• 제목/요약/키워드: Neutron spectroscopy

검색결과 69건 처리시간 0.022초

Neutron and gamma-ray energy reconstruction for characterization of special nuclear material

  • Clarke, Shaun D.;Hamel, Michael C.;Di fulvio, Angela;Pozzi, Sara A.
    • Nuclear Engineering and Technology
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    • 제49권6호
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    • pp.1354-1357
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    • 2017
  • Characterization of special nuclear material may be performed using energy spectroscopy of either the neutron or gamma-ray emissions from the sample. Gamma-ray spectroscopy can be performed relatively easily using high-resolution semiconductors such as high-purity germanium. Neutron spectroscopy, by contrast, is a complex inverse problem. Here, results are presented for $^{252}Cf$ and PuBe energy spectra unfolded using a single EJ309 organic scintillator; excellent agreement is observed with the reference spectra. Neutron energy spectroscopy is also possible using a two-plane detector array, whereby time-of-flight kinematics can be used. With this system, energy spectra can also be obtained as a function of position. Spatial-dependent energy spectra are presented for neutron and gamma-ray sources that are in excellent agreement with expectations.

Diamond-based neutron scatter camera

  • Alghamdi, Ahmed;Lukosi, Eric
    • Nuclear Engineering and Technology
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    • 제54권4호
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    • pp.1406-1413
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    • 2022
  • In this study, a diamond-based neutron scatter camera (DNSC) was developed for neutron spectroscopy in high flux environments. The DNSC was evaluated experimentally and through simulations. It was simulated using several Monte Carlo codes in a two-array layout. The two-array model included two diamond detectors. The simulation reconstructed the spectra of 252Cf and 239Pu-Be neutron sources with high accuracy (~93%). The two-diamond array system was experimentally evaluated, demonstrating the neutron spectroscopy capabilities of the DNSC. The reconstructed spectrum of the 239Pu-Be source manifested the characteristic peaks of the source. The advantage of a DNSC over a NSC is its ability to define any neutron double-scattering events without the need to absorb incident neutrons in the second detector, and atomic recoil energy information is not needed to determine the incident neutron energy.

Neutron spectroscopy using pure LaCl3 crystal and the dependence of pulse shape discrimination on Ce-doped concentrations

  • Vuong, Phan Quoc;Kim, Hongjoo;Luan, Nguyen Thanh;Kim, Sunghwan
    • Nuclear Engineering and Technology
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    • 제53권11호
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    • pp.3784-3789
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    • 2021
  • We report a simple technique for direct neutron spectroscopy using pure LaCl3 crystals. Pure LaCl3 crystals exhibit considerably better pulse shape discrimination (PSD) capabilities with relatively good energy resolution as compared with Ce-doped LaCl3 crystals. Single crystals of pure and Ce-doped LaCl3 were grown using an inhouse-developed Bridgman furnace. PSD capabilities of these crystals were investigated using 241Am and 137Cs sources. Fast neutron detection was tested using a252Cf source and three separate bands corresponding to electron, proton, and alpha were observed. The proton band induced by the 35Cl(n,p)35S reaction can be used for direct neutron spectroscopy because proton energy is proportional to incident neutron energy. Owing to good scintillation performance and excellent PSD capabilities, pure LaCl3 is a promising candidate for space detectors and other applications that necessitate gamma/fast neutron discrimination capability.

Electrical characteristics and deep-level transient spectroscopy of a fast-neutron-irradiated 4H-SiC Schottky barrier diode

  • Junesic Park;Byung-Gun Park;Hani Baek;Gwang-Min Sun
    • Nuclear Engineering and Technology
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    • 제55권1호
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    • pp.201-208
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    • 2023
  • The dependence of the electrical characteristics on the fast neutron fluence of an epitaxial 4H-SiC Schottky barrier diode (SBD) was investigated. The 30 MeV cyclotron was used for fast neutron irradiation. The neutron fluences evaluated through Monte Carlo simulation were in the 2.7 × 1011 to 1.45 × 1013 neutrons/cm2 range. Current-voltage and capacitance-voltage measurements were performed to characterize the samples by extracting the parameters of the irradiated SBDs. Neutron-induced defects in the epitaxial layer were identified and quantified using a deep-level transient spectroscopy measurement system developed at the Korea Atomic Energy Research Institute. As the neutron fluence increased from 2.7 × 1011 to 1.45 × 1013 neutrons/cm2, the concentration of the Z1/2 defects increased by approximately 20 times. The maximum defect concentration was estimated as 1.5 × 1014 cm-3 at a neutron fluence of 1.45 × 1013 neutrons/cm2.

Structural and component characterization of the B4C neutron conversion layer deposited by magnetron sputtering

  • Jingtao Zhu;Yang Liu;Jianrong Zhou;Zehua Yang;Hangyu Zhu;Xiaojuan Zhou;Jinhao Tan;Mingqi Cui;Zhijia Sun
    • Nuclear Engineering and Technology
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    • 제55권9호
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    • pp.3121-3125
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    • 2023
  • Neutron conversion detectors that use 10B-enriched boron carbide are feasible alternatives to 3He-based detectors. We prepared boron carbide films at micron-scale thickness using direct-current magnetron sputtering. The structural characteristics of natural B4C films, including density, roughness, crystallization, and purity, were analyzed using grazing incidence X-ray reflectivity, X-ray diffraction, X-ray photoelectron spectroscopy, time-of-flight secondary ion mass spectrometry, and scanning electron microscopy. A beam profile test was conducted to verify the practicality of the 10B-enriched B4C neutron conversion layer. A clear profile indicated the high quality of the neutron conversion of the boron carbide layer.

Thermal-annealing behavior of in-core neutron-irradiated epitaxial 4H-SiC

  • Junesic Park ;Byung-Gun Park;Gwang-Min Sun
    • Nuclear Engineering and Technology
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    • 제55권1호
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    • pp.209-214
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    • 2023
  • The effect of thermal annealing on defect recovery of in-core neutron-irradiated 4H-SiC was investigated. Au/SiC Schottky diodes were manufactured using a 4H-SiC epitaxial wafer that was neutron-irradiated at the HANARO research reactor. The electrical characteristics of their epitaxial layers were analyzed under various conditions, including different neutron fluences (1.3 × 1017 and 2.7 × 1017 neutrons/cm2) and annealing times (up to 2 h at 1700 ℃). Capacity-voltage measurements showed high carrier compensation in the neutron-irradiated samples and a recovery tendency that increased with annealing time. The carrier density could be recovered up to 77% of the bare sample. Deep-level-transient spectroscopy revealed intrinsic defects of 4H-SiC with energy levels 0.47 and 0.68 eV below the conduction-band edge, which were significantly increased by in-core neutron irradiation. A previously unknown defect with a high electron-capture cross-section was discovered at 0.36 eV below the conduction-band edge. All defect concentrations decreased with 1700 ℃ annealing; the decrease was faster when the defect level was shallow.

252Cf 선원을 이용한 즉발감마선 계측시스템 구성 (Development of Neutron Induced Prompt γ-ray Spectroscopy System Using 252Cf)

  • 박용준;송병철;지광용
    • 분석과학
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    • 제16권1호
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    • pp.12-24
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    • 2003
  • $^{252}Cf$ 중성자 선원을 이용한 즉발감마선 계측 시스템 (NIPS, Neutron Induced Promp ${\gamma}$-ray Spectroscopy)을 설계 및 구성하기 위하여, 시스템내의 감속제 및 차폐체등의 효과를 시험하고 감마선 바탕값과 Cl을 포함한 시료의 즉발 감마선을 계측하였다. 이를 위한 예비시험으로 한국원자력연구소 내에 있는 TLD 판독용 $^{252}Cf$ 선원을 이용하였으며 즉발감마선은 시스템 내부의 동축형 HPGe (GMX, 60% relative efficiency)과 시스템외부 (약 20m 거리)의 Notebook PC 중성자와 감마선의 바탕값을 측정하고, 바탕값을 최소로 할 수 있는 차폐체의 기하학적 구조를 고안하였다. 감마선 바탕값을 최소화하기 위하여 두 개의 HPGe 검출기를 이용한 감마-감마 동시계측법을 이용하였다. 이 실험 자료를 이용하여 최적의 NIPS 시스템을 구성하였다.

Study in Background Reduction for the Neutron Induced Prompt Gamma-ray Spectroscopy

  • Song, Byoung-Chul;Jee, Kwang-Yong;Park, Yong-Joon
    • 한국방사성폐기물학회:학술대회논문집
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    • 한국방사성폐기물학회 2004년도 학술논문집
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    • pp.433-433
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    • 2004
  • Neutron induced prompt gamma-ray spectroscopy (NIPS) system measures the prompt gamma-ray, emitting by the interaction of a neutron with various materials. This system will be of great benefit to scientists worldwide, since it provides the non-destructive measurement of many elements in either solid or liquid wastes. A NIPS facility has been developed in Nuclear Chemistry Research Division, at Korea Atomic Energy Research Institute (KAERI) with the aim of analyzing the major component elements in both aqueous and solid samples.(omitted)

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Monte Carlo 시물레이션에 기초한 포획모드 중성자-감마 스펙트럼 존데 설계 및 반응 분석 (Neutron Induced Capture Gamma Spectroscopy Sonde Design and Response Analysis Based on Monte Carlo Simulation)

  • 원병호;황세호;신제현;김종만;김기석;박창제
    • 지구물리와물리탐사
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    • 제18권3호
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    • pp.154-161
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    • 2015
  • 본 연구에서는 중성자-감마 스펙트럼검층 존데 설계를 목적으로 Monte Carlo 시물레이션을 이용하여 열중성자 반응의 우세한 영역 파악 및 포획감마 스펙트럼의 에너지피크 값에 기초한 지층 구성 원소 구분을 수행하였다. 14 MeV 에너지준위의 중성자를 방출하는 중성자발생장치를 선원으로 이용하여 선원으로부터 10 cm 간격으로 12개의 중성자 검출기들을 배열함으로써 거리에 따른 열중성자 양을 측정하였다. 시추공 영향 저감을 위해 존데모형에 차폐재를 적용하여 보다 정확한 열중성자 측정을 수행하여 열중성자 반응이 우세한 위치를 분석한 뒤, 이 위치에서 검출된 포획감마 에너지 스펙트럼을 분석하여 지층을 구성하는 주요 원소 및 그 양을 확인하였다. 본 연구 결과는 중성자-감마 스펙트럼검층 존데의 신호대잡음 비 향상과 포획감마 검출기 최적 위치 선정에 도움이 될 것으로 판단된다.