• Title/Summary/Keyword: Oxide nuclear fuel

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Neutronics study on small power ADS loaded with recycled inert matrix fuel for transuranic elements transmutation using Serpent code

  • Vu, Thanh Mai;Hartanto, Donny;Ha, Pham Nhu Viet
    • Nuclear Engineering and Technology
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    • v.53 no.7
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    • pp.2095-2103
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    • 2021
  • A small power ADS design using thorium oxide and diluent matrix reprocessed fuel is proposed for a high transmutation rate, small reactivity swing, and strong safety features. Two fuel matrices (CERCER and CERMET) and different recycled fuel compositions recovered from UO2 spent fuels with 45 GWd/tU and 60 GWd/tU burnup were investigated to determine the suitable fuel for the ADS. It was found that the transmutation of each isotope depends on TRU initial loading amount. After examining the cores, the results show that CERCER fueled ADS has a negative coolant void reactivity (CVR) and a smaller radiotoxicity at discharge compared to that of CERMET core. It implies that CERCER fuel has enhanced safety features and more flavor in terms of radiotoxicity management. To increase fuel utilization and core operation efficiency, a simple assembly shuffling pattern for the CERCER fueled ADS is also proposed. Eigenvalue and burnup calculations were conducted using Serpent 2 with ENDF/B-VII.0 library in both kcode and external source modes, and it indicates that the results of transmutation analyses obtained by kcode only is reliable to discuss the transmutation potential of ADS. Burnup calculation with the fixed-source mode is essential to be used for more practical results of the transmutation by ADS.

Mechanical and Thermal Analysis of Oxide Fuel Rods

  • Ilsoon Hwang;Lee, Byungho;Lee, Changkun
    • Nuclear Engineering and Technology
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    • v.9 no.4
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    • pp.223-236
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    • 1977
  • An integral computer code has been developed for a mechanical and thermal design and performance analysis of an oxide fuel rod in a pressurized water reactor. The code designated as FROD 1.0 takes into account the phenomena of radial power depression within the pellet, cracking, densification and swelling of the pellet, fission gas release, clad creep, pellet-clad contact, heat transfer to coolant and buildup of corrosion layers on the clad surface. The FROD 1.0 code yields two-dimensional temperature distributions, dimensional changes, stresses, and internal pressure of a fuel rod as a function of irradiation time within a reasonable computation time. The code may also be used for the analyses of oxide fuel rods in other thermal reactors. As an application of FROD 1.0 the behavior of fuel rod loaded in the first core of Go-ri Nuclear Power Plant Unit 1 is predicted for the two power histories corresponding to steady state operation and Codition II of the ANS Classification. The results are compared with the design criteria described in the Final Safety Analysis Report and a discrepancy between these two values is discussed herein.

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In-pile Test Results of HANA Claddings in Halden Research Reactor

  • Baek, Jong-Hyuk;Choi, Byoung-Kwon;Jeong, Yong-Hwan;Jung, Yun-Ho;Kim, Kyu-Tae
    • Proceedings of the Korean Nuclear Society Conference
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    • 2005.05a
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    • pp.425-426
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    • 2005
  • 1. The oxide thickness on the fuelled test rods was within the following range from 7 ${\mu}m$ to 17 ${\mu}m$. In general, the HANA claddings showed better corrosion behavior than the two reference alloys (A-Cladding and Zr-4). 2. The weight gains of corrosion coupons were ranged from 21 to 56 mg/$dm^2$.

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HIGH BURNUP FUEL TECHNOLOGY IN KOREA

  • Song, Kun-Woo;Jeong, Yong-Hwan;Kim, Keon-Sik;Bang, Je-Geon;Chun, Tae-Hyun;Kim, Hyung-Kyu;Song, Kee-Nam
    • Nuclear Engineering and Technology
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    • v.40 no.1
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    • pp.21-36
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    • 2008
  • High bum-up fuel technology has been developed through a national R&D program, which covers key technology areas such as claddings, $UO_2$ pellets, spacer grids, performance code, and fuel assembly tests. New cladding alloys were developed through alloy designs, tube fabrication, out-of-pile test and in-reactor test. The new Zr-Nb tubes are found to be much better in their corrosion resistance and creep strength than the Zircaloy-4 tube, owing to an optimized composition and heat treatment of the new Zr-Nb alloys. A new fabrication technology for large grain $UO_2$ pellets was developed using various uranium oxide seeds and a micro-doping of Al. The uranium oxide seeds, which were added to $UO_2$ powder, were prepared by oxidizing and heat-treating scrap $UO_2$ pellets. A $UO_2$ pellet containing tungsten channels was fabricated for a thermal conductivity enhancement. For the fuel performance analysis, new high burnup models were developed and implemented in a code. This code was verified by an international database and our own database. The developed spacer grid has two features of contoured contact spring and hybrid mixing vanes. Mechanical and hydraulic tests showed that the spacer grid is superior in its rodsupporting, wear resistance and CHF performance. Finally, fuel assembly test technology was also developed. Facilities for mechanical and thermal hydraulic tests were constructed and are now in operation. Several achievements are to be utilized soon by the Korea Nuclear Fuel and thereby contribute to the economy and safety of PWR fuel in Korea

The Effect of Hydrogen in the Nuclear Fuel Cladding on the Oxidation under High Temperature and High Pressure Steam (고압 수증기하 산화에서 핵연료 피복관내 수소효과 연구)

  • Jung, Yunmock;Jeong, Seonggi;Park, Kwangheon;Noh, Seonho
    • Journal of the Korean institute of surface engineering
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    • v.47 no.1
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    • pp.7-12
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    • 2014
  • The characteristics of oxidation for the Zry-4 was measured in the $800^{\circ}C$ and high steam pressure (50 bar, 75 bar, 100 bar) conditions, using an apparatus for high pressure steam oxidation. The effect of accelerated oxidation by high-pressure steam was increased more than 60% in hydrogen-charged cladding than normal cladding. This difference between hydrogen charged claddings and normal claddings tends to be larger as the higher pressure. The accelerated oxidation effect of hydrogen charging cladding is regarded as the hydrogen on the metal layer affects the formation of the protective oxide layer. The creation of the sound monoclinic phase in Zry-4 oxidation influences reinforcement of corrosion-resistance of the oxide layer. The oxidation is estimated to be accelerated due to the creation of equiaxial type oxide film with lower corrosion resistance than that of columnar type oxide film. When tetragonal oxide film transformed into the monoclinic oxide film, surface energy of the new monoclinic phase reduced by hydrogen in the metal layer.

Destructive Examination of 3 Cycle Burned 14$\times$14 PWR Fuel (삼주기연소 14$\times$14 PWR 핵연료의 핫셀 파괴시험)

  • 이기순;유길성;이영길;민덕기;서항석
    • Nuclear Engineering and Technology
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    • v.21 no.4
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    • pp.332-340
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    • 1989
  • Destructive examination of 14$\times$14 PWR fuel burned for 3 cycles are carried out to investigate the in-reactor fuel performance. The results obtained are as follows; 1) Grain growth is not occured at the fuel center. 2) Fuel density is decreased as the turnup increase, the density is down to 94.4% TD at burnup of 36,000 MWD/MTU. 3) Average thickness of oxide layer on cladding is less than 10 $\mu$m in the lower and middle section, while it is rapidly increased above 20 $\mu$m in the upper section. 4) The rate of hydride production in the cladding is large in the upper section than lower section and is related to the production of oxide on the cladding

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DEVELOPMENT OF PYROPROCESSING AND ITS FUTURE DIRECTION

  • Inoue, Tadashi;Koch, Lothar
    • Nuclear Engineering and Technology
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    • v.40 no.3
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    • pp.183-190
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    • 2008
  • Pyroprocessing is the optimal means of treating spent metal fuels from metal fast fuel reactors and is proposed as a potential option for GNEP in order to meet the requirements of the next generation fuel cycle. Currently, efforts for research and development are being made not only in the U.S., but also in Asian countries. Electrorefining, cathode processing by distillation, injection casting for fuel fabrication, and waste treatment must be verified by the use of genuine materials, and the engineering scale model of each device must be developed for commercial deployment. Pyroprocessing can be effectively extended to treat oxide fuels by applying an electrochemical reduction, for which various kinds of oxides are examined. A typical morphology change was observed following the electrochemical reduction, while the product composition was estimated through the process flow diagram. The products include much stronger radiation emitter than pure typical LWR Pu or weapon-grade Pu. Nevertheless, institutional measures are unavoidable to ensure proliferation-proof plant operations. The safeguard concept of a pyroprocessing plant was compared with that of a PUREX plant. The pyroprocessing is better adapted for a collocation system positioned with some reactors and a single processing facility rather than for a centralized reprocessing unit with a large scale throughput.

ESTIMATION OF ALUMINUM AND ARGON ACTIVATION SOURCES IN THE HANARO COOLANT

  • Jun, Byung-Jin;Lee, Byung-Chul;Kim, Myung-Seop
    • Nuclear Engineering and Technology
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    • v.42 no.4
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    • pp.434-441
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    • 2010
  • The activation products of aluminum and argon are key radionuclides for operational and environmental radiological safety during the normal operation of open-tank-in-pool type research reactors using aluminum-clad fuels. Their activities measured in the primary coolant and pool surface water of HANARO have been consistent. We estimated their sources from the measured activities and then compared these values with their production rates obtained by a core calculation. For each aluminum activation product, an equivalent aluminum thickness (EAT) in which its production rate is identical to its release rate into the coolant is determined. For the argon activation calculation, the saturated argon concentration in the water at the temperature of the pool surface is assumed. The EATs are 5680, 266 and 1.2 nm, respectively, for Na-24, Mg-27 and Al-28, which are much larger than the flight lengths of the respective recoil nuclides. These values coincide with the water solubility levels and with the half-lives. The EAT for Na-24 is similar to the average oxide layer thickness (OLT) of fuel cladding as well; hence, the majority of them in the oxide layer may be released to the coolant. However, while the average OLT clearly increases with the fuel burn-up during an operation cycle, its effect on the pool-top radiation is not distinguishable. The source of Ar-41 is in good agreement with the calculated reaction rate of Ar-40 dissolved in the coolant.

HIGH TEMPERATURE OXIDATION OF NB-CONTAINING ZR ALLOY CLADDING IN LOCA CONDITIONS

  • Chuto, Toshinori;Nagase, Fumihisa;Fuketa, Toyoshi
    • Nuclear Engineering and Technology
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    • v.41 no.2
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    • pp.163-170
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    • 2009
  • In order to evaluate high-temperature oxidation behavior of the advanced alloy cladding under LOCA conditions, isothermal oxidation tests in steam were performed with cladding specimens prepared from high burnup PWR fuel rods that were irradiated up to 79 MWd/kg. Cladding materials were $M5^{(R)}$ and $ZIRLO^{TM}$, which are Nb-containing alloys. Ring-shaped specimens were isothermally oxidized in flowing steam at temperatures from 1173 to 1473 K for the duration between 120 and 4000s. Oxidation rates were evaluated from measured oxide layer thickness and weight gain. A protective effect of the preformed corrosion layer is seen for the shorter time range at the lower temperatures. The influence of pre-hydriding is not significant for the examined range. Alloy composition change generally has small influence on oxidation in the examined temperature range, though $M5^{(R)}$ shows an obviously smaller oxidation constant at 1273 K. Consequently, the oxidation rates of the high burnup $M5^{(R)}$ and $ZIRLO^{TM}$ cladding are comparable or lower than that of unirradiated Zircaloy-4 cladding.