Korean Journal of Materials Research (한국재료학회지)

Materials Research Society of Korea (한국재료학회)
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Preparation and Electrochemical Characterization of Nitrogen-Doped Porous Carbon Textile from Waste Cotton T-Shirt for Supercapacitors

슈퍼커패시터용 폐면 티셔츠로부터 질소 도핑된 다공성 탄소 직물의 제조 및 전기화학 특성 평가

  • Chang, Hyeong-Seok (Department of Polymer Science and Engineering, Chungnam National University) ;
  • Hwang, Ahreum (Department of Polymer Science and Engineering, Chungnam National University) ;
  • Lee, Byoung-Min (Department of Polymer Science and Engineering, Chungnam National University) ;
  • Yun, Je Moon (Division of Advanced Materials Engineering, Dong-Eui University) ;
  • Choi, Jae-Hak (Department of Polymer Science and Engineering, Chungnam National University)
  • 장형석 (충남대학교 고분자공학과) ;
  • 황아름 (충남대학교 고분자공학과) ;
  • 이병민 (충남대학교 고분자공학과) ;
  • 윤제문 (동의대학교 신소재공학부) ;
  • 최재학 (충남대학교 고분자공학과)
  • Received : 2021.07.16
  • Accepted : 2021.08.20
  • Published : 2021.09.27
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Abstract

Hierarchically porous carbon materials with high nitrogen functionalities are extensively studied as high-performance supercapacitor electrode materials. In this study, nitrogen-doped porous carbon textile (N-PCT) with hierarchical pore structures is prepared as an electrode material for supercapacitors from a waste cotton T-shirt (WCT). Porous carbon textile (PCT) is first prepared from WCT by two-step heat treatment of stabilization and carbonization. The PCT is then nitrogen-doped with urea at various concentrations. The obtained N-PCT is found to have multi-modal pore structures with a high specific surface area of 1,299 m2 g-1 and large total pore volume of 1.01 cm3 g-1. The N-PCT-based electrode shows excellent electrochemical performance in a 3-electrode system, such as a specific capacitance of 235 F g-1 at 1 A g-1, excellent cycling stability of 100 % at 5 A g-1 after 1,000 cycles, and a power density of 2,500 W kg-1 at an energy density of 3.593 Wh kg-1. Thus, the prepared N-PCT can be used as an electrode material for supercapacitors.

Keywords

Acknowledgement

This research was supported by Chungnam National University (2020-2021).

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