• Title/Summary/Keyword: 중성자 측정

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하나로를 이용한 근접치료용 Ir-192 Seed의 제조

  • 조운갑;한현수;박울재;이영구;전상수
    • Proceedings of the Korean Nuclear Society Conference
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    • 1997.05b
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    • pp.373-378
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    • 1997
  • 시험가동중인 다목적연구용 '하나로'를 이용하여 근접치료용으로 사용되는 $^{192}$ IR seed 제조실험을 하였다. '하나로'의 특성을 고려하여 제작된 조사표적용기에 표적용 Ir seed를 넣고 밀봉한 후 He 누출시험을 통과한 표적만 원자로의 HTS 조사공에서 중성자 조사시켰다. HTS 조사공의 평균 열중성자속은 측정결과 원자로출력 15 MWt일 때 2.54 $\times$ $10^{13}$ n/$\textrm{cm}^2$.sec였다. 5회에 걸쳐 5개의 조사표적을 사용하여 총 200개의 $^{192}$ Ir seed를 제조, 실험하였으며 2시간 조사후 14일간 냉각시킨 Ir seed의 r-ray spectrum을 분석한 결과 $^{l92}$Ir외의 불순핵종은 검출되지 않았다. Ir seed의 방사능은 이온전리함을 사용하여 측정하였으며 방사능 측정결과 개별 $^{192}$ Ir seed의 방사능값은 평균 방사능값으로부터 $\pm$5 % 이내오차의 방사능 균일도를 갖는 것이 확인되었다.차의 방사능 균일도를 갖는 것이 확인되었다.

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Preliminary Study for Imaging of Therapy Region from Boron Neutron Capture Therapy (붕소 중성자 포획 치료에서 치료 영역 영상화를 위한 예비 연구)

  • Jung, Joo-Young;Yoon, Do-Kun;Han, Seong-Min;Jang, HongSeok;Suh, Tae Suk
    • Progress in Medical Physics
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    • v.25 no.3
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    • pp.151-156
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    • 2014
  • The purpose of this study was to confirm the feasibility of imaging of therapy region from the boron neutron capture therapy (BNCT) using the measurement of the prompt gamma ray depending on the neutron flux. Through the Monte Carlo simulation, we performed the verification of physical phenomena from the BNCT; (1) the effects of neutron according to the existence of boron uptake region (BUR), (2) the internal and external measurement of prompt gamma ray dose, (3) the energy spectrum by the prompt gamma ray. All simulation results were deducted using the Monte Carlo n-particle extended (MCNPX, Ver.2.6.0, Los Alamos National Laboratory, Los Alamos, NM, USA) simulation tool. The virtual water phantom, thermal neutron source, and BURs were simulated using the MCNPX. The energy of the thermal neutron source was defined as below 1 eV with 2,000,000 n/sec flux. The prompt gamma ray was measured with the direction of beam path in the water phantom. The detector material was defined as the lutetium-yttrium oxyorthosilicate (Lu0,6Y1,4Si0,5:Ce; LYSO) scintillator with lead shielding for the collimation. The BUR's height was 5 cm with the 28 frames (bin: 0.18 cm) for the dose calculation. The neutron flux was decreased dramatically at the shallow region of BUR. In addition, the dose of prompt gamma ray was confirmed at the 9 cm depth from water surface, which is the start point of the BUR. In the energy spectrum, the prompt gamma ray peak of the 478 keV was appeared clearly with full width at half maximum (FWHM) of the 41 keV (energy resolution: 8.5%). In conclusion, the therapy region can be monitored by the gamma camera and single photon emission computed tomography (SPECT) using the measurement of the prompt gamma ray during the BNCT.

경.중수로 연계 핵연료 주기 (DUPIC)관련 핵물질 보장조치 (Safeguards)

  • 나원우;이용덕;차홍렬;김호동;홍종숙;박현수
    • Nuclear Engineering and Technology
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    • v.27 no.3
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    • pp.447-452
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    • 1995
  • 경·중수로 연계 핵연료 주기 (Direct Use of Spent PWR Fuel in CANDU : DUPIC ) 기술개발의 핵물질 보장조치(Safeguards)는 경수로 사용후 핵연료를 중수로에 재 활용하기 위한 DUPIC 공정에 대한 최적 보장조치 시스템을 구축하여, 국제 원자력 기구(IAEA) 및 국제 원자력 사회에서 핵 투명성확보 및 신뢰도를 향상시키는 것을 기술개발의 목적으로 하고 있다. DUPIC 공정은 고립된 차폐시설내의 고준위 방사선장 하에서 가동되므로 타 시설에 비해 핵 물질 전용 가능성은 희박하지만, 전 공정이 원격제어 되야 하고, 조업조건이 정복해야 하므로 기존의 보장조치 기술보다 더욱 발전된 계량관리시스템, 측정시스템 및 감시시스템 등을 개발하여야 한다. 이를 위해 본 연구에서는 각 항목에 대한 요소 분석 및 각 항목별 향후 연구방향에 대해 분석하였다. DUPIC 공정 전반에 대한 핵물질 계량관리를 위해 물질수지구역 (Material Balance Area : MBA) 및 주요측정 지점 (Key Measurement Point : KMP )을 설정하여 각 측정지점별 측정방법 및 재고검증(Inventory Verification) 방법을 분석하였다. 최적 측정시스템을 개발하기 위해 적용 가능한 비파괴분석 방법들을 분석한 결과, 핵분열성 물질 함량을 정량적으로 측정할 수 있는 수동적 중성자 측정법이 가장 적합하다는 결론을 얻었다. 또한, 감시시스템을 개발하기 위해 전용전략의 주요 요소 및 전용경로 등을 분석하였으며, 핵물질 및 시설에 대한 물리적 방호체제를 DUPIC시설에 적용하기 위하여 물리적 방호에 필요한 방호체제 요소를 분석하여 DUPIC 시설을 위한 가상적인 방호체제를 구축하였다.

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The Rietveld Structure Refinement of Natural Phlogopite Using Neutron Powder Diffraction (중성자분말회절법을 이용한 금운모 결정에 대한 리트벨트 구조분석)

  • 이철규;송윤구;전철민;김신애;성기훈
    • Journal of the Mineralogical Society of Korea
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    • v.16 no.3
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    • pp.215-222
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    • 2003
  • The Rietveld structure refinement for the natural trioctahedral mica, phlogopite-1M (Parker Mine, Quebec, Canada) has been done by high resolution neutron powder diffraction at $25^{\circ}C$ and -263$^{\circ}C$. The structural formula of phlogopite determined by electron probe microanalysis is $K_2$(M $g_{4.46}$F $e_{0.83}$A $l_{0.34}$ $Ti_{0.22}$)(S $i_{5.51}$A $l_{2.49}$) $O_{20}$(O $H_{3.59}$ $F_{0.41}$). Cell parameters are a=5.30∼5.31 $\AA$, b=9.18∼9.20 $\AA$, c=10.18∼10.21 $\AA$, $\beta$=100.06∼100.08$^{\circ}$. Refinements converged to R values in the range of $R_{p}$=2.35%, $R_{wp}$=3.01%, respectively. In this study, the OH bond length is calculated to 0.93 $\AA$ at room temperature and 1.03 $\AA$ at -263$^{\circ}C$, and the angles between OH vector and (001) plane are obtained 93.4$^{\circ}$∼93.6$^{\circ}$. The decrease in the length of OH with the increase in temperature should be due to the hydrogen bonding in the structure of phogopite.e.e.f phogopite.e.e.

The Thermal and Mechanical Properties of Epoxy Composites Including Boron Carbide Surface Treated with Iron Oxide and Tungsten (철산화물과 텅스텐으로 표면 처리된 보론카바이드를 포함하는 에폭시 조성물의 열적·기계적 물성)

  • Kim, Taehee;Lee, Wonjoo;Seo, Bongkuk;Lim, Choong-Sun
    • Journal of Adhesion and Interface
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    • v.19 no.3
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    • pp.113-117
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    • 2018
  • Boron carbide is lower in hardness than diamond or boron nitride but has a hardness of more than 30 GPa and is used for manufacturing tank armors and ammo shells due to its high hardness. It is also used as a neutron absorber due to its ability to absorb neutrons, which is increasing its use in nuclear power projects. Neutrons have no interaction with electrons and are known to pass through the material without interactions. Along with boron carbide, the atoms with high interaction with neutrons are hydrogen, and high hydrogen concentration polyesters and epoxy polymers including boron are used as materials for manufacturing products for nuclear power generation waste. In this paper, the surface of boron carbide is treated with iron oxide and tungsten to improve interaction between modified boron carbide and epoxy polymer. XRD and XPS were used to confirm that iron oxide and tungsten are well attached on the surface of boron carbide, respectively. The mechanical strength of the surface treated boron carbide was measured by a universal testing machine (UTM) and the dynamic characteristics of the cured product were observed by using a dynamic analyzer (DMA).

Development of Sample Environment at High Temperature for the four Circle Diffractometer at HANARO: Structural Study of $LiTaO_3$ at Room and High Temperatures (하나로 4축 단결정 회절장치용 고온시료환경장치의 개발: $LiTaO_3$의 상온 및 고온 구조 연구)

  • 김신애;성기훈;이창희
    • Journal of the Mineralogical Society of Korea
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    • v.15 no.2
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    • pp.140-144
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    • 2002
  • The sample environment at high temperature for the four circle diffractometer at HANARO in Korea Atomic Energy Research Institute is developed. The performance test was carried out for a structurally known sample through the high temperature experiment with this equipment. In this study we found out that the developed sample environment is stable for a long time experiment at over 900 K. By the neutron diffraction from a single crystal of $LiTaO_3$(phase transition temperature about 900 K) at 298 and 913 K, the lithium atomic positions at both temperatures and disordered state of lithium atom at high temperature were confirmed. These are hardly possible to determine by the conventional X-ray diffraction method.

단순 노외계측기 교정법

  • 하창주;정선교;성기봉;우해석;이상희;박현택;조희봉;박재원;윤준구
    • Proceedings of the Korean Nuclear Society Conference
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    • 1996.05a
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    • pp.433-439
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    • 1996
  • 노심 외각에 설치되어 노심 외각으로 누설되는 중성자를 검출하여 노심내의 출력 변화를 지시해 주는 노외계측기(Excore Detector)는 운전중 노심의 변화를 정확히 감지하도록 정기적으로 교정되어져야 한다. 노외계측기는 노내계측기(Incore Detector)를 통하여 측정되어진 축방향 출력편차(Axial Offset)를 이용하여 교정하고 있다. 기존의 방법은 노내계측기로 최소한 4회 노심 출력을 측정하여 최소자승법(Least Square Method)으로 상수들을 구한후 노외계측기를 교정한다. 여기서 소개되는 단순 노외계측기 교정법은 노내계측기로 2회 측정되어진 자료들을 이용하는 2점 교정법과 1회 측정되어진 자료들을 이용하는 1점 교정법으로, 계측기 반응상수(Detector Response Factor)를 계산한후 교정되어진 노외계측기의 출력편차를 측정값과 비교하였다. 위의 두가지 방법을 고리 3호기 9주기, 10주기에 적용하여 노심 운전영역(~$\pm$10%)에서 2점 교정법은 최대 1.40 %, 1점 교정법은 최대 0.63 %의 오차를 보여주고 있다. 단순 노외계측기 교정법은 노심출력을 1회 또는 2회 측정하므로 교정시간을 줄이고 제어봉의 사용을 억제하여 방사성 폐기물을 감소시키는 효과와 기존의 교정 방법과 같은 정확성을 기대할수 있다.

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Experimental Study on the Determination of Absorbed dose Index (흡수선량지수결정(吸收線量指數決定)에 관한 실험적(實驗的) 연구(硏究))

  • Jun, Jae-Shik;Rho, Chae-Shik;Ro, Seung-Gy;Ha, Chung-Woo;Yoo, Young-Soo;Lee, Hyun-Duk
    • Journal of Radiation Protection and Research
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    • v.7 no.1
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    • pp.34-48
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    • 1982
  • The prime purpose of this study is to realize an index quantity, absorbed dose index, defined by the ICRU for the characterization of ambient radiation level at any location for the purpose of radiation protection. The experiment has been designed to be carried out in two phases, namely, preliminary and main experiment. In the primary study a 30cm diameter sphere of polyethylene was used, while in the main experiment that of tissue equivalent material was fabricated and used. Both experiments were performed in the gamma-ray fields of $^{137}Cs\;and\;^{60}Co$, and in a neutron beam of thermal column of the TRIGA MARK-II research reactor. In the measurement of gamma-ray absorbed dose TLD-700 $(^{7}LiF)$ chips were used, and for the neutron dose both Au activation foils and TLD chips (TLD-600 $(^{6}LiF)$ and TLD-700 for the discrimination of gamma-ray contribution) were used. Theoretical assessment of the absorbed dose in the sphere phantom has been carried out in accordance with the Ehrlich's idea that deduced on the basis of Burlin's cavity theory in the case of gamma-ray irradiation. For the analysis of neutron dose fluence-KERMA rate conversion method was used. The explanation on the dose assessment is given in detail. Results obtained were numerically and statistically analyzed and the depth dose distributions are presented in the graphic forms with normalized values. In the concluding remarks, the possibility and difficulty of realizing the index quantity, including questions and problems to be solved are mentioned.

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Determination of Trace Elements in $PM_{2.5}/PM_{10}$ of Dsejeon Region using Neutron Activation Analysis(IV) (중성자 방사화분석에 의한 대전지역의 $PM_{2.5}/PM_{10}$ 농도 밀 미량원소의 측정(IV))

  • 문종화;김선하;임종명;정용삼
    • Proceedings of the Korea Air Pollution Research Association Conference
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    • 2003.05b
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    • pp.259-260
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    • 2003
  • 대기환경에 대한 정보의 파악은 환경연구의 기본이 된다. 유해원소 및 미량원소에 의한 환경오염과 그로 인한 인체건강에 대한 영향은 인간생활에 심각한 문제가 되므로 대기, 수질, 토양등의 환경시료 중의 농도를 정확히 측정하는 것은 매우 중요한 일이다. 중성자방사화분석법은 핵반응을 통해 생성시킨 방사성동위원소로부터 방출되는 방사선을 검색하여 절대적으로 성분원소를 정량하는 핵분석기술(Nuclear Analytical Techniques)중의 하나로서 소량의 시료로부터 미소량원소의 비파괴, 동시다원소분석이 가능하고 분석감도($10^{-3}$ - $10^{-7}$$\mu\textrm{g}$)가 탁월한 분석기술이다. (중략)

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A Study of Boron Determination in High Purity Aluminum by Capture Gamma-Ray Measurement (즉발감마선 계측에 의한 고순도 알루미늄중의 붕소정량에 관한 연구)

  • Nak Bae Kim;Hae-Ill Bak
    • Nuclear Engineering and Technology
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    • v.13 no.4
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    • pp.229-236
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    • 1981
  • The boron content in reactor grade aluminum has been determined by means of a capture gamma-ray counting method. The experimental detection limit is found to be 5.7% ppm with 10% uncertainty. In order to improve the sensitivity, the boron is preconcentrated from aluminum by cation exchange resin system. The accuracies of both methods, i.e., one by the direct measurement and the other by the measurement after preconcentration, are checked by an additive method. The results show good agreements with less than 5% deviation.

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