• Title/Summary/Keyword: Gamma-ray Spectroscopy

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A comparative study of machine learning methods for automated identification of radioisotopes using NaI gamma-ray spectra

  • Galib, S.M.;Bhowmik, P.K.;Avachat, A.V.;Lee, H.K.
    • Nuclear Engineering and Technology
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    • v.53 no.12
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    • pp.4072-4079
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    • 2021
  • This article presents a study on the state-of-the-art methods for automated radioactive material detection and identification, using gamma-ray spectra and modern machine learning methods. The recent developments inspired this in deep learning algorithms, and the proposed method provided better performance than the current state-of-the-art models. Machine learning models such as: fully connected, recurrent, convolutional, and gradient boosted decision trees, are applied under a wide variety of testing conditions, and their advantage and disadvantage are discussed. Furthermore, a hybrid model is developed by combining the fully-connected and convolutional neural network, which shows the best performance among the different machine learning models. These improvements are represented by the model's test performance metric (i.e., F1 score) of 93.33% with an improvement of 2%-12% than the state-of-the-art model at various conditions. The experimental results show that fusion of classical neural networks and modern deep learning architecture is a suitable choice for interpreting gamma spectra data where real-time and remote detection is necessary.

Effect of Various Supports on the Physico-chemical Properties of V-Sb Oxides in the Oxidative Dehydrogenation of Isobutane

  • Shamilov, N.T.;Vislovskiy, V.P.
    • Journal of the Korean Chemical Society
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    • v.55 no.5
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    • pp.812-818
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    • 2011
  • [ $V_{0.9}Sb_{0.1}O_x$ ]systems, bulk and deposited on different supports (five types of ${\gamma}$-aluminas, ${\alpha}$-alumina, silica-alumina, silica gel, magnesium oxide), have been tested in the oxidative dehydrogenation (ODH) of iso-butane. This statement is derived from the data obtained by a set of characterisation techniques(specific surface area measurements, X-ray diffraction, X-ray photoelectron spectroscopy, laser Raman spectroscopy, in situ differential scanning calorimetry and in situ diffuse reflectance-absorption infrared Fourier transform spectroscopy).

A Comparative Study of Branching Ratio of 167Yb Radioactive Isotope from Gamma-ray Spectrum Produced by 169Tm(p,3n)167Yb Reaction with 100-MeV Proton Beam (100-MeV 양성자 빔을 이용하여 169Tm(p,3n)167Yb 반응에 의해 생성된 167Yb 방사성동위원소에서 방출되는 감마선 스펙트럼 비교 연구)

  • Sam-Yol, Lee
    • Journal of the Korean Society of Radiology
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    • v.16 no.7
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    • pp.953-960
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    • 2022
  • The measurement of branching ratio of 167Yb radioactive isotopes from gamma-ray spectrum of 169Tm(p,3n)167Yb reaction were performed by using a 100-MeV proton linear accelerator of the Korea Multi-purpose Accelerator Complex (KOMAC). The 167Yb isotope has a half-life of 17.5 minutes and decays to 169Tm. The gamma rays generated from the 167Yb isotope were measured using an HPGe detector gamma ray spectroscopy system. The energy calibration of the detector and the efficiency measurement of the detector were determined using a standard source. The gamma rays of known main energy (62.9, 106.2, 113.3, 143.5 and 176.3 keV) were measured. On the other hand, information about the intensity of the generated gamma rays is very inaccurate. Therefore, in this study, the decay strength of the main gamma rays was accurately measured. Overall, it was different from the previously known results, and in particular, it was found that the intensity of the main decay gamma ray, such as the 113.3 and 106.2 keV gamma ray, was overestimated, and it was found that the gamma ray, such as 62.9, 116.7 and 143.5 keV was underestimated. The present results are considered to be important information in the fields of nuclear fusion, astrophysics and nuclear physics in the future.

Flame Synthesis of Silica-Coated Iron Oxide Nanoparticles and Their Characterization

  • Jun, Kimin;Yang, Sangsun;Lee, Jeonghoon;Pikhitsa, Peter V.;Choi, Mansoo
    • Particle and aerosol research
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    • v.9 no.4
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    • pp.209-219
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    • 2013
  • We have used the modified diffusion flame burner to synthesize silica coated iron oxide nanoparticles having enhanced superparamagnetic property. Silica-encapsulated iron oxide particles were directly observed using a high resolution transmission electron microscope. From the energy dispersive X-ray spectroscopy (EDS) and zeta potential measurements, the iron oxide particles were found to be completely covered by a silica coating layer. X-ray photoelectron spectroscopy (XPS) and X-ray diffraction (XRD) measurements revealed that the iron oxide core consists of ${\gamma}-Fe_2O_3$ rather than ${\alpha}-Fe_2O_3$. Our magnetization measurements support this conclusion. Biocompatibility test of the silica-coated iron oxide nanoparticles is also conducted using the protein adsorption onto the coated particle.

GRB 140304A at z=5.283: Implications on the high redshift universe and the observed flaring activities

  • Jeong, Soomin
    • The Bulletin of The Korean Astronomical Society
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    • v.41 no.1
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    • pp.38.1-38.1
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    • 2016
  • Gamma ray burst, the most brightest explosion phenomena in the current universe is well suited for study of high redshift universe. We report the afterglow multi-wavelength observation and GTC spectroscopy follow up of GRB 140304A which was exploded at z=5.283. The spectrum was shown damped Lyman alpha features and a series of absorption lines S, Si, SiII*, Oi, CII, CII*, SiIV are clearly detected at common redshift. Clear optical flares are detected when X-ray flare happened and a possible gamma-ray excess also. At this conference, we report on implications for the GRB host and environments using its absorption features which place the results in context to other well studied high redshift GRBs and studies about the ejecta using its observed flaring activities.

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Analytical-numerical formula for estimating the characteristics of a cylindrical NaI(Tl) gamma-ray detector with a side-through hole

  • Thabet, Abouzeid A.;Badawi, Mohamed S.
    • Nuclear Engineering and Technology
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    • v.54 no.10
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    • pp.3795-3802
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    • 2022
  • NaI(Tl) scintillation materials are considered to be one of many materials that are used exclusively for γ-ray detection and spectroscopy. The gamma-ray spectrometer is not an easy-to-use device, and the accuracy of the numerical values must be carefully checked based on the rules of the calibration technique. Therefore, accurate information about the detection system and its effectiveness is of greater importance. The purpose of this study is to estimate, using an analytical-numerical formula (ANF), the purely geometric solid angle, geometric efficiency, and total efficiency of a cylindrical NaI(Tl) γ-ray detector with a side-through hole. This type of detector is ideal for scanning fuel rods and pipelines, as well as for performing radio-immunoassays. The study included the calculation of the complex solid angle, in combination with the use of various points like gamma sources, located axially and non-axially inside the through detector side hole, which can be applied in a hypothetical method for calibrating the facility. An extended γ-ray energy range, the detector, source dimensions, "source-to-detector" geometry inside the side-through hole, path lengths of γ-quanta photons crossing the facility, besides the photon average path length inside the detector medium itself, were studied and considered. This study is very important for an expanded future article where the radioactive point source can be replaced by a volume source located inside the side-trough hole of the detector, or by a radioactive pipeline passing through the well. The results provide a good and useful approach to a new generation of detectors that can be used for low-level radiation that needs to be measured efficiently.

Effect of ${\gamma}$-Ray Irradiation on Surface Oxidation of Ultra High Molecular Weight Polyethylene/Zirconia Composite Prepared by in situ Ziegler-Natta Polymerization

  • Kwak, Soon-Jong;Noh, Dong-Il;Chun, Heung-Jae;Lim, Youn-Mook;Nho, Young-Chang;Jang, Ju-Woong;Shim, Young-Bock
    • Macromolecular Research
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    • v.17 no.8
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    • pp.603-608
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    • 2009
  • Novel ultra-high molecular weight polyethylene (UHMWPE)/zirconia composites were previously prepared by the in situ polymerization of ethylene using a Ti-based Ziegler-Natta catalyst supported on to the surface of zirconia, as a bearing material for artificial joints. Tribological tests revealed that a uniform dispersion of zirconia in UHMWPE markedly increased the wear resistance. The effects of zirconia content on the oxidation behavior of the ${\gamma}$-ray-treated UHMWPE/zirconia composite surfaces were examined. The oxidation index that estimates the oxidation degree as the content of total carbonyl compounds was monitored using Fourier transform infrared spectroscopy-attenuated total reflectance. The changes in the surface composition due to the oxidation were confirmed by electron spectroscopy for chemical analysis. The extent of oxidation decreased with increasing zirconia content, which was attributed to the increased crystallinity as well as the decreased polymer portion of the UHMWPE/zirconia composites.

Detection of voluminous gamma-ray source with a collimation beam geometry and comparison with peak efficiency calculations of EXVol

  • Kang, M.Y.;Sun, G.M.;Choi, H.D.
    • Nuclear Engineering and Technology
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    • v.52 no.11
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    • pp.2601-2606
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    • 2020
  • In this study, we expanded the performance of the existing EXVol code and performed empirical experiments and calculations. A high-resolution gamma spectroscopy system was constructed, and a standard point source and a standard volume source were measured with an HPGe detector with 43.1% relative efficiency. EXVol was verified by quantitative comparison of the detection efficiencies determined by measurements and calculations. To introduce the concept of the detector scanning that occurs in the actual measurement into the EXVol code, a collimator was placed between the source and detector. The detection efficiency was determined in the asymmetric arrangement of the source and detector with a collimator. A collimator made of lead with a diameter of 15 mm and a thickness of 50 mm was installed between the source and the detector to determine the detection efficiency at a specific location. The calculation result was contour plotted so that the distribution of detection efficiency could be visually confirmed. The relative deviation between the measurements and calculations for the coaxial and asymmetric structures was 10%, and that for the collimation structure was 20%. The results of this study can be applied to research using γ-ray measurements.

Diagnostics of Diffuse Two-Phase Matter Using Techniques of Positron Annihilation Spectroscopy in Gamma-Ray and Optical Spectra

  • Doikov, Dmytry;Yushchenko, Alexander;Jeong, Yeuncheol
    • Journal of Astronomy and Space Sciences
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    • v.36 no.3
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    • pp.115-119
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    • 2019
  • This paper is a part of the series on positron annihilation spectroscopy of two-phase diffuse gas-and-dust aggregates, such as interstellar medium and the young remnants of type II supernovae. The results obtained from prior studies were applied here to detect the relationship between the processes of the annihilation of the K-shell electrons and incident positrons, and the effects of these processes on the optical spectra of their respective atoms. Particular attention was paid to the Doppler broadening of their optical lines. The relationship between the atomic mass of the elements and the Doppler broadening, ${\Delta}{\lambda}_D$ (${\AA}$), of their emission lines as produced in these processes was established. This relationship is also illustrated for isotope sets of light elements, namely $^3_2He$, $^6_3Li$, $^7_3Be$, $^{10}_5B$ and $^{11}_5B$. A direct correlation between the ${\gamma}-line$ luminosity ( $E_{\gamma}=1.022MeV$) and ${\Delta}{\lambda}_D$ (${\AA}$) was proved virtually. Qualitative estimates of the structure of such lines depending on the positron velocity distribution function, f(E), were made. The results are presented in tabular form and can be used to set up the objectives of further studies on active galactic nuclei and young remnants of type II supernovae.

Fixation of $\gamma$-Radionuclides by the PVA-PMAA System

  • Won, Hui-Jun;Ahn, Byung-Gil;Jung, Chong-Hun;Kim, Gye-Nam;Oh, Won-Zin
    • Nuclear Engineering and Technology
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    • v.32 no.3
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    • pp.205-213
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    • 2000
  • A series of laboratory experiments was conducted to investigate the fixation characteristics of poly(vinylalcohol)-poly(methacrylic acid)(PVA-PMAA) mixed solution on the soluble ${\gamma}$- radionuclides. Using the potentiometric titration technique, it was found out that the PVA and PMAA in a solution form intermacromolecular complex. The mobilized portion of each radionuclide by water from sand surface treated with a fixative was measured by ${\gamma}$-ray spectroscopy. The mobilized portion of minor radionuclides such as 241Am, 154Eu, 155Eu and 144Ce were higher than those of 134Cs and 137Cs. The capability of PVA-PMAA system was better among the candidate solutions for the fixation of total ${\gamma}$-radioactivity. 134,137Cs which is composed of more than 85 % of total ${\gamma}$-radioactivity could be fixed effectively by the PVA-PMAA solution.

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