• Title/Summary/Keyword: Burnup

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On the intra-granular behaviour of a cocktail of inert gases in oxide nuclear fuel: Methodological recommendation for accelerated experimental investigation

  • Romano, M.;Pizzocri, D.;Luzzi, L.
    • Nuclear Engineering and Technology
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    • v.54 no.5
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    • pp.1929-1934
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    • 2022
  • Besides recent progresses in the physics-based modelling of fission gas and helium behaviour, the scarcity of experimental data concerning their combined behaviour (i.e., cocktail) hinders further model developments. For this reason, in this work, we propose a modelling methodology aimed at providing recommendations for accelerated experimental investigations. By exploring a wide range of annealing temperatures and cocktail compositions with a physics-based modelling approach we identify the most interesting conditions to be targeted by future experiments. To corroborate the recommendations arising from the proposed methodology, we include a sensitivity analysis quantifying the impact of the model parameters on fission gas and helium release, in conditions representative of high and low burnup.

Novel homogeneous burnable poisons in pressurized water reactor ceramic fuel

  • Dodd, Brandon;Britt, Taylor;Lloyd, Cody;Shah, Manit;Goddard, Braden
    • Nuclear Engineering and Technology
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    • v.52 no.12
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    • pp.2874-2879
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    • 2020
  • Due to excess reactivity, fresh nuclear fuel often contains burnable poisons. This research looks at six different burnable poisons and their impacts on reactivity, material attractiveness, and waste management. An MCNP simulation of a PWR fuel pin was performed with a fuel burnup of 60 GWd/MTHM to determine when each burnable poison fuel type would decrease below a k of 1. For determining the plutonium material attractiveness in each burnable poison fuel type, the plutonium isotopic content of the used fuel was evaluated using Bathke's Figure of Merit formula. For the waste management analysis, the thermal output of each burnable poison fuel type was determined through ORIGEN decay simulations at 100 and 300 years after being discharged from the core. The performance of all six burnable poisons varied over the three criteria considered and no single burnable poison performed best in all three considerations.

Spent fuel characterization analysis using various nuclear data libraries

  • Calic, Dusan;Kromar, Marjan
    • Nuclear Engineering and Technology
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    • v.54 no.9
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    • pp.3260-3271
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    • 2022
  • Experience shows that the solution to waste management in any national programme is lengthy and burdened with uncertainties. There are several uncertainties that contribute to the costs associated with spent fuel management. In this work, we have analysed the impact of the current nuclear data on the isotopic composition of the spent fuel and consequently their influence on the main spent fuel observables such as decay heat, activity, neutron multiplication factor, and neutron and photon source terms. Nuclear libraries based on the most general nuclear data ENDF/B-VII.0, ENDF/B-VII.1, ENDF/B-VIII.0 and JEFF-3.3 are considered. A typical NPP Krško fuel assembly is analysed using the Monte Carlo code Serpent 2. The analysis considers burnup of up to 60 GWd/tU and cooling times of up to 100 years. The comparison of results showed significant differences, which should be taken into account when selecting the library and evaluating the uncertainty in determining the characteristics of the spent fuel.

Analyses on the recriticality and sub-critical boron concentrations during late phase of a severe accident of pressurized water reactors

  • Yoonhee Lee;Yong Jin Cho;Kukhee Lim
    • Nuclear Engineering and Technology
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    • v.55 no.9
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    • pp.3241-3251
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    • 2023
  • The potential for recriticality and sub-critical boron concentrations is analyzed during the relocation of the fuel rods in the assembly, which we call late phase of a severe accident, via coupling between MELCOR and whole-core Monte Carlo analyses by Serpent 2. The recriticality, initiated during the early phase, is found to maintain when the fuel assemblies containing intact fuel rods are submerged by the cooling water. It is also found that the effect of the negative reactivity insertion via remaining fission products in the fuel debris increases as the burnup increases. The sub-critical boron concentrations during the late phase are found to be 76~544 ppm lower than those during the early phase. Therefore, it can be concluded that the boron concentration that prevents recriticality not only during the early phase but also during the late phase is the sub-critical boron concentration during the early phase.

Real variance estimation in iDTMC-based depletion analysis

  • Inyup Kim;Yonghee Kim
    • Nuclear Engineering and Technology
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    • v.55 no.11
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    • pp.4228-4237
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    • 2023
  • The Improved Deterministic Truncation of Monte Carlo (iDTMC) is a powerful acceleration and variance reduction scheme in the Monte Carlo analysis. The concept of the iDTMC method and correlated sampling-based real variance estimation are briefly introduced. Moreover, the application of the iterative scheme to the correlated sampling is discussed. The iDTMC method is utilized in a 3-dimensional small modular reactor (SMR) model problem. The real variances of burnup-dependent criticality and power distribution are evaluated and compared with the ones obtained from 30 independent iDTMC calculations. The impact of the inactive cycles on the correlated sampling is also evaluated to investigate the consistency of the correlated sample scheme. In addition, numerical performances and sensitivity analysis on the real variance estimation are performed in view of the figure of merit of the iDTMC method. The numerical results show that the correlated sampling accurately estimates the real variances with high computational efficiencies.

A Study on Radiation Safety Evaluation for Spent Fuel Transportation Cask (사용후핵연료 운반용기 방사선적 안전성평가에 관한 연구)

  • Choi, Young-Hwan;Ko, Jae-Hun;Lee, Dong-Gyu;Jung, In-Su
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.17 no.4
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    • pp.375-387
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    • 2019
  • In this study, the radiation dose rates for the design basis fuel of 360 assemblies CANDU spent nuclear fuel transportation cask were evaluated, by measuring radiation source terms for the design basis fuel of a pressurized heavy water reactor. Additionally, radiological safety evaluation was carried out and the validity of the results was determined by radiological technical standards. To select the design basis fuel, which was the radiation source term for the spent fuel transportation cask, the design basis fuels from two spent fuel storage facilities were stored in a spent fuel transportation cask operating in Wolsung NPP. The design basis fuel for each transportation and storage system was based on the burnup of spent fuel, minimum cooling period, and time of transportation to the intermediate storage facility. A burnup of 7,800 MWD/MTU and a minimum cooling period of 6 years were set as the design basis fuel. The radiation source terms of the design basis fuel were evaluated using the ORIGEN-ARP computer module of SCALE computer code. The radiation shielding of the cask was evaluated using the MCNP6 computer code. In addition, the evaluation of the radiation dose rate outside the transport cask required by the technical standard was classified into normal and accident conditions. Thus, the maximum radiation dose rates calculated at the surface of the cask and at a point 2 m from the surface of the cask under normal transportation conditions were respectively 0.330 mSv·h-1 and 0.065 mSv·h-1. The maximum radiation dose rate 1 m from the surface of the cask under accident conditions was calculated as 0.321 mSv·h-1. Thus, it was confirmed that the spent fuel cask of the large capacity heavy water reactor had secured the radiation safety.

Investigation on the Allowable Transient Power Levels to Maintain the Mechanical Integrity of the 17$\times$17 KOFA Fuel Rod During the ANS Conditions I and II (ANS과도조건 I 및 II에서 17x17 KOFA 핵연료봉의 기계적 건전성이 유지되는 과도상태 허용 출력준위에 관한 연구)

  • Lee, Chan-Bock;Kim, Ki-Hang;Kim, Kyu-Tae
    • Nuclear Engineering and Technology
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    • v.26 no.1
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    • pp.119-125
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    • 1994
  • Transient power level of the fuel rod is one of the key parameters for the transient fuel behavior. Through the analysis of the fuel performance data bases and sensitivity analyses of such parameters as rod power history, fast neutron flux, fuel enrichment and cycle length, which can affect the transient fuel behavior, a methodology generally applicable to find the allowable transient power level during the ANS Conditions I and II below which the mechanical integrity of the fuel rod is maintained was derived, and allowable transient power levels for the 17$\times$17 KOFA fuel rod have been determined as a function of the burnup. With the introduction of this methodology, design analysis of the transient fuel behavior currently being calculated every cycle can be replaced by the simple check of the peak transient power level achievable during the cycle, and an operational flexibility of the reactor can be obtained by allowing higher transient power level up to 689.5 w/cm at low burnup range than current maximum allowable transient power level, 591 w/cm for the 17$\times$17 KOFA fuel.

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The Evaluation of Minimum Cooling Period for Loading of PWR Spent Nuclear Fuel of a Dual Purpose Metal Cask (국내 경수로 사용후핵연료의 금속 겸용용기 장전을 위한 최소 냉각기간 평가)

  • Dho, Ho-Seog;Kim, Tae-Man;Cho, Chun-Hyung
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.14 no.4
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    • pp.411-422
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    • 2016
  • Recently, because the wet pool storage facilities of NPPs in Korea has become saturated, there has been much active R&D on an interim dry storage system using a transportation and storage cask. Generally, the shielding evaluation for the design of a spent fuel transportation and storage cask is performed by the design basis fuel, which selects the most conservative fuel among the fuels to be loaded into the cask. However, the loading of actual spent fuel into the transportation metal cask is not limited to the design basis fuel used in the shielding evaluation; the loading feasibility of actual spent fuel is determined by the shielding evaluation that considers the characteristics of the initial enrichment, the maximum burnup and the minimum cooling period. This study describes a shielding analysis method for determining the minimum cooling period of spent fuel that meets the domestic transportation standard of the dual purpose metal cask. In particular, the spent fuel of 3.0~4.5wt% initial enrichment, which has a large amount of release, was evaluated by segmented shielding calculations for efficient improvement of the results. The shielding evaluation revealed that about 81% of generated spent fuel from the domestic nuclear power plants until 2008 could be transported by the dual purpose metal cask. The results of this study will be helpful in establishing a technical basis for developing operating procedures for transportation of the dual purpose metal cask.

Oxidation Behavior of $UO_2$ in Air ($UO_2$ 의 공기중 산화거동)

  • You, Gil-Sung;Kim, Keon-Sik;Min, Duck-Kee;Ro, Seung-Gy;Kim, Eun-Ka
    • Nuclear Engineering and Technology
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    • v.27 no.1
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    • pp.67-73
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    • 1995
  • To investigate the storage behavior of the defective LWR spent fuel, air-oxidation tests on non-irradiated and irradiated U $O_2$ were performed. The weight gains of non-irradiated U $O_2$ specimens are characterized by the S-shape curves at 250-40$0^{\circ}C$ temperature range. One hundred percent conversion of U $O_2$ to U$_3$ $O_{8}$ corresponds with about 4% weight increase. The activation energies are 110 kJ/mol above 35$0^{\circ}C$ and 153 kJ/mol below 35$0^{\circ}C$. The irradiated U $O_2$ specimens with about 35 GWD/MTU burnup were oxidized at 300-40$0^{\circ}C$ in air. They show a rapid increase of weight gain at the initial stage and a slow increase at the later stage when compared with non-irradiated U $O_2$. The activation energy under these conditions is 95 kJ/mol. Burnup and aging effects of irradiated U $O_2$ were also investigated at 35$0^{\circ}C$ in air environment, but the specimens appears insensitive to these variables.s.

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Current Status and Characterization of CANDU Spent Fuel for Geological Disposal System Design (심지층 처분시스템 설계를 위한 중수로 사용후핵연료 현황 및 선원항 분석)

  • Cho, Dong-Keun;Lee, Seung-Woo;Cha, Jeong-Hun;Choi, Jong-Won;Lee, Yang;Choi, Heui-Joo
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.6 no.2
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    • pp.155-162
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    • 2008
  • Inventories to be disposed of, reference turnup, and source terms for CANDU spent fuel were evaluated for geological disposal system design. The historical and projected inventory by 2040 is expected to be 14,600 MtU under the condition of 30-year lifetime for unit 1 and 40-year lifetime for other units in Wolsong site. As a result of statistical analysis for discharge burnup of the spent fuels generated by 2007, average and stand deviation revealed 6,987 MWD/MtU and 1,167, respectively. From this result, the reference burnup was determined as 8,100 MWD/MtU which covers 84% of spent fuels in total. Source terms such as nuclide concentration for a long-term safety analysis, decay heat, thermo-mechanical analysis, and radiation intenity and spectrum was characterized by using ORIGEN-ARP containing conservativeness in the aspect of decay heat up to several thousand years. The results from this study will be useful for the design of storage and disposal facilities.

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