DOI QR코드

DOI QR Code

Assessment of Exposure to and Risk of Formaldehyde and Particulate Matter (PM10 and PM2.5) by Time Activity Applying Real-Time Indoor and Outdoor Monitoring

실내·외 실시간 모니터링을 활용한 폼알데하이드 및 미세먼지(PM10, PM2.5)의 거주시간별 노출 및 위해도 평가

  • Yoon, Danki (Department of Nano and Biological Engineering, Seokyeong University) ;
  • Namgoung, Sunju (Institute of Risk Assessment, Seokyeong University) ;
  • Kong, Hyekwan (Department of Nano and Biological Engineering, Seokyeong University) ;
  • Hong, Hyungjin (Department of Nano and Biological Engineering, Seokyeong University) ;
  • Lim, Huibeen (Department of Chemical and Biological Engineering, Seokyeong University) ;
  • Park, Sihyun (Institute of Risk Assessment, Seokyeong University) ;
  • Lee, Hyewon (Institute of Risk Assessment, Seokyeong University) ;
  • Lee, Jungsub (Indoor Environment and Noise Research Division, National Institute of Environment Research) ;
  • Lee, Cheolmin (Department of Chemical and Biological Engineering, Seokyeong University)
  • 윤단기 (서경대학교 나노생명공학과) ;
  • 남궁선주 (서경대학교 위해성평가 연구소) ;
  • 공혜관 (서경대학교 나노생명공학과) ;
  • 홍형진 (서경대학교 나노생명공학과) ;
  • 임희빈 (서경대학교 화학생명공학과) ;
  • 박시현 (서경대학교 위해성평가 연구소) ;
  • 이혜원 (서경대학교 위해성평가 연구소) ;
  • 이정섭 (국립환경과학원 환경기반연구부 생활환경연구과) ;
  • 이철민 (서경대학교 화학생명공학과)
  • Received : 2019.11.05
  • Accepted : 2019.11.29
  • Published : 2019.12.31

Abstract

Objectives: The purpose of this study was to suggest methods to investigate continuous monitoring of concentration levels and assess the exposure of individuals considering the actual time activity of residents for formaldehyde and particulate matter (PM10, PM2.5) in the indoor and outdoor air of a house, assess the health risks of children and adults based on the results of the exposure assessment, and provide basic data on studies for assessing exposure and health risks in Korea in the future. Methods: The concentration levels of formaldehyde and particulate matter were measured in a family home in Gyeonggi-do Province from April 25 to July 31, 2019, using electrochemical sensors (formaldehyde) and light scattering sensors (PM10, PM2.5). Risk assessment by the duration of exposure by time activity was performed by dividing between weekdays and weekends, and indoors and outdoors. Results: The greatest level of carcinogenic risk from inhaling formaldehyde was indoors during the weekdays for both children and adults. For children, the risk was at 7.5 per approximately 10,000 people, and for adults, the risk was at 4.1 per approximately 10,000 people. PM10 and PM2.5 also showed the greatest values indoors during the weekdays, with children at 1.7 people and 1.4 per approximately 100 people, respectively, and adults at 8.2 per approximately 1,000 and 1.8 per approximately 100 people, respectively. Conclusions: The risks of formaldehyde, PM10 and PM2.5 were shown to be high indoors. Therefore, consideration of exposure assesment for each indoor pollutant and management of indoor air quality is necessary.

Keywords

References

  1. Cho EM, Jeon HJ, Yoon DK, Park SH, Hong HJ, Choi KY, et al. Reliability of Low-Cost, Sensor-Based Fine Dust Measurement Devices for Monitoring Atmospheric Particulate Matter Concentrations. International journal of environmental research and public health. 2019; 16(8): 1430. https://doi.org/10.3390/ijerph16081430
  2. Kampa M, Castanas E. Human health effects of air pollution. Environmental pollution. 2008; 151(2): 362-367. https://doi.org/10.1016/j.envpol.2007.06.012
  3. Honour SL, Bell JNB, Ashenden TW, Cape JN, Power SA. Responses of herbaceous plants to urban air pollution: effects on growth, phenology and leaf surface characteristics. Environmental pollution. 2009; 157(4): 1279-1286. https://doi.org/10.1016/j.envpol.2008.11.049
  4. Wang Y, Li J, Jing H, Zhang Q, Jiang J, Biswas P. Laboratory evaluation and calibration of three lowcost particle sensors for particulate matter measurement. Aerosol Science and Technology. 2015; 49(11): 1063-1077. https://doi.org/10.1080/02786826.2015.1100710
  5. MoE (Ministry of Environment). Atmosphere Environmental Standard. 2019.
  6. WHO (World Health Organization). Guideline for air quality. 2000.
  7. WHO (World Health Organization). Guidelines for Drinking-Water Quality. 2005.
  8. Kim, JB. Assessment and estimation of particulate matter formation potential and respiratory effects from air emission matters in industrial sectors and cities/regions. Journal of Korean Society of Environmental Engineers. 2017; 39(4): 220-228. https://doi.org/10.4491/KSEE.2017.39.4.220
  9. Park JH, Yang SY, Park YK, Ryu HS, Kim EC, Choe YT, et al. Exposure and Risk Assessment of Benzene and $PM_{10}$ for Sub-populations using Monte-Carlo Simulations. Korean Society of Environmental Health. 2019; 45(3): 247-257.
  10. Graedel TE. Chemical compounds in the Atmosphere, Academic Press Inc, New York, U.S.A. 1978; 161.
  11. Kitchens JF, Casner RE, Edwards GS, Harward WE, III, Macri BJ. Investigation of selected potential environmental contaminants: Formaldehyde. Washington, DC: United States Environmental Protection Agency. 1976.
  12. Verschueren, K. Handbook of environmental data on organic chemicals: Vol. 1 (No. Ed. 4). John Wiley and Sons, Inc. 2001.
  13. Chae HJ, Kim HK, Kim SK, Pyo HS, Hong JK. Analysis and Risk Assessment of Formaldehyde in Water from Water Purification Plant in Korea. Analytical Science & Technology. 2009; 22(5): 386-394.
  14. Calvert GJ. Formaldehyde and other Aldehydes. National Research Council, Washington, USA. 1981.
  15. ToxFAQs, A. T. S. D. R. Agency for Toxic Substances and Disease Registry (ATSDR): Formaldehyde. 1999.
  16. Mopper K, Stahovec WL. Sources and sinks of low molecular weight organic carbonyl compounds in seawater. Marine Chemistry. 1986; 19(4): 305-321. https://doi.org/10.1016/0304-4203(86)90052-6
  17. US EPA (United State Environmental Protection Agency). Indoor Air Quality (IAQ). 2007.
  18. MoE (Ministry of Environment). Multi-Media and Multi-Pathway Aggregate Risk Assessment (II)-Formaldehyde-. 2012.
  19. Liu W, Zhang J, Korn LR, Zhang L, Weisel CP, Turpin B, et al. Predicting personal exposure to airborne carbonyls using residential measurements and time/activity data. Atmospheric Environment. 2007; 41: 5280-5288. https://doi.org/10.1016/j.atmosenv.2006.05.089
  20. Sexton K, Mongin SJ, Adgate JL, Pratt GC, Ramachandran G, Stock TH, et al. Estimating volatile organic compound concentrations in selected microenvironments using time-activity and personal exposure data. Journal of Toxicology and Environmental Health, Part A. 2007; 70: 465-476. https://doi.org/10.1080/15287390600870858
  21. Yang WH, Lee KY, Park KH, Yoon CS, Son BS, Jeon JM, et al. Microenvrionmental Time Activity Patterns of Weekday and Weekend on Korean. Korean Society for Indoor Environment. 2009; 6(4): 267-274.
  22. Lai HK, Kendall M, Ferrier H, Lindup I, Alm S, Hanninen O, et al. Personal exposures and microenvironment concentrations of $PM_{2.5}$, VOC, $NO_2$ and CO in Oxford, UK. Atmospheric Environment. 2004; 38: 6399-6410. https://doi.org/10.1016/j.atmosenv.2004.07.013
  23. Schwab M, Colome SD, Spengler JD, Ryan PB, Billick IH. Activity patterns applied to pollutant exposure assessment: data from a personal monitoring study in Los Angeles. Toxicology and industrial health. 1990; 6(6): 517.
  24. Noy D, Brunekreef B, Boleij JS, Houthuijs D, De Koning R. The assessment of personal exposure to nitrogen dioxide in epidemiological studies. Atmospheric Environment. Part A. General Topics. 1990; 24(12): 2903-2909. https://doi.org/10.1016/0960-1686(90)90470-8
  25. Yoon HJ, Shuai JF, Kim TS, Seo JK, Jung DY, Ryu HS, et al. Microenvironmental Time-Activity Patterns of Weekday and Weekend on Korean Adults. 2017; 16(2): 182-186. https://doi.org/10.15250/joie.2017.16.2.182
  26. US EPA IRIS (United State Environmental Protection Agency Integrated Risk Infomation System). Formaldehyde; CASRN 50-00-0. Available: http://cfpub.epa.gov/ncea/iris/iris_documents/documents/subst/0419_summary.pdf [accessed 28 October 2019].
  27. Bae HJ, Kim MH, Lee AK, Park JI, Acute Effects of $PM_{10}$ on Asthma Hospitalization Among Children and Benefit Analysis at Four Major Cities in Korea. Korean Society of Environmental Health. 2009; 35(1): 1-10. https://doi.org/10.5668/JEHS.2009.35.1.001
  28. Korea Environment Institute. A Study on Children's Environmental Disease due to $PM_{2.5}$. 2014.
  29. Bae HJ. Effects of Short-term Exposure to $PM_{10}$ and $PM_{2.5}$ on Mortality in Seoul. Korean Society of Environmental Health. 2014; 40(5): 346-354. https://doi.org/10.5668/JEHS.2014.40.5.346
  30. MoE (Ministry of Environment). Korean Exposure Factors Handbook for Children, 2016.
  31. MoE (Ministry of Environment). Korean Exposure Factors Handbook, 2007.
  32. KOSTAT (Statistics Korea). Life Time Table 2019.
  33. Yoon CS, Park DW, Park DY, Jung JY, Lee GY. Variation of Formaldehyde Concentration in Preschool Facilities by Location and Indoor/Outdoor. Korean Society of Environmental Health. 2004; 30(3): 259-263.
  34. Kang DH, Choi DH. A Preliminary Study to Evaluate the Impact of Outdoor Dust on Indoor Air by Measuring Indoor/Outdoor Particle Concentration in a Residential Housing Unit. Journal of Korean Institute of Architectural Sustainable Environment and Building Systems. 2015; 9(6): 462-469.
  35. Yang JY, Kim HH, Shin DC, Kim YS, Sohn JR, Lim JH, et al. Health Risk Assessment of Occupants in the Small-Scale Public Facilites for Aldehydes and VOCs. Journal of the Environmental Sciences. 2008; 17(1): 45-56. https://doi.org/10.5322/JES.2008.17.1.045
  36. Huang L, Mo J, Sundell J, Fan Z, Zhang Y. Health risk assessment of inhalation exposure to formaldehyde and benzene in newly remodeled buildings, Beijing. PLoS One. 2013; 8(11): e79553. https://doi.org/10.1371/journal.pone.0079553
  37. Sax SN, Bennett DH, Chillrud SN, Ross J, Kinney PL, Spengler JD. A cancer risk assessment of innercity teenagers living in New York City and Los Angeles. Environmental health perspectives. 2006; 114(10): 1558-1566. https://doi.org/10.1289/ehp.8507
  38. MoE (Ministry of Environment). Survey on the Actual Condition of Indoor Air Quality in Non-Prosecuted Multi-use Facilities. 2015.