한 여름철 도시지역 시정 감쇄 현상의 광ㆍ화학적인 특성 분석)

  • 김경원;김영준
    • Journal of Korean Society for Atmospheric Environment
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    • v.19 no.6
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    • pp.647-661
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    • 2003
  • For continuous monitoring of atmospheric visibility in the city of Kwanaju, Korea, a transmissometer system consisting of a transmitter and a receiver was installed at a distance of 1.91 km across the downtown Kwanaju. At the transmitter site an integrating nephelometer and an aethalometer were also installed to measure the scattering and absorption coefficients of the atmosphere, respectively. At the receiver site. an URG PM$_{2.5}$ cyclone sampler and an URG-VAPS (Versatile Air Pollutant Sampler) with three filter packs and two denuders were used to collect both PM$_{2.5}$ and PM$_{10}$ samples at a 2-hour or 12-hour sampling interval for aerosol chemical analysis. Sulfate, organic mass by carbon (OMC), nitrate, elemental carbon (EC) components of fine aerosol were the major contributors to visibility impairment. Diurnal variation of visibility during best-case days showed rapid improvement in the morning hours, while it was delayed until afternoon during the worst-case days. Aerosol mass concentration of each aerosol component for the worst-case was calculated to be 11.2 times larger than the best-case for (NH$_4$)$_2$SO$_4$(NHSO), 19.0 times for NH$_4$NO$_3$ (NHNO), 2.2 times for OMC, respectively. Also result shows that elemental carbon and fine soil (FS) were 3.7 and 2.2 times more than those of best-case. respectively- Sum of total contributions of wet NHSO and NHNO to light extinction was calculated to be 301 Mm$^{-1}$ for the worst-case. However, sum of contributions by dry NHSO and NHNO was calculated to be 123 Mm$^{-1}$ for the best case. Mass extinction efficiencies of fine and coarse particles were calculated to be 5.8$\pm$0.3 $m^2$/g and 1.8$\pm$0.1 $m^2$/g, respectively.ely.

Localized Surface Plasmon Resonance Coupling in Self-Assembled Ag Nanoparticles by Using 3-Dimensional FDTD Simulation (3차원 FDTD Simulation을 이용한 자기조립된 Ag 나노입자의 국소표면플라즈몬공명 상호작용 현상 연구)

  • Lee, Kyung-Min;Yoon, Soon-Gil;Jeong, Jong-Ryul
    • Korean Journal of Materials Research
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    • v.24 no.8
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    • pp.417-422
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    • 2014
  • In this study, we investigated localized surface plasmon resonance and the related coupling phenomena with respect to various geometric parameters of Ag nanoparticles, including the size and inter-particle distance. The plasmon resonances of Ag nanoparticles were studied using three-dimensional finite difference time domain(FDTD) calculations. From the FDTD calculations, we discovered the existence of a symmetric and an anti-symmetric plasmon coupling modes in the coupled Ag nanoparticles. The dependence of the resonance wavelength with respect to the inter-particle distance was also investigated, revealing that the anti-symmetric mode is more closely correlated with the inter-particle distance of the Ag nanoparticles than the symmetric mode. We also found that higher order resonance modes are appeared in the extinction spectrum for closely spaced Ag nanoparticles. Plasmon resonance calculations for the Ag particles coated with a $SiO_2$ layer showed enhanced plasmon coupling due to the strengthened plasmon resonance, suggesting that the inter-particle distance of the Ag nanoparticles can be estimated by measuring the transmission and absorption spectra with the plasmon resonance of symmetric and anti-symmetric localized surface plasmons.